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Ren-Bao Liu

Publications and source records attributed to Ren-Bao Liu.

At least 37 records · Page 2Linked to original sources

Effects of local decoherence on quantum critical metrology

The diverging responses to parameter variations of systems at quantum critical points motivate schemes of quantum metrology that feature sub-Heisenberg scaling of the sensitivity with the system size (e.g., the number of particles). This sensitivity enhancement is fundamentally rooted in the formation of Schrödinger cat states, or macroscopic superposition states at the quantum critical points. The cat states, however, are fragile to decoherence caused by local noises on individual particles or coupling to local environments, since the local decoherence of any particle would cause the collapse of the whole cat state. Therefore, it is unclear whether the sub-Heisenberg scaling of quantum critical metrology is robust against the local decoherence. Here we study the effects of local decoherence on the quantum critical metrology, using a one-dimensional transverse-field Ising model as a representative example. Based on a previous work [Phys. Rev. Lett. 94, 047201 (2005)] on the critical behaviors of the noisy Ising model, which shows that the universality class of the quantum criticality is modified by the decoherence, we find that the standard quantum limit is recovered by the single-particle decoherence, which is equivalent to local quantum measurement conducted by the environment and destroys the many-body entanglement in the ground state at the quantum critical point. Following the renormalization group analysis [Phys. Rev. B 69, 054426 (2004)], we argue that the noise effects on quantum critical metrology should be universal. This works demonstrates the importance of protecting macroscopic quantum coherence for quantum sensing based on critical behaviors.

quant-ph↗

Collision-induced spin noise

Collision phenomena are ubiquitous and of importance in determining the microscopic structures and intermolecular interactions of atoms and molecules. The existing approaches are mostly based on atomic or molecular scatterings, which are hindered by the inconvenience of using ultra-high vacuum and low temperature systems. Here we demonstrate a new spin-noise spectroscopic approach by measuring optical polarization rotation noise of the probe light, which operates with simple apparatus and ambient conditions. Our approach features tens of gigahertz bandwidth and one part-per-million resolution, outperforming existing spin-noise techniques. Enabled by the new technique, we observe the collision-induced spin noise of alkali atoms, and precisely determine key collision parameters, such as collision diameter, well depth, and dominant interaction type. Our work provides a new tool to study a broad range of collision phenomena under ambient conditions.

quant-ph↗

Unification of valley and anomalous Hall effects in a strained lattice

Two dimensional lattices are an important stage for studying many aspects of quantum physics, in particular the topological phases. The valley Hall and anomalous Hall effects are two representative topological phenomena. Here we show that they can be unified in a strained honeycomb lattice, where the hopping strengths between neighboring sites are designed by mimicking those between the Fock states in a three-mode Jaynes-Cummings model. Such a strain induces an effective magnetic field which results in quantized Landau levels. The eigenstates in the zeroth Landau level can be represented by the eigenstates of a large pseudo-spin. We find that the valley Hall current and the chiral edge current in the Haldane model correspond to the spin precession around different axes. Our study sheds light on connection between seemingly unrelated topological phases in condensed matter physics.

cond-mat.mes-hall↗

Berry phases of higher spins due to internal geometry of Majorana constellation and relation to quantum entanglement

Majorana stars, the antipodal directions associated with the coherent states that are orthogonal to a spin state, provide a visualization and a geometric understanding of the structures of general quantum states. For example, the Berry phase of a spin-1/2 is given by half the solid angle enclosed by the close path of its Majorana star. It is conceivable that the Berry phase of higher spins may also be related to the geometry of the Majorana constellation. We find that for a spin-1 state, besides the expected contributions from the solid angles enclosed by the close paths of the two Majorana stars, the Berry phase includes a term related to the twist of the relative position vector around the barycenter vector of the two Majorana stars, i.e., the self-rotation of the constellation. Interestingly, if the spin-1 state is taken as a symmetrized two-qubit state, the extra contribution to the Berry phase is given by the self-rotation of the Majorana constellation weighted by the quantum entanglement of the two qubits. This discovery alludes to the relevance of the Majorana stellar geometry in representing the deep structures of quantum states and of quantum entanglement.

