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Randy S. Fishman

Publications and source records attributed to Randy S. Fishman.

At least 19 recordsLinked to original sources

Topological Magnons on the Ferromagnetic Zigzag Lattice

Motivated by the experimental identification of magnetic compounds consisting of zigzag chains, we analyze the band structure topology of magnons in ferromagnets on a zigzag lattice. We account for the general lattice geometry by including spatially anisotropic Heisenberg exchange interactions and by Dzyaloshinskii-Moriya interaction on inversion asymmetric bonds. Within the linear spin-wave theory, we find two magnon branches, whose band structure topology (i.e., Chern numbers) we map out in a comprehensive phase diagram. Notably, besides topologically trivial and gapless phases, we identify topologically nontrivial phases that support chiral edge magnons. We show that these edge states are robust against elastic defect scattering.

cond-mat.mes-hall

Topological and Magnetic Properties of a Non-collinear Spin State on a Honeycomb Lattice in a Magnetic Field

We study the Berry curvature and Chern number of a non-collinear spin state on a honeycomb lattice that evolves from coplanar to ferromagnetic with a magnetic field applied along the $z$ axis. The coplanar state is stabilized by nearest-neighbor ferromagnetic interactions, single-ion anisotropy along $z$, and Dzyalloshinskii-Moriya interactions between next-nearest neighbor sites. Below the critical field $H_c$ that aligns the spins, the magnetic unit cell contains $M=6$ sites and the spin dynamics contains six magnon subbands. Although the classical energy is degenerate wrt the twist angle $\phi $ between nearest-neighbor spins, the dependence of the free energy on $\phi $ at low temperatures is dominated by the magnon zero-point energy, which contains extremum at $\phi =\pi l/3$ for integer $l$. The only unique ground states GS($\phi )$ have $l=0$ or 1. For $H < H_c'$, the zero-point energy has minima at even $l$ and the ground state is GS(0). For $H_c' < H < H_c$, the zero-point energy has minima at odd $l$ and the ground state is GS($\pi/3$). In GS(0), the magnon density-of-states exhibits five distinct phases with increasing field associated with the opening and closing of energy gaps between the two or three magnonic bands, each containing between 1 and 4 four magnon subbands. While the Berry curvature vanishes for the coplanar $\phi=0$ phase in zero field, the Berry curvature and Chern numbers exhibit signatures of the five phases at nonzero fields below $H_c'$. If $\phi \ne \pi l/3$, the Chern numbers of the two or three magnonic bands are non-integer. We also evaluate the inelastic neutron-scattering spectrum $S(\vk ,\omega )$ produced by the six magnon subbands in all five phases of GS(0) and in GS($\pi/3$).

cond-mat.mtrl-sci

Gauge-Invariant Measure of the Magnon Orbital Angular Momentum

Unlike the Berry phase, the orbital angular momentum (OAM) of magnons with two-dimensional wavevector k in band n is not gauge invariant for arbitrary phase lambda_n(k). However, by integrating the OAM over the orientation $ϕ$ of wavevector k, we construct a gauge-invariant function F_n(k). Like F_n(k), the average OAM for magnon band n in a circle of radius k is also gauge invariant. We demonstrate these results for a ferromagnet on a honeycomb lattice with Dzyalloshinskii-Moriya interactions between next-nearest neighbor spins. With wavevectors k restricted to the first Brillouin zone, the angular averaged OAM F_n(k) then has opposite signs for lower and upper bands n=1 and 2 for all k.

cond-mat.mtrl-sci

Static and dynamical magnetic properties of the extended Kitaev-Heisenberg model with spin vacancies

Motivated by the potential to suppress the antiferromagnetic long-range order in favor of the long-sought-after Kitaev quantum spin liquid state, we study the effect of spin vacancies in the extended Kitaev-Heisenberg model. In particular, we focus on a realistic model obtained from fitting inelastic neutron scattering on $α$-RuCl$_3$. We observe that the long-range zigzag magnetic ordered state only survives when the doping concentration is smaller than 5\%. Upon further increasing the spin vacancy concentration, the ground state becomes a short-range ordered state at low temperatures. Compared with experiments, our classical solution over-stabilizes the zigzag correlation in the presence of spin vacancies. Our theoretical results provide guidance toward interpreting inelastic neutron scattering experiments on magnetically diluted Kitaev candidate materials.

