arXiv subjects

Ravitej Uppu

Publications and source records attributed to Ravitej Uppu.

At least 19 recordsLinked to original sources

arXiv2026

Geometric Control of Visible Emitter Creation in Hexagonal Boron Nitride by Oblique Ion Irradiation

Ion irradiation creates optically active defects in wide-bandgap van der Waals materials, yet most approaches tune defect formation by varying the ion species, energy, or fluence while leaving the incidence geometry fixed. The ion-incidence angle is established here as a geometric control parameter for engineering visible emitters in hexagonal boron nitride (hBN). The angle and ion fluence of a plasma-focused heavy-ion (Xe+) beam are varied across hBN flakes of different thickness, and the resulting photoluminescence is quantified. In thick flakes, oblique irradiation shifts the fluence for maximum emission by nearly two orders of magnitude relative to normal incidence, whereas thin flakes exhibit an angle-independent optimum. Ion-trajectory simulations attribute this thickness dependence to lateral redistribution of the collision cascade and enhanced oblique sputtering. Atomic force microscopy identifies distinct processing regimes that delineate the useful defect-creation window. Post-irradiation annealing quenches the emission and shifts the spectral weight toward the green-yellow band while preserving the angle-dependent activation trends. Spectrally resolved lifetime measurements show comparable biexponential dynamics for normal and oblique incidence, consistent with emission from related defect families rather than a geometry-specific emitter species. These results establish ion-incidence geometry as a materials-level knob for programming optical defect activation and spatial defect distributions in van der Waals photonic materials.

physics.optics↗

arXiv2025

Quantum Coherence of Rare-Earth Ions in Heterogeneous Photonic Interfaces

Harnessing rare-earth ions in oxides for quantum networks requires integration with bright emitters in III-V semiconductors, but local disorder and interfacial noise limit their optical coherence. Here, we investigate the microscopic origins of the ensemble spectrum in Er$^{3+}$:TiO$_2$ epitaxial thin films on GaAs and GaSb substrates. Ab initio calculations combined with noise-Hamiltonian modeling and Monte Carlo simulations quantify the effects of interfacial and bulk spin noise and local strain on erbium crystal-field energies and inhomogeneous linewidths. Photoluminescence excitation spectroscopy reveals that Er$^{3+}$ ions positioned at increasing distances from the III-V/oxide interface produce a systematic blue shift of the $Y_1\rightarrow Z_1$ transition, consistent with strain relaxation predicted by theory. Thermal annealing produces a compensating redshift and linewidth narrowing, isolating the roles of oxygen-vacancy and gallium-diffusion noise. These results provide microscopic insight into disorder-driven decoherence, offering pathways for precise control of hybrid quantum systems for scalable quantum technologies.

quant-ph↗

arXiv2025

Controlled growth of rare-earth-doped TiO$_{2}$ thin films on III-V semiconductors for hybrid quantum photonic interfaces

Quantum photonic networks require two distinct functionalities: bright single-photon sources and long-lived quantum memories. III-V semiconductor quantum dots excel as deterministic and coherent photon emitters, while rare-earth ions such as erbium (Er$^{3+}$) in crystalline oxides offer exceptional spin and optical coherence at telecom wavelengths. Combining these systems and their functionalities via direct epitaxy is challenging due to lattice mismatch and incompatible growth conditions. Here we demonstrate low-temperature pulsed laser deposition of Er$^{3+}$-doped TiO$_{2}$ thin films directly on GaAs and GaSb substrates. Controlled surface preparation with an arsenic cap and an oxygen-deficient buffer layer enables the growth of epitaxial anatase TiO$_{2}$ (001) at 390$^{o}$C with sub-300 pm surface roughness, while avoiding interface degradation. In contrast, high-temperature oxide desorption or growth temperatures drive the transition to rough, polycrystalline rutile film, as confirmed by transmission electron microscopy. Minimal coincident interface area (MCIA) modeling explains the orientation-selective growth on GaAs and GaSb. Raman and cryogenic photoluminescence excitation spectroscopy verify the crystal phase and optical activation of Er$^{3+}$ ions. This multi-parameter growth strategy helps preserve III-V quantum dot functionality and yields smooth surfaces suitable for low-loss nanophotonic structures. Our results establish a materials platform for monolithically integrating rare-earth quantum memories with semiconductor photon sources, paving the way toward scalable hybrid quantum photonic chips.

quant-ph↗

arXiv2023

Hardware requirements for realizing a quantum advantage with deterministic single-photon sources

