arXiv subjects

Ren-Bao Liu

Publications and source records attributed to Ren-Bao Liu.

At least 73 records · Page 4Linked to original sources

arXiv2014

Quantum coherence induced second plateau in high-sideband generation

Optically excited electron-hole pairs, driven by a strong terahertz (THz) field, create high-sidebands in the optical spectrum. The sideband spectrum exhibits a 'plateau' up to a cutoff of 3.17Up, where Up is the ponderomotive energy. This cutoff is determined, semi-classically, from the maximum kinetic energy an electron-hole pair can gain from the THz field along a closed trajectory. A full quantum treatment reveals a second, classically forbidden, plateau with a cutoff of 8Up, the maximum kinetic energy an electron-hole pair can gain from the THz field along an open trajectory. The second plateau appears because a spatially separated electron and hole can still recombine if the classical excursion is within the coherence length of the electron-hole wavefunction or, equivalently, the coherence time is longer than the excursion time (half the THz field period). This effect broadens the range of materials and excitation conditions where high-sideband generations can occur, thereby providing a wealth of novel systems for ultrafast electro-optical applications.

cond-mat.mes-hall↗

arXiv2014

Observation of Lee-Yang zeros

Lee-Yang zeros are points on the complex plane of magnetic field where the partition function of a spin system is zero and therefore the free energy diverges. Lee-Yang zeros and their generalizations are ubiquitous in many-body systems and they fully characterize the analytic properties of the free energy and hence thermodynamics of the systems. Determining the Lee-Yang zeros is not only fundamentally important for conceptual completeness of thermodynamics and statistical physics but also technically useful for studying many-body systems. However, Lee-Yang zeros have never been observed in experiments, due to the intrinsic difficulty that Lee-Yang zeros would occur only at complex values of magnetic field, which are unphysical. Here we report the first observation of Lee-Yang zeros, by measuring quantum coherence of a probe spin coupled to an Ising-type spin bath. As recently proposed, the quantum evolution of the probe spin introduces a complex phase factor, and therefore effectively realizes an imaginary magnetic field on the bath. From the measured Lee-Yang zeros, we reconstructed the free energy of the spin bath and determined its phase transition temperature. This experiment demonstrates quantum coherence probe as a useful approach to studying thermodynamics in the complex plane, which may reveal a broad range of new phenomena that would otherwise be inaccessible if physical parameters are restricted to be real numbers.

quant-ph↗

arXiv2014

Faraday rotation echo spectroscopy and detection of quantum fluctuations

Central spin decoherence is useful for detecting many-body physics in environments and moreover, the spin echo control can remove the effects of static thermal fluctuations so that the quantum fluctuations are revealed. The central spin decoherence approach, however, is feasible only in some special configurations and often requires uniform coupling between the central spin and individual spins in the baths, which are very challenging in experiments. Here, by making analogue between central spin decoherence and depolarization of photons, we propose a scheme of Faraday rotation echo spectroscopy (FRES) for studying quantum fluctuations in interacting spin systems. The echo control of the photon polarization is realized by flipping the polarization with a birefringence crystal. The FRES, similar to spin echo in magnetic resonance spectroscopy, can suppress the effects of the static magnetic fluctuations and therefore reveal dynamical magnetic fluctuations. We apply the scheme to a rare-earth compound LiHoF4 and calculate the echo signal, which is related to the quantum fluctuations of the system. We observe enhanced signals at the phase boundary. The FRES should be useful for studying quantum fluctuations in a broad range of spin systems, including cold atoms, quantum dots, solid-state impurities, and transparent magnetic materials.

cond-mat.mes-hall↗

arXiv2014

Dynamical decoupling design for identifying weakly coupled nuclear spins in a bath

Identifying weakly coupled nuclear spins around single electron spins is a key step of implementing quantum information processing using coupled electron-nuclei spin systems or sensing like single spin nuclear magnetic resonance detection using diamond defect spins. Dynamical decoupling control of the center electron spin with periodic pulse sequences [e.g., the Carre-Purcell-Meiboom-Gill (CPMG) sequence] has been successfully used to identify single nuclear spins and to resolve structure of nuclear spin clusters. Here, we design a new type of pulse sequences by replacing the repetition unit (a single $π$-pulse) of the CPMG sequence with a group of nonuniformly-spaced $π$-pulses. Using nitrogen-vacancy center system in diamond, we show that the designed pulse sequence improves the resolution of nuclear spin noise spectroscopy, and more information about the surrounding nuclear spins is extracted. The principle of dynamical decoupling design proposed in this paper is useful in many systems (e.g., defect spin qubit in solids, trapped ion and superconducting qubit) for high-resolution noise spectroscopy.

