Searcharxiv⌕ Search

arXiv subjects

Raphael Wittkowski

Publications and source records attributed to Raphael Wittkowski.

At least 37 records · Page 2Linked to original sources

Orientation-dependent propulsion of active Brownian spheres: from self-advection to programmable cluster shapes

Applications of active particles require a method for controlling their dynamics. While this is typically achieved via direct interventions, indirect interventions based, e.g., on an orientation-dependent self-propulsion speed of the particles, become increasingly popular. In this work, we investigate systems of interacting active Brownian spheres in two spatial dimensions with orientation-dependent propulsion using analytical modeling and Brownian dynamics simulations. It is found that the orientation-dependence leads to self-advection, circulating currents, and programmable cluster shapes.

cond-mat.soft↗

Acoustic propulsion of nano- and microcones: dependence on the viscosity of the surrounding fluid

This article investigates how the acoustic propulsion of cone-shaped colloidal particles that are exposed to a traveling ultrasound wave depends on the viscosity of the fluid surrounding the particles. Using acoustofluidic computer simulations, we found that the propulsion of such nano- and microcones decreases strongly and even changes sign for increasing shear viscosity. In contrast, we found only a weak dependence of the propulsion on the bulk viscosity. The obtained results are in line with the findings of previous theoretical and experimental studies.

cond-mat.soft↗

Propulsion of bullet- and cup-shaped nano- and microparticles by traveling ultrasound waves

The propulsion of colloidal particles via planar traveling ultrasound waves has attracted increasing attention in recent years. A frequently studied type of particles is bullet-shaped and cup-shaped nano- and microparticles. Based on acoustofluidic simulations, this article investigates how the propulsion of bullet-shaped particles depends on their length and diameter, where cup-shaped particles are included as limiting cases corresponding to the smallest particle length. The structure of the flow field generated by the particles is discussed and it is shown that the particles' propulsion strength increases with their length and diameter. When varying the diameter, we observed also a sign change of the propulsion. This work complements previous experimental studies that have addressed such particles only for particular aspect ratios, and the provided understanding of how the propulsion of the particles depends on their dimensions will prospectively be helpful for the choice of particle shapes that are most suitable for future experimental studies.

cond-mat.soft↗

ASEVis: Visual Exploration of Active System Ensembles to Define Characteristic Measures

Simulation ensembles are a common tool in physics for understanding how a model outcome depends on input parameters. We analyze an active particle system, where each particle can use energy from its surroundings to propel itself. A multi-dimensional feature vector containing all particles' motion information can describe the whole system at each time step. The system's behavior strongly depends on input parameters like the propulsion mechanism of the particles. To understand how the time-varying behavior depends on the input parameters, it is necessary to introduce new measures to quantify the difference of the dynamics of the ensemble members. We propose a tool that supports the interactive visual analysis of time-varying feature-vector ensembles. A core component of our tool allows for the interactive definition and refinement of new measures that can then be used to understand the system's behavior and compare the ensemble members. Different visualizations support the user in finding a characteristic measure for the system. By visualizing the user-defined measure, the user can then investigate the parameter dependencies and gain insights into the relationship between input parameters and simulation output.

cs.HC↗

Roadmap for Optical Tweezers

Optical tweezers are tools made of light that enable contactless pushing, trapping, and manipulation of objects ranging from atoms to space light sails. Since the pioneering work by Arthur Ashkin in the 1970s, optical tweezers have evolved into sophisticated instruments and have been employed in a broad range of applications in life sciences, physics, and engineering. These include accurate force and torque measurement at the femtonewton level, microrheology of complex fluids, single micro- and nanoparticle spectroscopy, single-cell analysis, and statistical-physics experiments. This roadmap provides insights into current investigations involving optical forces and optical tweezers from their theoretical foundations to designs and setups. It also offers perspectives for applications to a wide range of research fields, from biophysics to space exploration.

physics.optics↗

Inertial dynamics of an active Brownian particle

Active Brownian motion commonly assumes spherical overdamped particles. However, self-propelled particles are often neither symmetric nor overdamped yet underlie random fluctuations from their surroundings. Active Brownian motion has already been generalized to include asymmetric particles. Separately, recent findings have shown the importance of inertial effects for particles of macroscopic size or in low-friction environments. We aim to consolidate the previous findings into the general description of a self-propelled asymmetric particle with inertia. We derive the Langevin equation of such a particle as well as the corresponding Fokker-Planck equation. Furthermore, a formula is presented that allows reconstructing the hydrodynamic resistance matrix of the particle by measuring its trajectory. Numerical solutions of the Langevin equation show that, independently of the particle's shape, the noise-free trajectory at zero temperature starts with an inertial transition phase and converges to a circular helix. We discuss this universal convergence with respect to the helical motion that many microorganisms exhibit.

cond-mat.soft↗

Derivation and analysis of a phase field crystal model for a mixture of active and passive particles

