arXiv subjects

Rafael M. Fernandes

Publications and source records attributed to Rafael M. Fernandes.

At least 145 records · Page 8Linked to original sources

arXiv2018

Visualizing the Nonlinear Coupling between Strain and Electronic Nematicity in the Iron Pnictides by Elasto-Scanning Tunneling Spectroscopy

Mechanical strain is a powerful technique for tuning electronic structure and interactions in quantum materials. In a system with tetragonal symmetry, a tunable uniaxial in-plane strain can be used to probe nematic correlations in the same way that a tunable magnetic field is used to probe magnetic correlations. Here, we present a new spectroscopic scanned probe technique that provides atomic-resolution insight into the effect of anisotropic strain on the electronic structure. We use this technique to study nematic fluctuations and nematic order across the phase diagram of a prototypical iron-based superconductor. By extracting quantitatively the electronic anisotropy as function of applied strain, we show that while true long range nematic order is established at the tetragonal to orthorhombic structural transition temperature, sizable nematic fluctuations persist to high temperatures and also to the overdoped end of the superconducting dome. Remarkably, we find that uniaxial strain in the pnictides significantly enhances the amplitude of the nematic fluctuations, indicating a strong nonlinear coupling between structure and electronic nematicity.

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arXiv2018

Correlations and electronic order in a two-orbital honeycomb lattice model for twisted bilayer graphene

The recent observation of superconductivity in proximity to an insulating phase in twisted bilayer graphene (TBG) at small `magic' twist angles has been linked to the existence of nearly-flat bands, which make TBG a fresh playground to investigate the interplay between correlations and superconductivity. The low-energy narrow bands were shown to be well-described by an effective tight-binding model on the honeycomb lattice (the dual of the triangular Moiré superlattice) with a local orbital degree of freedom. In this paper, we perform a strong-coupling analysis of the proposed $\left(p_{x},\,p_{y}\right)$ two-orbital extended Hubbard model on the honeycomb lattice. By decomposing the interacting terms in the particle-particle and particle-hole channels, we classify the different possible superconducting, magnetic, and charge instabilities of the system. In the pairing case, we pay particular attention to the two-component ($d$-wave) pairing channels, which admit vestigial phases with nematic or chiral orders, and study their phenomenology. Furthermore, we explore the strong-regime by obtaining a simplified spin-orbital exchange model which may describe a putative Mott-like insulating state at quarter-filling. Our mean-field solution reveals a rich intertwinement between ferro- and antiferro-magnetic orders with different types of nematic and magnetic orbital orders. Overall, our work provides a solid framework for further investigations of the phase diagram of the two-orbital extended Hubbard model in both strong- and weak-coupling regimes.

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arXiv2018

Superconductivity at an antiferromagnetic quantum critical point: the role of energy fluctuations

Motivated by recent experiments reporting superconductivity only at very low temperature in a class of heavy fermion compounds, we study the impact of energy fluctuations with small momentum transfer on the pairing instability near an antiferromagnetic quantum critical point. While these fluctuations, formed by composite spin fluctuations, were proposed to explain the thermodynamic and transport properties near the quantum critical point of compounds such as YbRh$_{2}$Si$_{2}$ and CeCu$_{6-x}$Au$_{x}$ at $x\approx0.1$, here they are found to strongly suppress $T_{c}$ of the $d$-wave pairing of the hot quasiparticles promoted by the spin fluctuations. Interestingly, if energy fluctuations are strong enough, they can induce triplet pairing involving the quasiparticles of the cold regions of the Fermi surface. Overall, the opposing effects of energy and spin fluctuations lead to a suppression of $T_{c}$.

