arXiv subjects

Randy Lemons

Publications and source records attributed to Randy Lemons.

15 recordsLinked to original sources

arXiv2026

Mutually phase-stable tunable attosecond soft X-ray attosecond pulses from a free-electron laser

We demonstrate the production of mutually phase-stable attosecond X-ray pulse pairs with tunable relative time delays and phases in a cascaded X-ray free-electron laser. We showcase the method in an experiment at the LCLS-II, in which a shaped electron beam is used in a split undulator configuration to generate the two attosecond pulses. We achieve mutual phase stability by reusing microbunching generated in the first undulator in order to seed the FEL process in the second at a detuned frequency. We measure controllable temporal delays between the two pulses directly in the time domain using angular streaking of photoelectrons, with a step size of 250 attoseconds. We then show that the behavior of the X-ray spectrum is consistent with phase stability between the two pulses, with a relative phase that can be easily tuned using inter-undulator phase shifters. This method is particularly well-suited to few to ten eV energy separations and sub to few femtosecond time delays, which are ideal for experiments in the soft X-ray regime for pushing the limits of our models for molecular dynamics and exerting direct coherent control over quantum systems.

physics.acc-ph↗

arXiv2026

Advanced Control of Electron Beams: Tailoring X-ray Production with Programmable Laser Shaping

Leveraging the full scientific capabilities of next-generation high-repetition-rate free-electron lasers requires programmable control over electron-beam properties at their source. The photoinjector drive laser defines the electron beam's initial six-dimensional phase-space distribution, yet has historically been limited to Gaussian or static flat-top profiles, with most manipulation occurring downstream. Here we demonstrate software-programmable ultraviolet pulse shaping at the LCLS-II photoinjector as a source-level actuator that complements traditional accelerator controls. Using a coupled architecture combining dispersion-controlled nonlinear frequency conversion with spatial-light-modulator spectral shaping, we generate user-defined temporal structures and observe their imprint on electron bunches through high-resolution time-domain diagnostics. Laser-imposed multi-peaked modulation persists through acceleration, magnetic compression, and undulator transport with shot-to-shot repeatability, producing clearly resolved current structure in the compressed beam. Variance-based reconstruction from transverse deflecting cavity measurements reveals structured X-ray emission profiles exhibiting temporal features consistent with the programmed laser waveform. By providing rapid, software-controlled reconfiguration of electron-beam initial conditions, this source-level control approach establishes a programmable upstream actuator for future adaptive optimization and autonomous facility operation at high-repetition-rate light sources.

physics.acc-ph↗

arXiv2026

Physics-Guided Inverse Design of Optical Waveforms for Nonlinear Electromagnetic Dynamics

Structured optical waveforms are emerging as powerful control fields for the next generation of complex photonic and electromagnetic systems, where the temporal structure of light can determine the ultimate performance of scientific instruments. However, identifying optimal optical drive fields in strongly nonlinear regimes remains challenging because the mapping between optical inputs and system response is high-dimensional and typically accessible only through computationally expensive simulations. Here, we present a physics-guided deep learning framework for the inverse design of optical temporal waveforms. By training a light-weighted surrogate model on simulations, the method enables gradient-based synthesis of optical profiles that compensate nonlinear field distortions in driven particle-field systems. As a representative application, we apply the approach to the generation of electron beams used in advanced photon and particle sources. The learned optical waveform actively suppresses extrinsic emittance growth by more than 52% compared with conventional Gaussian operation and by approximately 9% relative to the theoretical flattop limit in simulation. We further demonstrate experimental feasibility by synthesizing the predicted waveform using a programmable pulse-shaping platform; incorporating the measured optical profile into beamline simulations yields a 31% reduction in the extrinsic emittance contribution. Beyond accelerator applications, this work establishes a general way for physics-guided inverse design of optical control fields, enabling structured light to approach fundamental performance limits in nonlinear photonic and high-frequency electromagnetic systems.

physics.optics↗

arXiv2026

Upstream Laser-based Longitudinal Enhancement of Relativistic Photoelectrons

Controlling the longitudinal phase space of high-brightness relativistic electron beams is crucial for advancing a broad spectrum of charged-particle-based instrumentation and scientific frontiers. A generalized method for achieving this control involves manipulating the photoemission laser's temporal distribution at the picosecond level, a long-standing technical challenge. Recent developments in laser shaping have enabled the creation of high-power, picosecond-scale symmetrical and asymmetrical temporal profiles, capable of fine-tuning complex space-charge dynamics and external field effects in relativistic charged-particle beams. Here, we demonstrate that rather than deviations from theorized, idealized laser distributions, a controlled asymmetry can be harnessed to counteract accelerator-induced distortions. By implementing spatiotemporal shaping of the ultraviolet photocathode laser at the LCLS-II superconducting injector, we achieve deterministic control over the longitudinal phase space without downstream corrections. We find that this optical asymmetry induces a self-linearizing effect across both low (40 pC) and high (80 pC) charge regimes, effectively suppressing nonlinear compression and energy chirp. Consequently, this approach is expected to preserve a low emittance comparable to that of ideal flattop or regular Gaussian profiles, while delivering superior current uniformity and shot-to-shot stability. These results establish spatiotemporal laser shaping as a compact, generalizable tool for directly optimizing beam brightness at the source.

