arXiv subjects

Rakhul Raj

Publications and source records attributed to Rakhul Raj.

3 recordsLinked to original sources

arXiv2026

Observation of large perpendicular magnetic anisotropy and excessive polar magneto-optical effect in Pt/CoFeB/Ru tri-layer system

Heterostructures comprising ferromagnet (FM) and heavy metals (HM) with perpendicular magnetic anisotropy (PMA) and interfacial Dzyaloshinskii-Moriya interaction (iDMI) can host chiral domain walls and topological spin textures, making them highly promising for various spintronics applications. In this paper, we have investigated the magneto-optical properties, the anomalous Hall effect (AHE), and PMA of Pt/CoFeB/Ru multilayers engineered to possess significant iDMI. We utilized the Anomalous Hall effect (AHE), and the polar magneto-optical Kerr effect (p-MOKE), Hall response and the domain wall motion in Pt/CoFeB/Ru-systems. Both MOKE and AHE measurements confirm that the films maintain strong perpendicular magnetization for CoFeB thicknesses below 1.2 nm. The effective magnetic anisotropy K_{\mathrm{eff}} of 0.88 \times 10^6 erg/cm^3 has been achieved without any post-annealing, highlighting the high-quality interface in this multilayer design. The angular dependence of the switching field deviates from the conventional Kondorsky model and is well described using a modified Kondorsky formalism, capturing the role of field-induced domain-wall softening and pinning effects in the reversal process. Furthermore, p-MOKE microscopy imaging during the magnetization reversal process provides detailed insight into domain nucleation and subsequent domain-wall propagation. The observations reveal well-defined, stable magnetic domains that evolve coherently under the applied magnetic field. Such a behavior is expected in the system where interfacial DMI, PMA interact to stabilize the chiral N\'eel-type domain walls, which are essential for fast, low-power domain-wall motion driven by spin-orbit torques.

cond-mat.mtrl-sci↗

arXiv2024

Growth-Induced Unconventional Magnetic Anisotropy in Co/Fullerene (C60) Bilayer Systems; Insights from a Two-Grain Stoner-Wohlfarth Model

Organic spintronics has drawn the interest of the science community due to various applications in spin-valve devices. However, an efficient room-temperature Organic Spin Valve device has not been experimentally realized due to the complicated spin transport at the metal-organic interfaces. The present study focuses on a comprehensive understanding of the interfacial properties essential for advancing device performance and functionality. The structural and magnetic properties of the ultra-thin Cobalt (Co) films deposited on the fullerene (C60) layer are studied to investigate the origin of magnetic anisotropy in the metal-organic bilayer structures. Due to the mechanical softness of C60, penetration of ferromagnetic Co atoms inside the C60 film is confirmed by the X-ray reflectivity and Secondary Ion Mass Spectroscopy measurements. Grazing incidence small-angle X-ray scattering and atomic force microscopy provided information regarding the structural and morphological properties of the Co/C60 bilayers, angular dependent Magneto-optic Kerr effect measurements with varying Co layer thickness provided information about the growth-induced uniaxial magnetic anisotropy. In contrast to the inorganic silicon substrates, magnetic anisotropy in Co film tends to develop at 25 {\AA} thickness on the C60 layer, which further increases with the thickness of Cobalt. The anomalous behavior in coercivity and remanence variation along the nominal hard axis is explained by a two-grain Stoner-Wohlfarth model with intergranular exchange coupling. It is further confirmed by a non-uniform spatial distribution of magnetic domains investigated through Kerr microscopy. These anomalies could be attributed to the distribution of magneto-crystalline anisotropy and inhomogeneous strain caused by the formation of a diffused layer at the Co/C60 interface.

cond-mat.mtrl-sci↗

arXiv2022

Light-induced giant and persistent changes in the converse magnetoelastic effects in Ni/BaTiO3 multiferroic heterostructure

Magnetoelastic and magnetoelectric coupling in the artificial multiferroic heterostructures facilitate valuable features for device applications such as magnetic field sensors and electric write magnetic-read memory devices. In a ferromagnetic/ferroelectric heterostructures, the strain mediated coupling exploits piezoelectricity/electrostriction in ferroelectric phase and magnetostriction/piezomagnetism in ferromagnetic phase. Such verity of these combined effect can be manipulated by an external perturbation, such as electric field, temperature or magnetic field. Here, we demonstrate the remote-controlled tunability of these effects under the visible, coherent and polarized light. The combined surface and bulk magnetic study of domain-correlated Ni/BaTiO3 heterostructure reveals that the system is strong sensitive about the light illumination via the combined effect of converse piezoelectric, magnetoelastic coupling and converse magnetostriction. Well-defined ferroelastic domain structure is fully transferred from a tetragonal ferroelectric to magnetostrictive layer via interface strain transfer during the film growth. The visible light illumination is used to manipulate the original ferromagnetic microstructure by the light-induced domain wall motion in ferroelectric, consequently the domain wall motion in the ferromagnetic layer. Our findings mimic the attractive remote-controlled ferroelectric random-access memory write and magnetic random-access memory read application scenarios, hence, can be proven as a novel perspective for room temperature device applications.

cond-mat.mtrl-sci↗