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arXiv2018

Impact of disorder on the superconducting transition temperature near a Lifshitz transition

Multi-band superconductivity is realized in a plethora of systems, from high-temperature superconductors to very diluted superconductors. While several properties of multi-band superconductors can be understood as straightforward generalizations of their single-band counterparts, recent works have unveiled rather unusual behaviors unique to the former case. In this regard, a regime that has received significant attention is that near a Lifshitz transition, in which one of the bands crosses the Fermi level. In this work, we investigate how impurity scattering $τ^{-1}$ affects the superconducting transition temperature $T_{c}$ across a Lifshitz transition, in the regime where intra-band pairing is dominant and inter-band pairing is subleading. This is accomplished by deriving analytic asymptotic expressions for $T_{c}$ and $\partial T_{c}/\partialτ^{-1}$ in a two-dimensional two-band system. When the inter-band pairing interaction is repulsive, we find that, despite the incipient nature of the band crossing the Fermi level, inter-band impurity scattering is extremely effective in breaking Cooper pairs, making $\partial T_{c}/\partialτ^{-1}$ quickly approach the limiting Abrikosov-Gor'kov value of the high-density regime. In contrast, when the inter-band pairing interaction is attractive, pair-breaking is much less efficient, affecting $T_{c}$ only mildly at the vicinity of the Lifshitz transition. The consequence of this general result is that the behavior of $T_{c}$ across a Lifshitz transition can be qualitatively changed in the presence of strong enough disorder: instead of displaying a sharp increase across the Lifshitz transition, as in the clean case, $T_{c}$ can actually display a maximum and be suppressed at the Lifshitz transition. These results shed new light on the non-trivial role of impurity scattering in multi-band superconductors.

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arXiv2018

Unconventional multi-band superconductivity in bulk SrTiO$_{3}$ and LaAlO$_{3}$/SrTiO$_{3}$ interfaces

Although discovered many decades ago, superconductivity in doped SrTiO$_{3}$ remains a topic of intense research. Recent experiments revealed that, upon increasing the carrier concentration, multiple bands cross the Fermi level, signaling the onset of Lifshitz transitions. Interestingly, $T_{c}$ was observed to be suppressed across the Lifshitz transition of oxygen-deficient SrTiO$_{3}$; a similar behavior was also observed in gated LaAlO$_{3}$/SrTiO$_{3}$ interfaces. Such a behavior is difficult to explain in the clean theory of two-band superconductivity, as the additional electronic states provided by the second band should enhance $T_{c}$. Here, we show that this unexpected behavior can be explained by the strong pair-breaking effect promoted by disorder, which takes place if the inter-band pairing interaction is subleading and repulsive. A consequence of this scenario is that, upon moving away from the Lifshitz transition, the two-band superconducting state changes from opposite-sign gaps to same-sign gaps.

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arXiv2018

Magnetic phase diagram of the iron pnictides in the presence of spin-orbit coupling: Frustration between $C_2$ and $C_4$ magnetic phases

We investigate the impact of spin anisotropic interactions, promoted by spin-orbit coupling, on the magnetic phase diagram of the iron-based superconductors. Three distinct magnetic phases with Bragg peaks at $(π,0)$ and $(0,π)$ are possible in these systems: one $C_2$ (i.e. orthorhombic) symmetric stripe magnetic phase and two $C_4$ (i.e. tetragonal) symmetric magnetic phases. While the spin anisotropic interactions allow the magnetic moments to point in any direction in the $C_2$ phase, they restrict the possible moment orientations in the $C_4$ phases. As a result, an interesting scenario arises in which the spin anisotropic interactions favor a $C_2$ phase, but the other spin isotropic interactions favor a $C_4$ phase. We study this frustration via both mean-field and renormalization-group approaches. We find that, to lift this frustration, a rich magnetic landscape emerges well below the magnetic transition temperature, with novel $C_2$, $C_4$, and mixed $C_2$-$C_4$ phases. Near the putative magnetic quantum critical point, spin anisotropies promote a stable Gaussian fixed point in the renormalization-group flow, which is absent in the spin isotropic case, and is associated with a near-degeneracy between $C_2$ and $C_4$ phases. We argue that this frustration is the reason why most $C_4$ phases in the iron pnictides only appear inside the $C_2$ phase, and discuss additional manifestations of this frustration in the phase diagrams of these materials.

