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Ran Holtzman

Publications and source records attributed to Ran Holtzman.

14 recordsLinked to original sources

Dynamics of fluid-fluid displacements in a model rough fracture beyond the quasistatic limit: A spectral approach

In fluid-fluid displacements in porous and fractured materials, viscous friction in microscale interfacial (Haines) jumps is intimately linked to macroscale energy dissipation and the associated pressure-saturation (retention) hysteresis. The mode of control (flow rate vs. pressure) and the driving rate (from quasistatic to finite) can substantially affect hysteresis. Despite the significance of hysteresis and dissipation in various technological and natural processes, a quantitative understanding of the link between the micro- and macro-scales, and of the impact of the inherent heterogeneity of porous media, remains elusive. An ``imperfect'' Hele-Shaw cell of variable aperture is a simple model system which allows to study all these in details. However, simulating fluid-fluid interface evolution in heterogeneous media, even in such a simple system, is computationally prohibitive, as multiple length and time scales need to be resolved simultaneously. We develop here a spectral computational approach for interface evolution and energy dissipation and validate it via comparison to computational fluid dynamics simulations and experiments. Computational efficiency is demonstrated by following interface evolution in a cell with a single ``defect'', as well as with random roughness; in both, disparate length scales lead to nontrivial dynamics over many orders of magnitude in time. We also show theoretically that while viscous forces during Haines jumps fully account for the energy dissipated between consecutive metastable equilibria, viscosity does not change the total dissipated amount, merely the relaxation time. Our approach provides a stepping stone towards upscaling of fluid-fluid flows in porous media.

physics.flu-dyn

Numerical Investigation of the Effect of an Oblique Flow Entry on the Pressure Losses in Square Channels

Flows in square channels are common in applications, such as automotive after-treatment systems and heat exchangers. Flows with axial flow entry are well understood, but for oblique flow entry, there is no clarity on the additional pressure loss magnitude or the flow regime. Laminar flow is often assumed, even though flow separation at the channel entrance can cause a transition to turbulence. Here, the impact of oblique flow entry on the flow is investigated using LES (Large Eddy Simulation) and RANS (Reynolds Averaged Navier Stokes) models, and their advantages and limitations are identified. The LES simulations show that the shear layer at the channel entrance produces continuous shedding of eddies that persist downstream even at moderate channel Reynolds numbers (~2000). The predicted pressure losses mostly agree with experimental data. The differences observed for some parameters are attributed to the difficulty of accurately replicating the experimental geometry. It is shown that LES results are susceptible to the rounding of the leading edge (present in experiments). Including edge rounding improves the pressure predictions. RANS simulations predicted pressure losses within 5% of experimental values for most cases, apart from where transitional flow was observed (resulting in differences up to 40%). This study provides insights into the flow structure and sources of pressure losses in square channels and highlights the importance of understanding key flow and geometric features when using LES to predict complex flows involving flow separation and shear layers.

physics.flu-dyn

Emergence of dissipation and hysteresis from interactions among reversible, non-dissipative units: The case of fluid-fluid interfaces

We examine the nonequilibrium nature of two-phase fluid displacements in a quasi-two-dimensional medium (a model open fracture), in the presence of localized constrictions ("defects"), from a theoretical and numerical standpoint. Our analysis predicts the capillary energy dissipated in abrupt interfacial displacements (jumps) across defects, and relates it to the corresponding hysteresis cycle, e.g. in pressure-saturation. We distinguish between "weak" (reversible interface displacement, exhibiting no hysteresis and dissipation) and "strong" (irreversible) defects. We expose the emergence of dissipation and irreversibility caused by spatial interactions, mediated by interfacial tension, among otherwise weak defects. We exemplify this cooperative behavior for a pair of weak defects and establish a critical separation distance, analytically and numerically, verified by a proof-of-concept experiment.

physics.flu-dyn

Interplay of viscosity and wettability controls fluid displacement in porous media