Boson sampling is a specialised algorithm native to the quantum photonic platform developed for near-term demonstrations of quantum advantage over classical computers. While clear useful applications for such near-term pre-fault-tolerance devices are not currently known, reaching a quantum advantage regime serves as a useful benchmark for the hardware. Here, we analyse and detail hardware requirements needed to reach quantum advantage with deterministic quantum emitters, a promising platform for photonic quantum computing. We elucidate key steps that can be taken in experiments to overcome practical constraints and establish quantitative hardware-level requirements. We find that quantum advantage is within reach using quantum emitters with an efficiency of 60%-70% and interferometers constructed according to a hybrid-mode-encoding architecture, constituted of Mach-Zehnder interferometers with an insertion loss of 0.0035 (a transmittance of 99.92%) per component.

quant-ph↗

arXiv2023

Independent operation of two waveguide-integrated quantum emitters

We demonstrate the resonant excitation of two quantum dots in a photonic integrated circuit for on-chip single-photon generation in multiple spatial modes. The two quantum dots are electrically tuned to the same emission wavelength using a pair of isolated $p$-$i$-$n$ junctions and excited by a resonant pump laser via dual-mode waveguides. We demonstrate two-photon quantum interference visibility of $(79\pm2)\%$ under continuous-wave excitation of narrow-linewidth quantum dots. Our work solves an outstanding challenge in quantum photonics by realizing the key enabling functionality of how to scale-up deterministic single-photon sources.

quant-ph↗

arXiv2023

Entanglement properties of a quantum-dot biexciton cascade in a chiral nanophotonic waveguide

We analyse the entanglement properties of deterministic path-entangled photonic states generated by coupling the emission of a quantum-dot biexciton cascade to a chiral nanophotonic waveguide, as implemented by Østfeldt et al. [PRX Quantum 3, 020363 (2022)]. We model the degree of entanglement through the concurrence of the two-photon entangled state in the presence of realistic experimental imperfections. The model accounts for imperfect chiral emitter-photon interactions in the waveguide and the asymmetric coupling of the exciton levels introduced by fine-structure splitting along with time-jitter in the detection of photons. The analysis shows that the approach offers a promising platform for deterministically generating entanglement in integrated nanophotonic systems in the presence of realistic experimental imperfections.

quant-ph↗

arXiv2023

Observation of light propagation through a three-dimensional cavity superlattice in a 3D photonic band gap

We experimentally investigate unusual light propagation inside a three-dimensional (3D) superlattice of resonant cavities that are confined within a 3D photonic band gap. Therefore, we fabricated 3D diamond-like photonic crystals from silicon with a broad 3D band gap in the near-infrared and doped them with a periodic array of point defects. In position-resolved reflectivity and scattering microscopy, we observe narrow spectral features that match well with superlattice bands in band structures computed with the plane wave expansion. The cavities are coupled in all three dimensions when they are closely spaced and uncoupled when they are further apart. The superlattice bands correspond to light that hops in high symmetry directions in 3D - so-called Cartesian Light - that opens applications in 3D photonic networks, 3D Anderson localization of light, and future 3D quantum photonic networks.

physics.optics↗

arXiv2022

On-demand source of dual-rail photon pairs based on chiral interaction in a nanophotonic waveguide

Entanglement is the fuel of advanced quantum technology. It is for instance consumed in measurement-based quantum computing and allows loss-tolerant encoding of quantum information. In photonics, entanglement has traditionally been generated probabilistically, requiring massive multiplexing for scaling up to many photons. An alternative approach utilizes quantum emitters in nanophotonic devices for deterministic generation of single photons, which an be extended to two- and multi-photon generation on demand. The proposed polarization-entanglement sources are, however, incompatible with spatial dual-rail qubit encoding, which is preferred in photonic quantum computing realized in scalable integrated photonic circuits. Here we propose and experimentally realize an on-demand source of dual-rail photon pairs using a quantum dot in a planar nanophotonic waveguide. The source exploits the cascaded decay of a biexciton state and chiral light-matter coupling to achieve deterministic generation of spatial dual-rail Bell pairs with the amount of entanglement determined by the chirality. The operational principle can readily be extended to multi-photon entanglement generation, and such sources may be interfaced with advanced photonic-integrated circuits, e.g., for efficient preparation of entanglement resource states for photonic quantum computing.

quant-ph↗

arXiv2022

A Pure and indistinguishable single-photon source at telecommunication wavelength

On-demand single-photon sources emitting pure and indistinguishable photons at the telecommunication wavelength are a critical asset towards the deployment of fiber-based quantum networks. Indeed, single photons may serve as flying qubits, allowing communication of quantum information over long distances. Self-assembled InAs quantum dots embedded in GaAs constitute an excellent nearly deterministic source of high quality single photons, but the vast majority of sources operate in the 900-950 nm wavelength range, precluding their adoption in a quantum network. Here, we present a quantum frequency conversion scheme for converting single photons from quantum dots to the telecommunication C band, around 1550 nm, achieving 40.8% end-to-end efficiency, while maintaining both high purity and a high degree of indistinguishability during conversion with measured values of $g^{(2)}(0)=2.4\%$ and $V^{\text{corr}}=94.8\%$, respectively.