cond-mat.str-el

Field Tunable Magnetic Transitions of CsCo2(MoO4)2(OH): A Triangular Chain Structure with a Frustrated Geometry

Identifying and characterizing new magnetic systems with Co2+ ions can enhance our understanding of quantum behavior since Co2+ can host a pseudospin-1/2 magnetic ground state. Understanding the magnetic ground state and the phase diagrams of such systems are central to the development of new theoretical models to described emergent quantum properties of complex magnetic systems. The sawtooth chain compound, CsCo2MoO4_2OH, is one such complex magnetic system and here, we present a comprehensive series of magnetic and neutron scattering measurements to determine its magnetic phase diagram. The magnetic properties of CsCo2MoO4_2OH exhibit a strong coupling to the crystal lattice and its magnetic ground state can be easily manipulated by applied magnetic fields. There are two unique Co2+ ions, base and vertex, with Jbb and Jbv magnetic exchange. The magnetism is highly anisotropic with the b-axis (chain) along the easy axis and the material orders antiferromagnetically at TN = 5 K. The zero field antiferromagnetic phase contains vertex magnetic vectors Co1 aligned parallel to the b-axis, while the base vectors Co2 are canted by 34 and aligned in an opposite direction to the vertex vectors. The spins in parallel adjacent chains align in opposite directions, creating an overall antiferromagnetic structure. At a 3 kOe applied magnetic field, adjacent chains flip by 180° to generate a ferrimagnetic phase. An increase in field gradually induces the Co(1) moment to rotate along the b-axis and align in the same direction with Co2 generating a ferromagnetic structure. Our results demonstrate that the CsCo2MoO4_2OH is a promising candidate to study new physics associated with sawtooth chain magnetism.

cond-mat.str-el

Exact Results for the Orbital Angular Momentum of Magnons on Honeycomb Lattices

We obtain exact results for the orbital angular momentum (OAM) of magnons at the high symmetry points of ferromagnetic (FM) and antiferromagnetic (AF) honeycomb lattices in the presence of Dzyallonshinskii-Moriya (DM) interactions. For the FM honeycomb lattice in the absence of DM interactions, the values of the OAM at the corners of the Brillouin zone (BZ) (${\bf k}_1^*=(0,2\sqrt{3}/9)2π/a $, ${\bf k}_2^*=(1/3,\sqrt{3}/9)2π/a ,\ldots $) are alternately $\pm 3\hbar /16$ for both magnon bands. The presence of DM interactions dramatically changes those values by breaking the degeneracy of the two magnon bands. The OAM values are alternately $3\hbar /8$ and 0 for the lower magnon band and $-3\hbar /8$ and 0 for the upper magnon band. For the AF honeycomb lattice, the values of the OAM at the corners of the BZ are $\mp (3\hbar /16)κ$ on one of the degenerate magnon bands and $\pm (3\hbar /8) (1+κ/2)$ on the other, where $κ$ measures the anisotropy and the result is independent of the DM interaction.

cond-mat.mtrl-sci

Orbital Angular Momentum of Magnons in Collinear Magnets

We study the orbital angular momentum of magnons for collinear ferromagnet (FM) and antiferromagnetic (AF) systems with nontrivial networks of exchange interactions. The orbital angular momentum of magnons for AF and FM zig-zag and honeycomb lattices becomes nonzero when the lattice contains two inequivalent sites and is largest at the avoided-crossing points or extremum of the frequency bands. Hence, the arrangement of exchange interactions may play a more important role at producing the orbital angular momentum of magnons than the spin-orbit coupling energy and the resulting non-collinear arrangement of spins.

cond-mat.str-el

NaCo2(SeO3)2(OH): Competing Magnetic Ground States of a New Sawtooth Structure with 3d7 Co2+ Ions

