arXiv subjects

Radu Malureanu

Publications and source records attributed to Radu Malureanu.

At least 19 recordsLinked to original sources

arXiv2026

Polarization-Sensitive Third Harmonic Generation in resonant silicon nitride Metasurfaces for deep-UV Emission

We present a combined experimental and theoretical study of enhanced third-harmonic generation (THG) in silicon nitride metasurfaces. These structures exhibit strong resonant nonlinear responses, enabling up to two orders of magnitude enhancement in THG compared to a flat silicon nitride etalon, driven by strong electromagnetic field localization. We investigate two polarization-selective metasurface geometries supporting transverse electric (TE) and transverse magnetic (TM) resonances, implemented in fully planar architecture. When driven by ultrafast near-infrared laser pulses, these resonances confine optical energy at the nanoscale, enabling efficient frequency up-conversion from the visible to the ultraviolet (UV) and deep-UV spectral regions. Through spectral mapping of the nonlinear response under both TE and TM excitation, we quantify field confinement, extract the effective nonlinear enhancement, and characterize the spectral dependence of the third-harmonic generation efficiency. This two-dimensional periodic platform provides a flexible design toolbox for engineering polarization-dependent UV and deep-UV light sources. More broadly, our results demonstrate that silicon nitride, a CMOS-compatible dielectric, can support efficient nonlinear up-conversion deep into the UV. This finding shows that access to short-wavelength nonlinear photonics does not require complex materials or architectures, but can instead be achieved using widely available dielectrics through careful structural design.

physics.optics↗

arXiv2026

Enhancing FRET through DNA-controlled Emitters and ENZ Metamaterials

The ability to significantly enhance energy transfer processes at the nanoscale requires the simultaneous optimization of molecular-scale orientation and macroscopic photonic enhancement between multiple quantum emitters. However, achieving this dual control has remained a significant experimental challenge, often limited by the stochastic arrangement of emitter assemblies and spatially non-uniform electromagnetic fields in conventional photonic platforms. In this work, we demonstrate a unified architecture that achieves this synergy by combining the structural precision of DNA nanotechnology with the unique field environment generated by epsilon-near-zero (ENZ) materials. Using DNA molecular beacons as programmable emitter scaffolds, we establish fixed donor-acceptor separations and emitter orientations (Atto425/Cy3.5) in two well-defined conformational states: closed hairpin (emitter separation 2 nm) and extended (8.16 nm) configurations. These structures are then embedded in the near-field of a multilayer ENZ metamaterial substrate, which facilitates spatially uniform, enhanced electromagnetic field coupling. Time-resolved photoluminescence measurements demonstrate a significant increase in FRET efficiency for DNA-programmed emitter pairs in the ENZ environment, compared to those on a glass substrate, corresponding to increased donor quenching and shortened donor lifetime. These results establish a scalable experimental pathway for engineering light-matter interactions at molecular scales with applications in next-generation biosensing and quantum photonic technologies.

physics.optics↗

arXiv2025

Integrated angstrom-tunable polarization-resolved solid-state photon sources

The development of high-quality solid-state photon sources is essential to nano optics, quantum photonics, and related fields. A key objective of this research area is to develop tunable photon sources that not only enhance the performance but also offer dynamic functionalities. However, the realization of compact and robust photon sources with precise and wide range tunability remains a long-standing challenge. Moreover, the lack of an effective approach to integrate nanoscale photon sources with dynamic systems has hindered tunability beyond mere spectral adjustments, such as simultaneous polarization control. Here we propose a platform based on quantum emitter (QE) embedded metasurfaces (QEMS) integrated with a microelectromechanical system (MEMS)-positioned microcavity, enabling on-chip multi-degree control of solid-state photon sources. Taking advantages of MEMS-QEMS, we show that typically broadband room-temperature emission from nanodiamonds containing nitrogen-vacancy centres can be narrowed to 3.7 nm and dynamically tuned with angstrom resolution. Furthermore, we design a wavelength-polarization-multiplexed QEMS and demonstrate polarization-resolved control of the MEMS-QEMS emission in a wide wavelength range (650 nm to 700 nm) along with polarization switching at sub-millisecond timescales. We believe that the proposed MEMS-QEMS platform can be adapted for most existing QEs, significantly expanding their room-temperature capabilities and thereby enhancing their potential for advanced photonic applications.