quant-ph↗

Cluster-correlation expansion for studying decoherence of clock transitions in spin baths

The clock transitions (CTs) of central spins have long coherence times because their frequency fluctuations vanish in the linear order of external field noise (such as Overhauser fields from nuclear spin baths). Therefore, CTs are useful for quantum technologies. Also, the quadratic dependence of frequencies on noises makes the CT decoherence an interesting physics problem. Thus we are motivated to study the decoherence of CTs. We consider noise from spin baths, which is one of the most relevant mechanisms of qubit decoherence. Various quantum many-body methods have been developed to study the decoherence of a central spin in spin baths. In particular, the cluster-correlation expansion (CCE) systematically accounts for the many-body correlations that cause the central spin decoherence. However, the CCE can not be straightforwardly applied to CTs in spin baths, for the expansion may fail to converge due to the effective long-range interactions resulting from the quadratic term of the noise (e.g., the second-order interaction mediated by hyperfine interactions for a nuclear spin bath). In this work, we develop a modified CCE method to tackle this class of decoherence problems. By diagonalizing the central spin Hamiltonian for each bath eigenstate of the hyperfine interaction, we find that the effects of long-range interactions are absorbed as fluctuations of central spin eigenenergies in the form of single-spin correlations. We apply the method to two specific systems, namely, nitrogen vacancy center electron spins in near zero magnetic field and singlet-triplet transition of two electrons in a double quantum dot. The numerical simulation shows that the modified CCE converges rapidly for the CTs.

quant-ph↗

Three-Tangle of a General Three-Qubit State in the Representation of Majorana Stars

Majorana stars, the $2j$ spin coherent states that are orthogonal to a spin-$j$ state, offer a visualization of general quantum states and may disclose deep structures in quantum states and their evolutions. In particular, the genuine tripartite entanglement - the three-tangle of a symmetric three-qubit state, which can be mapped to a spin-3/2 state, is measured by the normalized product of the distance between the Majorana stars. However, the Majorana representation cannot applied to general non-symmetric $n$-qubit states. We show that after a series of SL$(2,\mathbb{C})$ transformations, non-symmetric three-qubit states can be transformed to symmetric three-qubit states, while at the same time the three-tangle is unchanged. Thus the genuine tripartite entanglement of general three-qubit states has the geometric representation of the associated Majorana stars. The symmetrization and hence the Majorana star representation of certain genuine high-order entanglement for more qubits are possible for some special states. In general cases, however, the constraints on the symmetrization may prevent the Majorana star representation of the genuine entanglement.

quant-ph↗

Ultra-sensitive hybrid diamond nanothermometer

Nitrogen-vacancy (NV) centers in diamond are promising quantum sensors for their long spin coherence time under ambient conditions. However, their spin resonances are relatively insensitive to non-magnetic parameters such as temperature. A magnetic-nanoparticle-nanodiamond hybrid thermometer, where the temperature change is converted to the magnetic field variation near the Curie temperature, was demonstrated to have enhanced temperature sensitivity (11 mK Hz^{-1/2}) [Phys. Rev. X 8, 011042 (2018)], but the sensitivity was limited by the large spectral broadening of ensemble spins in nanodiamonds. To overcome this limitation, here we showed an improved design of a hybrid nanothermometer using a single NV center in a diamond nanopillar coupled with a single magnetic nanoparticle of copper-nickel alloy, and demonstrated a temperature sensitivity of 76 uK Hz^{-1/2}. This hybrid design enabled detection of 2 millikelvins temperature changes with temporal resolution of 5 milliseconds. The ultra-sensitive nanothermometer offers a new tool to investigate thermal processes in nanoscale systems.

