arXiv subjects

Randy K. Dumas

Publications and source records attributed to Randy K. Dumas.

16 recordsLinked to original sources

arXiv2026

Self-thermometry measurements of the adiabatic temperature change in first-order phase transition magnetocaloric materials

Accurately measuring the magnetocaloric effect is necessary to foster the development of magnetic refrigeration devices. However, current methods are inconvenient, requiring different instruments to measure each individual property or a custom-made setup. By measuring the time-varying magnetization in a commercially available VersaLab\textsuperscript{\textregistered} PPMS\textsuperscript{\textregistered} from Quantum Design, we have determined the adiabatic temperature change ($Δ$T$_{\textrm{ad}}$) of the first-order phase transition material Gd$_5$Si$_2$Ge$_2$, for a magnetic field change of 0 to 1 T, under high vacuum ($<$ 0.1 mTorr). For each temperature and magnetic field, the equilibrium magnetization is used as the magnetization-to-temperature conversion curve, allowing us to extend the validity of a previously proposed technique to the first-order phase transition material Gd$_5$Si$_2$Ge$_2$, which exhibits significant hysteresis. Our method thus enables full characterization (magnetic entropy change, adiabatic temperature change, and heat capacity) of any magnetocaloric material, whether it has a first-order or a second-order phase transition, using a single instrument. Comparing to a directly measured $Δ$T$_{\textrm{ad}}$, our method resulted in a peak $Δ$T$_{\textrm{ad}}$ value of 4.47 K, within 1\% of the directly measured value for a sample of the same composition.

cond-mat.mtrl-sci↗

arXiv2021

Spin diffusion length associated to out-of-plane resistivity of Pt thin films in spin pumping experiments

We present a broadband ferromagnetic resonance study of the Gilbert damping enhancement ($Δα$) due to spin pumping in NiFe/Pt bilayers. The bilayers, which have negligible interfacial spin memory loss, are studied as a function of the Pt layer thickness ($t_{\text{Pt}}$) and temperature (100-293 K). Within the framework of diffusive spin pumping theory, we demonstrate that Dyakonov-Perel (DP) or Elliot-Yaffet (EY) spin relaxation mechanisms acting alone are incompatible with our observations. In contrast, if we consider that the relation between spin relaxation characteristic time ($τ_{\text{s}}$) and momentum relaxation characteristic time ($τ_{\text{p}}$) is determined by a superposition of DP and EY mechanisms, the qualitative and quantitative agreement with experimental results is excellent. Remarkably, we found that $τ_{\text{p}}$ must be determined by the out-of-plane electrical resistivity ($ρ$) of the Pt film and hence its spin diffusion length ($λ_{\text{Pt}}$) is independent of $t_{\text{Pt}}$. Our work settles the controversy regarding the $t_{\text{Pt}}$ dependence of $λ_{\text{Pt}}$ by demonstrating its fundamental connection with $ρ$ considered along the same direction of spin current flow. \end{abstract}

cond-mat.mes-hall↗

arXiv2020

Reconstructing phase-resolved hysteresis loops from first-order reversal curves

The first order reversal curve (FORC) method is a magnetometry based technique used to capture nanoscale magnetic phase separation and interactions with macroscopic measurements using minor hysteresis loop analysis. This makes the FORC technique a powerful tool in the analysis of complex systems which cannot be effectively probed using localized techniques. However, recovering quantitative details about the identified phases which can be compared to traditionally measured metrics remains an enigmatic challenge. We demonstrate a technique to reconstruct phase-resolved magnetic hysteresis loops by selectively integrating the measured FORC distribution. From these minor loops, the traditional metrics - including the coercivity and saturation field, and the remanent and saturation magnetization - can be determined. In order to perform this analysis, special consideration must be paid to the accurate quantitative management of the so-called reversible features. This technique is demonstrated on three representative materials systems, high anisotropy FeCuPt thin-films, Fe nanodots, and SmCo/Fe exchange spring magnet films, and shows excellent agreement with the direct measured major loop, as well as the phase separated loops.

cond-mat.mtrl-sci↗

arXiv2015

Spin-Torque and Spin-Hall Nano-Oscillators

This paper reviews the state of the art in spin-torque and spin Hall effect driven nano-oscillators. After a brief introduction to the underlying physics, the authors discuss different implementations of these oscillators, their functional properties in terms of frequency range, output power, phase noise, and modulation rates, and their inherent propensity for mutual synchronization. Finally, the potential for these oscillators in a wide range of applications, from microwave signal sources and detectors to neuromorphic computation elements, is discussed together with the specific electronic circuitry that has so far been designed to harness this potential.

cond-mat.mes-hall↗

arXiv2015

Tunable damping, saturation magnetization, and exchange stiffness of half-Heusler NiMnSb thin films

