arXiv subjects

Raphael Holzinger

Publications and source records attributed to Raphael Holzinger.

At least 19 recordsLinked to original sources

arXiv2026

Continuous Narrow-Linewidth Superradiance in Waveguide QED

Superradiant lasers promise continuous, narrow-linewidth coherent emission at the bare atomic transition frequency, enabling frequency references of exceptional precision. Recent experiments have advanced the field, but achieving truly continuous operation remains technically challenging. Here we propose an alternative route to an active optical frequency reference with fewer emitters using all-to-all dipole-dipole interactions mediated by a nanophotonic waveguide. We show that selectively pumping only a sub-ensemble of emitters, rather than the full ensemble, substantially improves emission characteristics. The collective interactions with unpumped emitters provide narrowband frequency selection and establish an effective feedback mechanism analogous to the role of a macroscopic cavity. We find directional superradiant emission with strongly phase-synchronized emitter correlations and a narrow output spectrum close to the bare emitter resonance. Our results demonstrate a strong metrological gain from selective partial pumping of quantum emitters with the second-order intensity correlation $g^{(2)}(0)\simeq 1$, indicating reduced equal-time intensity fluctuations, and open a route to waveguide-based optical frequency references using small clock-atom ensembles for chip-scale precision metrology.

quant-ph↗

arXiv2026

Light-induced Self-Organization in Cooperative Free Space Atomic Arrays

We investigate how laser-driven, cooperative dipole-dipole interactions in weakly trapped atomic arrays give rise to self-organized configurations. Starting from an analytically tractable two-emitter system, we identify the possible steady-state spatial arrangements accessible to the atoms. We then extend this analysis to larger ensembles in both linear and ring geometries. In linear chains, we demonstrate the emergence of topologically nontrivial dimerized configurations across a range of initial interatomic spacings. In ring geometries, we find that the system undergoes self-organized contraction and expansion, enabling access to length scales below those set by the trapping lattice. Our results demonstrate that collective light-matter interactions in free space can spontaneously generate modified ordered geometries, even when the emitters are initially separated by distances larger than their transition wavelength.

quant-ph↗

arXiv2025

Symbolic Quantum-Trajectory Method for Multichannel Dicke Superradiance

We solve Dicke superradiance with two or more competing collective decay channels of tunable rates using a symbolic quantum-trajectory construction. The method yields closed time-domain populations and observables as finite combinations of exponential terms for arbitrary numbers of emitters and arbitrary decay rates. For two channels, the behavior of the stationary ground-state distribution resembles a first-order phase transition at the point where the channel-rate ratio is equal to unity. For balanced $d$-channel decay, we obtain scaling laws for the superradiant peak time and intensity. These results unify and extend single-channel Dicke dynamics to multilevel emitters and provide a compact tool for cavity and waveguide experiments, where permutation-symmetric reservoirs engineer multiple collective decay paths.

quant-ph↗

arXiv2025

Scaling of Superradiant Peak Emission in Spatially Extended Emitter Arrays

In quantum optics, superradiance is a phenomenon in which a system of $N$ fully excited quantum emitters radiate intense flashes of light during collective decay. However, computing its peak intensity exactly for many spatially separated emitters remains challenging due to the exponential growth of the underlying Hilbert space with system size $N$. Based on third-order cumulant expansion methods, we present general scaling laws for the expononent of the peak emission rate as a function of the emitter number in free-space emitter arrays and arrays coupled to one-dimensional waveguide reservoirs. We find, that for 1D chains in free-space the peak emission rate scales linearly with $N$, while for 2D and 3D arrays with finite emitter spacing it scales superlinearly but sub-quadratically. For emitter chains coupled to waveguide reservoirs we find that the peak emission rate scales quadratically with $N$.