quant-ph↗

arXiv2021

Single-photon quantum hardware: towards scalable photonic quantum technology with a quantum advantage

The scaling up of quantum hardware is the fundamental challenge ahead in order to realize the disruptive potential of quantum technology in information science. Among the plethora of hardware platforms, photonics stands out by offering a modular approach, where the main challenge is to construct sufficiently high-quality building blocks and develop methods to efficiently interface them. Importantly, the subsequent scaling-up will make full use of the mature integrated photonic technology provided by photonic foundry infrastructure to produce small foot-print quantum processors of immense complexity. A fully coherent and deterministic photon-emitter interface is a key enabler of quantum photonics, and can today be realized with solid-state quantum emitters with specifications reaching the quantitative benchmark referred to as Quantum Advantage. This light-matter interaction primer realizes a range of quantum photonic resources and functionalities, including on-demand single-photon and multi-photon entanglement sources, and photon-photon nonlinear quantum gates. We will present the current state-of-the-art in single-photon quantum hardware and the main photonic building blocks required in order to scale up. Furthermore, we will point out specific promising applications of the hardware building blocks within quantum communication and photonic quantum computing, laying out the road ahead for quantum photonics applications that could offer a genuine quantum advantage.

quant-ph↗

arXiv2021

Electroabsorption in gated GaAs nanophotonic waveguides

We report on the analysis of electroabsorption in thin GaAs/Al$_{0.3}$Ga$_{0.7}$As nanophotonic waveguides with an embedded $p$-$i$-$n$ junction. By measuring the transmission through waveguides of different lengths, we derive the propagation loss as a function of electric field, wavelength, and temperature. The results are in good agreement with the Franz-Keldysh model of electroabsorption extending over 200 meV below the GaAs bandgap, i.e. in the 910--970 nm wavelength range. We find a pronounced residual absorption in forward bias, which we attribute to Fermi-level pinning at the waveguide surface, producing over 20 dB/mm loss at room temperature. These results are essential for understanding the origin of loss in nanophotonic devices operating in the emission range of self-assembled InAs semiconductor quantum dots, towards the realization of scalable quantum photonic integrated circuits.

physics.optics↗

arXiv2020

Spatially shaping waves to penetrate deep inside a forbidden gap

It is well known that waves incident upon a crystal are transported only over a limited distance - the Bragg length - before being reflected by Bragg interference. Here, we demonstrate how to send waves much deeper into crystals, by studying light in exemplary two-dimensional silicon photonic crystals. By spatially shaping the optical wavefronts, we observe that the intensity of laterally scattered light, that probes the internal energy density, is enhanced at a tunable distance away from the front surface. The intensity is up to $100 \times$ enhanced compared to random wavefronts and extends as far as $8 \times$ the Bragg length. Our novel steering of waves inside a forbidden gap exploits the transport channels induced by unavoidable deviations from perfect periodicity, here unavoidable fabrication deviations.

physics.optics↗

arXiv2020

Near Transform-limited Quantum Dot Linewidths in a Broadband Photonic Crystal Waveguide

Planar nanophotonic structures enable broadband, near-unity coupling of emission from quantum dots embedded within, thereby realizing ideal singe-photon sources. The efficiency and coherence of the single-photon source is limited by charge noise, which results in the broadening of the emission spectrum.We report suppression of the noise by fabricating photonic crystal waveguides in a gallium arsenide membrane containing quantum dots embedded in a $p$-$i$-$n$ diode. Local electrical contacts in the vicinity of the waveguides minimize the leakage current and allow fast electrical control ($\approx$4 MHz bandwidth) of the quantum dot resonances. Resonant linewidth measurements of $79$ quantum dots coupled to the photonic crystal waveguides exhibit near transform-limited emission over a 6 nm wide range of emission wavelengths. Importantly, the local electrical contacts allow independent tuning of multiple quantum dots on the same chip, which together with the transform-limited emission are key components in realizing multiemitter-based quantum information processing.

quant-ph↗

arXiv2020

Scalable integrated single-photon source

Photonic qubits are key enablers for quantum-information processing deployable across a distributed quantum network. An on-demand and truly scalable source of indistinguishable single photons is the essential component enabling high-fidelity photonic quantum operations. A main challenge is to overcome noise and decoherence processes in order to reach the steep benchmarks on generation efficiency and photon indistinguishability required for scaling up the source. We report on the realization of a deterministic single-photon source featuring near-unity indistinguishability using a quantum dot in an 'on-chip' planar nanophotonic waveguide circuit. The device produces long strings of $>100$ single photons without any observable decrease in the mutual indistinguishability between photons. A total generation rate of $122$ million photons per second is achieved corresponding to an 'on-chip' source efficiency of $84 \%$. These specifications of the single-photon source are benchmarked for boson sampling and found to enable scaling into the regime of quantum advantage.