The half-metallic half-Heusler alloy NiMnSb is a promising candidate for applications in spintronic devices due to its low magnetic damping and its rich anisotropies. Here we use ferromagnetic resonance (FMR) measurements and calculations from first principles to investigate how the composition of the epitaxially grown NiMnSb influences the magnetodynamic properties of saturation magnetization $M_S$, Gilbert damping $α$, and exchange stiffness $A$. $M_S$ and $A$ are shown to have a maximum for stoichiometric composition, while the Gilbert damping is minimum. We find excellent quantitative agreement between theory and experiment for $M_S$ and $α$. The calculated $A$ shows the same trend as the experimental data, but has a larger magnitude. Additionally to the unique in-plane anisotropy of the material, these tunabilities of the magnetodynamic properties can be taken advantage of when employing NiMnSb films in magnonic devices.

cond-mat.mtrl-sci↗

arXiv2014

Magnetoplasmonic design rules for active magneto-optics

Light polarization rotators and non-reciprocal optical isolators are essential building blocks in photonics technology. These macroscopic passive devices are commonly based on magneto-optical Faraday and Kerr polarization rotation. Magnetoplasmonics - the combination of magnetism and plasmonics - is a promising route to bring these devices to the nanoscale. We introduce design rules for highly tunable active magnetoplasmonic elements in which we can tailor the amplitude and sign of the Kerr response over a broad spectral range.

physics.optics↗

arXiv2014

Accessing Different Spin-Disordered States using First Order Reversal Curves

Combined first order reversal curve (FORC) analyses of the magnetization (M-FORC) and magnetoresistance (MR-FORC) have been employed to provide a comprehensive study of the M-MR correlation in two canonical systems: a NiFe/Cu/FePt pseudo spin-valve (PSV) and a [Co/Cu]8 multilayer. In the PSV, due to the large difference in switching fields and minimal interactions between the NiFe and FePt layers, the M and MR show a simple one-to-one relationship during reversal. In the [Co/Cu]8 multilayer, the correlation between the magnetization reversal and MR evolution is more complex. This is primarily due to the similar switching fields of, and interactions between, the constituent Co layers. The FORC protocol accesses states with much higher spin disorders and larger MR than those found along the conventional major loop field-cycle. Unlike the M-FORC measurements, which only probe changes in the macroscopic magnetization, the MR-FORCs are more sensitive to the microscopic domain configurations, as those are most important in determining the resultant MR effect size. This approach is generally applicable to spintronic systems to realize the maximum spin-disorder and the largest MR.

cond-mat.mtrl-sci↗

arXiv2014

Quantitative Decoding of Interactions in Tunable Nanomagnet Arrays Using First Order Reversal Curves

To develop a full understanding of interactions in nanomagnet arrays is a persistent challenge, critically impacting their technological acceptance. This paper reports the experimental, numerical and analytical investigation of interactions in arrays of Co nanoellipses using the first-order reversal curve (FORC) technique. A mean-field analysis has revealed the physical mechanisms giving rise to all of the observed features: a shift of the non-interacting FORC-ridge at the low-H$_c$ end off the local coercivity H$_c$ axis; a stretch of the FORC-ridge at the high-H$_c$ end without shifting it off the H$_c$ axis; and a formation of a tilted edge connected to the ridge at the low-H$_c$ end. Changing from flat to Gaussian coercivity distribution produces a negative feature, bends the ridge, and broadens the edge. Finally, nearest neighbor interactions segment the FORC-ridge. These results demonstrate that the FORC approach provides a comprehensive framework to qualitatively and quantitatively decode interactions in nanomagnet arrays.

cond-mat.mtrl-sci↗

arXiv2013

Confined dissipative droplet solitons in spin-valve nanowires with perpendicular magnetic anisotropy

Magnetic dissipative droplets are localized, strongly nonlinear dynamical modes excited in nano-contact spin valves with perpendicular magnetic anisotropy. These modes find potential application in nanoscale structures for magnetic storage and computation, but dissipative droplet studies have so far been limited to extended thin films. Here, numerical and asymptotic analyses are used to demonstrate the existence and properties of novel solitons in confined structures. As a nanowire's width is decreased with a nano-contact of fixed size at its center, the observed modes undergo transitions from a fully localized two-dimensional droplet into a two-dimensional droplet edge mode and then a pulsating one-dimensional droplet. These solitons are interpreted as dissipative versions of classical, conservative solitons, allowing for an analytical description of the modes and the mechanisms of bifurcation. The presented results open up new possibilities for the study of low-dimensional solitons and droplet applications in nanostructures.

cond-mat.mes-hall↗

arXiv2013

Spin wave mode coexistence on the nano-scale: A consequence of the Oersted field induced asymmetric energy landscape

It has been argued that if multiple spin wave modes are competing for the same centrally located energy source, as in a nanocontact spin torque oscillator, that only one mode should survive in the steady state. Here, the experimental conditions necessary for mode coexistence are explored. Mode coexistence is facilitated by the local field asymmetries induced by the spatially inhomogeneous Oersted field, which leads to a physical separation of the modes, and is further promoted by spin wave localization at reduced applied field angles. Finally, both simulation and experiment reveal a low frequency signal consistent with the intermodulation of two coexistent modes.