physics.optics↗

arXiv2025

Deep Learning Assisted Modeling for $\chi^{(2)}$ Nonlinear Optics

Modeling second-order ($\chi^{(2)}$) nonlinear optical processes remains computationally expensive due to the need to resolve fast field oscillations and simulate wave propagation using methods like the split-step Fourier method (SSFM). This can become a bottleneck in real-time applications, such as high-repetition-rate laser systems requiring rapid feedback and control. We present an LSTM-based surrogate model trained on SSFM simulations generated from a start-to-end model of the photocathode drive laser at SLAC National Accelerator Laboratory's Linac Coherent Light Source II. The model achieves over 250x speedup while maintaining high fidelity, enabling future real-time optimization and laying the foundation for data-integrated modeling frameworks and digital twins of laser systems.

physics.optics↗

arXiv2024

Nonlinear Shaping in the Picosecond Gap

Lightwave pulse shaping in the picosecond regime has remained unaddressed because it resides beyond the limits of state-of-the-art techniques, either due to its inherently narrow spectral content or fundamental speed limitations in electronic devices. The so-called picosecond shaping gap hampers progress in all areas correlated with time-modulated light-matter interactions, such as photoelectronics, health and medical technologies, and energy and material sciences. We report on a novel nonlinear method to simultaneously frequency-convert and adaptably shape the envelope of light wavepackets in the picosecond regime by balancing spectral engineering and nonlinear conversion in solid-state nonlinear media, without requiring active devices. We capture computationally the versatility of this methodology across a diverse set of nonlinear conversion chains and initial conditions. We also provide experimental evidence of this framework producing picosecond-shaped, ultra-narrowband, near-transform limited light pulses from broadband, femtosecond input pulses, paving the way toward programmable lightwave shaping at GHz-to-THz frequencies.

physics.optics↗

arXiv2024

Spectrotemporal shaping of attosecond x-ray pulses with a fresh-slice free-electron laser

We propose a scheme allowing coherent shaping, i.e., controlling both the amplitude and phase, of attosecond x-ray pulses at free-electron lasers. We show that by seeding an FEL with a short coherent seed that overfills the amplification bandwidth, one can shape the Wigner function of the pulse by controlling the undulator taper profile. The examples of controllable pulse pairs and trains, as well as isolated spectrotemporally shaped pulses with very broad bandwidths are examined in detail. Existing attosecond XFELs can achieve these experimental conditions in a two-stage cascade, in which the seed is generated by a short current spike in an electron bunch and shaped in an unspoiled region within the same bunch. We experimentally demonstrate the production and control of phase-stable pulse trains using this method at the Linac Coherent Light Source II.

physics.acc-ph↗

arXiv2023

The LCLS-II Photoinjector Laser Infrastructure

This paper presents a comprehensive technical overview of the Linac Coherent Light Source II (LCLS-II) photoinjector laser system, its first and foremost component. The LCLS-II photoinjector laser system serves as an upgrade to the original LCLS at SLAC National Accelerator Laboratory. This advanced laser system generates high-quality laser beams for LCLS-II, contributing to the instrument's unprecedented brightness, precision, and flexibility. Our discussion extends to the various subsystems that comprise the photoinjector, including the photocathode laser, laser heater, and beam transport systems. Lastly, we draw attention to the ongoing research and development infrastructure underway to enhance the functionality and efficiency of the LCLS-II, and similar X-ray free-electron laser facilities around the world, thereby contributing to the future of laser technology and its applications.

physics.acc-ph↗

arXiv2023

Nonlinearly Shaped Pulses in Photoinjectors and Free-Electron Lasers

Photoinjectors and Free Electron Lasers (FEL) are amongst the most advanced systems in accelerator physics and have consistently pushed the boundaries of emittance and x-ray peak power. In this paper, laser shaping at the cathode is proposed to further lower the emittance and reduce electron beam tails, which would result in brighter x-ray production. Using dispersion controlled nonlinear shaping (DCNS), laser pulses and beam dynamics were simulated in LCLS-II. The photoinjector emittance was optimized and the resulting e-beam profiles were then simulated and optimized in the linac. Finally, the expected FEL performance is estimated and compared to the current technology: Gaussian laser pulses on the cathode. The e-beams produced by DCNS pulses show a potential for 35% increase in x-ray power per pulse during SASE when compared to the standard Gaussian laser pulses.

