arXiv subjects

Rachel Grange

Publications and source records attributed to Rachel Grange.

At least 19 recordsLinked to original sources

arXiv2026

Cryogenic nonlinear processes in thin-film lithium niobate

Photonic integrated circuits operating at cryogenic temperatures are necessary for many quantum technologies such as quantum transduction, integrated single-photon emitters and detectors, as well as deep-space communication and sensing devices. Thin-film lithium niobate (TFLN) is an emerging platform that is a strong candidate for fully integrated quantum photonics, offering low loss, fast electro-optic reconfigurability, nonlinear quantum light sources, and the ability to host quantum emitters and single-photon detectors. To interface TFLN with technologies that require cryogenic operation, like superconducting single-photon detectors, microwave-to-optical transducers, and solid-state quantum emitters, it is important to study its optical and electrical properties from room temperature down to cryogenic temperatures. Here, we investigate linear and nonlinear photonic devices, including racetrack resonators, Mach-Zehnder modulators and periodically poled waveguides in TFLN using a cryogenic fiber probe station with full temperature control down to 5 K. We quantify a shift in resonances, a 22% increase in electro-optic modulator half-wave voltage, a blue shift of 18 nm for Type-0 phase-matching as well as a red shift of 64 nm for Type-II phase-matching as the sample temperature decreases. Our study of nonlinear processes in a cryogenic environment will contribute towards developing novel devices for inter-platform quantum information processing, secure communication, and enhanced sensing.

physics.optics↗

arXiv2026

Integrated tunable mid-infrared electro-optic frequency comb generator based on nonlinear conversion

Mid-infrared frequency combs enable highly selective and sensitive molecular spectroscopy by leveraging the strong vibrational transitions in this spectral region. Among these, there is a particular need for compact, tunable sources with electronic control over comb parameters for integrated sensing platforms. In this work, we demonstrate a mid-infrared electro-optic frequency comb source based on nonlinear frequency conversion in thin film lithium niobate. The system combines a near-infrared pump, amplitude-modulated using an integrated Mach-Zehnder modulator for lock-in detection, with a telecom-band electro-optic comb generated via a double-pass phase modulation scheme. Mid-infrared comb generation is achieved through difference frequency generation in a periodically poled waveguide. By tuning the telecom seed laser and the chip temperature, we obtain mid-infrared combs with a bandwidth of approximately 6 nm and center wavelength tunability of over 200 nm. The comb free spectral range is directly controlled via the applied radio-frequency modulation. Operation across multiple integrated photonic circuits reaching wavelengths up to 3.7 $\mu$m is demonstrated. Furthermore, dual-tone EO comb generation in the mid-infrared is realized. To our knowledge, this is the first integrated mid-infrared electro-optic comb source offering independent electronic control of both center wavelength and comb spacing.

physics.optics↗

arXiv2026

Integrated electro-optic attention nonlinearities for transformers

Transformers have emerged as the dominant neural-network architecture, achieving state-of-the-art performance in language processing and computer vision. At the core of these models lies the attention mechanism, which requires a nonlinear, non-negative mapping using the Softmax function. However, although Softmax operations account for less than 1% of the total operation count, they can disproportionately bottleneck overall inference latency. Here, we use thin-film lithium niobate (TFLN) Mach-Zehnder modulators (MZMs) as analog nonlinear computational elements to drastically reduce the latency of nonlinear computations. We implement electro-optic alternatives to digital Softmax and Sigmoid, and evaluate their performance in Vision Transformers and Large Language Models. Our system maintains highly competitive accuracy, even under aggressive 4-bit input-output quantization of the analog units. We further characterize system noise at encoding speeds up to 10 GBaud and assess model robustness under various noise conditions. Our findings suggest that TFLN modulators can serve as nonlinear function units within hybrid co-packaged hardware, enabling high-speed and energy-efficient nonlinear computation.

cs.LG↗

arXiv2026

Wavelength-selective nonlinear wavefront control in resonant thin-film lithium niobate metasurfaces

