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Raimund Ricken

Publications and source records attributed to Raimund Ricken.

At least 19 recordsLinked to original sources

Photorefraction Management in Lithium Niobate Waveguides: High-Temperature vs. Cryogenic Solutions

Lithium niobate sees widespread use in nonlinear and quantum optical devices, such as for sum- and difference-frequency generation or spontaneous parametric down-conversion. In lithium niobate waveguides, nonlinear optical processes are often limited by the so-called photorefractive effect, which limits the maximum input or output powers and impacts the nonlinear spectral response. Therefore, strategies for the management of photorefractive damage are a key consideration in device design. Usually, the photorefractive damage threshold, i.e. the maximal permissible operating power, can be increased by high temperature operation of devices. This approach, however, is not applicable in cryogenic environments, which may be required for specialized applications. To better understand the impact of photorefraction in nonlinear optical applications, we study the impact of photorefraction on the phase-matching spectra of two nonlinear-optical sum-frequency generation experiments at 1) high temperatures and 2) cryogenic temperatures. Furthermore, we present an approach to reduce the impact of photorefraction which is compatible with cryogenic operation. This comprises an auxiliary light source, propagating in the same waveguide, which is used to restore phase-matching spectra impacted by photorefraction, as well as reduce pyroelectric effects. Our work provides an alternative route to photorefraction management applicable to cryogenic environments, as well as in situations with tight energy budgets like space applications.

physics.optics

Integrated, bright, broadband parametric down-conversion source for quantum metrology and spectroscopy

Broadband quantum light is a vital resource for quantum metrology and spectroscopy applications such as quantum optical coherence tomography or entangled two photon absorption. For entangled two photon absorption in particular, very high photon flux combined with high time-frequency entanglement is crucial for observing a signal. So far these conditions could be met by using high power lasers driving degenerate, type 0 bulk-crystal spontaneous parametric down conversion (SPDC) sources. This naturally limits the available wavelength ranges and precludes deterministic splitting of the generated output photons. In this work we demonstrate an integrated two-colour SPDC source utilising a group-velocity matched lithium niobate waveguide, reaching both exceptional brightness $1.52\cdot10^6\frac{\mathrm{pairs}}{\mathrm{s\,mW\,GHz}}$ and large bandwidth ($7.8\,$THz FWHM) while pumped with a few mW of continuous wave (CW) laser light. By converting a narrow band pump to broadband pulses the created photon pairs show correlation times of $Δτ\approx 120\,\text{fs}$ while maintaining the narrow bandwidth $Δω_p \ll 1\,\text{MHz}$ of the CW pump light, yielding strong time-frequency entanglement. Furthermore our process can be adapted to a wide range of central wavelengths.

quant-ph

Realization of a multi-output quantum pulse gate for decoding high-dimensional temporal modes of single-photon states

Temporal modes (TMs) of photons provide an appealing high-dimensional encoding basis for quantum information. While techniques to generate TM states have been established, high-dimensional decoding of single-photon TMs remains an open challenge. In this work, we experimentally demonstrate demultiplexing of five-dimensional TMs of single photons with an average fidelity of 0.96 $\pm$ 0.01, characterized via measurement tomography. This is achieved using a newly developed device, the multi-output quantum pulse gate (mQPG). We demonstrate a proof-of-principle complete decoder based on the mQPG that operates on any basis from a set of 6 five-dimensional MUBs and is therefore suitable as a receiver for high-dimensional quantum key distribution. Furthermore, we confirm the high-quality operation of the mQPG by performing resource-efficient state tomography with an average fidelity of 0.98 $\pm$ 0.02.

quant-ph

Cryogenic electro-optic modulation in titanium in-diffused lithium niobate waveguides

Lithium niobate is a promising platform for integrated quantum optics. In this platform we aim to efficiently manipulate and detect quantum states by combining superconducting single photon detectors and modulators. The cryogenic operation of a superconducting single photon detector dictates the optimisation of the electro-optic modulators under the same operating conditions. To that end, we characterise a phase modulator, directional coupler, and polarisation converter at both ambient and cryogenic temperatures. The operation voltage $V_{π/2}$ of these modulators increases due to the decrease of the electro-optic effect by 74% for the phase modulator, 84% for the directional coupler and 35% for the polarisation converter below 8.5$\,\mathrm{K}$. The phase modulator preserves its broadband nature and modulates light in the characterised wavelength range. The unbiased bar state of the directional coupler changed by a wavelength shift of 85$\,\mathrm{nm}$ while cooling the device down to 5$\,\mathrm{K}$. The polarisation converter uses periodic poling to phasematch the two orthogonal polarisations. The phasematched wavelength of the used poling changes by 112$\,\mathrm{nm}$ when cooling to 5$\,\mathrm{K}$

physics.optics

Cryogenic integrated spontaneous parametric down-conversion

Scalable quantum photonics relies on interfacing many optical components under mutually compatible operating conditions. To that end, we demonstrate that spontaneous parametric down-conversion (SPDC) in nonlinear waveguides, a standard technology for generating entangled photon pairs, squeezed states, and heralded single photons, is fully compatible with cryogenic operating conditions required for superconducting detectors. This is necessary for the proliferation of integrated quantum photonics in integration platforms exploiting quasi-phase-matched second-order nonlinear interactions. We investigate how cryogenic operation at 4 K affects the SPDC process by comparing the heralding efficiency, second-order correlation function and spectral properties with operation at room temperature.