cond-mat.mes-hall↗

arXiv2014

Phase transitions in the complex plane of physical parameters

At low temperature a thermodynamic system undergoes a phase transition when a physical parameter passes through a singularity point of the free energy, corresponding to formation of a new order. At high temperature the thermal fluctuations destroy the orders; correspondingly the free energy is a smooth function of the physical parameter and the singularity would occur only at complex values of the parameter. Since a complex parameter is unphysical, at high temperature no phase transition is expected with varying the physical parameter. Here we show that the quantum evolution, driven by a designed interaction, of a system initialized in thermal equilibrium is equivalent to the partition function of a complex parameter. Therefore we can access the complex singularity points of thermodynamic functions and observe phase transitions even at high temperatures. This discovery makes it possible to study thermodynamics in the complex plane of physical parameters.

cond-mat.stat-mech↗

arXiv2013

Noise-resilient quantum evolution steered by dynamical decoupling

Realistic quantum computing is subjected to noise. A most important frontier in research of quantum computing is to implement noise-resilient quantum control over qubits. Dynamical decoupling can protect coherence of qubits. Here we demonstrate non-trivial quantum evolution steered by dynamical decoupling control, which automatically suppresses the noise effect. We designed and implemented a self-protected controlled-NOT gate on the electron spin of a nitrogen-vacancy centre and a nearby carbon-13 nuclear spin in diamond at room temperature, by employing an engineered dynamical decoupling control on the electron spin. Final state fidelities of 0.91 and 0.88 were observed even with imperfect initial states. In the mean time, the qubit coherence time has been elongated by at least 30 folds. The design scheme does not require that the dynamical decoupling control commute with the qubit interaction and works for general systems. This work marks a step toward realistic quantum computing.

quant-ph↗

arXiv2013

Sensing and atomic-scale structure analysis of single nuclear spin clusters in diamond

Single-molecule nuclear magnetic resonance (NMR) is a crown-jewel challenge in the field of magnetic resonance spectroscopy and has important applications in chemical analysis and in quantum computing. Recently, it becomes possible to tackle this grand challenge thanks to experimental advances in preserving quantum coherence of nitrogen-vacancy (NV) center spins in diamond as a sensitive probe and theoretical proposals on atomic-scale magnetometry via dynamical decoupling control. Through decoherence measurement of NV centers under dynamical decoupling control, sensing of single $^{13}\textbf{C}$ at nanometer distance has been realized. Toward the ultimate goal of structure analysis of single molecules, it is highly desirable to directly measure the interactions within single nuclear spin clusters. Here we sensed a single $^{13}\textbf{C}$-$^{13}\textbf{C}$ nuclear spin dimer located about 1 nm from the NV center and characterized the interaction between the two nuclear spins, by measuring NV center spin decoherence under various dynamical decoupling control. From the measured interaction we derived the spatial configuration of the dimer with atomic-scale resolution. These results demonstrate that central spin decoherence under dynamical decoupling control is a feasible probe for NMR structure analysis of single molecules.

cond-mat.mes-hall↗

arXiv2013

Suppression of electron spin decoherence of the diamond NV center by a transverse magnetic field

We demonstrate that the spin decoherence of nitrogen vacancy (NV) centers in diamond can be suppressed by a transverse magnetic field if the electron spin bath is the primary decoherence source. The NV spin coherence, created in "a decoherence-free subspace" is protected by the transverse component of the zero-field splitting, increasing the spin-coherence time about twofold. The decoherence due to the electron spin bath is also suppressed at magnetic fields stronger than ~25 gauss when applied parallel to the NV symmetry axis. Our method can be used to extend the spin-coherence time of similar spin systems for applications in quantum computing, field sensing, and other metrologies.

quant-ph↗

arXiv2013

Giant Faraday rotation induced by Berry phase in bilayer graphene under strong terahertz fields

High-order terahertz (THz) sideband generation (HSG) in semiconductors is a phenomenon with physics similar to high-order harmonic generation but in a much lower frequency regime. It was found that the electron-hole pairs excited by a weak optical laser can accumulate Berry phases along a cyclic path under the driving of a strong THz field. The Berry phases appear as the Faraday rotation angles of the emission signal under short-pulse excitation in monolayer MoS$_2$. In this paper, the theory of Berry phase in THz extreme nonlinear optics is applied to biased bilayer graphene with Bernal stacking, which has similar Bloch band features and optical properties to the monolayer MoS$_2$, such as time-reversal related valleys and valley contrasting optical selection rules. The bilayer graphene has much larger Berry curvature than monolayer MoS$_2$, which leads to a giant Faraday rotation of the optical emission ($\sim$ 1 rad for a THz field with frequency 1 THz and strength 8 kV/cm). This provides opportunities to use bilayer graphene and low-power THz lasers for ultrafast electro-optical devices.