Nonlinear metasurfaces offer compact control over frequency conversion and wavefront shaping. However, existing approaches, often based on geometric phase, lack wavelength selectivity, resulting in static nonlinear responses. Here, we demonstrate a thin-film lithium niobate metasurface that enables spectrally selective shaping of second-harmonic generation through resonance-engineered phase control. The structure consists of two regions with distinct phase responses, realized via spectral tuning of Mie-type resonances. This design enables simultaneous frequency conversion and spatial mode shaping, transforming a Gaussian pump near 1100 nm into a first-order Hermite-Gaussian mode at 550 nm, while maintaining the pump profile. The demonstrated approach offers a pathway toward ultracompact and tunable components for nonlinear holography and related applications.

physics.optics↗

arXiv2026

Electro-Optic Modulation in Polycrystalline Barium Titanate Metasurfaces Enhanced by Poling

Electrically tunable metasurfaces leveraging the strong Pockel's effect in barium titanate (BaTiO$_3$ or BTO) are a promising platform for reconfigurable free-space optical devices. However, the high cost, limited scalability, and restricted substrate compatibility of epitaxial BTO films hinder its exploitation. Here, we demonstrate free-space optical modulators based on imprinted BTO metasurfaces with targeted designs for optical and electric field confinement within the active material. With resonances exhibiting high quality factors of up to 200, we demonstrate improved transmission modulation at sub-volt driving amplitudes and frequencies up to 5 MHz. Additional enhancement is achieved via ferroelectric domain alignment, resulting in up to 25 % higher modulation strength compared to the unbiased case and up to 75 % compared to previous demonstrations. This enhanced EO response, arising from the effective permittivity engineering and domain orientation in these polycrystalline metasurfaces, holds significant potential for scalable and efficient EO modulators and active metasurfaces.

physics.optics↗

arXiv2026

Solution-derived barium titanate waveguides for integrated electro-optic modulation

Metal oxides with strong nonlinear optical properties and wide transparency window are key materials for the development of compact and efficient photonic integrated circuits used for electro-optic modulators and entangled photon sources. Among them, barium titanate (BaTiO$_{3}$) is particularly attractive due to its large Pockels coefficient. However, its use has been limited by challenges in material synthesis and in nanopatterning, owing to its chemical stability and inertness. Here, we demonstrate a monolithic electro-optic modulator entirely based on solution-deposited BaTiO$_{3}$, fabricated through a bottom-up soft nanoimprinting lithography process. Fine-tuning the synthesis and nanofabrication enhances the optical properties of the polycrystalline material. By optimizing the process parameters, we achieve a reduction in propagation losses of two orders of magnitude, enabling efficient electro-optic modulation. This scalable, etch-free approach enables direct patterning of high-quality BaTiO$_{3}$ structures, establishing a new route for low-cost, large-scale integrated electro-optic devices entirely based on oxide material compatible with a wide range of substrates.

physics.optics↗

arXiv2025

Order-disorder duality of high entropy alloys extends non-linear optics

Order versus disorder in the structure of materials plays a key role in the theoretical prediction of their properties. However, this structural description appears to be ineffective for new families of materials such as high entropy alloys (HEAs), which combine crystallographic order with chemical disorder. Here, we demonstrate for five-element HEAs as pure solid solutions that the chemical disorder of the elements decorating their cubic structure underlies the generation of second optical harmonics, overcoming the theoretical limit imposed on centrosymmetric crystals. Moreover, we discover that this disorder, inherent to HEAs, sets a threshold for non-linear light emission from the 4th to the 26th order. As a consequence of the 0.5 eV broadening of the energy levels of the five elements of the HEA, the emission spectrum covers broad visible (400-650 nm) and infrared (800-1600 nm) ranges. In addition to the challenge of theoretically predicting non-linear effects in unconventional materials, the duality of structural order and chemical disorder in HEAs offers the opportunity to design sustainable alternatives to urgently needed optical materials.

cond-mat.mtrl-sci↗

arXiv2025

Electro-optical modulation of light polarization in a nonlocal lithium niobate metasurface

