arXiv subjects

Raj Chakrabarti

Publications and source records attributed to Raj Chakrabarti.

15 recordsLinked to original sources

arXiv2021

Robust Control of Quantum Dynamics under Input and Parameter Uncertainty

Despite significant progress in theoretical and laboratory quantum control, engineering quantum systems remains principally challenging due to manifestation of noise and uncertainties associated with the field and Hamiltonian parameters. In this paper, we extend and generalize the asymptotic quantum control robustness analysis method -- which provides more accurate estimates of quantum control objective moments than standard leading order techniques -- to diverse quantum observables, gates and moments thereof, and also introduce the Pontryagin Maximum Principle for quantum robust control. In addition, we present a Pareto optimization framework for achieving robust control via evolutionary open loop (model-based) and closed loop (model-free) approaches with the mechanisms of robustness and convergence described using asymptotic quantum control robustness analysis. In the open loop approach, a multiobjective genetic algorithm is used to obtain Pareto solutions in terms of the expectation and variance of the transition probability under Hamiltonian parameter uncertainty. The set of numerically determined solutions can then be used as a starting population for model-free learning control in a feedback loop. The closed loop approach utilizes real-coded genetic algorithm with adaptive exploration and exploitation operators in order to preserve solution diversity and dynamically optimize the transition probability in the presence of field noise. Together, these methods provide a foundation for high fidelity adaptive feedback control of quantum systems wherein open loop control predictions are iteratively improved based on data from closed loop experiments.

quant-ph↗

arXiv2014

Dynamics and Control of DNA Sequence Amplification

DNA amplification is the process of replication of a specified DNA sequence \emph{in vitro} through time-dependent manipulation of its external environment. A theoretical framework for determination of the optimal dynamic operating conditions of DNA amplification reactions, for any specified amplification objective, is presented based on first-principles biophysical modeling and control theory. Amplification of DNA is formulated as a problem in control theory with optimal solutions that can differ considerably from strategies typically used in practice. Using the Polymerase Chain Reaction (PCR) as an example, sequence-dependent biophysical models for DNA amplification are cast as control systems, wherein the dynamics of the reaction are controlled by a manipulated input variable. Using these control systems, we demonstrate that there exists an optimal temperature cycling strategy for geometric amplification of any DNA sequence and formulate optimal control problems that can be used to derive the optimal temperature profile. Strategies for the optimal synthesis of the DNA amplification control trajectory are proposed. Analogous methods can be used to formulate control problems for more advanced amplification objectives corresponding to the design of new types of DNA amplification reactions.

physics.bio-ph↗

arXiv2014

Robustness of Controlled Quantum Dynamics

Control of multi-level quantum systems is sensitive to implementation errors in the control field and uncertainties associated with system Hamiltonian parameters. A small variation in the control field spectrum or the system Hamiltonian can cause an otherwise optimal field to deviate from controlling desired quantum state transitions and reaching a particular objective. An accurate analysis of robustness is thus essential in understanding and achieving model-based quantum control, such as in control of chemical reactions based on ab initio or experimental estimates of the molecular Hamiltonian. In this paper, theoretical foundations for quantum control robustness analysis are presented from both a distributional perspective - in terms of moments of the transition amplitude, interferences, and transition probability - and a worst-case perspective. Based on this theory, analytical expressions and a computationally efficient method for determining the robustness of coherently controlled quantum dynamics are derived. The robustness analysis reveals that there generally exists a set of control pathways that are more resistant to destructive interferences in the presence of control field and system parameter uncertainty. These robust pathways interfere and combine to yield a relatively accurate transition amplitude and high transition probability when uncertainty is present.

quant-ph↗

arXiv2011

Asymptotic Efficiency and Finite Sample Performance of Frequentist Quantum State Estimation

We undertake a detailed study of the performance of maximum likelihood (ML) estimators of the density matrix of finite-dimensional quantum systems, in order to interrogate generic properties of frequentist quantum state estimation. Existing literature on frequentist quantum estimation has not rigorously examined the finite sample performance of the estimators and associated methods of hypothesis testing. While ML is usually preferred on the basis of its asymptotic properties - it achieves the Cramer-Rao (CR) lower bound - the finite sample properties are often less than optimal. We compare the asymptotic and finite-sample properties of the ML estimators and test statistics for two different choices of measurement bases: the average case optimal or mutually unbiased bases (MUB) and a representative set of suboptimal bases, for spin-1/2 and spin-1 systems. We show that, in both cases, the standard errors of the ML estimators sometimes do not contain the true value of the parameter, which can render inference based on the asymptotic properties of the ML unreliable for experimentally realistic sample sizes. The results indicate that in order to fully exploit the information geometry of quantum states and achieve smaller reconstruction errors, the use of Bayesian state reconstruction methods - which, unlike frequentist methods, do not rely on asymptotic properties - is desirable, since the estimation error is typically lower due to the incorporation of prior knowledge.

