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Rafael Sánchez

Publications and source records attributed to Rafael Sánchez.

At least 55 records · Page 3Linked to original sources

Dynamical Coulomb blockade of thermal transport

The role of energy exchange between a quantum system and its environment is investigated from the perspective of the Onsager conductance matrix. We consider the thermoelectric linear transport of an interacting quantum dot coupled to two terminals under the influence of an electrical potential and a thermal bias. We implement in our model the effect of coupling to electromagnetic environmental modes created by nearby electrons within the P(E)-theory of dynamical Coulomb blockade. Our findings relate the lack of some symmetries among the Onsager matrix coefficients with an enhancement of the efficiency at maximum power and the occurrence of the heat rectification phenomenon.

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Thermoelectrics with Coulomb coupled quantum dots

In this article we review the thermoelectric properties of three terminal devices with Coulomb coupled quantum dots (QDs) as observed in recent experiments [1,2]. The system we consider consists of two Coulomb-blockade QDs one of which can exchange electrons with only a single reservoir (heat reservoir) while the other dot is tunnel coupled to two reservoirs at a lower temperature (conductor). The heat reservoir and the conductor interact only via the Coulomb-coupling of the quantum dots. It has been found that two regimes have to be considered. In the first one heat flow between the two systems is small. In this regime thermally driven occupation fluctuations of the hot QD modify the transport properties of the conductor system. This leads to an effect called thermal gating. Experiment have shown how this can be used to control charge flow in the conductor by means of temperature in a remote reservoir. We further substantiate the observations with model calculations and implications for the realization of an all-thermal transistor are discussed. In the second regime, heat flow between the two systems is relevant. Here the system works as a nano scale heat engine, as proposed recently [3]. We review the conceptual idea, its experimental realization and the novel features arising in this new kind of thermoelectric device such as decoupling of heat and charge flow.

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Three-Terminal Energy Harvester with Coupled Quantum Dots

Rectification of thermal fluctuations in mesoscopic conductors is the key idea of today's attempts to build nanoscale thermoelectric energy harvesters in order to convert heat into a useful electric power. So far, most concepts make use of the Seebeck effect in a two-terminal geometry where heat and charge are both carried by the same particles. Here, we experimentally demonstrate the working principle of a new kind of energy harvester, proposed recently using two capacitively coupled quantum dots. We show that due to its novel three-terminal design which spatially separates the heat reservoir from the conductor circuit, the directions of charge and heat flow become decoupled in our device. This enables us to manipulate the direction of the generated charge current by means of external gate voltages while leaving the direction of heat flow unaffected. Our results pave the way for a new generation of multi-terminal, highly efficient nanoscale heat engines.

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Coupled Landau-Zener-Stuckelberg Quantum Dot Interferometers

We investigate the interplay between long-range and direct photon-assisted transport in a triple quantum dot chain where local ac voltages are applied to the outer dots. We propose the phase difference between the two ac voltages as an external parameter, which can be easily tuned to manipulate the current characteristics. For gate voltages in phase opposition we find quantum destructive interferences analogous to the interferences in closed-loop undriven triple dots. As the voltages oscillate in phase, interferences between multiple paths give rise to dark states. Those totally cancel the current, and could be experimentally resolved.

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Thermoelectricity without absorbing energy from the heat sources

We analyze the power output of a quantum dot machine coupled to two electronic reservoirs via thermoelectric contacts, and to two thermal reservoirs - one hot and one cold. This machine is a nanoscale analogue of a conventional thermocouple heat-engine, in which the active region being heated is unavoidably also exchanging heat with its cold environment. Heat exchange between the dot and the thermal reservoirs is treated as a capacitive coupling to electronic fluctuations in localized levels, modeled as two additional quantum dots. The resulting multiple-dot setup is described using a master equation approach. We observe an "exotic" power generation, which remains finite even when the heat absorbed from the thermal reservoirs is zero (in other words the heat coming from the hot reservoir all escapes into the cold environment). This effect can be understood in terms of a non-local effect in which the heat flow from heat source to the cold environment generates power via a mechanism which we refer to as Coulomb heat drag. It relies on the fact that there is no relaxation in the quantum dot system, so electrons within it have a non-thermal energy distribution. More poetically, one can say that we find a spatial separation of the first-law of thermodynamics (heat to work conversion) from the second-law of thermodynamics (generation of entropy). We present circumstances in which this non-thermal system can generate more power than any conventional macroscopic thermocouple (with local thermalization), even when the latter works with Carnot efficiency.