physics.optics↗

arXiv2020

Near-Zero Index Photonic Crystals with Directive Bound States in the Continuum

Near-zero-index platforms arise as a new opportunity for light manipulation with boosting of optical nonlinearities, transmission properties in waveguides and constant phase distribution. In addition, they represent a solution to impedance mismatch faced in photonic circuitry offering several applications in quantum photonics, communication and sensing. However, their realization is limited to availability of materials that could exhibit such low-index. For materials used in the visible and near-infrared wavelengths, the intrinsic losses annihilate most of near-zero index properties. The design of all-dielectric photonic crystals with specific electromagnetic modes overcame the issue of intrinsic losses while showing effective mode index near-zero. Nonetheless, these modes strongly radiate to the surrounding environment, greatly limiting the devices applications. Here, we explore a novel all-dielectric photonic crystal structure that is able to sustain effective near-zero-index modes coupled to directive bound-states in the continuum in order to decrease radiative losses, opening extraordinary opportunities for radiation manipulation in nanophotonic circuits. Moreover, its relatively simple design and phase stability facilitates integration and reproducibility with other photonic components.

physics.optics↗

arXiv2020

Experimental verification of a plasmonic hook in a dielectric Janus particle

We report on a very first experimental observation of a new curved plasmonic beam, a plasmonic hook (PH), for surface plasmon-polariton (SPP) waves. We demonstrate that the SPP PH effect could be realized within a trapezoidal dielectric microstructure with the relative ease of fabrication compared to the generation of the Airy SPP waves which require complex techniques to compensate the wave vectors mismatch. Using numerical analysis, we predicted the PH phenomenon, optimized the microstructure and then confirmed the SPP PH existence via amplitude and phase-resolved scattering scanning near-field optical microscopy at the telecom wavelengths of 1530-1570 nm. The experimental results are in reasonable agreement with our predictions. Importantly, the SPP PH demonstrates the smallest radius of curvature ever recorded for SPP waves compared to that for the Airy-family plasmonic beams providing many useful applications spreading from nanoparticles manipulation toward bio-sensing within a nanoscale.

physics.optics↗

arXiv2020

Engineering nanoparticles with pure high-order multipole scattering

The ability to control scattering directionality of nanoparticles is in high demand for many nanophotonic applications. One of the challenges is to design nanoparticles producing pure high-order multipole scattering (e.g., octopole, hexadecapole), whose contribution is usually negligible compared to strong low-order multipole scattering (i.e., dipole or quadrupole). Here we present an intuitive way to design such nanoparticles by introducing a void inside them. We show that both shell and ring nanostructures allow regimes with nearly pure high-order multipole scattering. Experimentally measured scattering diagrams from properly designed silicon rings at near-infrared wavelengths (~ 800 nm) reproduce well scattering patterns of an electric octopole and magnetic hexadecapole. Our findings advance significantly inverse engineering of nanoparticles from given complex scattering characteristics, with possible applications in biosensing, optical metasurfaces, and quantum communications.

physics.optics↗

arXiv2019

Magnetic and Electric Mie-Exciton Polaritons in Silicon Nanodisks

Light-matter interactions at the nanoscale constitute a fundamental ingredient for engineering applications in nanophotonics and quantum optics. To this regard electromagnetic Mie resonances excited in high-refractive index dielectric nanoparticles have recently attracted interest because of their lower losses and better control over the scattering patterns compared to their plasmonic metallic counterparts. The emergence of several resonances in those systems results in an overall high complexity, where the electric and magnetic dipoles have significant overlap in the case of spherical symmetry, thus concealing the contributions of each resonance separately. Here we show, experimentally and theoretically, the emergence of strong light-matter coupling between the magnetic and electric-dipole resonances of individual silicon nanodisks coupled to a J-aggregated organic semiconductor resonating at optical frequencies, evidencing how the different properties of the two resonances results in two different coupling strengths. The energy splittings observed are of the same order of magnitude as in similar plasmonic systems, thus confirming dielectric nanoparticles as promising alternatives for localized strong coupling studies. The coupling of both the electric and magnetic dipole resonances can offer interesting possibilities for the control of directional light scattering in the strong-coupling regime and the dynamic tuning of nanoscale light-matter coupled states by external fields.

physics.optics↗

arXiv2018

Photonic spin Hall effect in hyperbolic metamaterials at visible

Photonic spin Hall effect in transmission is a transverse beam shift of the out-coming beam depending on polarization of the in-coming beam. The effect can be significantly enhanced by materials with high anisotropy. We report the first experimental demonstration of the photonic spin Hall effect in a multilayer hyperbolic metamaterial at visible wavelengths (wavelengths of 520 nm and 633 nm). The metamaterial is composed of alternating layers of gold and alumina with deeply-subwavelength thicknesses, exhibiting extremely large anisotropy. The angle resolved polarimetric measurements showed the shift of 165 $μm$ for the metamaterial of 176 nm in thickness. Additionally the transverse beam shift is extremely sensitive to the variations of the incident angle changing theoretically by 270 $μm$ with one milli-radian ($0.057^\circ$). These features can lead to minituarized spin Hall switches and filters with high angular resolution.

