arXiv subjects

Ralu Divan

Publications and source records attributed to Ralu Divan.

At least 19 recordsLinked to original sources

arXiv2026

Strong coupling between propagating spin wave and microwave photons in a superconducting resonator

We demonstrate strong coupling between propagating spin wave modes and microwave photons in superconducting resonator-magnetic thin film hybrid circuits. By fabricating the resonator directly on yttrium iron garnet thin films grown on rare-earth-free Y$_3$Sc$_2$Ga$_3$O$_{12}$ substrates, we achieve strong coupling of both Damon-Eshbach and backward-volume spin wave modes to the resonator, with coupling strengths exceeding both the magnon and photon damping rates. Furthermore, we observe nonreciprocal spin wave radiation of the hybrid magnonic mode in the Damon-Eshbach configuration, highlighting the potential for incorporating intrinsic spin-wave nonreciprocity into hybrid magnonic systems. These results open new avenues for integrating spin-wave magnonics with cavity magnonics, and for harnessing spin waves for potential applications in quantum information science.

cond-mat.mes-hall↗

arXiv2026

Magnonic spontaneous oscillation induced by parametric pumping

Spontaneous dynamic systems have attracted significant attention for their rich underlying physics such as phase-locking and synchronization. In this work, we report a new mechanism of generating magnetic spontaneous oscillation via parametric pumping. By applying a pump tone to excite propagating spin waves in a yttrium iron garnet delay line, four-wave mixing converts the pump mode into two phase-autonomous propagating magnon modes, i.e. a spontaneous mode with nearly twice the wavenumber of the pump mode and an idler mode with nearly zero wavenumber. This allows us to reliably generate ultrasharp spin wave dynamics with broad frequency tunability from the pump and magnetic field. We show that the spontaneous mode can be phase-locked to a probe tone, similar to an auto-oscillator. Furthermore, the spontaneous dynamics can be used to implement a high-gain magnonic parametric amplifier with a gain up to 40 dB. Our results open a new avenue for studying nonlinear magnonics and synchronization physics in propagating magnon geometry and for developing new magnonic devices.

cond-mat.mes-hall↗

arXiv2025

A15 Phase Ta3Sb Thin Films: Direct Synthesis, Charge Transport and Spin-Orbit Torque

Ta3Sb is one of the A15 compounds that have been predicted to have giant spin Hall conductivities due to the gapped Dirac-like band crossings in their electronic structures. We use co-sputtering to directly synthesize thin films of Ta3Sb and identify a large window of Ta:Sb flux ratio that permits the formation of single-phase A15 structure. These sputtered films have an actual Ta:Sb atomic ratio of 4:1 as determined from Rutherford backscattering spectrometry. Their high resistivity, at the Mott-Ioffe-Regel limit, suggests that the electron mean free path is comparable to interatomic distances. From harmonic Hall and spin-torque ferromagnetic resonance measurements, the intrinsic spin Hall conductivity of thin film Ta3Sb is estimated to be in the range of -526 to -1230 (hbar/e) S/cm at 300 K, lower in magnitude than the predicted value of -1400 (hbar/e) S/cm. First-principles calculations of the electronic structure show that the discrepancy is consistent with an increase of the Fermi level due to the non-ideal stoichiometry needed to stabilize the A15 structure.

cond-mat.mtrl-sci↗

arXiv2025

Adaptive AI decision interface for autonomous electronic material discovery

AI-powered autonomous experimentation (AI/AE) can accelerate materials discovery but its effectiveness for electronic materials is hindered by data scarcity from lengthy and complex design-fabricate-test-analyze cycles. Unlike experienced human scientists, even advanced AI algorithms in AI/AE lack the adaptability to make informative real-time decisions with limited datasets. Here, we address this challenge by developing and implementing an AI decision interface on our AI/AE system. The central element of the interface is an AI advisor that performs real-time progress monitoring, data analysis, and interactive human-AI collaboration for actively adapting to experiments in different stages and types. We applied this platform to an emerging type of electronic materials-mixed ion-electron conducting polymers (MIECPs) -- to engineer and study the relationships between multiscale morphology and properties. Using organic electrochemical transistors (OECT) as the testing-bed device for evaluating the mixed-conducting figure-of-merit -- the product of charge-carrier mobility and the volumetric capacitance (μC*), our adaptive AI/AE platform achieved a 150% increase in μC* compared to the commonly used spin-coating method, reaching 1,275 F cm-1 V-1 s-1 in just 64 autonomous experimental trials. A study of 10 statistically selected samples identifies two key structural factors for achieving higher volumetric capacitance: larger crystalline lamellar spacing and higher specific surface area, while also uncovering a new polymer polymorph in this material.