quant-ph↗

Characterization of arbitrary-order correlations in quantum baths by weak measurement

Correlations of fluctuations are the driving forces behind the dynamics and thermodynamics in quantum many-body systems. For qubits embedded in a quantum bath, the correlations in the bath are the key to understanding and combating decoherence -a critical issue in quantum information technology. However, there is no systematic method for characterizing the many-body correlations in quantum baths beyond the second order or the Gaussian approximation. Here we present a scheme to characterize the correlations in a quantum bath to arbitrary order. The scheme employs weak measurement of the bath via projective measurement of a central system. The bath correlations, including both the "classical" and the "quantum" parts, can be reconstructed from the correlations of the measurement outputs. The possibility of full characterization of many-body correlations in a quantum bath forms the basis for optimizing quantum control against decoherence in realistic environments, for studying the quantum characteristics of baths, and for quantum sensing of correlated clusters in quantum baths.

quant-ph↗

Nanometer-precision non-local deformation reconstruction using nanodiamond orientation sensing

Information of material deformation upon loading is critical to evaluate mechanical properties of materials in general, and key to understand fundamental mechano-stimuli induced response of live systems in particular. Conventionally, such information is obtained at macroscopic scale about averaged properties, which misses the important details of deformation at individual structures; or at nanoscale with localized properties accessed, which misses the information of deformation at locations away from the force-loading positions. Here we demonstrate that an integration of nanodiamond orientation sensing and AFM nanoindentation offers a complementary approach to the nonlocal reconstruction of material deformation. This approach features a 5 nm precision in the loading direction and a sub-hundred nanometer lateral resolution. Using this tool, we mapped out the deformation of a PDMS thin film in air and that of the gelatin microgel particles in water, with precision high enough to disclose the significance of the surface/interface effects in the material deformation. The non-local nanometer-precision sensing of deformation upon a local impact brings in new opportunities in studying mechanical response of complex material systems.

cond-mat.mes-hall↗

Quantum coherence control at near 1000 K

Quantum coherence control usually requires extremely low temperature environments. Even for spins in diamond, a remarkable exception, the coherence signal is lost as temperature approaches 700 K. Here we demonstrate quantum coherence control of the electron spins of nitrogen-vacancy centers in nanodiamonds at temperatures near 1000 K. The scheme is based on initialization and readout of the spins at room temperature and control at high temperature, which is enabled by pulse laser heating and rapid diffusion cooling of nanodiamonds on amorphous carbon films. Using high-temperature spin control, we observe the magnetic phase transition of a single nickel nanoparticle at about 615 K. This work enables nano-thermometry and nano-magnetometry in the high-temperature regime.

quant-ph↗

Sensitivity of parameter estimation near the exceptional point of a non-Hermitian system

The exceptional points of non-Hermitian systems, where $n$ different energy eigenstates merge into an identical one, have many intriguing properties that have no counterparts in Hermitian systems. In particular, the $ε^{1/n}$ dependence of the energy level splitting on a perturbative parameter $ε$ near an $n$-th order exceptional point stimulates the idea of metrology with arbitrarily high sensitivity, since the susceptibility $dε^{1/n}/dε$ diverges at the exceptional point. Here we theoretically study the sensitivity of parameter estimation near the exceptional points, using the exact formalism of quantum Fisher information. The quantum Fisher information formalism allows the highest sensitivity to be determined without specifying a specific measurement approach. We find that the exceptional point bears no dramatic enhancement of the sensitivity. Instead, the coalescence of the eigenstates exactly counteracts the eigenvalue susceptibility divergence and makes the sensitivity a smooth function of the perturbative parameter.

quant-ph↗

High-resolution spectroscopy of single nuclear spins via sequential weak measurements

