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Raj K. Gupta

Publications and source records attributed to Raj K. Gupta.

At least 19 recordsLinked to original sources

Decay analysis of compound nuclei with mass A$\sim 30-200$ formed in the reactions involving loosely bound projectiles

The dynamics of the reactions forming compound nuclei using loosely bound projectiles is analysed within the framework of dynamical cluster decay model (DCM) of Gupta and Collaborators. We have analysed different reactions with $^{7}Li$, $^{9}Be$ and $^{7}Be$ as neutron rich and neutron deficient projectiles, respectively, on different targets at the three $E_{lab}$ values, forming compound nuclei within the mass region A$\sim 30-200$. The contributions of light particles LPs ($A\le4$) cross sections $σ_{LP}$, energetically favoured intermediate mass fragments IMFs ($5 \le A_2 \le 20$) cross sections $σ_{IMF}$ as well as fusion-fission $\it{ff}$ cross sections $σ_{ff}$ constitute the $σ_{fus}$ (=$σ_{LP}$+$σ_{IMF}$+$σ_{ff}$) for these reactions. The contribution of the emitted LPs, IMFs and ff fragments is added for all the angular momentum upto the $\ell_{max}$ value, for the resepctive reactions. Interestingly, we find that the $ΔR^{emp}$, the only parameter of model and uniquely fixed to address the $σ_{fus}$ for all other reactions having $\it same$ loosely bound projectile at the chosen incident energy. It may be noted that the dynamical collective mass motion of preformed LPs, IMFs and ff fragments or clusters through the modified interaction potential barrier are treated on parallel footing. We see that the values of modified interaction barrier heights $ΔV_{B}^{emp}$ for such reactions are almost of the same amount specifically at the respective $\ell_{max}$ values.

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The evaporation residue in the fission state of Barium nuclei within relativistic mean-field theory

The evaporation residue of Barium isotopes are investigated in a microscopic study using relativistic mean field theory. The investigation includes the isotopes of Barium from the valley of stability to exotic proton-rich region. The ground as well as neck configurations for these nuclei are generated from their total nucleonic density distributions of the corresponding state. We have estimated the constituents (number of nucleons) in the elongated neck region of the fission state. We found the $α$-particle as the constituent of neck of Ba-isotopes, referred to as the evaporated residue in heavy-ion reaction studies. A strong correlation between the neutron and proton is observed throughout the isotopic chain.

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Structure effects in the region of superheavy elements via the $α$-decay chain of $^{293}$118

The $α$-decay chain of $^{293}$118, first proposed in the Berkeley cold fusion experiment $^{208}$Pb($^{86}$Kr,1n) and now retracted, is calculated by using the preformed cluster model (PCM) of one of us (RKG). Also, the possible branchings of $α$-particles to heavier cluster decays of all the parents in this chain are calculated for the first time. The calculated Q-values, penetrabilities and preformation factors for $α$-decays suggest that the $^{285}$114 nucleus with Z=114, N=171 is a magic nucleus, either due to the magicity of Z=114, or of N=172 or of both. The N=172 is proposed to be a magic number in certain relativistic mean-field calculations, but with Z=120. The calculated cluster decays point to new interesting possibilities of $^{14}$C decay of the $^{281}$112 parent, giving rise to a (reasonably) deformed Z=106, N=161, $^{267}$106 daughter (N=162 being now established as the deformed magic shell) or to a doubly magic $^{48}$Ca cluster emitted from any of the parent nucleus in the $α$-decay chain. Apparently, these are exciting new directions for future experiments.

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The cluster-core model for halo-structure of light nuclei at the drip lines

Nuclei at both the neutron- and proton-drip lines are studied. In the cluster-core model, the halo-structure of all the observed and proposed cases of neutron- or proton-halos is investigated in terms of simple potential energy surfaces calculated as the sum of binding energies, Coulomb repulsion, nuclear proximity attraction and the centrifugal potential for all the possible cluster+core configurations of a nucleus. The clusters of neutrons and protons are taken to be unbound, with additional Coulomb energy added for proton-clusters. The model predictions agree with the available experimental studies but show some differences with the nucleon separation energy hypothesis, particularly for proton-halo nuclei. Of particular interest are the halo-structures of $^{11}N$ and $^{20}Mg$. The calculated potential energy surfaces are also useful to identify the new magic numbers and molecular structures in exotic nuclei. In particular, N=6 is a possible new magic number for very neutron-deficient nuclei, but Z=N=2 and Z=8 seem to remain magic even for such nuclei, near the drip line.