While certain magnetic sublattices have long been known theoretically to give rise to emergent physics via competing magnetic interactions and quantum effects, finding such configurations in real materials is often deeply challenging. Here we report the synthesis and characterization of a new such material, NaCo2(SeO3)2(OH) which crystallizes with a highly frustrated sublattice of sawtooth Co2+ chains. Single crystals of NaCo2(SeO3)2(OH) were synthesized using a low-temperature hydrothermal method. X-ray single crystal structure analysis reveals that the material crystallizes in orthorhombic space group of Pnma (no. 62). Its crystal structure exhibits one-dimensional chains of corner-sharing isosceles triangles that are made of two crystallographically distinct 3d7 Co2+ sites (Co(1) and Co(2)). The chains run along the b-axis and are interconnected via [SeO3] groups to form a three-dimensional structure mediating super-exchange interactions. The temperature dependent magnetization data show a ferromagnetic-like (FM) transition at 11 K (T1) followed by an antiferromagnetic (AFM) transition at about 6 K (T2). Neutron-powder diffraction measurements reveal that at T1 = 11 K only Co(2) site orders magnetically, forming ferromagnetic zigzag chains along the b-axis. Below T2 = 6 K, both Co(1) and Co(2) sites order in an nearly orthogonal configuration, with Co(1) moments lying inside the plane of the sawtooth chain while Co(2) moments cant out of the plane. The canting of the magnetic moments leads to a net ferromagnetic component along b-axis, parallel to the chain direction. The ordered moments are fully compensated in the ac-plane.

cond-mat.str-el

Confined Magnons

Magnetic structures are known to possess magnon excitations confined to their surfaces and interfaces, but these spatially localized modes are often not resolved in spectroscopy experiments. We develop a theory to calculate the confined magnon spectra and its associated spin scattering function, which is the physical observable in neutron and electron scattering, and a proxy for photon spectroscopy based on X-ray, Raman and THz sources. We show that extra anisotropy at the surface or interface plays a key role in magnon confinement. We obtain analytical expressions for the confinement length scale, and show that it is qualitatively similar for ferromagnets and antiferromagnets in dimension d>=2. For d=1 we find remarkable differences between ferromagnetic and antiferromagnetic models. The theory indicates the presence of several confined magnon resonances in addition to the usual magnons thought to explain the excitations of magnetic nanostructures. Detecting these modes may elucidate the impact of the interface on spin anisotropy and magnetic order.

cond-mat.mtrl-sci

Magnetic Excitations of the Hybrid Multiferroic (ND4)2FeCl5D2O

We report a comprehensive inelastic neutron scattering study of the hybrid molecule-based multiferroic compound (ND4)2FeCl5D2O in the zero-field incommensurate cycloidal phase and the high-field quasi-collinear phase. The spontaneous electric polarization changes its direction concurrently with the field-induced magnetic transition, from mostly aligned with the crystallographic a-axis to the c-axis. To account for such change of polarization direction, the underlying multiferroic mechanism was proposed to switch from the spin-current model induced via the inverse Dzyalloshinskii-Moriya interaction to the p-d hybridization model. We perform a detailed analysis of the inelastic neutron data of (ND4)2FeCl5D2O using linear spin-wave theory to quantify magnetic interaction strengths and investigate possible impact of different multiferroic mechanisms on the magnetic couplings. Our result reveals that the spin dynamics of both multiferroic phases can be well-described by a Heisenberg Hamiltonian with an easy-plane anisotropy. We do not find notable differences between the optimal model parameters of the two phases. The hierarchy of exchange couplings and the balance among frustrated interactions remain the same between two phases, suggesting that magnetic interactions in (ND4)2FeCl5D2O are much more robust than the electric polarization in response to delicate reorganizations of the electronic degrees of freedom in an applied magnetic field.

cond-mat.str-el

Phase transitions of the ferroelectric $(\mathrm{ND}_4)_2\mathrm{FeCl}_5\cdot\mathrm{D}_2\mathrm{O}$ under a magnetic field