physics.optics↗

arXiv2017

Effective surface conductivity of plasmonic metasurfaces: from far-field characterization to surface wave analysis

Metasurfaces offer great potential to control near- and far-fields through engineering of optical properties of elementary cells or meta-atoms. Such perspective opens a route to efficient manipulation of the optical signals both at nanoscale and in photonics applications. In this paper we show that by using an effective surface conductivity tensor it is possible to unambigiously describe optical properties of an anisotropic metasurface in the far- and near-field regimes. We begin with retrieving the effective surface conductivity tensor from the comparative analysis of experimental and numerical reflectance spectra of a metasurface composed of elliptical gold nanoparticles. Afterwards restored conductivities are validated in the crosscheck versus semianalytic parameters obtained with the discrete dipole model with and without dipoles interaction contribution. The obtained effective parameters are further used for the dispersion analysis of surface plasmons localized at the metasurface. The effective medium model predicts existence of both TE- and TM-polarized plasmons in a wide range of optical frequencies and describes peculiarities of their dispersion, in particularly, topological transition from the elliptical to hyperbolic regime with eligible accuracy. The analysis in question offers a simple practical way to describe properties of metasurfaces including ones in the near-field zone by extracting effective parameters from the convenient far-field characterisation.

physics.optics↗

arXiv2017

Direct amplitude-phase near-field observation of higher-order anapole states

Anapole states associated with the resonant suppression of electric-dipole scattering exhibit minimized extinction and maximized storage of electromagnetic energy inside a particle. Using numerical simulations, optical extinction spectroscopy and amplitude-phase near-field mapping of silicon dielectric disks, we demonstrate high-order anapole states in the near-infrared wavelength range (900-1700 nm). We develop the procedure for unambiguously identifying anapole states by monitoring the normal component of the electric near-field and experimentally detect the first two anapole states as verified by far-field extinction spectroscopy and confirmed with the numerical simulations. We demonstrate that higher order anapole states possess stronger energy concentration and narrower resonances, a remarkable feature that is advantageous for their applications in metasurfaces and nanophotonics components, such as non-linear higher-harmonic generators and nanoscale lasers.

physics.optics↗

arXiv2017

Two-dimensional optical plasmons with mixed polarization on anisotropic resonant metasurface

Optical metasurfaces have great potential to form the platform for manipulation of surface waves. A plethora of advanced surface-wave phenomena utilizing negative refraction, self-collimation and channeling of 2D waves can be realized through on-demand engineering of dispersion properties of a periodic metasurface. In this letter, we report on the first-time direct experimental polarization-resolved measurement of dispersion of 2D optical plasmons supported by an anisotropic metasurface. We demonstrate that a subdiffractive array of strongly coupled resonant anisotropic plasmonic nanoparticles supports unusual optical surface waves with mixed TE- and TM-like polarizations. With the assistance of numerical simulations we identify dipole and quadrupole dispersion bands. The shape of isofrequency contours changes drastically with frequency exhibiting nontrivial transformations of their curvature and topology that is consistently confirmed by the experimental data. By revealing polarization degree of freedom for surface waves, our results open new routes for designing of planar on-chip devices for surface photonics.

physics.optics↗

arXiv2017

Mid-infrared directional surface waves on a high aspect ratio nano-trench platform

Optical surface waves, highly localized modes bound to the surface of media, enable manipulation of light at nanoscale, thus impacting a wide range of areas in nanoscience. By applying metamaterials, artificially designed optical materials, as contacting media at the interface, we can significantly ameliorate surface wave propagation and even generate new types of waves. Here, we demonstrate that high aspect ratio (1:20) grating structures with plasmonic lamellas in deep nanoscale trenches function as a versatile platform supporting both surface and volume infrared waves. The surface waves exhibit a unique combination of properties, such as directionality, broadband existence (from 4 μm to at least 14 μm and beyond) and high localization, making them an attractive tool for effective control of light in an extended range of infrared frequencies.

physics.optics↗

arXiv2017

Laguerre-Gauss beam generation in IR and UV by subwavelength surface-relief gratings

The angular momentum of light can be described by the states of spin angular momentum, associated with polarization, and orbital angular momentum, related to the helical structure of the wave front. Laguerre-Gaussian beams carry orbital angular momentum and their generation can be done by using an optical device known as q-plate. However, due to the usage of liquid crystals, these components may be restricted to operate in specific wavelengths and low power sources. Here we present the fabrication and characterization of q-plates made without liquid crystals, using processes of e-beam lithography, atomic layer depositions and dry etch techniques. We exploit the phenomenon of form birefringence to give rise to the spin-to-orbital angular momentum conversion. We demonstrate that these plates can generate beams with high quality for the UV and IR range, allowing them to interact with high power laser sources or inside laser cavities.