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The formation and decay of superheavy nuclei produced in $^{48}Ca$-induced reactions

The formation of superheavy nuclei in $^{48}Ca+^{232}Th$, $^{238}U$, $^{242,244}Pu$ and $^{248}Cm$ reactions and their subsequent decay are studied within the quantum mechanical fragmentation theory (QMFT) and the QMFT based preformed cluster-decay model (PCM) of Gupta and collaborators. According to QMFT, all these $^{48}Ca$-induced reactions are cold fusion reactions with relative excitation energies larger than for the $Pb$-induced cold fusion reactions and smaller than for the lighter beam i.e. $Mg$, $Si$ or $S$-induced hot fusion reactions. The same reactions were first suggested by Gupta et al. in 1977 on the basis of QMFT, and this study re-establishes the same result. In fact, for such heavy isotopes of Z=110 to 116, $^{50}Ca$ is shown to be a better beam for cold fusion, but $^{50}Ca$ is a radioactive nucleus. The $α$-decay half-lives of these nuclei after 3n and/ or 4n evaporations, i.e. of the evaporation residues of these compound systems, calculated on PCM compare reasonably well with experiments published by Dubna group and another recent calculation. As expected for such rare decays, PCM calculations show that the $α$-preformation factors are small, $\sim 10^{-8}$ to $10^{-10}$. The possible competition of $α$-decays with heavy cluster emissions from these superheavy nuclei is also probed from the point of view of searching for new nuclear structure information and possible future experiments with such exotic nuclei. The decay half-lives for some clusters are in fact shown to be lower than the limits of experiments for nuclei with enough available atoms.

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Barrier modification in sub-barrier fusion reactions using Dynamical cluster-decay and extended-Wong models

Fusion-evaporation cross-sections σevr in reactions known for fusion hindrance phenomenon in coupled-channels calculations at below-barrier energies, are studied in terms of the dynamical cluster-decay model (DCM) of one of us (RKG) and Collaborators and the Wong formula extended by us, both based on proximity potential, by using the concept of "barrier modification" at sub-barrier energies, first advocated by Misicu and Esbensen for M3Y potential. The DCM is shown to contain the "barrier lowering" as its inbuilt characteristic, and the same is found essential, and introduced empirically, in the extended-Wong formula.

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A new microscopic nucleon-nucleon interaction derived from relativistic mean field theory

A new microscopic nucleon-nucleon (NN) interaction has been derived for the first time from the popular relativistic mean field theory (RMFT) Lagrangian. The NN interaction so obtained remarkably relate to the inbuilt fundamental parameters of RMFT. Furthermore, by folding it with the RMFT-densities of cluster and daughter nuclei to obtain the optical potential, it's application is also examined to study the exotic cluster radioactive decays, and results obtained found comparable with the successfully used M3Y phenomenological effective NN interactions. The presently derived NN-interaction can also be used to calculate a number of other nuclear observables.

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Temeprature-dependent Seeger's liquid drop energy for nuclei up to Z=118

Seeger's semi-empirical mass formula is revisited for two of its constants (bulk constant α(0) and neutron-proton asymmetry constant a_{a}) readjusted to obtain the ground-state (g.s.) binding energies of nuclei within a precision of <1.5 MeV and for nuclei up to Z=118. The aim is to include the temperature T-dependence on experimental binding energies, and not to obtain the new parameter set of Seeger's liquid drop energy VLDM . Our proceedure is to define the g.s. binding energy B = V_{LDM} + δU, as per Strutinsky renormalization procedure, and using the empirical shell corrections δU of Myers and Swiatecki, fit the constants of V_{LDM} to obtain the experimental binding energy Bexpt or theoretically calculated Btheo if data were not available. The T-dependence of the constants of V_{LDM}, is introduced as per the work of Davidson et al., where the pairing energy δ(T) is modified as per new calculations on compound nucleus decays. The newly fitted constants of V_{LDM} at T=0 are made available here for use of other workers interested in nuclear dynamics of hot and rotating nuclei.

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Sudden- or Frozen-density approximation in Semi-classical extended Thomas Fermi model for Wong formula used in 64Ni+64Ni reaction

The {\ell}-summed Wong expression is applied in the semiclassical extended Thomas Fermi (ETF) method of Skyrme energy density formalism (SEDF), using both the sudden and frozen-density approximations, to the case of 64Ni+64Ni reaction data. We find that a very much improved fit (almost exact, point to point) to the data is obtained for the frozen-density approximation with {\ell}max (Ec.m.) varying smoothly. On the other hand, the same could not be achieved in the sudden case, still requiring a modification of the barrier at both the below- and above-barrier energies. This result means to say that the phenomenon of hindrance, observed in coupled channel calculations for 64Ni+64Ni reaction, could be explained simply on the basis of the {\ell}-summed Wong expression, at least for the frozen-density approximation in ETF method of SEDF.