Due to the strong coupling between magnetism and ferroelectricity, $(\mathrm{ND}_4)_2\mathrm{FeCl}_5\cdot\mathrm{D}_2\mathrm{O}$ exhibits several intriguing magnetic and electric phases. In this letter, we include high-order onsite spin anisotropic interactions in a spin model that successfully captures the ferroelectric phase transitions of $(\mathrm{ND}_4)_2\mathrm{FeCl}_5\cdot\mathrm{D}_2\mathrm{O}$ under a magnetic field and produces the large weights of high-order harmonic components in the cycloid structure that are observed from neutron diffraction experiments. Moreover, we predict a new ferroelectric phase sandwiched between the FE II and FE III phases in a magnetic field. Our results emphasize the importance of the high-order spin anisotropic interactions and provide a guideline to understand multiferroic materials with rich phase diagrams.

cond-mat.mtrl-sci

The Magnetoelastic Distortion of Multiferroic BiFeO$_3$ in the Canted Antiferromagnetic State

Using THz spectroscopy, we show that the spin-wave spectrum of multiferroic BiFeO$_3$ in its high-field canted antiferromagnetic state is well described by a spin model that violates rhombohedral symmetry. We demonstrate that the monoclinic distortion of the canted antiferromagnetic state is induced by the single-ion magnetoelastic coupling between the lattice and the two nearly anti-parallel spins. The revised spin model for BiFeO$_3$ contains two new single-ion anisotropy terms that violate rhombohedral symmetry and depend on the direction of the magnetic field.

cond-mat.str-el

Simulating Spin Waves in Entropy Stabilized Oxides

The entropy stabilized oxide Mg$_{0.2}$Co$_{0.2}$Ni$_{0.2}$Cu$_{0.2}$Zn$_{0.2}$O exhibits antiferromagnetic order and magnetic excitations, as revealed by recent neutron scattering experiments. This observation raises the question of the nature of spin wave excitations in such disordered systems. Here, we investigate theoretically the magnetic ground state and the spin-wave excitations using linear spin-wave theory in combination with the supercell approximation to take into account the extreme disorder in this magnetic system. We find that the experimentally observed antiferromagnetic structure can be stabilized by a rhombohedral distortion together with large second nearest neighbor interactions. Our calculations show that the spin-wave spectrum consists of a well-defined low-energy coherent spectrum in the background of an incoherent continuum that extends to higher energies.

cond-mat.dis-nn

Stripe antiferromagnetic ground state of ideal triangular lattice KErSe$_2$

Rare earth triangular lattice materials have been proposed as a good platform for the investigation of frustrated magnetic ground states. KErSe$_2$ with the delafossite structure, contains perfect two-dimensional Er$^{3+}$ triangular layers separated by potassium ions, realizing this ideal configuration and inviting study. Here we investigate the magnetism of KErSe$_2$ at miliKelvin temperatures by heat capacity and neutron powder diffraction. Heat capacity results reveal a magnetic transition at 0.2 K in zero applied field. This long-range order is suppressed by an applied magnetic field of 0.5 T below 0.08 K. Neutron powder diffraction suggests that the zero-field magnetic structure orders with $k=(\frac{1}{2},0,\frac{1}{2})$ in a stripe spin structure. Unexpectedly, Er is found to have a reduced moment of 3.06(1) $μ_B$/Er in the ordered state and diffuse magnetic scattering, which originates at higher temperatures, is found to persist in the ordered state potentially indicating magnetic fluctuations. Neutron diffraction collected under an applied field shows a metamagnetic transition at $\sim$ 0.5 T to ferromagnetic order with $k$=(0,0,0) and two possible structures, which are likely dependent on the applied field direction. First principle calculations show that the zero field stripe spin structure can be explained by the first, second and third neighbor couplings in the antiferromagnetic triangular lattice.