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Effect of incoherent scattering on three-terminal quantum Hall thermoelectrics

A three-terminal conductor presents peculiar thermoelectric and thermal properties in the quantum Hall regime: it can behave as a symmetric rectifier and as an ideal thermal diode. These properties rely on the coherent propagation along chiral edge channels. We investigate the effect of breaking the coherent propagation by the introduction of a probe terminal. It is shown that chiral effects not only survive the presence of incoherence but they can even improve the thermoelectric performance in the totally incoherent regime.

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Heat diode and engine based on quantum Hall edge states

We investigate charge and energy transport in a three-terminal quantum Hall conductor. The peculiar properties of chiral propagation along the edges of the sample have important consequences on the response to thermal biases. Based on the separation of charge and heat flows, thermoelectric conversion and heat rectification can be manipulated by tuning the scattering at gate-modulated constrictions. Chiral motion in a magnetic field allows for a different behaviour of left- and right-moving carriers giving rise to thermal rectification by redirecting the heat flows. We propose our system both as an efficient heat-to-work converter and as a heat diode.

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Chiral thermoelectrics with quantum Hall edge states

The thermoelectric properties of a three-terminal quantum Hall conductor are investigated. We identify a contribution to the thermoelectric response that relies on the chirality of the carrier motion rather than on spatial asymmetries. The Onsager matrix becomes maximally asymmetric with configurations where either the Seebeck or the Peltier coefficients are zero while the other one remains finite. Reversing the magnetic field direction exchanges these effects, which originate from the chiral nature of the quantum Hall edge states. The possibility to generate spin-polarized currents in quantum spin Hall samples is discussed.

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Thermoelectric energy harvesting with quantum dots

We review recent theoretical work on thermoelectric energy harvesting in multi-terminal quantum-dot setups. We first discuss several examples of nanoscale heat engines based on Coulomb-coupled conductors. In particular, we focus on quantum dots in the Coulomb-blockade regime, chaotic cavities and resonant tunneling through quantum dots and wells. We then turn towards quantum-dot heat engines that are driven by bosonic degrees of freedom such as phonons, magnons and microwave photons. These systems provide interesting connections to spin caloritronics and circuit quantum electrodynamics.

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Photon assisted long-range tunneling

We analyze long-range transport through an ac driven triple quantum dot with one single electron. An effective model is proposed for the analysis of photoassisted cotunnel in order to account for the virtual processes which dominate the long-range transport, which takes place at n-photon resonances between the edge quantum dots. The AC field renormalizes the inter dot hopping, modifying the levels hybridization. It results in a non trivial behavior of the current with the frequency and intensity of the external ac field.

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Quantum Nernst engines

We theoretically propose Nernst engines based on quantum Hall edge states. We identify a setup that exhibits an extreme asymmetry between the off-diagonal Onsager coefficients for heat and charge transport. In terms of thermodynamic efficiency, this engine outperforms a recently proposed classical Nernst engine. A second setup using an anti-dot is found to be more efficient as energy filtering becomes less strong.

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Superexchange blockade in triple quantum dots

We propose the interaction of two electrons in a triple quantum dot as a minimal system to control long range superexchange transitions. These are probed by transport spectroscopy. Narrow resonances appear indicating the transfer of charge from one side of the sample to the other with the central one being occupied only virtually. We predict that two different intermediate states establish the two arms of a one dimensional interferometer. Configurations of destructive interference of the two superexchage trajectories totally block the current through the system. We emphasize the role of spin correlations giving rise to lifetime-enhanced resonances.