We report the experimental realization of a LiNbO3 metasurface for electro-optic modulation of light polarization in the telecommunication band. High-Q quasi-bound states in the continuum are emploied to enhance the modulation of amplitude and phase of an impinging beam by a driving electric field, leading to efficient polarization rotation and conversion. We quantified modulation effects under a CMOS-compatible bias at 1 MHz frequency, achieving a variation of 5% in the Stokes parameters and a variation of the polarization ellipse angles of about 3{\deg} for the transmitted light. These results demonstrate that dynamic polarization and phase modulation can be attained in a compact platform, highlighting the potential of high-Q resonant LiNbO3 metasurfaces for enhanced light-matter interaction in subwavelength electro-optic devices.

physics.optics↗

arXiv2025

Tunable polarization-entangled near-infrared photons from orthogonal GaAs nanowires

Quantum entanglement is a fundamental resource for emerging quantum technologies, enabling secure communication and enhanced sensing. For decades, generating polarization entangled states has been mainly achieved using bulk crystals with spontaneous parametric down conversion (SPDC), preventing scalability and on-chip integration. Miniaturizing the quantum source provides access to more versatility and tunability while enabling an easier integration to other devices, notably necessary for satellite-based quantum communication, and eventually reducing fabrication costs. This challenging task can be achieved with Zinc Blende GaAs nanowires. They already have shown an efficient photon pairs generation via SPDC at 1550 nm. Here we demonstrate that a pair of orthogonal GaAs nanowires constitutes a new nanoscale platform to control the quantum state at telecommunication wavelength, enabling a transition from polarization entangled to separable states as a function of the pump polarization, with fidelities reaching 90%

physics.optics↗

arXiv2025

Fostering cultural change in research through innovative knowledge sharing, evaluation, and community engagement strategies

Bringing together researchers, funders, industry partners, and publishers from 14 countries across 5 continents, we advance the debate around open-science, assessment and learning. We introduce an integrative "open knowledge system" framework linking knowledge production, validation, assessment, and reuse into one ecosystem view, and translate it into actionable recommendations for each stakeholder. Shifting focus to modular, machine-readable knowledge objects, these recommendations are intended to help diagnose misaligned incentives and guide reforms that properly value all scientific contributions.

cs.SI↗

arXiv2025

High-temperature growth of ultra thin NbTiN films on lithium niobate for integrated single photon detection

Lithium niobate-on-insulator (LNOI) is an emerging photonic platform with high potential for scalable quantum information processing due to its strong second-order nonlinearity. However, little progress has been made in developing on-chip single-photon detectors on LNOI. Niobium titanium nitride (NbTiN) superconducting nanowire single-photon detectors (SNSPDs) are a promising candidate for this application. In this work, we use DC reactive magnetron sputtering to grow high-quality NbTiN thin films using an ultra-high vacuum deposition system with a base pressure lower than $2\times 10^{-10}$ mbar. Enabled by the low concentration of background impurities in this system, we investigate the impact of substrate temperature during NbTiN growth. We achieve four nm thick superconducting films with a critical temperature ($T_{c}$) of 12.3 K grown at a substrate temperature of 825 K. We find that the NbTiN films grow in the (111) orientation and evolve from a porous pillar structure when grown at low temperatures to densely packed fibrous grains at higher temperatures. Furthermore, we demonstrate that the increased substrate temperature reduces the oxygen concentration in our films and improves the overall stoichiometry. In addition, we integrate these films with the LNOI platform and investigate the obtained interface quality. Lastly, we fabricate SNSPDs from the NbTiN film on LNOI and characterize the detector performance.

cond-mat.supr-con↗

arXiv2025

Nanodomain poling unlocking backward nonlinear light generation in thin film lithium niobate

Nonlinear frequency conversion offers powerful capabilities for applications in telecommunications, signal processing, and computing. Thin-film lithium niobate (TFLN) has emerged as a promising integrated photonics platform due to its strong electro-optic effect and second-order nonlinearity, which can be exploited through periodic poling. However, conventional poling techniques in x-cut TFLN are limited to minimum period sizes on the order of microns, preventing the efficient generation of interactions involving counter-propagating waves. Here we report scalable periodic poling of x-cut TFLN with periods down to 215 nm and realize devices for counter- and back-propagating phase matching. We estimate conversion efficiencies of 1474 $\%$/W/cm$^2$ and 45 $\%$/W/cm$^2$ respectively, and measuring sum frequency generation we confirm that the nonlinear generation takes place in the desired direction. We report spontaneous parametric down conversion for the counter-propagating and, for the first time, for a backward propagating device. This technological advance provides the control of domain geometry in TFLN with an unprecedented precision and leads into the generation of photon pairs with spatial and spectral properties tailored for quantum signal processing, quantum computing and metrology.