cond-mat.mes-hall↗

arXiv2013

Effects of excitation frequency on high-order terahertz sideband generation in semiconductors

We theoretically investigate the effects of the excitation frequency on the plateau of high-order terahertz sideband generation (HSG) in semiconductors driven by intense terahertz (THz) fields. We find that the plateau of the sideband spectrum strongly depends on the detuning between the NIR laser field and the band gap. We use the quantum trajectory theory (three-step model) to understand the HSG. In the three-step model, an electron-hole pair is first excited by a weak laser, then driven by the strong THz field, and finally recombine to emit a photon with energy gain. When the laser is tuned below the band gap (negative detuning), the electron-hole generation is a virtual process that requires quantum tunneling to occur. When the energy gained by the electron-hole pair from the THz field is less than 3.2 times the ponderomotive energy, the electron and the hole can be driven to the same position and recombine without quantum tunneling, so the HSG will have large probability amplitude. This leads to a plateau feature of the HSG spectrum with a high-frequency cutoff at about 3.2 times the ponderomotive energy above the band gap. Such a plateau feature is similar to the case of high-order harmonics generation in atoms where electrons have to overcome the binding energy to escape the atomic core. A particularly interesting excitation condition in HSG is that the laser can be tuned above the band gap (positive detuning), corresponding to the unphysical "negative" binding energy in atoms for high-order harmonic generation. Now the electron-hole pair is generation by real excitation, but the recombination process can be real or virtual depending on the energy gained from the THz field, which determines the plateau feature in HSG.

cond-mat.mes-hall↗

arXiv2013

Single Dirac point and helical states in a one-dimensional system

Odd numbers of Dirac points and helical states can exist at edges (surfaces) of two-dimensional (three-dimensional) topological insulators. In the bulk of a one-dimensional lattice (not an edge) with time reversal symmetry, however, a no-go theorem forbids the existence of an odd number of Dirac points or helical states. Introducing a magnetic field can violate the time reversal condition but would usually lift the degeneracy at the Dirac points. We find that a spatially periodic magnetic field with zero mean value can induce a single Dirac point in a one-dimensional system with spin-orbit coupling. A wealth of new physics may emerge due to the existence of a single Dirac point and helical states in the bulk of a one-dimensional lattice (rather than edge states). A series of quantized numbers emerge due to the non-trivial topology of the 1D helical states, including the doubled period of helical Bloch oscillations, quantized conductance near the Dirac point, and 1/2-charge solitons at mass kinks. Such a system can be realized in one-dimensional semiconductor systems or in optical traps of atoms.

cond-mat.mes-hall↗

arXiv2013

No-go theorem and optimization of dynamical decoupling against noise with soft cutoff

We study the performance of dynamical decoupling in suppressing decoherence caused by soft-cutoff Gaussian noise, using short-time expansion of the noise correlations and numerical optimization. For the noise with soft cutoff at high frequencies, there exists no dynamical decoupling scheme to eliminate the decoherence to arbitrary orders of the short time, regardless of the timing or pulse shaping of the control under the population conserving condition. We formulate the equations for optimizing pulse sequences that minimizes decoherence up to the highest possible order of the short time for the noise correlations with odd power terms in the short-time expansion. In particular, we show that the Carr-Purcell-Meiboom-Gill sequence is optimal in short-time limit for the noise correlations with a linear order term in the time expansion.

quant-ph↗

arXiv2012

Berry phases of quantum trajectories in semiconductors under strong terahertz fields

Quantum evolution of particles under strong fields can be essentially captured by a small number of quantum trajectories that satisfy the stationary phase condition in the Dirac-Feynmann path integrals. The quantum trajectories are the key concept to understand extreme nonlinear optical phenomena, such as high-order harmonic generation (HHG), above-threshold ionization (ATI), and high-order terahertz sideband generation (HSG). While HHG and ATI have been mostly studied in atoms and molecules, the HSG in semiconductors can have interesting effects due to possible nontrivial "vacuum" states of band materials. We find that in a semiconductor with non-vanishing Berry curvature in its energy bands, the cyclic quantum trajectories of an electron-hole pair under a strong terahertz field can accumulate Berry phases. Taking monolayer MoS$_2$ as a model system, we show that the Berry phases appear as the Faraday rotation angles of the pulse emission from the material under short-pulse excitation. This finding reveals an interesting transport effect in the extreme nonlinear optics regime.