cond-mat.mtrl-sci

Cluster Frustration in the Breathing Pyrochlore Magnet LiGaCr4S8

We present a comprehensive neutron scattering study of the breathing pyrochlore magnet LiGaCr4S8. We observe an unconventional magnetic excitation spectrum with a separation of high and low-energy spin dynamics in the correlated paramagnetic regime above a spin-freezing transition at 12(2) K. By fitting to magnetic diffuse-scattering data, we parameterize the spin Hamiltonian. We find that interactions are ferromagnetic within the large and small tetrahedra of the breathing pyrochlore lattice, but antiferromagnetic further-neighbor interactions are also essential to explain our data, in qualitative agreement with density-functional theory predictions [Ghoshet al.,npj Quantum Mater.4, 63 (2019)]. We explain the origin of geometrical frustration in LiGaCr4S8 interms of net antiferromagnetic coupling between emergent tetrahedral spin clusters that occupy a face-centered lattice. Our results provide insight into the emergence of frustration in the presence of strong further-neighbor couplings, and a blueprint for the determination of magnetic interactions in classical spin liquids.

cond-mat.str-el

Steplike metamagnetic transitions in a honeycomb lattice antiferromagnet Tb$_2$Ir$_3$Ga$_9$

Single crystals of a honeycomb lattice antiferromagnet, Tb$_2$Ir$_3$Ga$_9$ were synthesized, and the physical properties have been studied. From magnetometry, a long-range antiferromagnetic ordering at $\approx$12.5 K with highly anisotropic magnetic behavior was found. Neutron powder diffraction confirms that the Tb spins lie along the $\va $-axis, parallel to the shortest Tb-Tb contact. Two field-induced spin-flip transitions are observed when the field is applied parallel to this axis, separated by a plateau corresponding roughly to M$\approx$M$_{\rm{s}}$/2. Transport measurements show the resistivity to be metallic with a discontinuity at the onset of Néel order. Heat capacity shows a $λ$-like transition confirming the bulk nature of the magnetism. We propose a phenomenological spin-Hamiltonian that describes the magnetization plateau as a result of strong Ising character arising from a quasidoublet ground state of the Tb$^{3+}$ ion in a site of \textit{C$_s$} symmetry and expressing a significant bond dependent anisotropy.

cond-mat.mes-hall

Normal Modes of a Spin Cycloid or Helix

Although spin cycloids and helices are quite common, remarkably little is known about the normal modes of a spin cycloid or helix with finite length on a discrete lattice. Based on simple one-dimensional lattice models, we numerically evaluate the normal modes of a spin cycloid or helix produced by either Dzyaloshinskii-Moriya (DM) or competing exchange (CE) interactions. The normal modes depend on the type of interaction and on whether the nearest-neighbor exchange is antiferromagnetic (AF) or ferromagnetic (FM). In the AF/DM and FM/DM cases, there is only a single Goldstone mode; in the AF/CE and FM/CE cases, there are three. For FM exchange, the spin oscillations produced by non-Goldstone modes contain a mixture of tangential and transverse components. For the DM cases, we compare our numerical results with analytic results in the continuum limit. Examples are given of materials that fall into all four cases.

cond-mat.mtrl-sci

Pinning, Rotation, and Metastability of BiFeO$_3$ Cycloidal Domains in a Magnetic Field

Earlier models for the room-temperature multiferroic BiFeO3 implicitly assumed that a very strong anisotropy restricts the domain wavevectors q to the three-fold symmetric axis normal to the static polarization P. However, recent measurements demonstrate that the domain wavevectors rotate so that q rotates within the hexagonal plane normal to P away from the field orientation m. We show that the previously neglected three-fold anisotropy K3 restricts the wavevectors to lie along the three-fold axis in zero field. For m along a three-fold axis, the domain with q parallel to m remains metastable below Bc1 = 7 T. Due to the pinning of domains by non-magnetic impurities, the wavevectors of the other two domains start to rotate away from m above 5.6 T, when the component of the torque t = M x B along P exceeds a threshold value tpin. Since t =0 when m is perpendicular to q, the wavevectors of those domains never become completely perpendicular to the magnetic field. Our results explain recent measurements of the critical field as a function of field orientation, small-angle neutron scattering measurements of the wavevectors, as well as spectroscopic measurements with m along a three-fold axis.

cond-mat.mtrl-sci