physics.optics↗

arXiv2025

Counter-propagating spontaneous parametric down-conversion source in lithium niobate on insulator

Quantum photonic technologies rely on the ability to generate, manipulate, and interfere indistinguishable single photons on a scalable platform. Among the various approaches, spontaneous parametric down-conversion (SPDC) remains one of the most widely used methods for generating entangled or pure photon pairs. However most integrated SPDC sources relying on co-propagating geometries have a limited purity of heralded photons, or require lossy filtering. Type-2 SPDC processes can produce pure separable photons but typically suffer from lower efficiency and added complexity due to polarisation management. Here we show the first integrated counter-propagating photon-pair source on lithium niobate on insulator, where signal and idler photons are generated in opposite directions. The counter-propagating geometry leads to spectrally uncorrelated photon pairs without spectral filtering. The joint spectral intensity measurements and unheralded $g^{(2)}$ correlations, yield purities of (92$\pm$3)%. Interference between two independent sources achieves heralded visibilities of (71$\pm$3)%, confirming the scalability of the platform. These results establish a new route toward integrated, high-purity, and tunable photon sources. The demonstrated counter-propagating geometry offers a scalable solution for quantum photonic networks.

quant-ph↗

arXiv2025

Scalable quantum interference in integrated lithium niobate nanophotonics

Photonics has emerged as one of the leading platforms for the implementation of real-world-applicable quantum technologies, enabling secure communication, enhanced sensing capabilities, as well as resolving previously intractable computational challenges. However, to harness the full potential of the photonics platform, several engineering feats need to be accomplished, among those is the quest for a scalable source of pure single photons. While single photon sources can be implemented in a variety of different ways, integrated lithium niobate stands out as a prime contender for a monolithic quantum photonics platform, given its second-order nonlinearity and proven classical scalability. Despite the extensive effort put into developing the platform, integrating suitable photon pair sources remains a hurdle limiting the scalability of quantum photonic systems in lithium niobate. We engineer three-wave-mixing in a nanophotonic lithium niobate device, integrating multiple near-perfect spectrally separable heralded single photon sources. By mixing photons generated via the developed sources, we show bosonic interference between indistinguishable photons, a crucial interaction for many photonic quantum computing protocols. This demonstration of the first proof-of-principle multi-source interference in integrated lithium niobate contributes to developing a truly scalable quantum photonics platform.

quant-ph↗

arXiv2025

Programmable Bell State Generation in an Integrated Thin Film Lithium Niobate Circuit

Entanglement is central to quantum technologies such as cryptography, sensing, and computing. Photon pairs generated via nonlinear optical processes are excellent for preparing entangled states due to their long coherence times and compatibility with fiber optic networks. Steady progress in nanofabrication has positioned lithium niobate-on-insulator (LNOI) as a leading platform for monolithic integration of photon pair sources into optical circuits, leveraging its strong second-order nonlinearity. Here, we present a reconfigurable photonic integrated circuit on LNOI, which combines two on-chip photon pair sources with programmable interferometers, enabling generation of entangled states. The pair sources achieve a source brightness of 26 MHz nm$^{-1}$ mW$^{-1}$ while maintaining a coincidence-to-accidental ratio above 100. We successfully interfere the two sources with $99 \pm 0.7$ % visibility, demonstrating the indistinguishability required for producing entanglement on-chip. We show preparation of any of the maximally entangled Bell states with fidelity above 90 % verified by quantum state tomography. These results establish LNOI as a compelling, scalable platform to explore integrated quantum photonic technologies enabled by high-brightness sources of entangled quantum states.