Quantum sensors have recently achieved to detect the magnetic moment of few or single nuclear spins and measure their magnetic resonance (NMR) signal. However, the spectral resolution, a key feature of NMR, has been limited by relaxation of the sensor to a few kHz at room temperature. The spectral resolution of NMR signals from single nuclear spins can be improved by, e.g., using quantum memories, however at the expense of sensitivity. Classical signals on the other hand can be measured with exceptional spectral resolution by using continuous measurement techniques, without compromising sensitivity. To apply these techniques to single-spin NMR, it is critical to overcome the impact of back action inherent of quantum measurements. Here we report sequential weak measurements on a single $^{13}$C nuclear spin. The back-action of repetitive weak measurements causes the spin to undergo a quantum dynamics phase transition from coherent trapping to coherent oscillation. Single-spin NMR at room-temperature with a spectral resolution of 3.8 Hz is achieved. These results enable the use of measurement-correlation schemes for the detection of very weakly coupled single spins.

quant-ph↗

Phase transitions in sequential weak measurements

Quantum measurements and phase transitions are seemingly uncorrelated topics, but here we show that phase transitions occur in sequential quantum measurements. We find that the probability distribution of the measurement results of a sequence of quantum measurements on a two-level system (e.g. a qubit) is equivalent to the Boltzmann distribution of a classical lattice spin model. So the measurement results present phase transitions similar to those in the lattice spin model. In sequential commuting positive-operator valued measurements, the probability distribution is mapped to a long-range Ising model in the weak-measurement regime, and a projective measurement emerges from a sequence of weak measurement when the strength or the number of measurements becomes above certain critical values, which correspond to a second-order ferromagnetic phase transition of the lattice spin model. These findings not only provide new insights on sequential quantum measurements, but may also have potential applications in quantum technologies.

quant-ph↗

Dynamical birefringence: Electron-hole recollisions as probes of Berry curvature

The direct measurement of Berry phases is still a great challenge in condensed matter systems. The bottleneck has been the ability to adiabatically drive an electron coherently across a large portion of the Brillouin zone in a solid where the scattering is strong and complicated. We break through this bottleneck and show that high-order sideband generation (HSG) in semiconductors is intimately affected by Berry phases. Electron-hole recollisions and HSG occur when a near-band gap laser beam excites a semiconductor that is driven by sufficiently strong terahertz (THz)-frequency electric fields. We carried out experimental and theoretical studies of HSG from three GaAs/AlGaAs quantum wells. The observed HSG spectra contain sidebands up to the 90th order, to our knowledge the highest-order optical nonlinearity observed in solids. The highest-order sidebands are associated with electron-hole pairs driven coherently across roughly 10% of the Brillouin zone around the Γpoint. The principal experimental claim is a dynamical birefringence: the sidebands, when the order is high enough (> 20), are usually stronger when the exciting near-infrared (NIR) and the THz electric fields are polarized perpendicular than parallel; the sideband intensities depend on the angles between the THz field and the crystal axes in samples with sufficiently weak quenched disorder; and the sidebands exhibit significant ellipticity that increases with increasing sideband order, despite nearly linear excitation and driving fields. We explain dynamical birefringence by generalizing the three-step model for high order harmonic generation. The hole accumulates Berry phases due to variation of its internal state as the quasi-momentum changes under the THz field. Dynamical birefringence arises from quantum interference between time-reversed pairs of electron-hole recollision pathways.

cond-mat.mtrl-sci↗

Magnetic criticality-enhanced hybrid nanodiamond-thermometer under ambient conditions