physics.acc-ph↗

arXiv2022

Design, Optimization, and Blackbox Optimization of Laser Systems

Chirped pulse amplification (CPA) and subsequent nonlinear optical (NLO) systems constitute the backbone of myriad advancements in semiconductor and additive manufacturing, communication networks, biology and medicine, defense and national security, and a host of other sectors over the past decades. Accurately and efficiently modeling CPA and NLO-based laser systems is challenging because of the multitude of coupled linear and nonlinear processes and high variability in simulation frameworks. The lack of fully-integrated models severely hampers further advances in tailoring existing or materializing new CPA+NLO systems. Such tools are the key to enabling emerging optimization and inverse design approaches reliant on data-driven machine learning methods. Here, we present a modular start-to-end software model encompassing an array of amplifier designs and nonlinear optics techniques. The simulator renders time- and frequency-resolved electromagnetic fields alongside essential physical characteristics of energy, fluence, and spectral distribution. To demonstrate its robustness and real-world applicability -- specifically, reverse engineering, system optimization, and inverse design -- we present a case study on the LCLS-II photo-injector laser, representative of a high-power and spectro-temporally non-trivial CPA+NLO system.

physics.optics↗

arXiv2020

Temporal shaping of narrow-band picosecond pulses via non-colinear sum-frequency mixing of dispersion-controlled pulses

A long sought-after goal for photocathode electron sources has been to improve performance by temporally shaping the incident exitation laser pulse. The narrow bandwidth, short wavelength, and picosecond pulse duration make it challenging to employ conventional spectral pulse shaping techniques. We present a novel and efficient intensity-envelope shaping technique achieved during nonlinear upconversion through opposite-chirp sum-frequency mixing. We also present a numerical case-study of the LCLS-II photoinjector where transverse electron emittance is improved by at least 25%.

physics.optics↗

arXiv2020

Long-term Hybrid Stabilization of the Carrier-Envelope Phase

Controlling the carrier envelope phase (CEP) in mode-locked lasers over practically long timescales is crucial for real-world applications in ultrafast optics and precision metrology. We present a hybrid solution that combines a feed-forward technique to stabilize the phase offset in fast timescales and a feedback technique that addresses slowly varying sources of interference and locking bandwidth limitations associated with gain media with long upper-state lifetimes. We experimentally realize the hybrid stabilization system in an Er:Yb:glass mode-locked laser and demonstrate 75 hours of stabilization with integrated phase noise of 14 mrad (1 Hz to 3 MHz), corresponding to around 11 as of carrier to envelope jitter. Additionally, we examine the impact of environmental factors, such as humidity and pressure, on the long-term stability and performance of the system.

physics.optics↗

arXiv2020

Reconstruction and Optimization of Coherent Synthesis by Fourier Optics Based Genetic Algorithm

We present a numerical method for the reconstruction and optimization of complex field synthesis using coherent pulse combination systems. A genetic algorithm utilizing a Fourier optics based propagation method is developed for accurate convergence and modeling of near and far field distributions, achieving better than $\pi/10$ phase accuracy in reconstructed input parameters.

physics.optics↗

arXiv2020

Integrated Structured Light Architectures

The structural versatility of light underpins an outstanding collection of optical phenomena where both geometrical and topological states of light can dictate how matter will respond or display. Light possesses multiple degrees of freedom such as amplitude, and linear, spin angular, and orbital angular momenta, but the ability to adaptively engineer the spatio-temporal distribution of all these characteristics is primarily curtailed by technologies used to impose any desired structure to light. We describe a foundational demonstration that examines a laser architecture offering integrated spatio-temporal field control and programmability, thereby presenting unique opportunities for generating light by design to exploit its topology.

physics.optics↗

arXiv2019

Carrier-envelope phase stabilization of an Er:Yb:glass laser via feed-forward technique

Few-cycle pulsed laser technology highlights the need for control and stabilization of the carrier-envelope phase (CEP) for applications requiring shot-to-shot timing and phase consistency. This general requirement has been achieved successfully in a number of free space and fiber lasers via feedback and feed-forward methods. Expanding upon existing results, we demonstrate CEP stabilization through the feed-forward method applied to a SESAM mode-locked Er:Yb:glass laser at 1.55 um with a measured ultralow timing jitter of 2.9 as (1 Hz - 3 MHz) and long-term stabilization over a duration of eight hours. Single-digit attosecond stabilization at telecom wavelengths opens a new direction in applications requiring ultra-stable frequency and time precision such as high-resolution spectroscopy and fiber timing networks.

physics.ins-det↗