quant-ph

Integrated superconducting nanowire single-photon detectors on titanium in-diffused lithium niobate waveguides

We demonstrate the integration of amorphous tungsten silicide superconducting nanowire single-photon detectors on titanium in-diffused lithium niobate waveguides. We show proof-of-principle detection of evanescently-coupled photons of 1550nm wavelength using bidirectional waveguide coupling for two orthogonal polarization directions. We investigate the internal detection efficiency as well as detector absorption using coupling-independent characterization measurements. Furthermore, we describe strategies to improve the yield and efficiency of these devices.

quant-ph

Improved non-linear devices for quantum applications

In this paper, we review the state of the art of mode selective, integrated sum-frequency generation devices tailored for quantum optical technologies. We explore benchmarks to asses their performance and discuss the current limitations of these devices, outlining possible strategies to overcome them. Finally, we present the fabrication of a new, improved device and its characterization. We analyse the fabrication quality of this device and discuss the next steps towards improved non-linear devices for quantum applications.

quant-ph

Waveguide Resonator with Integrated Phase Modulator for Second Harmonic Generation

We report second harmonic generation from a titanium indiffused lithium niobate waveguide resonator device whose cavity length is locked to the fundamental pump laser using an on-chip phase modulator. The device remains locked for more than 5 minutes, producing more than 80\% of the initial second harmonic power. The stability of the system is seen to be limited by DC-drift, a known effect in many lithium niobate systems that include deposited electrodes. The presented device explores the suitability of waveguide resonators in this platform for use in larger integrated networks.

physics.optics

Cryogenic Electro-Optic Polarisation Conversion in Titanium in-diffused Lithium Niobate Waveguides

Many technologies in quantum photonics require cryogenic conditions to operate. However, the underlying platform behind active components such as switches, modulators and phase shifters must be compatible with these operating conditions. To address this, we demonstrate an electro-optic polarisation converter for 1550nm light at 0.8K in titanium in-diffused lithium niobate waveguides. To do so, we exploit the electro-optic properties of lithium niobate to convert between orthogonal polarisation modes with a fiber-to-fiber transmission >43%. We achieve a modulation depth of 23.6 +/-3.3dB and a conversion voltage-length product of 28.8 V cm. This enables the combination of cryogenic photonics and active components on a single integration platform.

physics.optics

Cryogenic second harmonic generation in periodically-poled lithium niobate waveguides

Prospective integrated quantum optical technologies will combine nonlinear optics and components requiring cryogenic operating temperatures. Despite the prevalence of integrated platforms exploiting $χ^{(2)}$-nonlinearities for quantum optics, for example used for quantum state generation and frequency conversion, their material properties at low temperatures are largely unstudied. Here, we demonstrate the first second harmonic generation in a fiber-coupled lithium niobate waveguide at temperatures down to 4.4K. We observe a reproducible shift in the phase-matched pump wavelength within the telecom band, in addition to transient discontinuities while temperature cycling. Our results establish lithium niobate as a versatile nonlinear photonic integration platform compatible with cryogenic quantum technologies.

physics.optics

Counter-propagating photon pair generation in a nonlinear waveguide

Counter-propagating parametric conversion processes in non-linear bulk crystals have been shown to feature unique properties for efficient narrowband frequency conversion. In quantum optics, the generation of photon pairs with a counter-propagating parametric down-conversion process (PDC) in a waveguide, where signal and idler photons propagate in opposite directions, offers unique material-independent engineering capabilities. However, realizing counter-propagating PDC necessitates quasi-phase-matching (QPM) with extremely short poling periods. Here, we report on the generation of counter-propagating single-photon pairs in a self-made periodically poled lithium niobate waveguide with a poling period on the same order of magnitude as the generated wavelength. The single photons of the biphoton state bridge GHz and THz bandwidths with a separable joint temporal-spectral behavior. Furthermore, they allow the direct observation of the temporal envelope of heralded single photons with state-of-the art photon counters.

quant-ph

Nonlinear integrated quantum electro-optic circuits

Future quantum computation and networks require scalable monolithic circuits, which incorporate various advanced functionalities on a single physical substrate. Although substantial progress for various applications has already been demonstrated on different platforms, the range of diversified manipulation of photonic states on demand on a single chip has remained limited, especially dynamic time management. Here, we demonstrate an electro-optic device, including photon pair generation, propagation, electro-optical path routing, as well as a voltage-controllable time delay of up to ~ 12 ps on a single Ti:LIbO3 waveguide chip. As an example, we demonstrate Hong-Ou-Mandel interference with a visibility of more than 93$\pm$ 1.8\%. Our chip not only enables the deliberate manipulation of photonic states by rotating the polarization but also provides precise time control. Our experiment reveals that we have full flexible control over single-qubit operations by harnessing the complete potential of fast on-chip electro-optic modulation.