We discuss an active phase field crystal (PFC) model that describes a mixture of active and passive particles. First, a microscopic derivation from dynamical density functional theory (DDFT) is presented that includes a systematic treatment of the relevant orientational degrees of freedom. Of particular interest is the construction of the nonlinear and coupling terms. This allows for interesting insights into the microscopic justification of phenomenological constructions used in PFC models for active particles and mixtures, the approximations required for obtaining them, and possible generalizations. Second, the derived model is investigated using linear stability analysis and nonlinear methods. It is found that the model allows for a rich nonlinear behavior with states ranging from steady periodic and localized states to various time-periodic states. The latter include standing, traveling, and modulated waves corresponding to spatially periodic and localized traveling, wiggling, and alternating peak patterns and their combinations.

cond-mat.soft↗

Perspective: New directions in dynamical density functional theory

Classical dynamical density functional theory (DDFT) has become one of the central modeling approaches in nonequilibrium soft matter physics. Recent years have seen the emergence of novel and interesting fields of application for DDFT. In particular, there has been a remarkable growth in the amount of work related to chemistry. Moreover, DDFT has stimulated research on other theories such as phase field crystal models and power functional theory. In this perspective, we summarize the latest developments in the field of DDFT and discuss a variety of possible directions for future research.

cond-mat.soft↗

From a microscopic inertial active matter model to the Schrödinger equation

Field theories for the one-body density of an active fluid, such as the paradigmatic active model B+, are simple yet very powerful tools for describing phenomena such as motility-induced phase separation. No comparable theory has been derived yet for the underdamped case. In this work, we introduce active model I+, an extension of active model B+ to particles with inertia. The governing equations of active model I+ are systematically derived from the microscopic Langevin equations. We show that, for underdamped active particles, thermodynamic and mechanical definitions of the velocity field no longer coincide and that the density-dependent swimming speed plays the role of an effective viscosity. Moreover, active model I+ contains the Schrödinger equation in Madelung form as a limiting case, allowing to find analoga of the quantum-mechanical tunnel effect and of fuzzy dark matter in the active fluid. We investigate the active tunnel effect analytically and via numerical continuation.

cond-mat.soft↗

Orientation-dependent propulsion of cone-shaped nano- and microparticles by a traveling ultrasound wave

Previous studies on ultrasound-propelled nano- and microparticles have considered only systems where the particle orientation is perpendicular to the direction of propagation of the ultrasound. However, in future applications of these particles, they will typically be able to attain also other orientations. Therefore, using direct acoustofluidic simulations, we here study how the propulsion of cone-shaped nano- and microparticles, which are known to have a particularly efficient acoustic propulsion and are therefore promising candidates for future applications, depends on their orientation relative to the propagation direction of a traveling ultrasound wave. Our results reveal that the propulsion of the particles depends strongly on their orientation relative to the direction of wave propagation and that the particles tend to orient perpendicularly to the wave direction. We also present the orientation-averaged translational and angular velocities of the particles, which correspond to the particles' effective propulsion for an isotropic exposure to ultrasound. Our results allow assessing how free ultrasound-propelled colloidal particles move in three spatial dimensions and thus constitute an important step towards the realization of the envisaged future applications of such particles.

cond-mat.soft↗

Active Brownian particles in external force fields: field-theoretical models, generalized barometric law, and programmable density patterns

We investigate the influence of external forces on the collective dynamics of interacting active Brownian particles in two as well as three spatial dimensions. Via explicit coarse graining, we derive predictive models that are applicable for space- and time-dependent external force fields. We study these models for the cases of gravity and harmonic traps. In particular, we derive a generalized barometric formula for interacting active Brownian particles under gravity that is valid for low to high concentrations and activities of the particles. Furthermore, we show that one can use an external harmonic trap to induce motility-induced phase separation in systems that, without external fields, remain in a homogeneous state. This finding makes it possible to realize programmable density patterns in systems of active Brownian particles. Our analytic predictions are found to be in very good agreement with Brownian dynamics simulations.

cond-mat.soft↗

Topological fine structure of smectic grain boundaries and tetratic disclination lines within three-dimensional smectic liquid crystals

Observing and characterizing the complex ordering phenomena of liquid crystals subjected to external constraints constitutes an ongoing challenge for chemists and physicists alike. To elucidate the delicate balance appearing when the intrinsic positional order of smectic liquid crystals comes into play, we perform Monte-Carlo simulations of rod-like particles in a range of cavities with a cylindrical symmetry. Based on recent insights into the topology of smectic orientational grain boundaries in two dimensions, we analyze the emerging three-dimensional defect structures from the perspective of tetratic symmetry. Using an appropriate three-dimensional tetratic order parameter constructed from the Steinhardt order parameters, we show that those grain boundaries can be interpreted as a pair of tetratic disclination lines that are located on the edges of the nematic domain boundary. Thereby, we shed light on the fine structure of grain boundaries in three-dimensional confined smectics.

cond-mat.soft↗

Collective guiding of acoustically propelled nano- and microparticles for medical applications