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arXiv2018

Emergent magnetic degeneracy in iron pnictides due to the interplay between spin-orbit coupling and quantum fluctuations

Recent experiments in iron pnictide superconductors reveal that, as the putative magnetic quantum critical point is approached, different types of magnetic order coexist over a narrow region of the phase diagram. Although these magnetic configurations share the same wave-vectors, they break distinct symmetries of the lattice. Importantly, the highest superconducting transition temperature takes place close to this proliferation of near-degenerate magnetic states. In this paper, we employ a renormalization group calculation to show that such a behavior naturally arises due to the effects of spin-orbit coupling on the quantum magnetic fluctuations. Formally, the enhanced magnetic degeneracy near the quantum critical point is manifested as a stable Gaussian fixed point with a large basin of attraction. Implications of our findings to the superconductivity of the iron pnictides are also discussed.

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arXiv2018

Superconductivity in FeSe: the role of nematic order

Bulk FeSe is a special iron-based material in which superconductivity emerges inside a well-developed nematic phase. We present a microscopic model for this nematic superconducting state, which takes into account the mixing between $s-$wave and $d-$wave pairing channels and the changes in the orbital spectral weight promoted by the sign-changing nematic order parameter. We show that nematicity gives rise to a $\cos2θ$ variation of the pairing gap on the hole pocket that agrees with ARPES and STM data for experimentally-extracted Fermi surface parameters. We further argue that, in BCS theory, $d_{xz}$ and $d_{yz}$ orbitals give nearly equal contributions to the pairing glue, i.e. nematic order alone accounts for the gap anisotropy, but has little effect on $T_{c}$. This result questions the validity of the concept of orbital-selective pairing. Self-energy corrections, however, make $d_{xz}$ orbital more incoherent and reduce its contribution to pairing.

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arXiv2018

Time-reversal symmetry-breaking nematic superconductivity in FeSe

FeSe is a unique member of the family of iron-based superconductors, not only because of the high values of $T_{c}$ in FeSe monolayer, but also because in bulk FeSe superconductivity emerges inside a nematic phase without competing with long-range magnetic order. Near $T_{c}$, superconducting order necessarily has $s+d$ symmetry, because nematic order couples linearly the $s$-wave and $d$-wave harmonics of the superconducting order parameter. Here we argue that the near-degeneracy between $s$-wave and $d$-wave pairing instabilities in FeSe, combined with the sign-change of the nematic order parameter between hole and electron pockets, allows the superconducting order to break time-reversal symmetry at a temperature $T^{*}<T_{c}$. The transition from an $s+d$ state to an $s+\mathrm{e}^{iα}d$ state should give rise to a peak in the specific heat and to the emergence of a soft collective mode that can be potentially detected by Raman spectroscopy.

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arXiv2018

Impact of damping on superconducting gap oscillations induced by intense Terahertz pulses

We investigate the interplay between gap oscillations and damping in the dynamics of superconductors taken out of equilibrium by strong optical pulses with sub-gap Terahertz frequencies. A semi-phenomenological formalism is developed to include the damping within the electronic subsystem that arises from effects beyond BCS, such as interactions between Bogoliubov quasiparticles and decay of the Higgs mode. Such processes are conveniently expressed as $T_{1}$ and $T_{2}$ times in the standard pseudospin language for superconductors. Comparing with data on NbN that we report here, we argue that the superconducting dynamics in the picosecond time scale, after the pump is turned off, is governed by the $T_{2}$ process.