Direct numerical simulations are used to elucidate the interplay of wettability and fluid viscosities on immiscible fluid displacements in a heterogeneous porous medium.We classify the flow regimes based using qualitative and quantitative analysis into viscous fingering (low $M$), compact displacement (high $M$), and an intermediate transition regime ($M \approx 1$). We use stability analysis to obtain theoretical phase boundaries between these regimes, which agree well with our analyses. At the macroscopic (sample) scale, we find that wettability strongly controls the threshold $M$ (at which the regimes change). At the pore scale, wettability alters the dominant pore-filling mechanism. At very small $M$ (viscous fingering regime), smaller pore spaces are preferentially invaded during imbibition, with flow of films of invading fluid along the pore walls. In contrast, during drainage, bursts result in filling of pores irrespective of their size. As $M$ increases, the effect of wettability decreases as cooperative filling becomes the dominant mechanism regardless of wettability. This suggest that for imbibition at a given contact angle, decreasing $M$ is associated with change in effective wetting from neutral-wet (cooperative filling) to strong-wet (film flow).

physics.flu-dyn

Onset of convective instability in an inclined porous medium

The diffusion of a solute from a concentrated source into a horizontal, stationary, fluid-saturated porous medium can lead to a convective motion when a gravitationally unstable density stratification evolves. In an inclined porous medium, the convective flow becomes intricate as it originates from a combination of diffusion and lateral flow, which is dominant near the source of the solute. Here, we investigate the role of inclination on the onset of convective instability by linear stability analyses of Darcy's law and mass conservation for the flow and the concentration field. We find that the onset time increases with the angle of inclination ($θ$) until it reaches a cut-off angle beyond which the system remains stable. The cut-off angle increases with the Rayleigh number, $Ra$. The evolving wavenumber at the onset exhibits a lateral velocity that depends non-monotonically on $θ$ and linearly on $Ra$. Instabilities are observed in gravitationally stable configurations ($θ\geq 90^{\circ}$) solely due to the non-uniform base flow generating a velocity shear commonly associated with Kelvin-Helmholtz instability. These results quantify the role of medium tilt on convective instabilities, which is of great importance to geological CO$_2$ sequestration.

physics.flu-dyn

Onset of transient convection in a porous medium with an embedded low-permeability layer

Deep saline aquifers used for CO$_2$ sequestration are commonly made of sedimentary formations consisting of several layers of distinguishable permeability. In this work, the effect of a non-monotonic, vertically varying permeability profile on the onset of convective instability is studied theoretically using linear stability analyses. The onset time depends on the interaction between the permeability profile and the location of the concentration perturbation peak beyond which the concentration of CO$_2$ decays. A thin low-permeability layer can either accelerate or delay the onset time of the convective instability depending on the nature of the permeability variation - whether the permeability transition is smooth or layered, the Rayleigh number (Ra), and the location of the permeability change ($\hat{a}$) relative to the perturbation peak ($\hat{a}_{c^{*}}$), which scales as $\hat{a}_{c^{*}}\approx 14Ra^{-1}$ for homogeneous systems. However, the low permeable layer has no effect on the onset time when it is near the lower boundary of a medium with sufficiently large Ra ($\hat{a}_{c^{*}} \ll \hat{a}$). This nontrivial dependence highlights the implication of ignoring geological features of a small spatial extent, indicating the importance of a detailed characterization of CO$_2$ storage sites.

physics.flu-dyn

Immiscible fluid displacement in porous media with spatially correlated particle sizes

