arXiv subjects

Radu Coldea

Publications and source records attributed to Radu Coldea.

22 records · Page 2Linked to original sources

arXiv2006

Excitation spectra and ground state properties of the layered spin-1/2 frustrated antiferromagnets Cs_2CuCl_4 and Cs_2CuBr_4

We use series expansion methods to study ground- and excited-state properties in the helically ordered phase of spin-1/2 frustrated antiferromagnets on an anisotropic triangular lattice. We calculate the ground state energy, ordering wavevector, sublattice magnetization and one-magnon excitation spectrum for parameters relevant to Cs_2CuCl_4 and Cs_2CuBr_4. Both materials are modeled in terms of a Heisenberg model with spatially anisotropic exchange constants; for Cs_2CuCl_4 we also take into account the additional Dzyaloshinskii-Moriya (DM) interaction. We compare our results for Cs_2CuCl_4 with unpolarized neutron scattering experiments and find good agreement. In particular, the large quantum renormalizations of the one-magnon dispersion are well accounted for in our analysis, and inclusion of the DM interaction brings the theoretical predictions for the ordering wavevector and the magnon dispersion closer to the experimental results.

cond-mat.str-el↗

arXiv2006

Excitation spectra of the spin-1/2 triangular-lattice Heisenberg antiferromagnet

We use series expansion methods to calculate the dispersion relation of the one-magnon excitations for the spin-1/2 triangular-lattice nearest-neighbor Heisenberg antiferromagnet above a three-sublattice ordered ground state. Several striking features are observed compared to the classical (large-S) spin-wave spectra. Whereas at low energies the dispersion is only weakly renormalized by quantum fluctuations, significant anomalies are observed at high energies. In particular, we find roton-like minima at special wave-vectors and strong downward renormalization in large parts of the Brillouin zone, leading to very flat or dispersionless modes. We present detailed comparison of our calculated excitation energies in the Brillouin zone with the spin-wave dispersion to order 1/S calculated recently by Starykh, Chubukov, and Abanov [cond-mat/0608002]. We find many common features but also some quantitative and qualitative differences. We show that at temperatures as low as 0.1J the thermally excited rotons make a significant contribution to the entropy. Consequently, unlike for the square lattice model, a non-linear sigma model description of the finite-temperature properties is only applicable at extremely low temperatures.

cond-mat.str-el↗

arXiv2006

Anomalous Excitation Spectra of Frustrated Quantum Antiferromagnets

We use series expansions to study the excitation spectra of spin-1/2 antiferromagnets on anisotropic triangular lattices. For the isotropic triangular lattice model (TLM) the high-energy spectra show several anomalous features that differ strongly from linear spin-wave theory (LSWT). Even in the Neel phase, the deviations from LSWT increase sharply with frustration, leading to roton-like minima at special wavevectors. We argue that these results can be interpreted naturally in a spinon language, and provide an explanation for the previously observed anomalous finite-temperature properties of the TLM. In the coupled-chains limit, quantum renormalizations strongly enhance the one-dimensionality of the spectra, in agreement with experiments on Cs_2CuCl_4.

cond-mat.str-el↗

arXiv2005

Temperature Dependence of the Magnetic Susceptibility for Triangular-Lattice Antiferromagnets with spatially anisotropic exchange constants

We present the temperature dependence of the uniform susceptibility of spin-half quantum antiferromagnets on spatially anisotropic triangular-lattices, using high temperature series expansions. We consider a model with two exchange constants, $J_1$ and $J_2$ on a lattice that interpolates between the limits of a square-lattice ($J_1=0$), a triangular-lattice ($J_2=J_1$), and decoupled linear chains ($J_2=0$). In all cases, the susceptibility which has a Curie-Weiss behavior at high temperatures, rolls over and begins to decrease below a peak temperature, $T_p$. Scaling the exchange constants to get the same peak temperature, shows that the susceptibilities for the square-lattice and linear chain limits have similar magnitudes near the peak. Maximum deviation arises near the triangular-lattice limit, where frustration leads to much smaller susceptibility and with a flatter temperature dependence. We compare our results to the inorganic materials Cs$_2$CuCl$_4$ and Cs$_2$CuBr$_4$ and to a number of organic molecular crystals. We find that the former (Cs$_2$CuCl$_4$ and Cs$_2$CuBr$_4$) are weakly frustrated and their exchange parameters determined through the temperature dependence of the susceptibility are in agreement with neutron-scattering measurements. In contrast, the organic materials are strongly frustrated with exchange parameters near the isotropic triangular-lattice limit.

cond-mat.str-el↗