cond-mat.mtrl-sci↗

arXiv2023

Extended Kohler's Rule of Magnetoresistance in TaCo$_2$Te$_2$

TaCo$_2$Te$_2$ is recently reported to be an air-stable, high mobility Van der Waals material with probable magnetic order. Here we investigate the scaling behavior of its magnetoresistance. We measured both the longitudinal ($ρ_{xx}$) and Hall ($ρ_{xy}$) magnetoresistivities of TaCo$_2$Te$_2$ crystals in magnetic fields parallel to the c-axis and found that the magnetoresistance violates the Kohler's rule $MR \sim f[H/ρ_0]$ while obeying the extended Kohler's rule $MR \sim f[H/(n_Tρ_0)]$, where $MR \sim [ρ_{xx}(H)-ρ_0]/ρ_0$, $H$ is the magnetic field, $n_T$ is a thermal factor, $ρ_{xx}(H)$ and $ρ_0$ are the resistivities at $H$ and zero field, respectively. While deviating from those of the densities of electrons ($n_e$) and holes ($n_h$) obtained from the two-band model analysis of the magnetoconductivities, the temperature dependence of $n_T$ is close to that of the Hall carrier densities $n_H$ calculated from the slopes of $ρ_{xy}(H)$ curves at low magnetic fields, providing a new way to obtain the thermal factor in the extended Kohler's rule.

cond-mat.mtrl-sci↗

arXiv2023

Field Orientation Dependent Magnetic Phases In Weyl Semimetal Co3Sn2S2

Magnetism plays a key role in the emergence of topological phenomena in the Weyl semimetal Co3Sn2S2, which exhibits a ferromagnetic (FM) interactions along the c-axis of the crystal and an antiferromagnetic (AFM) interactions within the ab plane. Extensive studies on the temperature dependence of the magnetism with the magnetic field along the c-axis have uncovered a number of magnetic phases. Currently, the nature and origins of the reported magnetic phases are under debate. Here we report on magnetic field orientation effects on the magnetism in Co3Sn2S2. The shape of the hysteresis loop of the Hall resistance at a fixed temperature is found to change from rectangular to bow-tie-like as the magnetic field is tilted from the c-axis towards the ab plane, resembling that reported for magnetic fields along the c-axis as the temperature approaches the Curie temperature from below. Unlike their temperature-dependent counterparts, the newly observed bow-tie-like hysteresis loops show exchange bias. Our results showcase the contribution of the in-plane AFM interactions to the magnetism in Co3Sn2S2 and demonstrate a new way to tune its magnetic phases. They also shed light on the temperature-dependent magnetic phases occurring in the magnetic field along the c-axis of the crystal.

cond-mat.mtrl-sci↗

arXiv2023

Programmable Real-Time Magnon Interference in Two Remotely Coupled Magnonic Resonators

Magnon interference is a signature of coherent magnon interactions for coherent information processing. In this work, we demonstrate programmable real-time magnon interference, with examples of nearly perfect constructive and destructive interference, between two remotely coupled yttrium iron garnet spheres mediated by a coplanar superconducting resonator. Exciting one of the coupled resonators by injecting single- and double-microwave pulse leads to the coherent energy exchange between the remote magnonic resonators and allows us to realize a programmable magnon interference that can define an arbitrary state of coupled magnon oscillation. The demonstration of time-domain coherent control of remotely coupled magnon dynamics offers new avenues for advancing coherent information processing with circuit-integrated hybrid magnonic networks.

cond-mat.mes-hall↗

arXiv2023

Tunable Magnon-Photon Coupling by Magnon Band Gap in a Layered Hybrid Perovskite Antiferromagnet

Tunability of coherent coupling between fundamental excitations is an important prerequisite for expanding their functionality in hybrid quantum systems. In hybrid magnonics, the dipolar interaction between magnon and photon usually persists and cannot be switched off. Here, we demonstrate this capability by coupling a superconducting resonator to a layered hybrid perovskite antiferromagnet, which exhibits a magnon band gap due to its intrinsic Dzyaloshinskii-Moriya interaction. The pronounced temperature sensitivity of the magnon band gap location allows us to set the photon mode within the gap and to disable magnon-photon hybridization. When the resonator mode falls into the magnon band gap, the resonator damping rate increases due to the nonzero coupling to the detuned magnon mode. This phenomena can be used to quantify the magnon band gap using an analytical model. Our work brings new opportunities in controlling coherent information processing with quantum properties in complex magnetic materials.