Immiscible fluid displacement in porous media is fundamental for many environmental processes, including infiltration of water in soils, groundwater remediation, enhanced recovery of hydrocarbons and carbon geosequestration. Microstructural heterogeneity, in particular of particle sizes, can significantly impact immiscible displacement. For instance, it may lead to unstable flow and preferential displacement patterns. We present a systematic, quantitative pore-scale study of the impact of spatial correlations in particle sizes on the drainage of a partially-wetting fluid. We perform pore-network simulations with varying flow rates and different degrees of spatial correlation, complemented with microfluidic experiments. Simulated and experimental displacement patterns show that spatial correlation leads to more preferential invasion, with reduced trapping of the defending fluid, especially at low flow rates. Numerically, we find that increasing the correlation length reduces the fluid-fluid interfacial area and the trapping of the defending fluid, and increases the invasion pattern asymmetry and selectivity. Our experiments, conducted for low capillary numbers, support these findings. Our results delineate the significant effect of spatial correlations on fluid displacement in porous media, of relevance to a wide range of natural and engineered processes.

physics.flu-dyn

Drying and percolation in spatially correlated porous media

We study how the dynamics of a drying front propagating through a porous medium are affected by small-scale correlations in material properties. For this, we first present drying experiments in micro-fluidic micro-models of porous media. Here, the fluid pressures develop more intermittent dynamics as local correlations are added to the structure of the pore spaces. We also consider this problem numerically, using a model of invasion percolation with trapping, and find that there is a crossover in invasion behaviour associated with the length-scale of the disorder in the system. The critical exponents associated with large enough events are similar to the classic invasion percolation problem, whereas the addition of a finite correlation length significantly affects the exponent values of avalanches and bursts, up to some characteristic size. This implies that the even a weak local structure can interfere with the universality of invasion percolation phenomena.

cond-mat.soft

The Effect of Gravitational Settling on Concentration Profiles and Dispersion Within and Above Fractured Media

The transport of heavy particles in a medium that consists of fluid and solid phases such as stream gravel beds, cracked soils and wetlands is affected by processes such as attachment-detachment, gravity and drag, and by mixing processes that are induced by Taylor dispersion and mechanical dispersion. This paper addresses an additional dispersion mechanism which is induced by gravitational settling and is a result of the coupling between the modified particle concentration (the change of particle number density due to settling) and the lateral velocity profiles at the subscale. Heavy particles that move in areas of low horizontal velocity (e.g., near solid surfaces and wake regions) settle closer to the release source as compared to particles in high velocity regions. The macroscopic concentration field of such suspensions is influenced by the ratio between the settling velocity and the subscale distribution of the horizontal velocities. The objective of the study is to isolate and quantify this type of dispersion using controlled flow scenarios. We used a Taylor brush geometry (an array of vertical grooves) to numerically solve the flow. Particles were released from a vertical plane, generating a constant flux. The subscale Eulerian concentration was compiled from simulated trajectories and then spatially averaged to generate macroscopic concentration fields. The results show that this settling-induced dispersion is significant in regions near the source and that it cannot be modeled using Fick's law type of formulations. A parametric investigation shows that the location of the highest dispersion flux is linearly proportional to both the groove spacing and depth. A proposed model that estimates this location is used to evaluate where settling-induced dispersion should not be ignored.

physics.flu-dyn

Reactive transport under stress: Permeability evolution in deformable porous media

We study reactive transport in a stressed porous media, where dissolution of the solid matrix causes two simultaneous, competing effects: pore enlargement (chemical deformation), and pore compaction due to mechanical weakening. A novel, mechanistic pore-scale model simulates flooding of a sample under fixed confining stress, showing that increasing stress inhibits permeability enhancement, increasing the injected volume required to reach a certain permeability, in agreement with recent experiments. We explain this behavior by stress concentration downstream, in the less dissolved (hence stiffer) region. As this region is also less conductive, even its small compaction has a strong bottleneck effect that curbs the permeability. Our results also elucidate that the impact of stress depends on the dissolution regime. Under wormholing conditions (slow injection, i.e. high Damkohler, $Da$), the development of a sharp dissolution front and high porosity contrast accentuates the bottleneck effect. This reduces transport heterogeneity, promoting wormhole competition. Once the outlet starts eroding, the extreme focusing of transport and hence dissolution--characteristic of wormholing--becomes dominant, diminishing the bottleneck effect and hence the impact of stress. In contrast, at low $Da$, incomplete reaction upstream allows the reagent to traverse the sample, causing a more uniform dissolution. The continuous dissolution and its partial counteraction by compaction downstream provides a steady, gradual increase in the effect of stress. Consequently, the impact of stress is more pronounced at high $Da$ during early stages (low permeability), and at low $Da$ close to breakthrough. Our work promotes understanding of the hydromechanical property evolution, with important implications for processes ranging from diagenesis and weathering of rocks, to well stimulation and carbon geosequetration.