cond-mat.mes-hall↗

arXiv2012

Deconvoluting Reversal Modes in Exchange Biased Nanodots

Ensemble-averaged exchange bias in arrays of Fe/FeF2 nanodots has been deconvoluted into local, microscopic, bias separately experienced by nanodots going through different reversal modes. The relative fraction of dots in each mode can be modified by exchange bias. Single domain dots exhibit a simple loop shift, while vortex state dots have asymmetric shifts in the vortex nucleation and annihilation fields, manifesting local incomplete domain walls in these nanodots as magnetic vortices with tilted cores.

cond-mat.mtrl-sci↗

arXiv2011

Chirality control via double vortices in asymmetric Co dots

Reproducible control of the magnetic vortex state in nanomagnets is of critical importance. We report on chirality control by manipulating the size and/or thickness of asymmetric Co dots. Below a critical diameter and/or thickness, chirality control is achieved by the nucleation of single vortex. Interestingly, above these critical dimensions chirality control is realized by the nucleation and subsequent coalescence of two vortices, resulting in a single vortex with the opposite chirality as found in smaller dots. Micromagnetic simulations and magnetic force microscopy highlight the role of edge-bound halfvortices in facilitating the coalescence process.

cond-mat.mtrl-sci↗

arXiv2009

Angular Dependence of Vortex Annihilation Fields in Asymmetric Co Dots

Shape asymmetries in nominally circular nanomagnets provide a potential means for vortex chirality control. However, in realistic arrays their effects are challenging to probe since asymmetric magnetization reversal processes are often averaged to include distributions over all angles. Here we investigate how shape asymmetry influences the vortex reversal in arrays of sub-micron edge-cut Co dots. We find that the vortices can be manipulated to annihilate at particular sites under different field orientations and cycle sequences. The vortex annihilation field and degree of chirality control depend sensitively on the angular position of the applied field relative to the flat edge of the dots. For small angles, the major loop annihilation field is significantly larger than that found from the half loop and the vortex chirality can be well controlled. At intermediate angles the chirality control is lost and an interesting crossover in the annihilation field is found: the half loop actually extrudes outside of the major loop, exhibiting a larger vortex annihilation field. At large angles the annihilation fields along major and half loops become degenerate.

cond-mat.mtrl-sci↗

arXiv2009

Controlling magnetization reversal in Co/Pt nanostructures with perpendicular anisotropy

We demonstrate a simple method to tailor the magnetization reversal mechanisms of Co/Pt multilayers by depositing them onto large area nanoporous anodized alumina (AAO) with various aspect ratios, A = pore depth/diameter. Magnetization reversal of composite (Co/Pt)/AAO films with large A is governed by strong domain-wall pinning which gradually transforms into a rotation-dominated reversal for samples with smaller A, as investigated by a first-order reversal curve method in conjunction with analysis of the angular dependent switching fields. The change of the magnetization reversal mode is attributed to topographical changes induced by the aspect ratio of the AAO templates.

cond-mat.mtrl-sci↗

arXiv2009

Probing Magnetic Configurations in Co/Cu Multilayered Nanowires

Magnetic configurations in heterostructures are often difficult to probe when the magnetic entities are buried inside. In this study we have captured magnetic and magnetoresistance "fingerprints" of Co nanodiscs embedded in Co/Cu multilayered nanowires using a first-order reversal curve method. In 200nm diameter nanowires, the magnetic configurations can be tuned by adjusting the Co nanodisc aspect ratio. Nanowires with the thinnest Co nanodiscs exhibit single domain behavior, while those with thicker Co reverse via vortex states. A superposition of giant and anisotropic magnetoresistance is observed, which corresponds to the different magnetic configurations of the Co nanodiscs.

cond-mat.mtrl-sci↗

arXiv2007

Magnetic Fingerprints of sub-100 nm Fe Nanodots

Sub-100 nm nanomagnets not only are technologically important, but also exhibit complex magnetization reversal behaviors as their dimensions are comparable to typical magnetic domain wall widths. Here we capture magnetic "fingerprints" of 1 billion Fe nanodots as they undergo a single domain to vortex state transition, using a first-order reversal curve (FORC) method. As the nanodot size increases from 52 nm to 67 nm, the FORC diagrams reveal striking differences, despite only subtle changes in their major hysteresis loops. The 52 nm nanodots exhibit single domain behavior and the coercivity distribution extracted from the FORC distribution agrees well with a calculation based on the measured nanodot size distribution. The 58 and 67 nm nanodots exhibit vortex states, where the nucleation and annihilation of the vortices are manifested as butterfly-like features in the FORC distribution and confirmed by micromagnetic simulations. Furthermore, the FORC method gives quantitative measures of the magnetic phase fractions, and vortex nucleation and annihilation fields.

cond-mat.mtrl-sci↗