quant-ph↗

arXiv2025

Integrated thin film lithium niobate mid-infrared modulator

The mid-infrared spectral range holds great promise for applications such as molecular spectroscopy and telecommunications. Many key molecules exhibit strong absorption features in this range, and free-space optical communication benefits from reduced atmospheric attenuation and low transmission losses in specific wavelength bands spanning from 3 to 14 $\mu m$. Recent progress in MIR photonics has been fuelled by the rapid development of efficient light sources and detectors. However, further advancement is hindered by the lack of low-loss, high-performance integrated photonic platforms and modulators. Lithium niobate on sapphire is a promising candidate, operating across a broad spectral range from 0.4 $\mu m$ to 4.5 $\mu m$. We demonstrate a broadband, high-speed lithium niobate on sapphire Mach-Zehnder electro-optic modulator operating from 3.95 to 4.3 $\mu m$. The device achieves a 3 dB bandwidth exceeding 20 GHz, an extinction ratio of 34 dB, and a half-wave voltage of 22 V$\cdot$cm, delivering optical output power at the half-milliwatt level. These properties are leveraged to demonstrate data transmission at 10 Gbit/s. The modulator is also used to generate a frequency comb with a width of 80 GHz. Furthermore, we demonstrate full $\pi$-phase modulation in the MIR, representing a key milestone for integrated MIR photonics. These results establish a pathway toward high-speed, energy-efficient MIR photonic systems for applications in telecommunications, sensing, and quantum technologies.

physics.optics↗

arXiv2025

Low threshold integrated optical parametric oscillator with a compact Bragg resonator

Optical parametric oscillators (OPOs) have been studied as basic components for optical computing with phase encoding and Ising machines. Integrated photonics offers a scalable solution to incorporate a progressively larger number of devices towards a functional computing module. Among the available platforms, lithium niobate on insulator is an excellent candidate for this goal thanks to its large second order nonlinearity, which can be leveraged via periodic poling of the thin film. In this work, we show a device with a 2.5 mW threshold for parametric oscillation, which is the lowest reported to date among double-resonant OPOs. We use a novel configuration with a Fabry-P\'erot cavity, which reduces the footprint compared to a typical ring resonator by a factor 10. Tuning our devices using pump wavelength and local heating, we can operate the oscillators at degeneracy, which is crucial for logical operations requiring phase bistability. Our results showcase the device as an ideal building block for phase-encoded integrated optical computing, enabling spatial multiplexing with reduced footprint and power consumption.

physics.optics↗

arXiv2024

Efficient GHz electro-optical modulation with a nonlocal lithium niobate metasurface in the linear and nonlinear regime

Electro-optical modulation is widely employed for optical signal processing and in laser technology. To date, it is efficiently realized in integrated photonic systems as well as in bulk optics devices. Yet, the achievement of modulators exploiting Pockels effect in flat optics, essential to scale down the electric radiation-optical control in free space, currently lag behind bulk and on-chip integrated platforms in terms efficiency and speed. We bridge this gap realizing a metasurface based on lithium niobate (LiNbO3) on insulator that leverages on resonances with quality-factor as high as 8e3 to achieve fast electrical modulation of both linear and nonlinear optical properties. LiNbO3, well known for its high nonlinear susceptibility and wide transparency window across the infrared and visible spectrum, is employed to realize an asymmetric, one-dimensional array of nanowires, exhibiting resonances with linewidth < 0.2 nm. By applying a CMOS-compatible electrical bias, the metasurface imparts a relative reflectivity modulation around 0.1, with a modulation efficiency, defined as relative modulation per applied Volt, larger than 0.01 V^-1 on a bandwidth of about 1 GHz. We also demonstrated more than one order of magnitude intensity modulation of the second harmonic seeded by a continuous-wave laser, with a modulation efficiency of about 0.12 V^-1. This dual modulation capability, rooted in the interplay between optical resonances and electric field manipulation, holds significant potential for cutting-edge applications in high-speed photonics, nonlinear optics, and reconfigurable communication systems. Our findings highlight the transformative potential of LiNbO3-based metasurfaces for integration into next-generation optical technologies that demand rapid, efficient electrical control of light.

physics.optics↗