One of the most important potential applications of self-propelled nano- and microdevices is targeted drug delivery. To realize this, biocompatible particles that can be guided collectively towards a target inside a patient's body are required. Acoustically propelled nano- and microparticles constitute a promising candidate for such biocompatible, artificial motile particles. The main remaining obstacle to targeted drug delivery by self-propelled nano- and microdevices is to also achieve a reliable and biocompatible method for guiding them collectively to their target. Here, we propose such a method. As we confirm by computer simulations, it allows for the remote guiding of large numbers of acoustically propelled particles to a prescribed target by combining a space- and time-dependent acoustic field and a time-dependent magnetic field. The method works without detailed knowledge about the particle positions and for arbitrary initial particle distributions. With these features, it paves the way for the future application of self-propelled particles as vehicles for targeted drug delivery in nanomedicine.

cond-mat.soft↗

A colloidal time crystal and its tempomechanical properties

The spontaneous breaking of symmetries is a widespread phenomenon in physics. When time translational symmetry is spontaneously broken, an exotic nonequilibrium state of matter in which the same structures repeat themselves in time can arise. This state, known as "time crystal", attracted a lot of interest recently. Another relatively new research area deals with active matter. Materials consisting of colloidal particles that consume energy from their environment and propel themselves forward can exhibit intriguing properties like superfluidity that were previously known only from quantum-mechanical systems. Here, we bring together these - at first glance completely different - research fields by showing that self-propelled colloidal particles can form classical continuous time crystals. We present a state diagram showing where this new state of matter arises. Furthermore, we investigate its tempomechanical properties and present a temporal stress-strain diagram showing parallels to conventional materials science but also remarkable new properties that do not have a counterpart in common materials.

cond-mat.soft↗

Mori-Zwanzig formalism for general relativity: a new approach to the averaging problem

Cosmology relies on a coarse-grained description of the universe, assumed to be valid on large length scales. However, the nonlinearity of general relativity makes coarse-graining extremely difficult. We here address this problem by extending the Mori-Zwanzig projection operator formalism, a highly successful coarse-graining method from statistical mechanics, towards general relativity. Using the Buchert equations, we derive a new dynamic equation for the Hubble parameter which captures the effects of averaging through a memory function. This gives an empirical prediction for the cosmic jerk.

gr-qc↗

Master equations for Wigner functions with spontaneous collapse and their relation to thermodynamic irreversibility

Wigner functions, allowing for a reformulation of quantum mechanics in phase space, are of central importance for the study of the quantum-classical transition. A full understanding of the quantum-classical transition, however, also requires an explanation for the absence of macroscopic superpositions to solve the quantum measurement problem. Stochastic reformulations of quantum mechanics based on spontaneous collapses of the wavefunction are a popular approach to this issue. In this article, we derive the dynamic equations for the four most important spontaneous collapse models - Ghirardi-Rimini-Weber (GRW) theory, continuous spontaneous localization (CSL) model, Diósi-Penrose model, and dissipative GRW model - in the Wigner framework. The resulting master equations are approximated by Fokker-Planck equations. Moreover, we use the phase-space form of GRW theory to test, via molecular dynamics simulations, David Albert's suggestion that the stochasticity induced by spontaneous collapses is responsible for the emergence of thermodynamic irreversibility. The simulations show that, for initial conditions leading to anti-thermodynamic behavior in the classical case, GRW-type perturbations do not lead to thermodynamic behavior. Consequently, the GRW-based equilibration mechanism proposed by Albert is not observed.

quant-ph↗

Acoustically propelled nano- and microcones: fast forward and backward motion

We focus on cone-shaped nano- and microparticles, which have recently been found to show particularly strong propulsion when they are exposed to a traveling ultrasound wave, and study based on direct acoustofluidic computer simulations how their propulsion depends on the cones' aspect ratio. The simulations reveal that the propulsion velocity and even its sign are very sensitive to the aspect ratio, where short particles move forward whereas elongated particles move backward. Furthermore, we identify a cone shape that allows for a particularly large propulsion speed. Our results contribute to the understanding of the propulsion of ultrasound-propelled colloidal particles, suggest a method for separation and sorting of nano- and microcones concerning their aspect ratio, and provide useful guidance for future experiments and applications.

cond-mat.soft↗

Jerky active matter: a phase field crystal model with translational and orientational memory

Most field theories for active matter neglect effects of memory and inertia. However, recent experiments have found inertial delay to be important for the motion of self-propelled particles. A major challenge in the theoretical description of these effects, which makes the application of standard methods very difficult, is the fact that orientable particles have both translational and orientational degrees of freedom which do not necessarily relax on the same time scale. In this work, we derive the general mathematical form of a field theory for soft matter systems with two different time scales. This allows to obtain a phase field crystal model for polar (i.e., nonspherical or active) particles with translational and orientational memory. Notably, this theory is of third order in temporal derivatives and can thus be seen as a spatiotemporal jerky dynamics. We obtain the phase diagram of this model, which shows that, unlike in the passive case, the linear stability of the liquid state depends on the damping coefficients. Moreover, we investigate sound waves in active matter. It is found that, in active fluids, there are two different mechanisms for sound propagation. For certain parameter values and sufficiently high frequencies, sound mediated by polarization waves experiences less damping than usual passive sound mediated by pressure waves of the same frequency. By combining the different modes, acoustic frequency filters based on active fluids could be realized.

cond-mat.soft↗