cond-mat.mtrl-sci↗

arXiv2023

Unidirectional Microwave Transduction with Chirality Selected Short-Wavelength Magnon Excitations

Nonreciprocal magnon propagation has recently become a highly potential approach of developing chip-embedded microwave isolators for advanced information processing. However, it is challenging to achieve large nonreciprocity in miniaturized magnetic thin-film devices because of the difficulty of distinguishing propagating surface spin waves along the opposite directions when the film thickness is small. In this work, we experimentally realize unidirectional microwave transduction with sub-micron-wavelength propagating magnons in a yttrium iron garnet (YIG) thin film delay line. We achieve a non-decaying isolation of 30 dB with a broad field-tunable band-pass frequency range up to 14 GHz. The large isolation is due to the selection of chiral magnetostatic surface spin waves with the Oersted field generated from the coplanar waveguide antenna. Increasing the geometry ratio between the antenna width and YIG thickness drastically reduces the nonreciprocity and introduces additional magnon transmission bands. Our results pave the way for on-chip microwave isolation and tunable delay line with short-wavelength magnonic excitations.

cond-mat.mes-hall↗

arXiv2022

Temperature-driven changes in the Fermi surface of graphite

We report on temperature-dependent size and anisotropy of the Fermi pockets in graphite revealed by magnetotransport measurements. The magnetoresistances obtained in fields along the c-axis obey an extended Kohler's rule, with the carrier density following prediction of a temperature-dependent Fermi energy, indicating a change in the Fermi pocket size with temperature. The angle-dependent magnetoresistivities at a given temperature exhibit a scaling behavior. The scaling factor that reflects the anisotropy of the Fermi surface is also found to vary with temperature. Our results demonstrate that temperature-driven changes in Fermi surface can be ubiquitous and need to be considered in understanding the temperature-dependent carrier density and magnetoresistance anisotropy in semimetals.

cond-mat.mtrl-sci↗

arXiv2022

Coherent coupling of two remote magnonic resonators mediated by superconducting circuits

We demonstrate microwave-mediated distant magnon-magnon coupling on a superconducting circuit platform, incorporating chip-mounted single-crystal Y$_3$Fe$_5$O$_{12}$ (YIG) spheres. Coherent level repulsion and dissipative level attraction between the magnon modes of the two YIG spheres are demonstrated. The former is mediated by cavity photons of a superconducting resonator, and the latter is mediated by propagating photons of a coplanar waveguide. Our results open new avenues towards exploring integrated hybrid magnonic networks for coherent information processing on a quantum-compatible superconducting platform.

cond-mat.mes-hall↗

arXiv2021

Devices for Thermal Conductivity Measurements of Electroplated Bi for X-ray TES Absorbers

Electroplated Bismuth (Bi) is commonly used in Transition-Edge Sensors (TESs) for X-rays because of its high stopping power and low heat capacity. Electroplated Bi is usually grown on top of another metal that acts as seed layer, typically gold (Au), making it challenging to extrapolate its thermoelectric properties. In this work, we present four-wire resistance measurement structures that allow us to measure resistance as a function of temperature of electroplated Bi independently of Au. The results show that the thermal conductivity of the Bi at 3 K is high enough to guarantee the correct thermalization of X-ray photons when used as an absorber for TESs.

physics.ins-det↗

arXiv2021

Phase-resolved electrical detection of coherently coupled magnonic devices

We demonstrate the electrical detection of magnon-magnon hybrid dynamics in yttrium iron garnet/permalloy (YIG/Py) thin film bilayer devices. Direct microwave current injection through the conductive Py layer excites the hybrid dynamics consisting of the uniform mode of Py and the first standing spin wave ($n=1$) mode of YIG, which are coupled via interfacial exchange. Both the two hybrid modes, with Py or YIG dominated excitations, can be detected via the spin rectification signals from the conductive Py layer, providing phase resolution of the coupled dynamics. The phase characterization is also applied to a nonlocally excited Py device, revealing the additional phase shift due to the perpendicular Oersted field. Our results provide a device platform for exploring hybrid magnonic dynamics and probing their phases, which are crucial for implementing coherent information processing with magnon excitations

