arXiv subjects

Ramon Aguado

Publications and source records attributed to Ramon Aguado.

At least 19 recordsLinked to original sources

arXiv2026

Granular aluminum induced superconductivity in germanium for hole spin-based hybrid devices

In superconductor-semiconductor hybrid structures, superconductivity and spin polarization are competing effects as magnetic fields break Cooper pairs. They can be combined using thin films and in-plane magnetic fields, an approach that enabled the pursuit of Majorana zero modes, Kitaev chains, and Andreev spin qubits (ASQs), but remains challenging for materials with small in-plane $g$-factors or when out-of-plane fields are required. We demonstrate that granular aluminium (grAl), composed of nanometre-scale aluminium grains embedded in an amorphous oxide matrix, can overcome this limitation. By depositing grAl on Ge/SiGe heterostructures, we induce a hard superconducting gap with BCS peaks at $305~\mu\mathrm{eV}$ and magnetic-field resilience for both the in-plane and out-of-plane directions, allowing Zeeman splitting of Yu-Shiba-Rusinov (YSR) states beyond $50~\mu\mathrm{eV}$ (12 GHz). Leveraging this robustness, we reveal signatures of hole physics and discuss a driving mechanism for ASQs regardless of the strength of the Rashba spin-orbit coupling in planar germanium.

cond-mat.mes-hall↗

arXiv2025

Coherent subgap transport in spin-split Josephson junctions

We report the first experimental observation of subgap transport in ferromagnetic insulator/superconductor/insulator/superconductor junctions realized in EuS/Al/AlOx/Al vertical stacks. Differential conductance measurements reveal multiple Andreev reflection peaks, with odd-order peaks split by the spin-splitting induced in the superconductor adjacent to EuS, while even-order peaks remain unaffected. Combining experiments with quasiclassical transport modeling, we extract the spin-splitting and the distribution of transmission channels, finding that a significant fraction ($\sim 23\%$) of highly transparent channels ($\tau \approx 0.9$) dominates transport. The observation of a Josephson current further confirms strong superconducting coupling through these channels. Our results demonstrate that a single spin-split superconductor is sufficient to observe the even-odd MAR effect. Our work establishes EuS/Al junctions as a versatile platform to study subgap transport, Josephson coupling, and spin-polarized superconducting phenomena.

cond-mat.supr-con↗

arXiv2025

Flux-tunable parity-protected qubit based on a single full-shell nanowire Josephson junction

Leveraging the higher harmonics content of the Josephson potential in a superconducting circuit offers a promising route in the search for new qubits with increased protection against decoherence. In this work, we demonstrate how the flux tunability of a hybrid semiconductor-superconductor Josephson junction based on a single full-shell nanowire enables this possibility. Near one flux quantum, $\Phi\approx \Phi_0=h/2e$, we find that the qubit system can be tuned from a gatemon regime to a parity-protected regime with qubit eigenstates localized in phase space in the $0$ and $\pi$ minima of the Josephson potential ($\cos 2\varphi_0$). Estimates of qubit coherence and relaxation times due to different noise sources are presented.

cond-mat.mes-hall↗

arXiv2022

Majorana-like Coulomb spectroscopy in the absence of zero bias peaks

Hybrid semiconductor-superconductor devices hold great promise for realizing topological quantum computing with Majorana zero modes (MZMs). However, multiple claims of Majorana detection, based on either tunneling or Coulomb blockade (CB) spectroscopy, remain disputed. Here we devise an experimental protocol that allows to perform both types of measurements on the same hybrid island by adjusting its charging energy via tunable junctions to the normal leads. This method reduces ambiguities of Majorana detections by checking the consistency between CB spectroscopy and zero bias peaks (ZBPs) in non-blockaded transport.Specifically, we observe junction-dependent, even-odd modulated, single-electron CB peaks in InAs/Al hybrid nanowires (NWs) without concomitant low-bias peaks in tunneling spectroscopy. We provide a theoretical interpretation of the experimental observations in terms of low-energy, longitudinally-confined island states rather than overlapping Majorana modes. Our results highlight the importance of combined measurements on the same device for the identification of topological MZMs.