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arXiv2018

Orbital loop currents in iron-based superconductors

We show that the antiferromagnetic state commonly observed in the phase diagrams of the iron-based superconductors necessarily triggers loop currents characterized by charge transfer between different Fe $ 3d $ orbitals. This effect is rooted on the glide-plane symmetry of these materials and on the existence of an atomic spin-orbit coupling that couples states at the $X$ and $Y$ points of the 1-Fe Brillouin zone. In the particular case in which the magnetic moments are aligned parallel to the magnetic ordering vector direction which is the moment configuration most commonly found in the iron-based superconductors these loop currents involve the $d_{xy}$ orbital and either the $d_{yz}$ orbital (if the moments point along the $y$ axis) or the $d_{xz}$ orbitals (if the moments point along the $x$ axis). We show that the two main manifestations of the orbital loop currents are the emergence of magnetic moments in the pnictide/chalcogen site and an orbital-selective band splitting in the magnetically ordered state, both of which could be detected experimentally. Our results highlight the unique intertwining between orbital and spin degrees of freedom in the iron-based superconductors, and reveal the emergence of an unusual correlated phase that may impact the normal state and superconducting properties of these materials.

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arXiv2018

Magnetic tricritical point and nematicity in FeSe under pressure

Magnetism induced by external pressure ($p$) was studied in a FeSe crystal sample by means of muon-spin rotation. The magnetic transition changes from second-order to first-order for pressures exceeding the critical value $p_{\rm c}\simeq2.4-2.5$ GPa. The magnetic ordering temperature ($T_{\rm N}$) and the value of the magnetic moment per Fe site ($m_{\rm Fe}$) increase continuously with increasing pressure, reaching $T_{\rm N}\simeq50$~K and $m_{\rm Fe}\simeq0.25$ $μ_{\rm B}$ at $p\simeq2.6$ GPa, respectively. No pronounced features at both $T_{\rm N}(p)$ and $m_{\rm Fe}(p)$ are detected at $p\simeq p_{\rm c}$, thus suggesting that the stripe-type magnetic order in FeSe remains unchanged above and below the critical pressure $p_{\rm c}$. A phenomenological model for the $(p,T)$ phase diagram of FeSe reveals that these observations are consistent with a scenario where the nematic transitions of FeSe at low and high pressures are driven by different mechanisms.

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arXiv2018

Intertwined vestigial order in quantum materials: nematicity and beyond

A hallmark of the phase diagrams of quantum materials is the existence of multiple electronic ordered states, which, in many cases, are not independent competing phases, but instead display a complex intertwinement. In this review, we focus on a particular realization of intertwined orders: a primary phase characterized by a multi-component order parameter and a fluctuation-driven vestigial phase characterized by a composite order parameter. This concept has been widely employed to elucidate nematicity in iron-based and cuprate superconductors. Here we present a group-theoretical framework that extends this notion to a variety of phases, providing a classification of vestigial orders of unconventional superconductors and density-waves. Electronic states with scalar and vector chiral order, spin-nematic order, Ising-nematic order, time-reversal symmetry-breaking order, and algebraic vestigial order emerge from one underlying principle. The formalism provides a framework to understand the complexity of quantum materials based on symmetry, largely without resorting to microscopic models.

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arXiv2018

Disentangling superconducting and magnetic orders in NaFe_1-xNi_xAs using muon spin rotation

Muon spin rotation and relaxation studies have been performed on a "111" family of iron-based superconductors NaFe_1-xNi_xAs. Static magnetic order was characterized by obtaining the temperature and doping dependences of the local ordered magnetic moment size and the volume fraction of the magnetically ordered regions. For x = 0 and 0.4 %, a transition to a nearly-homogeneous long range magnetically ordered state is observed, while for higher x than 0.4 % magnetic order becomes more disordered and is completely suppressed for x = 1.5 %. The magnetic volume fraction continuously decreases with increasing x. The combination of magnetic and superconducting volumes implies that a spatially-overlapping coexistence of magnetism and superconductivity spans a large region of the T-x phase diagram for NaFe_1-xNi_xAs . A strong reduction of both the ordered moment size and the volume fraction is observed below the superconducting T_C for x = 0.6, 1.0, and 1.3 %, in contrast to other iron pnictides in which one of these two parameters exhibits a reduction below TC, but not both. The suppression of magnetic order is further enhanced with increased Ni doping, leading to a reentrant non-magnetic state below T_C for x = 1.3 %. The reentrant behavior indicates an interplay between antiferromagnetism and superconductivity involving competition for the same electrons. These observations are consistent with the sign-changing s-wave superconducting state, which is expected to appear on the verge of microscopic coexistence and phase separation with magnetism. We also present a universal linear relationship between the local ordered moment size and the antiferromagnetic ordering temperature TN across a variety of iron-based superconductors. We argue that this linear relationship is consistent with an itinerant-electron approach, in which Fermi surface nesting drives antiferromagnetic ordering.