quant-ph↗

arXiv2020

On-chip deterministic operation of quantum dots in dual-mode waveguides for a plug-and-play single-photon source

A deterministic source of coherent single photons is an enabling device of quantum-information processing for quantum simulators, and ultimately a full-fledged quantum internet. Quantum dots (QDs) in nanophotonic structures have been employed as excellent sources of single photons, and planar waveguides are well suited for scaling up to multiple photons and emitters exploring near-unity photon-emitter coupling and advanced active on-chip functionalities. An ideal single-photon source requires suppressing noise and decoherence, which notably has been demonstrated in electrically-contacted heterostructures. It remains a challenge to implement deterministic resonant excitation of the QD required for generating coherent single photons, since residual light from the excitation laser should be suppressed without compromising source efficiency and scalability. Here, we present the design and realization of a novel planar nanophotonic device that enables deterministic pulsed resonant excitation of QDs through the waveguide. Through nanostructure engineering, the excitation light and collected photons are guided in two orthogonal waveguide modes enabling deterministic operation. We demonstrate a coherent single-photon source that simultaneously achieves high-purity ($g^{(2)}(0)$ = 0.020 $\pm$ 0.005), high-indistinguishability ($V$ = 96 $\pm$ 2 %), and $>$80 % coupling efficiency into the waveguide. The novel `plug-and-play' coherent single-photon source could be operated unmanned for several days and will find immediate applications, e.g., for constructing heralded multi-photon entanglement sources for photonic quantum computing or sensing.

quant-ph↗

arXiv2019

On-chip nanomechanical filtering of quantum-dot single-photon sources

Semiconductor quantum dots in photonic integrated circuits enable scaling quantum-information processing to many single photons and quantum-optical gates. On-chip spectral filters are essential to achieve high-purity and coherent photon emission from quantum dots embedded in waveguides, without resorting to free-space optics. Such spectral filters should be tunable, to compensate for the inhomogeneous spectral distribution of the quantum dots transitions. Here, we report an on-chip filter monolithically integrated with quantum dots, that uses nanomechanical motion for tuning its resonant wavelength over 10 nm, enabling operation at cryogenic temperatures and avoiding cross-talk with the emitter. We demonstrate single-photon emission from a quantum dot under non-resonant excitation by employing only the on-chip filter. These results are key for the development of fully-integrated de-multiplexing, multi-path photon encoding schemes, and multi-emitter circuits.

physics.app-ph↗

arXiv2019

Experimental probe of a complete 3D photonic band gap

The identification of a complete three-dimensional (3D) photonic band gap in real crystals always employs theoretical or numerical models that invoke idealized crystal structures. Thus, this approach is prone to false positives (gap wrongly assigned) or false negatives (gap missed). Therefore, we propose a purely experimental probe of the 3D photonic band gap that pertains to many different classes of photonic materials. We study position and polarization-resolved reflectivity spectra of 3D inverse woodpile structures that consist of two perpendicular nanopore arrays etched in silicon. We observe intense reflectivity peaks $(R > 90\%)$ typical of high-quality crystals with broad stopbands. We track the stopband width versus pore radius, which agrees much better with the predicted 3D photonic band gap than with a directional stop gap on account of the large numerical aperture used. A parametric plot of s-polarized versus p-polarized stopband width agrees very well with the 3D band gap and is model-free. This practical probe provides fast feedback on the advanced nanofabrication needed for 3D photonic crystals and stimulates practical applications of band gaps in 3D silicon nanophotonics and photonic integrated circuits, photovoltaics, cavity QED, and quantum information processing.

physics.optics↗

arXiv2019

Suspended Spot-Size Converters for Scalable Single-Photon Devices

We report on the realization of a highly efficient optical spot-size converter for the end-face coupling of single photons from GaAs-based nanophotonic waveguides with embedded quantum dots. The converter is realized using an inverted taper and an epoxy polymer overlay providing a 1.3~$μ$m output mode field diameter. We demonstrate the collection of single photons from a quantum dot into a lensed fiber with a rate of 5.84$\pm0.01$~MHz and estimate a chip-to-fiber coupling efficiency of $\sim48$~\%. The stability and compatibility with cryogenic temperatures make the epoxy waveguides a promising material to realize efficient and scalable interconnects between heterogeneous quantum photonic integrated circuits.

physics.app-ph↗