cond-mat.mes-hall↗

arXiv2017

Dynamic current susceptibility as a probe of Majorana bound states in nanowire-based Josephson junctions

We theoretically study a Josephson junction based on a semiconducting nanowire subject to a time-dependent flux bias. We establish a general density matrix approach for the dynamical response of the Majorana junction and calculate the resulting flux-dependent susceptibility using both microscopic and effective low-energy descriptions for the nanowire. We find that the diagonal component of the susceptibility, associated with the dynamics of the Majorana states populations, dominates over the standard Kubo contribution for a wide range of experimentally relevant parameters. The diagonal term, thus far unexplored in the context of Majorana physics, allows to probe accurately the presence of Majorana bound states in the junction.

cond-mat.mes-hall↗

arXiv2017

Proximity-induced Shiba states in a molecular junction

Superconductors containing magnetic impurities exhibit intriguing phenomena derived from the competition between Cooper pairing and Kondo screening. At the heart of this competition are the Yu-Shiba-Rusinov (Shiba) states which arise from the pair breaking effects a magnetic impurity has on a superconducting host. Hybrid superconductor-molecular junctions offer unique access to these states but the added complexity in fabricating such devices has kept their exploration to a minimum. Here, we report on the successful integration of a model spin 1/2 impurity, in the form of a neutral and stable all organic radical molecule, in proximity-induced superconducting break-junctions. Our measurements reveal excitations which are characteristic of a spin-induced Shiba state due to the radical's unpaired spin strongly coupled to a superconductor. By virtue of a variable molecule-electrode coupling, we access both the singlet and doublet ground states of the hybrid system which give rise to the doublet and singlet Shiba excited states, respectively. Our results show that Shiba states are a robust feature of the interaction between a paramagnetic impurity and a proximity-induced superconductor where the excited state is mediated by correlated electron-hole (Andreev) pairs instead of Cooper pairs.

cond-mat.mes-hall↗

arXiv2016

Scaling of sub-gap excitations in a superconductor-semiconductor nanowire quantum dot

A quantum dot coupled to a superconducting contact provides a tunable artificial analogue of a magnetic atom in a superconductor, a paradigmatic quantum impurity problem. We realize such a system with an InAs semiconductor nanowire contacted by an Al-based superconducting electrode. We use an additional normal-type contact as weakly coupled tunnel probe to perform tunneling spectroscopy measurements of the elementary sub-gap excitations, known as Andreev bound states or Yu-Shiba-Rusinov states. We demonstrate that the energy of these states, $ζ$, scales with the ratio between the Kondo temperature, $T_K$, and the superconducting gap, $Δ$. $ζ$ vanishes for $T_K/Δ\approx 0.6$, denoting a quantum phase transition between spin singlet and doublet ground states. By further leveraging the gate control over the quantum dot parameters, we determine the singlet-doublet phase boundary in the stability diagram of the system. Our experimental results show remarkable quantitative agreement with numerical renormalization group calculations.

cond-mat.mes-hall↗

arXiv2015

Shiba states and zero-bias anomalies in the hybrid normal-superconductor Anderson model

We determine the phase diagram of an Anderson impurity in contact with superconducting and normal-state leads for arbitrary ratio of the gap $Δ$ to the Kondo temperature $T_K$. We observe a considerable effect of even very weak coupling to the normal lead that is usually considered as a non-perturbing tunneling probe. The numerical renormalization group results are analyzed in the context of relevant experimental scenarios such as parity crossing (doublet-singlet) quantum phase transitions induced by a gap reduction as well as novel Kondo features induced by the normal lead. We point out the important role of finite temperatures and magnetic fields. Overall, we find a very rich behavior of spectral functions with zero-bias anomalies which can emerge irrespective of whether the ground state is a doublet or a singlet. Our findings are pertinent to the tunnelling-spectroscopy experiments aiming at detecting Majorana modes in nanowires.

cond-mat.mes-hall↗

arXiv2014

Spin-resolved Andreev levels and parity crossings in hybrid superconductor-semiconductor nanostructures