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arXiv2018

Smeared nematic quantum phase transitions due to rare-region effects in inhomogeneous systems

The concept of a vestigial nematic order emerging from a "mother" spin or charge density-wave state has been applied to describe the phase diagrams of several systems, including unconventional superconductors. In a perfectly clean system, the two orders appear simultaneously via a first-order quantum phase transition, implying the absence of quantum criticality. Here, we investigate how this behavior is affected by impurity-free droplets that are naturally present in inhomogeneous systems. Due to their quantum dynamics, finite-size droplets sustain long-range nematic order but not long-range density-wave order. Interestingly, rare droplets with moderately large sizes undergo a second-order nematic transition even before the first-order quantum transition of the clean system. This gives rise to an extended regime of inhomogeneous nematic order, which is followed by a density-wave quantum Griffiths phase. As a result, a smeared quantum nematic transition, separated from the density-wave quantum transition, emerges in moderately disordered systems.

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arXiv2017

Controlling competing orders via non-equilibrium acoustic phonons: emergence of anisotropic electronic temperature

Ultrafast perturbations offer a unique tool to manipulate correlated systems due to their ability to promote transient behaviors with no equilibrium counterpart. A widely employed strategy is the excitation of coherent optical phonons, as they can cause significant changes in the electronic structure and interactions on short time scales. Here, we explore a promising alternative route: the non-equilibrium excitation of acoustic phonons. We demonstrate that it leads to the remarkable phenomenon of a momentum-dependent temperature, by which electronic states at different regions of the Fermi surface are subject to distinct local temperatures. Such an anisotropic electronic temperature can have a profound effect on the delicate balance between competing ordered states in unconventional superconductors, opening a novel avenue to control correlated phases.

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arXiv2017

Is charge order induced near an antiferromagnetic quantum critical point?

We investigate the interplay between charge order and superconductivity near an antiferromagnetic quantum critical point using sign-problem-free Quantum Monte Carlo simulations. We establish that, when the electronic dispersion is particle-hole symmetric, the system has an emergent SU(2) symmetry that implies a degeneracy between $d$-wave superconductivity and charge order with $d$-wave form factor. Deviations from particle-hole symmetry, however, rapidly lift this degeneracy, despite the fact that the SU(2) symmetry is preserved at low energies. As a result, we find a strong suppression of charge order caused by the competing, leading superconducting instability. Across the antiferromagnetic phase transition, we also observe a shift in the charge order wave-vector from diagonal to axial. We discuss the implications of our results to the universal phase diagram of antiferromagnetic quantum-critical metals and to the elucidation of the charge order experimentally observed in the cuprates.

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arXiv2017

Dynamic Elastoresistivity Evidence for Slow Nematic Fluctuations in BaFe$_2$As$_2$

An instrumentation problem with the signal acquisition at high frequencies was discovered and we no longer believe that the experimental data presented in the manuscript, showing a frequency enhancement of the elastoresistivity, are correct. After correcting the problem, the elastoresistivity data is frequency independent in the range investigated. Therefore, the authors have withdrawn this submission. We would like to thank Alex Hristov, Johanna Palmstrom, Josh Straquadine and Ian Fisher (Stanford) for the kind discussions and assistance we received which helped us identify these problems.

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