Nitrogen vacancy (NV) centres in diamond are attractive as quantum sensors owing to their superb coherence under ambient conditions. However, the NV centre spin resonances are relatively insensitive to some important parameters such as temperature. Here we design and experimentally demonstrate a hybrid nano-thermometer composed of NV centres and a magnetic nanoparticle (MNP), in which the temperature sensitivity is enhanced by the critical magnetization of the MNP near the ferromagnetic-paramagnetic transition temperature. The temperature susceptibility of the NV center spin resonance reached 14 MHz/K, enhanced from the value without the MNP by two orders of magnitude. The sensitivity of a hybrid nano-thermometer composed of a Cu_{1-x}Ni_{x} MNP and a nanodiamond was measured to be 11 mK/Hz^{1/2} under ambient conditions. With such high-sensitivity, we monitored nanometer-scale temperature variation of 0.3 degree with a time resolution of 60 msec. This hybrid nano-thermometer provides a novel approach to studying a broad range of thermal processes at nanoscales such as nano-plasmonics, sub-cellular heat-stimulated processes, thermodynamics of nanostructures, and thermal remanent magnetization of nanoparticles.

quant-ph↗

Quantum many-body theory for electron spin decoherence in nanoscale nuclear spin baths

Decoherence of electron spins in nanoscale systems is important to quantum technologies such as quantum information processing and magnetometry. It is also an ideal model problem for studying the crossover between quantum and classical phenomena. At low temperatures or in light-element materials where the spin-orbit coupling is weak, the phonon scattering in nanostructures is less important and the fluctuations of nuclear spins become the dominant decoherence mechanism for electron spins. Since 1950s, semiclassical noise theories have been developed for understanding electron spin decoherence. In spin-based solid-state quantum technologies, the relevant systems are in the nanometer scale and the nuclear spin baths are quantum objects which require a quantum description. Recently, quantum pictures have been established to understand the decoherence and quantum many-body theories have been developed to quantitatively describe this phenomenon. Anomalous quantum effects have been predicted and some have been experimentally confirmed. A systematically truncated cluster correlation expansion theory has been developed to account for the many-body correlations in nanoscale nuclear spin baths that are built up during the electron spin decoherence. The theory has successfully predicted and explained a number of experimental results in a wide range of physical systems. In this review, we will cover these recent progresses. The limitations of the present quantum many-body theories and possible directions for future development will also be discussed.

cond-mat.mes-hall↗

Single-Shot Readout of a Nuclear Spin Weakly Coupled to a Nitrogen-Vacancy Center

Single-shot readout of qubits is required for scalable quantum computing. Nuclear spins are superb quantum memories due to their long coherence times but are difficult to be read out in single shot due to their weak interaction with probes. Here we demonstrate single-shot readout of a weakly coupled $^{13}$C nuclear spin, which is unresolvable in traditional protocols. We use dynamical decoupling pulse sequences to selectively enhance the entanglement between the nuclear spin and a nitrogen-vacancy center electron spin, tuning the weak measurement of the nuclear spin to a strong, projective one. A nuclear spin coupled to the NV center with strength 330 kHz is read out in 200 ms with fidelity 95.5\%. This work provides a general protocol for single-shot readout of weakly coupled qubits and therefore largely extends the range of physical systems for scalable quantum computing.

quant-ph↗

Proposal for Quantum Sensing Based on Two-Dimensional Dynamical Decoupling: NMR Correlation Spectroscopy of Single Molecules

Nuclear magnetic resonance (NMR) has enormous applications. Two-dimensional NMR is an essential technique to characterize correlations between nuclei and, hence, molecule structures. Towards the ultimate goal of single-molecule NMR, dynamical-decoupling- (DD) enhanced diamond quantum sensing enables the detection of single nuclear spins and nanoscale NMR. However, there is still the lack of a standard method in DD-based quantum sensing to characterize correlations between nuclear spins in single molecules. Here we present a scheme of two-dimensional DD-based quantum sensing, as a universal method for correlation spectroscopy of single molecules. We design two-dimensional DD sequences composed of two sets of periodic DD sequences with different periods, which can be independently set to match two different transition frequencies for resonant DD. We find that under the resonant DD condition the sensor coherence patterns, as functions of the two independent pulse numbers of DD subsequences, can fully determine different types of correlations between nuclear spin transitions. This work offers a systematic approach to correlation spectroscopy for single-molecule NMR.

quant-ph↗