The hybrid combination of superconductors and low-dimensional semiconductors offers a versatile ground for novel device concepts, such as sources of spin-entangled electrons, nanoscale superconducting magnetometers, or recently proposed qubits based on topologically protected Majorana fermions. The underlying physics behind such hybrid devices ultimately rely on the magnetic properties of sub-gap excitations, known as Andreev levels. Here we report the Zeeman effect on the Andreev levels of a semiconductor nanowire quantum dot (QD) strongly coupled to a conventional superconductor. The combination of the large QD g-factor with the large superconductor critical magnetic field allows spin degeneracy to be lifted without suppressing superconductivity. We show that a Zeeman-split Andreev level crossing the Fermi energy signals a quantum phase transition in the ground state of the superconductivity-induced QD, denoting a change in the fermionic parity of the system. This transition manifests itself as a zero-bias conductance anomaly appearing at a finite magnetic field, with properties that resemble those expected for Majorana fermions in a topological superconductor. Although the herein reported zero-bias anomalies do not hold any relation with topological superconductivity, the observed parity transitions can be regarded as precursors of Majorana modes in the long-wire limit.

cond-mat.mes-hall↗

arXiv2012

Transport spectroscopy of NS nanowire junctions with Majorana fermions

We investigate transport though normal-superconductor nanowire junctions in the presence of spin-orbit coupling and magnetic field. As the Zeeman field crosses the critical bulk value B_c of the topological transition, a Majorana bound state (MBS) is formed, giving rise to a sharp zero-bias anomaly (ZBA) in the tunneling differential conductance. We identify novel features beyond this picture in wires with inhomogeneous depletion, like the appearance of two MBSs inside a long depleted region for B<B_c. The resulting ZBA is in most cases weakly split and may coexist with Andreev bound states near zero energy. The ZBA may appear without evidence of a topological gap closing. This latter aspect is more evident in the multiband case and stems from a smooth pinch-off barrier. Most of these features are in qualitative agreement with recent experiments [Mourik et al, Science 336, 1003 (2012)]. We also discuss the rich phenomenology of the problem in other regimes which remain experimentally unexplored.

cond-mat.mes-hall↗

arXiv2012

Magnetic-field instability of Majorana modes in multiband quantum wires

We investigate the occurrence of Majorana modes in semiconductor quantum wires in close proximity with a superconductor and when both, Rashba interaction and magnetic field, are present. We consider long, but finite, multiband wires (namely, planar wires with dimensions $L_x\gg L_y$). Our results demonstrate that interband mixing coming from Rashba spin orbit term hybridizes Majorana pairs originating from different transverse modes while simultaneously closing the effective gap. Consequently, multiple Majorana modes do not coexist in general. On the contrary, Majorana physics is robust provided that only one single transverse mode contributes with a Majorana pair. Finally, we analyse the robustness of Majorana physics with respect to magnetic orbital effects.

cond-mat.mes-hall↗

arXiv2012

Zero-bias anomaly in a nanowire quantum dot coupled to superconductors

We studied the low-energy states of spin-1/2 quantum dots defined in InAs/InP nanowires and coupled to aluminium superconducting leads. By varying the superconducting gap, Δ, with a magnetic field, B, we investigated the transition from strong coupling, Δ<< T_{K}, to weak coupling, Δ>> T_{K}, where T_{K} is the Kondo temperature. Below the critical field, we observe a persisting zero-bias Kondo resonance that vanishes only for low B or higher temperatures, leaving the room to more robust sub-gap structures at bias voltages between Δand 2Δ. For strong and approximately symmetric tunnel couplings, a Josephson supercurrent is observed in addition to the Kondo peak. We ascribe the coexistence of a Kondo resonance and a superconducting gap to a significant density of intra-gap quasiparticle states, and the finite-bias sub-gap structures to tunneling through Shiba states. Our results, supported by numerical calculations, own relevance also in relation to tunnel-spectroscopy experiments aiming at the observation of Majorana fermions in hybrid nanostructures.