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Barrier modification in sub-barrier fusion reactions using Wong formula with Skyrme forces in semiclassical formalism

We obtain the nuclear proximity potential by using semiclassical extended Thomas Fermi (ETF) approach in Skyrme energy density formalism (SEDF), and use it in the extended $\ell$-summed Wong formula under frozen density approximation. This method has the advantage of allowing the use of different Skyrme forces, giving different barriers. Thus, for a given reaction, we could choose a Skyrme force with proper barrier characteristics, not-requiring extra ``barrier lowering" or ``barrier narrowing" for a best fit to data. For the $^{64}$Ni+$^{100}$Mo reaction, the $\ell$-summed Wong formula, with effects of deformations and orientations of nuclei included, fits the fusion-evaporation cross section data exactly for the force GSkI, requiring additional barrier modifications for forces SIII and SV. However, the same for other similar reactions, like $^{58,64}$Ni+$^{58,64}$Ni, fits the data best for SIII force. Hence, the barrier modification effects in $\ell$-summed Wong expression depends on the choice of Skyrme force in extended ETF method.

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Role of non-coplanarity in nuclear reactions using the Wong formula based on the proximity potential

we assessed Wong's formula for its angular momentum $\ell$-summation and "barrier modification" effects at sub-barrier energies in the dominant fusion-evaporation and capture (equivalently, quasi-fission) reaction cross-sections. For use of the multipole deformations (up to $β_4$) and (in-plane, $Φ$=0$^0$) orientations-dependent proximity potential in fusion-evaporation cross-sections of $^{58}$Ni+$^{58}$Ni, $^{64}$Ni+$^{64}$Ni and $^{100}$Mo, known for fusion hindrance phenomenon in coupled-channels calculations, and the capture cross-sections of $^{48}$Ca+$^{238}$U, $^{244}$Pu and $^{248}$Cm reactions, forming superheavy nuclei, though the simple $\ell$=0 barrier-based Wong formula is found inadequate, its extended version, the $\ell$-summed Wong expression fits very well the above noted capture cross-sections at all center-of-mass energies $E_{c.m.}$'s, but require (additional) modifications of the barriers to fit the fusion-evaporation cross-sections in the Ni-based reactions at below-barrier energies. Some barrier modification effects are shown \cite{kumar09} to be already present in Wong expression due to its inbuilt $\ell$-dependence via $\ell$-summation.

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Internal stucture of clusters in $^{112-122}$Ba nuclei within relativistic mean field theory

We study the clustering structure and the internal or sub-structure of clusters in $^{112-122}$Ba nuclei within the framework of relativistic mean field theory in an axially deformed cylindrical co-ordinate. We calculate the total density distribution, and the individual neutrons and protons density distributions. From the analysis of the clustering confugurations of the density distributions of various shapes, we find different sub-structures inside the Ba nuclei considered here. The important step, carried out for the first time, is the counting of number of protons and neutrons present in the clustering region(s). $^{12}$C is shown to consitute the cluster configuration of Ba nuclei in most cases, with $^{2,3}$H and $^4$He constituting the neck between two fissioning symmetrical fragments.

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Superdeformed and Hyperdeformed States in Z=122 Isotopes

We calculate the binding energy, root-mean-square radius and quadrupole deformation parameter for the recent, possibly discovered superheavey element Z=122, using the axially deformed relativistic mean field (RMF) and non-relativistic Skyrme Hartree-Fock (SHF) formalisms. The calculation is extended to include various isotopes of Z=122 element, strarting from A=282 to A=320. We predict highly deformed structures in the ground state for all the isotopes. A shape transition appears at about A=290 from a highly oblate to a large prolate shape, which may be considered as the superdeformed and hyperdeformed structures of Z=122 nucleus in the mean field approaches. The most stable isotope (largest binding energy per nucleon) is found to be $^{302}$122, instead of the experimentally observed $^{292}$122.

