arXiv subjects

Rahul Gogna

Publications and source records attributed to Rahul Gogna.

5 recordsLinked to original sources

arXiv2019

Moiré lattice-induced formation and tuning of hybrid dipolar excitons in twisted WS$_2$/MoSe$_2$ heterobilayers

Moiré superlattices formed in van der Waals bilayers have enabled the creation and manipulation of new quantum states, as is exemplified by the discovery of superconducting and correlated insulating states in twisted bilayer graphene near the magic angle. Twisted bilayer semiconductors may lead to tunable exciton lattices and topological states, yet signatures of moiré excitons have been reported only in closely angularly-aligned bilayers. Here we report tuning of moiré lattice in WS$_{2}$ /MoSe$_{2}$ bilayers over a wide range of twist angles, leading to the continuous tuning of moiré lattice induced interlayer excitons and their hybridization with optically bright intralayer excitons. A pronounced revival of the hybrid excitons takes place near commensurate twist angles, 21.8°and 38.2°, due to interlayer tunneling between states connected by a moiré reciprocal lattice vector. From the angle dependence, we obtain the effective mass of the interlayer excitons and the electron inter-layer tunneling strength. These findings pave the way for understanding and engineering rich moiré-lattice induced phenomena in angle-twisted semiconductor van dar Waals heterostructures.

cond-mat.mes-hall↗

arXiv2019

Highly Valley-Polarized Singlet and Triplet Interlayer Excitons in van der Waals Heterostructure

Two-dimensional semiconductors feature valleytronics phenomena due to locking of the spin and momentum valley of the electrons. However, the valley polarization is intrinsically limited in monolayer crystals by the fast intervalley electron-hole exchange. Hetero-bilayer crystals have been shown to have a longer exciton lifetime and valley depolarization time. But the reported valley polarization was low; the valley selection rules and mechanisms of valley depolarization remains controversial. Here, we report singlet and brightened triplet interlayer excitons both with over 80% valley polarizations, cross- and co-polarized with the pump laser, respectively. This is achieved in WSe2/MoSe2 hetero-bilayers with precise momentum valley alignment and narrow emission linewidth. The high valley polarizations allow us to identify the band minima in a hetero-structure and con_rm unambiguously the direct band-gap exciton transition, ultrafast charge separation, strongly suppressed valley depolarization. Our results pave the way for using semiconductor heterobilayers to control valley selection rules for valleytronic applications.

cond-mat.mes-hall↗

arXiv2019

Interlayer Exciton Laser with Extended Spatial Coherence in an Atomically-Thin Heterostructure

Two-dimensional semiconductors have emerged as a new class of materials for nanophotonics for their strong exciton-photon interaction and flexibility for engineering and integration. Taking advantage of these properties, we engineer an efficient lasing medium based on dipolar interlayer excitons, in rotationally aligned atomically thin heterostructures. Lasing is measured from a transition metal dichalcogenide hetero-bilayer integrated in a silicon nitride grating resonator. A sharp increase in the spatial coherence of the emission was observed across the lasing threshold. The work establishes interlayer excitons in two-dimensional heterostructures as a silicon-compatible coherent medium. With electrically tunable light-matter interaction strength and long-range dipolar interactions, these interlayer excitons promise both applications to low-power, ultrafast laser and modulators and rich many-body quantum phenomena.

cond-mat.mes-hall↗

arXiv2017

Photonic-Crystal Exciton-Polaritons in Monolayer Semiconductors

Semiconductor microcavity polaritons, formed via strong exciton-photon coupling, provide a quantum many-body system on a chip, featuring rich physics phenomena for better photonic technology. However, conventional polariton cavities are bulky, difficult to integrate, and inflexible for mode control, especially for room temperature materials. Here we demonstrate sub-wavelength thick one-dimensional photonic crystals (PCs) as a designable, compact and practical platform for strong coupling with atomically thin van der Waals Crystals (vdWCs). Polariton dispersions and mode anti-crossings are measured up to room temperature. Non-radiative decay to dark excitons was suppressed due to polariton enhancement of the radiative decay. Unusual features, including highly anisotropic dispersions and adjustable Fano resonances in reflectance, may facilitate high temperature polariton condensation in variable dimensions. Combining slab PCs and vdWCs in the strong coupling regime allows unprecedented engineering flexibility for exploring novel polariton phenomena and device concepts.

cond-mat.mes-hall↗

arXiv2017

What is the best planar cavity for maximizing coherent exciton-photon coupling

We compare alternative planar cavity structures for strong exciton$-$photon coupling, where the conventional distributed Bragg reflector (DBR) and three unconventional types of cavity mirrors$-$ air/GaAs DBR, Tamm $-$ plasmon mirror and sub$-$wavelength grating mirror. We design and optimize the planar cavities built with each type of mirror at one side or both sides for maximum vacuum field strength. We discuss the trade$-$off between performance and fabrication difficulty for each cavity structure. We show that cavities with sub$-$wavelength grating mirrors allow simultaneously strongest field and high cavity quality. The optimization principles and techniques developed in this work will guide the cavity design for research and applications of matter$-$light coupled semiconductors, especially new material systems that require greater flexibility in the choice of cavity materials and cavity fabrication procedures.

cond-mat.mes-hall↗