quant-ph

Integrated transition edge sensors on lithium niobate waveguides

We show the proof-of-principle detection of light at 1550 nm coupled evanescently from a titanium in-diffused lithium niobate waveguide to a superconducting transition edge sensor. The coupling efficiency strongly depends on the polarization, the overlap between the evanescent field, and the detector structure. We experimentally demonstrate polarization sensitivity of this coupling as well as photon-number resolution of the integrated detector. The combination of transition edge sensors and lithium niobate waveguides can open the field for a variety of new quantum optics experiments.

physics.ins-det

Pulse shaping using dispersion-engineered difference frequency generation

The temporal-mode (TM) basis is a prime candidate to perform high-dimensional quantum encoding. Quantum frequency conversion has been employed as a tool to perform tomographic analysis and manipulation of ultrafast states of quantum light necessary to implement a TM-based encoding protocol. While demultiplexing of such states of light has been demonstrated in the Quantum Pulse Gate (QPG), a multiplexing device is needed to complete an experimental framework for TM encoding. In this work we demonstrate the reverse process of the QPG. A dispersion-engineered difference frequency generation in non-linear optical waveguides is employed to imprint the pulse shape of the pump pulse onto the output. This transformation is unitary and can be more efficient than classical pulse shaping methods. We experimentally study the process by shaping the first five orders of Hermite-Gauss modes of various bandwidths. Finally, we establish and model the limits of practical, reliable shaping operation.

quant-ph

Towards integrated superconducting detectors on lithium niobate waveguides

Superconducting detectors are now well-established tools for low-light optics, and in particular quantum optics, boasting high-efficiency, fast response and low noise. Similarly, lithium niobate is an important platform for integrated optics given its high second-order nonlinearity, used for high-speed electro-optic modulation and polarization conversion, as well as frequency conversion and sources of quantum light. Combining these technologies addresses the requirements for a single platform capable of generating, manipulating and measuring quantum light in many degrees of freedom, in a compact and potentially scalable manner. We will report on progress integrating tungsten transition-edge sensors (TESs) and amorphous tungsten silicide superconducting nanowire single-photon detectors (SNSPDs) on titanium in-diffused lithium niobate waveguides. The travelling-wave design couples the evanescent field from the waveguides into the superconducting absorber. We will report on simulations and measurements of the absorption, which we can characterize at room temperature prior to cooling down the devices. Independently, we show how the detectors respond to flood illumination, normally incident on the devices, demonstrating their functionality.

physics.ins-det

Streak-camera measurements of single photons at telecom wavelength

Up to this point streak-cameras have been a powerful tool for temporal characterization of ultrafast light pulses even at the single photon level. However, the low signal-to-noise ratio in the infrared range prevents measurement on weak light sources in the telecom regime. We present an approach to circumvent this problem. The method utilizes an up-conversion process in periodically poled waveguides in Lithium Niobate. We convert single photons from a parametric down-conversion source in order to reach the point of maximum detection efficiency of commercially available streak-cameras. We explore phase-matching configurations to investigate the up-conversion scheme in real-world applications.

quant-ph

High efficiency 'plug & play' source of heralded single photons

Reliable generation of single photons is of key importance for fundamental physical experiments and to demonstrate quantum technologies. Waveguide-based photon pair sources have shown great promise in this regard due to their large degree of spectral tunability, high generation rates and long photon coherence times. However, for such a source to have real world applications it needs to be efficiently integrated with fiber-optic networks. We answer this challenge by presenting an alignment-free source of photon pairs in the telecommunications band that maintains heralding efficiency > 50 % even after fiber pigtailing, photon separation, and pump suppression. The source combines this outstanding performance in heralding efficiency and brightness with a compact, stable, and easy-to-use 'plug & play' package: one simply connects a laser to the input and detectors to the output and the source is ready to use. This high performance can be achieved even outside the lab without the need for alignment which makes the source extremely useful for any experiment or demonstration needing heralded single photons.

quant-ph

Fast time-domain measurements on telecom single photons

Direct measurements on the temporal envelope of quantum light are a challenging task and not many examples are known since most classical pulse characterisation methods do not work on the single photon level. Knowledge of both spectrum and timing can however give insights on properties that cannot be determined by the spectrum alone. While temporal measurements on single photons on timescales of tens of picoseconds are possible with superconducting photon detectors and picosecond measurements have been performed using streak cameras, there are no commercial single photon sensitive devices with femtosecond resolution available. While time-domain sampling using sum-frequency generation has been already exploited for such measurement, inefficient conversion has necessitated long integration times to build the temporal profile. We demonstrate a highly efficient waveguided sum-frequency generation process in Lithium Niobate to measure the temporal envelope of single photons with femtosecond resolution with short enough acquisition time to provide a live-view of the measurement. We demonstrate the measurement technique and combine it with spectral measurements using a dispersive fiber time-of-flight spectrometer to determine upper and lower bounds for the spectral purity of heralded single photons. The approach complements the joint spectral intensity measurements as a measure on the purity can be given without knowledge of the spectral phase.

quant-ph