quant-ph↗

arXiv2025

Nanoscale Mirrorless Superradiant Lasing

We predict collective 'free-space' lasing in a dense nanoscopic emitter arrangement where dipole-dipole coupled atomic emitters synchronize their emission and exhibit lasing behavior without the need for an optical resonator. At the example of a subwavelength-spaced linear emitter chain with varying fractions of pumped and unpumped emitters, we present a comprehensive study of this mirrorless lasing phenomenon. The total radiated power transitions from subradiant suppression under weak pumping to superradiant enhancement at stronger pumping, while exhibiting directional emission confined to a narrow spatial angle. At the same time multiple independent spectral emission lines below the lasing threshold merge towards a single narrow spectral line at high pump power. The most substantial enhancement and line narrowing occur when a fraction of unpumped atoms is present. We show that this leads to superradiant lasing near the bare atomic frequency, making the system a promising candidate for a minimalist active optical frequency reference.

quant-ph↗

arXiv2025

Superradiant Peak Emission Rate and Time in Quantum Emitter Arrays

Determining the peak photon emission time and rate for an ensemble of $N$ quantum systems undergoing collective superradiant decay typically requires tracking the time evolution of the density operator. Generally, the dimension of the density operator grows exponentially ($\sim \! 2^N$) with the number of emitters, in the absence of any symmetries such as in Dicke superradiance with full or partial permutational symmetry. We present a detailed study of the superradiant peak emission rate and time for initially fully excited quantum emitter ensembles, for one-, two- and three-dimensional arrays in free-space and emitter chains coupled to waveguide reservoirs. For few emitters ($N\lesssim 14$) we utilize the full quantum master equation, and for mesoscopic emitter numbers ($N\lesssim 400$) we use a second- and third-order cumulant expansion of the operator averages to track the time evolution of the system.

quant-ph↗

arXiv2025

Solving Dicke superradiance analytically: A compendium of methods

We present several analytical approaches to the Dicke superradiance problem, which involves determining the time evolution of the density operator for an initially inverted ensemble of $N$ identical two-level systems undergoing collective spontaneous emission. This serves as one of the simplest cases of open quantum system dynamics that allows for a fully analytical solution. We explore multiple methods to tackle this problem, yielding a solution valid for any time and any number of spins. These approaches range from solving coupled rate equations and identifying exceptional points in non-Hermitian evolution to employing combinatorial and probabilistic techniques, as well as utilizing a quantum jump unraveling of the master equation. The analytical solution is expressed as a residue sum obtained from a contour integral in the complex plane, suggesting the possibility of fully analytical solutions for a broader class of open quantum system dynamics problems.

quant-ph↗

arXiv2024

An exact analytical solution for Dicke superradiance

We revisit the Dicke superradiance problem, where an ensemble of N identical two-level systems undergoes collective spontaneous decay. While an exact analytical solution has been known since 1977, its algebraic complexity has hindered practical use. Here we present a compact, closed-form solution that expresses the dynamics as a finite sum over residues or, equivalently, a complex contour integral. The method yields explicit populations of all Dicke states at arbitrary times and system sizes, and generalizes naturally to arbitrary initial conditions. Our formulation is computationally efficient and offers structural insights into the role of spectral degeneracies and Lindbladian eigenmodes in collective decay.

quant-ph↗

arXiv2024

Symmetry based efficient simulation of dissipative quantum many-body dynamics in subwavelength quantum emitter arrays

We propose an efficient method to numerically simulate the dissipative dynamics of large numbers of quantum emitters in ordered arrays in the presence of long-range dipole-dipole interactions mediated by the vacuum electromagnetic field. Using the spatial symmetries of the system, we rewrite the equations of motion in a collective spin basis and subsequently apply a higher-order cumulant expansion for the collective operators. By truncating the subradiant collective modes with a heavily suppressed decay rate and keeping only the effect from the radiating collective modes, we reduce the numerical complexity significantly. This allows to efficiently compute the dissipative dynamics of the observables of interest for a linear, ring-shaped and planar arrays of quantum emitters. In particular, we characterize the excited population, the total photon emission rate and the second order intensity correlation function $g^{(2)}(\tau =0)$, which are challenging to compute for large systems with traditional cumulant expansion methods based on the individual spins.