quant-ph↗

arXiv2010

Search complexity and resource scaling for the quantum optimal control of unitary transformations

The optimal control of unitary transformations is a fundamental problem in quantum control theory and quantum information processing. The feasibility of performing such optimizations is determined by the computational and control resources required, particularly for systems with large Hilbert spaces. Prior work on unitary transformation control indicates that (i) for controllable systems, local extrema in the search landscape for optimal control of quantum gates have null measure, facilitating the convergence of local search algorithms; but (ii) the required time for convergence to optimal controls can scale exponentially with Hilbert space dimension. Depending on the control system Hamiltonian, the landscape structure and scaling may vary. This work introduces methods for quantifying Hamiltonian-dependent and kinematic effects on control optimization dynamics in order to classify quantum systems according to the search effort and control resources required to implement arbitrary unitary transformations.

quant-ph↗

arXiv2010

General unifying features of controlled quantum phenomena

Many proposals have been put forth for controlling quantum phenomena, including open-loop, adaptive feedback, and real-time feedback control. Each of these approaches has been viewed as operationally, and even physically, distinct from the others. This work shows that all such scenarios inherently share the same fundamental control features residing in the topology of the landscape relating the target physical observable to the applied controls. This unified foundation may provide a basis for development of hybrid control schemes that would combine the advantages of the existing approaches to achieve the best overall performance.

quant-ph↗

arXiv2010

Control of quantum phenomena: Past, present, and future

Quantum control is concerned with active manipulation of physical and chemical processes on the atomic and molecular scale. This work presents a perspective of progress in the field of control over quantum phenomena, tracing the evolution of theoretical concepts and experimental methods from early developments to the most recent advances. The current experimental successes would be impossible without the development of intense femtosecond laser sources and pulse shapers. The two most critical theoretical insights were (1) realizing that ultrafast atomic and molecular dynamics can be controlled via manipulation of quantum interferences and (2) understanding that optimally shaped ultrafast laser pulses are the most effective means for producing the desired quantum interference patterns in the controlled system. Finally, these theoretical and experimental advances were brought together by the crucial concept of adaptive feedback control, which is a laboratory procedure employing measurement-driven, closed-loop optimization to identify the best shapes of femtosecond laser control pulses for steering quantum dynamics towards the desired objective. Optimization in adaptive feedback control experiments is guided by a learning algorithm, with stochastic methods proving to be especially effective. Adaptive feedback control of quantum phenomena has found numerous applications in many areas of the physical and chemical sciences, and this paper reviews the extensive experiments. Other subjects discussed include quantum optimal control theory, quantum control landscapes, the role of theoretical control designs in experimental realizations, and real-time quantum feedback control. The paper concludes with a prospective of open research directions that are likely to attract significant attention in the future.

quant-ph↗

arXiv2008

Optimal Control of Evolutionary Dynamics

Elucidating the fitness measures optimized during the evolution of complex biological systems is a major challenge in evolutionary theory. We present experimental evidence and an analytical framework demonstrating how biochemical networks exploit optimal control strategies in their evolutionary dynamics. Optimal control theory explains a striking pattern of extremization in the redox potentials of electron transport proteins, assuming only that their fitness measure is a control objective functional with bounded controls.

q-bio.MN↗

arXiv2008

Quantum Pareto Optimal Control

We describe algorithms, and experimental strategies, for the Pareto optimal control problem of simultaneously driving an arbitrary number of quantum observable expectation values to their respective extrema. Conventional quantum optimal control strategies are less effective at sampling points on the Pareto frontier of multiobservable control landscapes than they are at locating optimal solutions to single observable control problems. The present algorithms facilitate multiobservable optimization by following direct paths to the Pareto front, and are capable of continuously tracing the front once it is found to explore families of viable solutions. The numerical and experimental methodologies introduced are also applicable to other problems that require the simultaneous control of large numbers of observables, such as quantum optimal mixed state preparation.