cond-mat.mes-hall↗

arXiv2012

AC Josephson effect in finite-length nanowire junctions with Majorana modes

It has been predicted that superconducting junctions made with topological nanowires hosting Majorana bound states (MBS) exhibit an anomalous 4π-periodic Josephson effect. Finding an experimental setup with these unconventional properties poses, however, a serious challenge: for finite-length wires, the equilibrium supercurrents are always 2π-periodic as anticrossings of states with the same fermionic parity are possible. We show, however, that the anomaly survives in the transient regime of the ac Josephson effect. Transients are moreover protected against decay by quasiparticle poisoning as a consequence of the quantum Zeno effect, which fixes the parity of Majorana qubits. The resulting long-lived ac Josephson transients may be effectively used to detect MBS.

cond-mat.mes-hall↗

arXiv2011

Quantum versus classical counting in nonMarkovian master equations

We discuss the description of full counting statistics in quantum transport with a nonMarkovian master equation. We focus on differences arising from whether charge is considered as a classical or a quantum degree of freedom. These differences manifest themselves in the inhomogeneous term of the master equation which describes initial correlations. We describe the influence on current and in particular, the finite-frequency shotnoise. We illustrate these ideas by studying transport through a quantum dot and give results that include both sequential and cotunneling processes. Importantly, the noise spectra derived from the classical description are essentially frequency-independent and all quantum noise effects are absent. These effects are fully recovered when charge is considered as a quantum degree of freedom.

cond-mat.mes-hall↗

arXiv2011

Josephson current in carbon nanotubes with spin-orbit interaction

We demonstrate that curvature-induced spin-orbit (SO) coupling induces a $0-π$ transition in the Josephson current through a carbon nanotube quantum dot coupled to superconducting leads. In the non-interacting regime, the transition can be tuned by applying parallel magnetic field near the critical field where orbital states become degenerate. Moreover, the interplay between charging and SO effects in the Coulomb Blockade and cotunneling regimes leads to a rich phase diagram with well-defined (analytical) boundaries in parameter space. Finally, the 0 phase always prevails in the Kondo regime. Our calculations are relevant in view of recent experimental advances in transport through ultra-clean carbon nanotubes.

cond-mat.mes-hall↗

arXiv2010

Josephson current in strongly correlated double quantum dots

We study the transport properties of a serial double quantum dot (DQD) coupled to two superconducting leads, focusing on the Josephson current through the DQD and the associated 0-$π$ transitions which result from the subtle interplay between the superconductivity, the Kondo physics, and the inter-dot superexchange interaction. We examine the competition between the superconductivity and the Kondo physics by tuning the relative strength $Δ/T_K$ of the superconducting gap $Δ$ and the Kondo temperature $T_K$, for different strengths of the superexchange coupling determined by the interdot tunneling $t$ relative to the dot level broadening $Γ$. We find strong renormalization of $t$, a significant role of the superexchange coupling $J$, and a rich phase diagram of the 0 and $π$-junction regimes. In particular, when both the superconductivity and the exchange interaction are in close competion with the Kondo physics ($Δ\sim J\sim T_K$), there appears an island of $π'$-phase at large values of the superconducting phase difference.

cond-mat.mes-hall↗

arXiv2009

The Two-impurity Anderson Model Revisited: Competition between Kondo Effect and Reservoir-mediated Superexchange in Double Quantum Dots

We study a series-coupled double quantum dot in the Kondo regime modeled by the two-impurity Anderson model and find a new conduction-band mediated superexchange interaction that competes with Kondo physics in the strong Coulomb interaction limit. Our numerical renormalization group results, complemented with the higher-order Rayleigh-Schrödinger perturbation theory, show that the novel exchange mechanism leads to clear experimental consequences that can be checked in transport measurements through double quantum dots.

cond-mat.mes-hall↗

arXiv2007

Mn-doped II-VI quantum dots: artificial molecular magnets

The notion of artifical atom relies on the capability to change the number of carriers one by one in semiconductor quantum dots, and the resulting changes in their electronic structure. Organic molecules with transition metal atoms that have a net magnetic moment and display hysteretic behaviour are known as single molecule magnets (SMM). The fabrication of CdTe quantum dots chemically doped with a controlled number of Mn atoms and with a number of carriers controlled either electrically or optically paves the way towards a new concept in nanomagnetism: the artificial single molecule magnet. Here we study the magnetic properties of a Mn-doped CdTe quantum dot for different charge states and show to what extent they behave like a single molecule magnet.

cond-mat.mes-hall↗