quant-ph↗

arXiv2024

Efficient excitation transfer in an LH2-inspired nanoscale stacked ring geometry

Subwavelength ring-shaped structures of quantum emitters exhibit outstanding radiation properties and are useful for antennas, excitation transport, and storage. Taking inspiration from the oligomeric geometry of biological light-harvesting 2 (LH2) complexes, we study here generic examples and predict highly efficient excitation transfer in a three-dimensional (3D) subwavelength concentric stacked ring structure with a diameter of 400 $nm$, formed by two-level atoms. Utilizing the quantum optical open system master equation approach for the collective dipole dynamics, we demonstrate that, depending on the system parameters, our bio-mimicked 3D ring enables efficient excitation transfer between two ring layers. Our findings open prospects for engineering other biomimetic light-matter platforms and emitter arrays to achieve efficient energy transfer.

physics.optics↗

arXiv2024

Collectively enhanced ground-state cooling in subwavelength atomic arrays

Subwavelength atomic arrays feature strong light-induced dipole-dipole interactions, resulting in subradiant collective resonances characterized by narrowed linewidths. In this work, we present a sideband cooling scheme for atoms trapped in subwavelength arrays that utilizes these narrow collective resonances. Working in the Lamb-Dicke regime, we derive an effective master equation for the atomic motion by adiabatically eliminating the internal degrees of freedom of the atoms, and validate its prediction with numerical simulations of the full system. Our results demonstrate that subradiant resonances enable the cooling of ensembles of atoms to temperatures lower than those achievable without dipole interactions, provided the atoms have different trap frequencies. Remarkably, narrow collective resonances can be sideband-resolved even when the individual atomic transition is not. In such scenarios, ground-state cooling becomes feasible solely due to light-induced dipole-dipole interactions. This approach could be utilized for future quantum technologies based on dense ensembles of emitters, and paves the way towards harnessing many-body cooperative decay for enhanced motional control.

quant-ph↗

arXiv2024

Examining the quantum signatures of optimal excitation energy transfer

Light-harvesting via the transport and trapping of optically-induced electronic excitations is of fundamental interest to the design of new energy efficient quantum technologies. Using a paradigmatic quantum optical model, we study the influence of coherence, entanglement, and cooperative dissipation on the transport and capture of excitation energy. In particular, we demonstrate that the rate of energy extraction is optimized under conditions that minimize the quantum coherence and entanglement of the system. We show that this finding is not limited to disordered or high temperature systems but is instead a fundamental consequence of spontaneous parity time-reversal symmetry breaking associated with the quantum-to-classical transition. We then examine the effects of vibrational fluctuations, revealing a strong dephasing assisted transport enhancement for delocalized excitations in the presence of cooperative interactions. Our results highlight the rich, emergent behavior associated with decoherence and may be relevant to the study of biological photosynthetic antenna complexes or to the design of room-temperature quantum devices.

quant-ph↗

arXiv2023

Harnessing quantum emitter rings for efficient energy transport and trapping

Efficient transport and harvesting of excitation energy under low light conditions is an important process in nature and quantum technologies alike. Here we formulate a quantum optics perspective to excitation energy transport in configurations of two-level quantum emitters with a particular emphasis on efficiency and robustness against disorder. We study a periodic geometry of emitter rings with subwavelength spacing, where collective electronic states emerge due to near-field dipole-dipole interactions. The system gives rise to collective subradiant states that are particularly suited to excitation transport and are protected from energy disorder and radiative decoherence. Comparing ring geometries with other configurations shows that that the former are more efficient in absorbing, transporting, and trapping incident light. Because our findings are agnostic as to the specific choice of quantum emitters, they indicate general design principles for quantum technologies with superior photon transport properties and may elucidate potential mechanisms resulting in the highly efficient energy transport efficiencies in natural light-harvesting systems.

quant-ph↗

arXiv2023

Scaling law for Kasha's rule in photoexcited molecular aggregates

We study the photophysics of molecular aggregates from a quantum optics perspective, with emphasis on deriving scaling laws for the fast non-radiative relaxation of collective electronic excitations, referred to as Kasha's rule. Aggregates exhibit an energetically broad manifold of collective states with delocalized electronic excitations originating from near field dipole-dipole exchanges between neighboring monomers. Photo-excitation at optical wavelengths, much larger than the monomer-monomer average separation, addresses almost exclusively symmetric collective states, which for an arrangement known as H-aggregate, show an upward hypsochromic shift. The extremely fast subsequent non-radiative relaxation via intramolecular vibrational modes populates lower energy, subradiant states, resulting in an effective inhibition of fluorescence. Our analytical treatment allows for the derivation of an approximate scaling law of this relaxation process, linear in the number of available low energy vibrational modes and directly proportional to the dipole-dipole interaction strength between neighbouring monomers.