quant-ph↗

arXiv2008

Quantum Multiobservable Control

We present deterministic algorithms for the simultaneous control of an arbitrary number of quantum observables. Unlike optimal control approaches based on cost function optimization, quantum multiobservable tracking control (MOTC) is capable of tracking predetermined homotopic trajectories to target expectation values in the space of multiobservables. The convergence of these algorithms is facilitated by the favorable critical topology of quantum control landscapes. Fundamental properties of quantum multiobservable control landscapes that underlie the efficiency of MOTC, including the multiobservable controllability Gramian, are introduced. The effects of multiple control objectives on the structure and complexity of optimal fields are examined. With minor modifications, the techniques described herein can be applied to general quantum multiobjective control problems.

quant-ph↗

arXiv2007

Quantum Control Landscapes

Numerous lines of experimental, numerical and analytical evidence indicate that it is surprisingly easy to locate optimal controls steering quantum dynamical systems to desired objectives. This has enabled the control of complex quantum systems despite the expense of solving the Schrodinger equation in simulations and the complicating effects of environmental decoherence in the laboratory. Recent work indicates that this simplicity originates in universal properties of the solution sets to quantum control problems that are fundamentally different from their classical counterparts. Here, we review studies that aim to systematically characterize these properties, enabling the classification of quantum control mechanisms and the design of globally efficient quantum control algorithms.

quant-ph↗

arXiv2007

Critical Topology for Optimization on the Symplectic Group

Optimization problems over compact Lie groups have been extensively studied due to their broad applications in linear programming and optimal control. This paper analyzes least square problems over a noncompact Lie group, the symplectic group $\Sp(2N,\R)$, which can be used to assess the optimality of control over dynamical transformations in classical mechanics and quantum optics. The critical topology for minimizing the Frobenius distance from a target symplectic transformation is solved. It is shown that the critical points include a unique local minimum and a number of saddle points. The topology is more complicated than those of previously studied problems on compact Lie groups such as the orthogonal and unitary groups because the incompatibility of the Frobenius norm with the pseudo-Riemannian structure on the symplectic group brings significant nonlinearity to the problem. Nonetheless, the lack of traps guarantees the global convergence of local optimization algorithms.

math-ph↗

arXiv2007

Computational complexity of quantum optimal control landscapes

We study the Hamiltonian-independent contribution to the complexity of quantum optimal control problems. The optimization of controls that steer quantum systems to desired objectives can itself be considered a classical dynamical system that executes an analog computation. The system-independent component of the equations of motion of this dynamical system can be integrated analytically for various classes of discrete quantum control problems. For the maximization of observable expectation values from an initial pure state and the maximization of the fidelity of quantum gates, the time complexity of the corresponding computation belongs to the class continuous log (CLOG), the lowest analog complexity class, equivalent to the discrete complexity class NC. The simple scaling of the Hamiltonian-independent contribution to these problems with quantum system dimension indicates that with appropriately designed search algorithms, quantum optimal control can be rendered efficient even for large systems.

quant-ph↗

arXiv2007

Orthogonal measurement-assisted quantum control

Existing algorithms for the optimal control of quantum observables are based on locally optimal steps in the space of control fields, or as in the case of genetic algorithms, operate on the basis of heuristics that do not explicitly take into account details pertaining to the geometry of the search space. We present globally efficient algorithms for quantum observable control that follow direct or close-to-direct paths in the domain of unitary dynamical propagators, based on partial reconstruction of these propagators at successive points along the search trajectory through orthogonal observable measurements. These algorithms can be implemented experimentally and offer an alternative to the adaptive learning control approach to optimal control experiments (OCE). Their performance is compared to that of local gradient-based control optimization.

quant-ph↗

arXiv2007

Optimal Control Theory for Continuous Variable Quantum Gates

We apply the methodology of optimal control theory to the problem of implementing quantum gates in continuous variable systems with quadratic Hamiltonians. We demonstrate that it is possible to define a fidelity measure for continuous variable (CV) gate optimization that is devoid of traps, such that the search for optimal control fields using local algorithms will not be hindered. The optimal control of several quantum computing gates, as well as that of algorithms composed of these primitives, is investigated using several typical physical models and compared for discrete and continuous quantum systems. Numerical simulations indicate that the optimization of generic CV quantum gates is inherently more expensive than that of generic discrete variable quantum gates, and that the exact-time controllability of CV systems plays an important role in determining the maximum achievable gate fidelity. The resulting optimal control fields typically display more complicated Fourier spectra that suggest a richer variety of possible control mechanisms. Moreover, the ability to control interactions between qunits is important for delimiting the total control fluence. The comparative ability of current experimental protocols to implement such time-dependent controls may help determine which physical incarnations of CV quantum information processing will be the easiest to implement with optimal fidelity.

quant-ph↗