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Raymond C. Ashoori

Publications and source records attributed to Raymond C. Ashoori.

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1/3 Fractional and Gapless Integer Quantum Anomalous Hall States in Rhombohedral Graphene

The fractional quantum anomalous Hall (FQAH) effect occurs in moiré superlattices in both twisted bilayer MoTe$_2$ and rhombohedral $n$-layer graphene aligned to hexagonal boron nitride (R$n$G/hBN) as a novel quantum phase driven by intertwined electron correlation and topology. Although several fractional states in the Jain sequence have been identified, the $1/3$ state, the most robust and fundamental state in conventional fractional quantum Hall (FQH) systems, was missing in either FQAH system. Determining whether it exists would have a major impact on understanding the mechanism of FQAH, especially in the theoretically still-debated R$n$G/hBN system. Here we report the FQAH effect at moiré filling factor $ν= 1/3$ in R$5$G/hBN moiré superlattice devices, through a combination of quantum capacitance and transport measurements. By tuning the displacement field, we observed a topological phase transition from a $1/3$ fractional Chern insulator (FCI) to a trivial charge density wave state. With the inclusion of the $1/3$ state, the FQAH states in R$5$G/hBN now exhibit a surprising level of particle-hole symmetry about half-filling, closely resembling the behavior of FQH states in the lowest Landau level. Additionally, we perform compressibility and transport measurements at a filling of one electron per moiré unit cell, $ν=1$, and also for $ν\lesssim 1$, where previous transport measurements displayed the extended quantum anomalous Hall (EQAH) effect. While our transport measurements show no change between the integer quantum anomalous Hall state (IQAH) and the EQAH region, compressibility measurements reveal a distinct transition from a gapped IQAH state to a gapless and highly compressible EQAH state. Our direct thermodynamic characterization of the rich phase diagram paves the way to engineering of anyon braiding and non-Abelian quasiparticles at zero magnetic field.

cond-mat.mes-hall

Displacement field-controlled fractional Chern insulators and charge density waves in a graphene/hBN moiré superlattice

Rhombohedral multilayer graphene, with its flat electronic bands and concentrated Berry curvature, is a promising material for the realization of correlated topological phases of matter. When aligned to an adjacent hexagonal boron nitride (hBN) layer, the graphene develops narrow minibands with non-trivial topology. By tuning an externally-applied electric displacement field, the conduction electrons can either be pushed towards or away from the moiré superlattice. Motivated by the recent observation of the fractional quantum anomalous Hall effect (FQAHE) in the moiré-distant case, we study the opposite moiré-proximal case, where the superlattice potential is considerably stronger. We explore the physics within the moiré conduction bands through capacitance measurements that allow us to determine the inverse electronic compressibility and extract energy gaps of incompressible states. We observe integer and fractional Chern insulator states at superlattice filling factors v = 1, 2/3, and 1/3 with Streda slopes of -1, -2/3, and -1/3, respectively. Remarkably, the v = 1/3 state persists down to a magnetic field of 0.2 T. In addition, we also observe numerous trivial and topological charge density waves. We map out a phase diagram that is highly sensitive to both displacement and magnetic fields, which tune the system between various ground states by modifying the band dispersion and the structure of the electronic wavefunctions. This work demonstrates displacement field control of topological phase transitions in the moiré-proximal limit of rhombohedral pentalayer graphene, creating a highly-tunable platform for studying the interplay between intrinsic band topology and strong lattice effects.

cond-mat.mes-hall

Superconductivity and strong interactions in a tunable moiré quasiperiodic crystal

Electronic states in quasiperiodic crystals generally preclude a Bloch description, rendering them simultaneously fascinating and enigmatic. Owing to their complexity and relative scarcity, quasiperiodic crystals are underexplored relative to periodic and amorphous structures. Here, we introduce a new type of highly tunable quasiperiodic crystal easily assembled from periodic components. By twisting three layers of graphene with two different twist angles, we form two moiré patterns with incommensurate moiré unit cells. In contrast to many common quasiperiodic structures that are defined on the atomic scale, the quasiperiodicity in our system is defined on moiré length scales of several nanometers. This novel "moiré quasiperiodic crystal" allows us to tune the chemical potential and thus the electronic system between a periodic-like regime at low energies and a strongly quasiperiodic regime at higher energies, the latter hosting a large density of weakly dispersing states. Interestingly, in the quasiperiodic regime we observe superconductivity near a flavor-symmetry-breaking phase transition, the latter indicative of the important role electronic interactions play in that regime. The prevalence of interacting phenomena in future systems with in situ tunability is not only useful for the study of quasiperiodic systems, but it may also provide insights into electronic ordering in related periodic moiré crystals. We anticipate that extending this new platform to engineer quasiperiodic crystals by varying the number of layers and twist angles, and by using different two-dimensional components, will lead to a new family of quantum materials to investigate the properties of strongly interacting quasiperiodic crystals.

cond-mat.mes-hall

Strong interlayer charge transfer due to exciton condensation in an electrically-isolated GaAs quantum well bilayer

We introduce a design of electrically isolated floating bilayer GaAs quantum wells (QW) in which application of a large gating voltage controllably and highly reproducibly induces charges that remain trapped in the bilayer after removal of the gating voltage. At smaller gate voltages, the bilayer is fully electrically isolated from external electrodes by thick insulating barriers. This design permits full control of the total and differential densities of two coupled 2D electron systems. The floating bilayer design provides a unique approach for studying systems inaccessible by simple transport measurements. It also provides the ability to measure the charge transfer between the layers, even when the in-plane resistivities of the 2D systems diverge. We measure the capacitance and inter-layer tunneling spectra of the QW bilayer with independent control of the top and bottom layer electron densities. Our measurements display strongly enhanced inter-layer tunneling current at the total filling factor of 1, a signature of exciton condensation of a strongly interlayer-correlated bilayer system. With fully tunable densities of individual layers, the floating bilayer QW system provides a versatile platform to access previously unavailable information on the quantum phases in electron bilayer systems.

cond-mat.mes-hall

Sharp Tunneling Resonance from the Vibrations of an Electronic Wigner Crystal

Photoemission and tunneling spectroscopies measure the energies at which single electrons can be added to or removed from an electronic system. Features observed in such spectra have revealed electrons coupling to vibrational modes of ions both in solids and in individual molecules. Here we report the discovery of a sharp resonance in the tunneling spectrum of a 2D electron system. Its behavior suggests that it originates from vibrational modes, not involving ionic motion, but instead arising from vibrations of spatial ordering of the electrons themselves. In a two-dimensional electronic system at very low temperatures and high magnetic fields, electrons can either condense into a variety of quantum Hall phases or arrange themselves into a highly ordered Wigner crystal lattice. Such spatially ordered phases of electrons are often electrically insulating and delicate and have proven very challenging to probe with conventional methods. Using a unique pulsed tunneling method capable of probing electron tunneling into insulating phases, we observe a sharp peak with dependencies on energy and other parameters that fit to models for vibrations of a Wigner crystal. The remarkable sharpness of the structure presents strong evidence of the existence of a Wigner crystal with long correlation length.

cond-mat.str-el