quant-ph↗

arXiv2023

Optical Properties of Concentric Nanorings of Quantum Emitters

A ring of sub-wavelength spaced dipole-coupled quantum emitters features extraordinary optical properties when compared to a one-dimensional chain or a random collection of emitters. One finds the emergence of extremely subradiant collective eigenmodes similar to an optical resonator, which feature strong 3D sub-wavelength field confinement. Motivated by structures commonly appearing in natural light harvesting complexes, we extend these studies to stacked concentric multi-ring geometries. We predict that double rings allow to engineer significantly darker and better confined collective excitation states over a broader energy band compared to the single ring case. These potentially enhance weak field absorption and low loss excitation energy transport. For the specific geometry of the three rings appearing in the natural LH2 antenna we show that the coupling between the lower double ring structure and the higher energy blue shifted single ring is very close to a critical value for the actual size of the molecule. This creates collective excitations with significant contributions from all three rings as a vital ingredient for efficient and fast coherent inter-ring transport. Such a geometry thus should prove useful for the design of sub-wavelength weak field antennas.

quant-ph↗

arXiv2022

Control of Localized Multiple Excitation Dark States in Waveguide QED

Subradiant excited states in finite chains of two-level quantum emitters coupled to a one-dimensional reservoir are a resource for superior photon storage and controlled photon manipulation. Typically, states storing multiple excitations exhibit fermionic correlations and are thus characterized by an anti-symmetric wavefunction, which makes them hard to prepare experimentally. Here we identify a class of quasi-localized dark states with up to half of the qubits excited, which appear for lattice constants that are an integer multiple of the guided-mode wavelength. They allow for a high-fidelity preparation and minimally invasive read out in state-of-the-art setups. In particular, we suggest an experimental implementation using a coplanar wave-guide coupled to superconducting transmon qubits on a chip. As free space and intrinsic losses are minimal, virtually perfect dark states can be achieved even for a low number of qubits, enabling fast preparation and manipulation with high fidelity.

quant-ph↗

arXiv2022

Cooperative subwavelength molecular quantum emitter arrays

Dipole-coupled subwavelength quantum emitter arrays respond cooperatively to external light fields as they may host collective delocalized excitations (a form of excitons) with super- or subradiant character. Deeply subwavelength separations typically occur in molecular ensembles, where in addition to photon-electron interactions, electron-vibron couplings and vibrational relaxation processes play an important role. We provide analytical and numerical results on the modification of super- and subradiance in molecular rings of dipoles including excitations of the vibrational degrees of freedom. While vibrations are typically considered detrimental to coherent dynamics, we show that molecular dimers or rings can be operated as platforms for the preparation of long-lived dark superposition states aided by vibrational relaxation. In closed ring configurations, we extend previous predictions for the generation of coherent light from ideal quantum emitters to molecular emitters, quantifying the role of vibronic coupling onto the output intensity and coherence.

quant-ph↗

arXiv2021

Nanoscale continuous quantum light sources based on driven dipole emitter arrays

Regular arrays of two-level emitters at distances smaller that the transition wavelength collectively scatter, absorb and emit photons. The strong inter-particle dipole coupling creates large energy shifts of the collective delocalized excitations, which generates a highly nonlinear response at the single and few photon level. This should allow to implement nanoscale non-classical light sources via weak coherent illumination. At the generic tailored examples of regular chains or polygons we show that the fields emitted perpendicular to the illumination direction exhibit a strong directional confinement with genuine quantum properties as antibunching. For short interparticle distances superradiant directional emission can enhance the radiated intensity by an order of magnitude compared to a single atom focused to a strongly confined solid angle but still keeping the anti-bunching parameter at the level of $g^{(2)}(0) \approx 10^{-2}$.

quant-ph↗