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Detection of single-electron heat transfer statistics

We consider a quantum dot system whose charge fluctuations are monitored by a quantum point contact allowing for the detection of both charge and transferred heat statistics. Our system consists of two nearby conductors that exchange energy via Coulomb interaction. In interfaces consisting of capacitively coupled quantum dots, energy transfer is discrete and can be measured by charge counting statistics. We investigate gate dependent deviations away from a charge fluctuation theorem in the presence of local temperature gradients (hot spots). Non universal relations are found for state dependent charge counting. A fluctuation theorem holds for coupled dot configurations with heat exchange and no net particle flow.

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Correlations of heat and charge currents in quantum-dot thermoelectric engines

We analyze the noise properties of both electric charge and heat currents as well as their correlations in a quantum-dot based thermoelectric engine. The engine is a three-terminal conductor with crossed heat and charge flows where heat fluctuations can be monitored by a charge detector. We investigate the mutual influence of charge and heat dynamics and how it is manifested in the current and noise properties. In the presence of energy-dependent tunneling, operating conditions are discussed where a charge current can be generated by heat conversion. In addition, heat can be pumped into the hot source by driving a charge current in the coupled conductor. An optimal configuration is found for structures in which the energy dependence of tunneling maximizes asymmetric transmission with maximal charge-heat cross-correlations. Remarkably, at a voltage that stalls the heat engine we find that in the optimal case the non-equilibrium state is maintained by fluctuations in the heat and charge current only.

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Powerful energy harvester based on resonant-tunneling quantum wells

We analyze a heat engine based on a hot cavity connected via quantum wells to electronic reservoirs. We discuss the output power as well as the efficiency both in the linear and nonlinear regime. We find that the device delivers a large power of about 0.18 W/cm^2 for a temperature difference of 1 K nearly doubling the power than can be extracted from a similar heat engine based on quantum dots. At the same time, the heat engine also has a good efficiency although reduced from the quantum dot case. Due to the large level spacings that can be achieved in quantum wells, our proposal opens the route towards room-temperature applications of nanoscale heat engines.

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Powerful and efficient energy harvester with resonant-tunneling quantum dots

We propose a nanoscale heat engine that utilizes the physics of resonant tunneling in quantum dots in order to transfer electrons only at specific energies. The nanoengine converts heat into electrical current in a multiterminal geometry which permits one to separate current and heat flows. By putting two quantum dots in series with a hot cavity, electrons that enter one lead are forced to gain a prescribed energy in order to exit the opposite lead, transporting a single electron charge. This condition yields an ideally efficient heat engine. The energy gain is a property of the composite system rather than of the individual dots. It is therefore tunable to optimize the power while keeping a much larger level spacing for the individual quantum dots. Despite the simplicity of the physical model, the optimized rectified current and power is larger than any other candidate nano-engine. The ability to scale the power by putting many such engines into a two-dimensional layered structure gives a paradigmatic system for harvesting thermal energy at the nanoscale. We demonstrate that the high power and efficiency of the layered structure persists even if the quantum dots exhibit some randomness.

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Dark Bell states in tunnel-coupled spin qubits

We investigate the dynamical purification of maximally entangled electron states by transport through coupled quantum dots. Under resonant ac driving and coherent tunneling, even-parity Bell states perform Rabi oscillations that decouple from the environment, leading to a dark state. The two electrons remain spatially separated, one in each quantum dot. We propose configurations where this effect will prove as antiresonances in transport spectroscopy experiments.

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Rectification of thermal fluctuations in a chaotic cavity heat engine

We investigate the rectification of thermal fluctuations in a mesoscopic on-chip heat engine. The engine consists of a hot chaotic cavity capacitively coupled to a cold cavity which rectifies the excess noise and generates a directed current. The fluctuation-induced directed current depends on the energy asymmetry of the transmissions of the contacts of the cold cavity to the leads and is proportional to the temperature difference. We discuss the maximal power output of the heat engine and its efficiency.

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