physics.flu-dyn

Impact of spatially correlated pore-scale heterogeneity on drying porous media

We study the effect of spatially-correlated heterogeneity on isothermal drying of porous media. We combine a minimal pore-scale model with microfluidic experiments with the same pore geometry. Our simulated drying behavior compare favorably with experiments, considering the large sensitivity of the emergent behavior to the uncertainty associated with even small manufacturing errors. We show that increasing the correlation length in particle sizes promotes preferential drying of clusters of large pores, prolonging liquid connectivity and surface wetness and thus higher drying rates for longer periods. Our findings improve our quantitative understanding of how pore-scale heterogeneity impacts drying, which plays a role in a wide range of processes ranging from fuel cells to curing of paints and cements to global budgets of energy, water and solutes in soils.

physics.flu-dyn

Validating pore-scale models of drying using microfluidic experiments

We present an experimental micro-model of drying porous media, based on microfluidic cells made of arrays of pillars on a regular grid, and complement these experiments with a matching two-dimensional pore-network model of drying. Disorder, or small-scale heterogeneity, was introduced into the cells by randomly varying the radii of the pillars, around their average value. The microfluidic chips were filled with a volatile oil and then dried horizontally, such that gravitational effects were excluded. The experimental and simulated drying rates and drying patterns were then compared in detail, for various levels of disorder, in order to verify the predictive capabilities of our model. The geometrical features were reproduced well, while reproducing drying rates proved to be more challenging.

physics.flu-dyn

Effects of Pore-Scale Disorder on Fluid Displacement in Partially-Wettable Porous Media

We present a systematic, quantitative assessment of the impact of pore size disorder and its interplay with flow rates and wettability on immiscible displacement of a viscous fluid. Pore-scale simulations and micromodel experiments show that reducing disorder increases the displacement efficiency and compactness, minimizing the fluid-fluid interfacial area, through (i) trapping at low rates and (ii) viscous fingering at high rates. Increasing the wetting angle suppresses both trapping and fingering, hence reducing the sensitivity of the displacement to the underlying disorder. A modified capillary number $\mathrm{Ca^*}$ that includes the impact of disorder $λ$ on viscous forces (through pore connectivity) is direct related to $λ$, in par with previous works. Our findings bear important consequences on sweep efficiency and fluid mixing and reactions, which are key in applications such as microfluidics to carbon geosequestration, energy recovery, and soil aeration and remediation.

physics.flu-dyn

Wettability stabilizes fluid invasion into porous media via nonlocal, cooperative pore filling

We study the impact of the wetting properties on the immiscible displacement of a viscous fluid in disordered porous media. We present a novel pore-scale model that captures wettability and dynamic effects, including the spatiotemporal nonlocality associated with interface readjustments. Our simulations show that increasing the wettability of the invading fluid (the contact angle) promotes cooperative pore filling that stabilizes the invasion, and that this effect is suppressed as the flow rate increases, due to viscous instabilities. We use scaling analysis to derive two dimensionless numbers that predict the mode of displacement. By elucidating the underlying mechanisms, we explain classical yet intriguing experimental observations. These insights could be used to improve technologies such as hydraulic fracturing, CO$_{2}$ geo-sequestration, and microfluidics.

physics.flu-dyn