physics.optics↗

arXiv2016

Direct characterization of plasmonic slot waveguides and nanocouplers

We demonstrate the use of amplitude- and phase-resolved near-field mapping for direct characterization of plasmonic slot waveguide mode propagation and excitation with nanocouplers in the telecom wavelength range. We measure mode's propagation length, effective index and field distribution and directly evaluate the relative coupling efficiencies for various couplers configurations. We report 26- and 15-fold improvements in the coupling efficiency with two serially connected dipole and modified bow-tie antennas, respectively, as compared to that of the short-circuited waveguide termination.

physics.optics↗

arXiv2016

Boosting local field enhancement by on-chip nanofocusing and impedance-matched plasmonic antennas

Strongly confined surface plasmon-polariton modes can be used for efficiently delivering the electromagnetic energy to nano-sized volumes by reducing the cross sections of propagating modes far beyond the diffraction limit, i.e., by nanofocusing. This process results in significant local-field enhancement that can advantageously be exploited in modern optical nanotechnologies, including signal processing, biochemical sensing, imaging and spectroscopy. Here, we propose, analyze, and experimentally demonstrate on-chip nanofocusing followed by impedance-matched nanowire antenna excitation in the end-fire geometry at telecom wavelengths. Numerical and experimental evidences of the efficient excitation of dipole and quadrupole (dark) antenna modes are provided, revealing underlying physical mechanisms and analogies with the operation of plane-wave Fabry-Pérot interferometers. The unique combination of efficient nanofocusing and nanoantenna resonant excitation realized in our experiments offers a major boost to the field intensity enhancement up to $\sim 12000$, with the enhanced field being evenly distributed over the gap volume of $30\times 30\times 10\ {\rm nm}^3$, and promises thereby a variety of useful on-chip functionalities within sensing, nonlinear spectroscopy and signal processing.

physics.optics↗

arXiv2015

Experimental Demonstration of Effective Medium Approximation Breakdown in Deeply Subwavelength All-Dielectric Multilayers

We experimentally demonstrate the effect of anomalous breakdown of the effective medium approximation in all-dielectric deeply subwavelength thickness ($d \simλ/160-λ/30$) multilayers, as recently predicted theoretically [H.H. Sheinfux et al., Phys. Rev. Lett. 113, 243901 (2014)]. Multilayer stacks are composed of alternating alumina and titania layers fabricated using atomic layer deposition. For light incident on such multilayers at angles near the total internal reflection we observe pronounced differences in the reflectance spectra for structures with 10-nm versus 20-nm thick layers, as well as for structures with different layers ordering, contrary to the predictions of the effective medium approximation. The reflectance difference can reach values up to 0.5, owing to the chosen geometrical configuration with an additional resonator layer employed for the enhancement of the effect. Our results are important for the development of new high-precision multilayer ellipsometry methods and schemes, as well as in a broad range of sensing applications.

physics.optics↗

arXiv2013

Plasmonic finite-thickness metal-semiconductor-metal waveguide as ultra-compact modulator

We propose a plasmonic modulator with semiconductor gain material for optoelectronic integrated circuits. We analyze properties of a finite-thickness metal-semiconductor-metal (F-MSM) waveguide to be utilized as an ultra-compact and fast plasmonic modulator. The InP-based semiconductor core allows electrical control of signal propagation. By pumping the core we can vary the gain level and thus the transmittance of the whole system. The study of the device was made using both analytical approaches for planar two-dimensional case as well as numerical simulations for finite-width waveguides. We analyze the eigenmodes of the F-MSM waveguide, propagation constant, confinement factor, Purcell factor, absorption coefficient, and extinction ratio of the structure. We show that using thin metal layers instead of thick ones we can obtain higher extinction ratio of the device.

physics.optics↗

arXiv2012

Metamaterial Polarization Converter Analysis: Limits of Performance

In this paper we analyze the theoretical limits of a metamaterial converter that allows for linear-to- elliptical polarization transformation with any desired ellipticity and ellipse orientation. We employ the transmission line approach providing a needed level of the design generalization. Our analysis reveals that the maximal conversion efficiency for transmission through a single metamaterial layer is 50%, while the realistic re ection configuration can give the conversion efficiency up to 90%. We show that a double layer transmission converter and a single layer with a ground plane can have 100% polarization conversion efficiency. We tested our conclusions numerically reaching the designated limits of efficiency using a simple metamaterial design. Our general analysis provides useful guidelines for the metamaterial polarization converter design for virtually any frequency range of the electromagnetic waves.

physics.optics↗