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Probing the density dependence of the symmetry potential in intermediate energy heavy ion collisions

Based on the ultrarelativistic quantum molecular dynamics (UrQMD) model, the effects of the density-dependent symmetry potential for baryons and of the Coulomb potential for produced mesons are investigated for neutron-rich heavy ion collisions at intermediate energies. The calculated results of the $Δ^-/Δ^{++}$ and $π^{-}/π^{+}$ production ratios show a clear beam-energy dependence on the density-dependent symmetry potential, which is stronger for the $π^{-}/π^{+}$ ratio close to the pion production threshold. The Coulomb potential of the mesons changes the transverse momentum distribution of the $π^{-}/π^{+}$ ratio significantly, though it alters only slightly the $π^-$ and $π^+$ total yields. The $π^-$ yields, especially at midrapidity or at low transverse momenta and the $π^-/π^+$ ratios at low transverse momenta, are shown to be sensitive probes of the density-dependent symmetry potential in dense nuclear matter. The effect of the density-dependent symmetry potential on the production of both, K$^0$ and K$^+$ mesons, is also investigated.

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$Σ^-/Σ^+$ ratio as a candidate for probing the density dependence of the symmetry potential at high nuclear densities

Based on the UrQMD model, we have investigated the influence of the symmetry potential on the negatively and positively charged $π$ and $Σ$ hyperon production ratios in heavy ion collisions at the SIS energies. We find that, in addition to $π^-/π^+$ ratio, the $Σ^-/Σ^+$ ratio can be taken as a sensitive probe for investigating the density dependence of the symmetry potential of nuclear matter at high densities (1-4 times of normal baryon density). This sensitivity of the symmetry potential to both the $π^-/π^+$ and $Σ^-/Σ^+$ ratios is found to depend strongly on the incident beam energy. Furthermore, the $Σ^-/Σ^+$ ratio is shown to carry the information about the isospin-dependent part of the $Σ$ hyperon single-particle potential.

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Dynamical cluster-decay model for hot and rotating light-mass nuclear systems, applied to low-energy $^{32}$S + $^{24}$Mg $\to ^{56}$Ni reaction

The dynamical cluster-decay model (DCM) is developed further for the decay of hot and rotating compound nuclei (CN) formed in light heavy-ion reactions. The model is worked out in terms of only one parameter, namely the neck-length parameter, which is related to the total kinetic energy TKE(T) or effective Q-value $Q_{eff}(T)$ at temperature T of the hot CN, defined in terms of the both the light-particles (LP), with $A \leq$ 4, Z $\leq$ 2, as well as the complex intermediate mass fragments (IMF), with $4 < A < 20, Z > 2$, is considered as the dynamical collective mass motion of preformed clusters through the barrier. Within the same dynamical model treatment, the LPs are shown to have different characteristics as compared to the IMFs. The systematic variation of the LP emission cross section $σ_{LP}$, and IMF emission cross section $σ_{IMF}$, calculated on the present DCM match exactly the statistical fission model predictions. It is for the first time that a non-statistical dynamical description is developed for the emission of light-particles from the hot and rotating CN. The model is applied to the decay of $^{56}$Ni formed in the $^{32}$S + $^{24}$Mg reaction at two incident energies E$_{c.m.}$ = 51.6 and 60.5 MeV. Both the IMFs and average $\bar{TKE}$ spectra are found to compare reasonably nicely with the experimental data, favoring asymmetric mass distributions. The LPs emission cross section is shown to depend strongly on the type of emitted particles and their multiplicities.

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The island of deformation and shape co-existence in neutron-deficient nuclei of the Pb region using relativistic mean field model

We have investigated the ground-state structures of even-even neutron-deficient isotopes of Hg and Pb nuclei within the framework of a deformed relativistic mean field formalism for a number of commonly used parameter sets, namely NL1, NL3, NL-SH, NL-RA1 and TM1. The ground states of a bunch of Hg and Pb-isotopes towards the proton-dripline are found to be deformed for all the forces, with a constant pairing gap. The small differences in the ground- and the first-excited state binding energies predict a sea of low-lying excited states, and hence of shape co-existence, for both the Hg and Pb nuclei. In general, a discrepancy between the experimentally observed and theoretically predicted (sign of) quadrupole deformations is noticed in this mass region. The constrained potential energy surfaces and the single-particle energy spectra analyzed for some selected nuclei show that the known large shell gap for Pb nuclei at Z=82 is almost extinguished for its proton-rich isotopes.

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Collective clusterization effects in light heavy ion reactions

The collective clusterization process, proposed for intermediate mass fragments (IMFs, 4$<$A$\le$28, 2$<$Z$\le$14) emitted from the hot and rotating compound nuclei formed in low energy reactions, is extended further to include also the emission of light particles (LPs, A$\le$4, Z$\le$2) from the fusion-evaporation residues. Both the LPs and IMFs are treated as the dynamical collective mass motion of preformed clusters through the barrier. Compared to IMFs, LPs are shown to have different characteristics, and the predictions of our, so-called, dynamical cluster-decay model are similar to those of the statistical fission model.

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