cond-mat.mes-hall↗

arXiv2021

Superconducting diode effect via conformal-mapped nanoholes

A superconducting diode is an electronic device that conducts supercurrent and exhibits zero resistance primarily for one direction of applied current. Such a dissipationless diode is a desirable unit for constructing electronic circuits with ultralow power consumption. However, realizing a superconducting diode is fundamentally and technologically challenging, as it usually requires a material structure without a centre of inversion, which is scarce among superconducting materials. Here, we demonstrate a superconducting diode achieved in a conventional superconducting film patterned with a conformal array of nanoscale holes, which breaks the spatial inversion symmetry. We showcase the superconducting diode effect through switchable and reversible rectification signals, which can be three orders of magnitude larger than that from a flux-quantum diode. The introduction of conformal potential landscapes for creating a superconducting diode is thereby proven as a convenient, tunable, yet vastly advantageous tool for superconducting electronics. This could be readily applicable to any superconducting materials, including cuprates and iron-based superconductors that have higher transition temperatures and are desirable in device applications.

cond-mat.supr-con↗

arXiv2021

Non-Ohmic negative longitudinal magnetoresistance in two-dimensional electron gas

Negative longitudinal magnetoresistance (NLMR) has been reported in a variety of materials and has attracted extensive attention as an electrotransport hallmark of topological Weyl semimetals. However, its origin is still under debate. Here, we demonstrate that the NLMR in a two dimensional electron gas can be influenced by the measurement current. While the NLMR persists up to 130 K, its magnitude and magnetic field response become dependent on the applied current below 60 K. The tunable NLMR at low and high currents can be best attributed to quantum interference and disorder scattering effects, respectively. This work uncovers non-Ohmic NLMR in a non-Weyl material and highlights potential effects of the measurement current in elucidating electrotransport phenomena. We also demonstrate that NLMRs can be a valuable phenomenon in revealing the origins of other properties, such as negative MRs in perpendicular magnetic fields.

cond-mat.mtrl-sci↗

arXiv2020

Reconfigurable pinwheel artificial-spin-ice and superconductor hybrid device

The ability to control the potential landscape in a medium of interacting particles could lead to intriguing collective behavior and innovative functionalities. Here, we utilize spatially reconfigurable magnetic potentials of a pinwheel artificial spin ice structure to tailor the motion of superconducting vortices. The reconstituted chain structures of the magnetic charges in the artificial pinwheel spin ice and the strong interaction between magnetic charges and superconducting vortices allow significant modification of the transport properties of the underlying superconducting thin film, resulting in a reprogrammable resistance state that enables a reversible and switchable vortex Hall effect. Our results highlight an effective and simple method of using artificial spin ice as an in-situ reconfigurable nanoscale energy landscape to design reprogrammable superconducting electronics, which could also be applied to the in-situ control of properties and functionalities in other magnetic particle systems, such as magnetic skyrmions.

cond-mat.supr-con↗

arXiv2020

Direct Imaging of Resonant Phonon-Magnon Coupling

Direct detection of phonons is important for the investigation of information interconversion between the resonantly coupled magnons and phonons. Here we report resonant coupling of magnons and phonons, which can be directly visualized by using micro focused Brillouin light scattering in Ni/LiNbO3 hybrid heterostructures. The patterns of surface acoustic wave phonons, originating from the interference between the original wave ψ0(A_0,k) and reflected wave ψ1(A_1,-k), can be modulated by magnetic field due to the magnon-phonon coupling. By analyzing the information of phonons obtained from Brillouin spectroscopy, the properties of the magnon system (Ni film), e.g., ferromagnetic resonance field and resonance linewidth can be determined. The results provide spatially resolved information about phonon manipulation and detection in a coupled magnon-phonon system.

physics.app-ph↗

arXiv2019

Magnetic damping modulation in $IrMn_{3}/Ni_{80}Fe_{20}$ via the magnetic spin Hall effect

Non-collinear antiferromagnets can have additional spin Hall effects due to the net chirality of their magnetic spin structure, which provides for more complex spin-transport phenomena compared to ordinary non-magnetic materials. Here we investigated how ferromagnetic resonance of permalloy ($Ni_{80}Fe_{20}$) is modulated by spin Hall effects in adjacent epitaxial $IrMn_{3}$ films. We observe a large dc modulation of the ferromagnetic resonance linewidth for currents applied along the [001] $IrMn_{3}$ direction. This very strong angular dependence of spin-orbit torques from dc currents through the bilayers can be explained by the magnetic spin Hall effect where $IrMn_{3}$ provides novel pathways for modulating magnetization dynamics electrically.

cond-mat.mtrl-sci↗