cond-mat.mes-hall↗

arXiv2012

Quantum criticality at infinite temperature

Quantum criticality, being important as an indicator of new quantum matters emerging, is known to occur only at zero or low temperature. We find that a quantum probe, if its coherence time is long, can detect quantum criticality at infinitely high temperature. In particular, the echo control over a spin probe can remove the thermal fluctuation effects and hence reveals the quantum fluctuation effects. Probes with quantum coherence time of milliseconds or seconds can be used to study emerging quantum orders that would occur at extremely low temperatures of nano- or pico-Kelvin. This discovery establishes a physical link between time and inverse temperature and provides a new route to the wonderland of quantum matters.

cond-mat.mes-hall↗

arXiv2012

Probing Lee-Yang zeros and coherence sudden death

As a foundation of statistical physics, Lee and Yang in 1952 proved that the partition functions of thermal systems can be zero at certain points (called Lee-Yang zeros) on the complex plane of temperature. In the thermodynamic limit, the Lee-Yang zeros approach to real numbers at the critical temperature. However, the imaginary Lee-Yang zeros have not been regarded as experimentally observable since they occur at imaginary field or temperature, which are unphysical. Here we show that the coherence of a probe spin weakly coupled to a many-body system presents zeros as a function of time that are one-to-one mapped to the Lee-Yang zeros of the many-body system. In the thermodynamic limit, of which the Lee-Yang zeros form a continuum, the probe spin coherence presents a sudden death at the edge singularities of the Lee-Yang zeros. By measuring the probe spin coherence, one can directly reconstruct the partition function of a many-body system. These discoveries establish a profound relation between two most fundamental quantities in the physical world, time and temperature, and also provide a universal approach to studying interacting many-body systems through measuring coherence of only one probe spin (or one qubit in quantum computing).

cond-mat.stat-mech↗

arXiv2012

Optical effects of spin currents in semiconductors

A spin current has novel linear and second-order nonlinear optical effects due to its symmetry properties. With the symmetry analysis and the eight-band microscopic calculation we have systematically investigated the interaction between a spin current and a polarized light beam (or the "photon spin current") in direct-gap semiconductors. This interaction is rooted in the intrinsic spin-orbit coupling in valence bands and does not rely on the Rashba or Dresselhaus effect. The light-spin current interaction results in an optical birefringence effect of the spin current. The symmetry analysis indicates that in a semiconductor with inversion symmetry, the linear birefringence effect vanishes and only the circular birefringence effect exists. The circular birefringence effect is similar to the Faraday rotation in magneto-optics but involves no net magnetization nor breaking the time-reversal symmetry. Moreover, a spin current can induce the second-order nonlinear optical processes due to the inversion-symmetry breaking. These findings form a basis of measuring a pure spin current where and when it flows with the standard optical spectroscopy, which may provide a toolbox to explore a wealth of physics connecting the spintronics and photonics.

cond-mat.mes-hall↗

arXiv2012

Sensing remote nuclear spins

Sensing single nuclear spins is a central challenge in magnetic resonance based imaging techniques. Although different methods and especially diamond defect based sensing and imaging techniques in principle have shown sufficient sensitivity, signals from single nuclear spins are usually too weak to be distinguished from background noise. Here, we present the detection and identification of remote single C-13 nuclear spins embedded in nuclear spin baths surrounding a single electron spins of a nitrogen-vacancy centre in diamond. With dynamical decoupling control of the centre electron spin, the weak magnetic field ~10 nT from a single nuclear spin located ~3 nm from the centre with hyperfine coupling as weak as ~500 Hz is amplified and detected. The quantum nature of the coupling is confirmed and precise position and the vector components of the nuclear field are determined. Given the distance over which nuclear magnetic fields can be detected the technique marks a firm step towards imaging, detecting and controlling nuclear spin species external to the diamond sensor.

cond-mat.mes-hall↗

arXiv2011

Non-Markovian dynamics and strong coupling between atomic transitions and a waveguide continuum edge

In quantum communication and distributed quantum computing, one-dimensional waveguides provide directional transfer of quantum information. A single-mode waveguide has a density-of-states singularity at the lower cut-off frequency, which resembles sharp resonances of a cavity but with non-Markovian dynamics. Thus we put forward schemes of coupling atomic transitions and a waveguide continuum edge. We first present a scheme of spin-photon quantum interface operating in the non-Markovian regime for a $Λ$-type three-level system coupled to a waveguide. Then we show that strong coupling between atomic transitions and a waveguide continuum edge can lead to vacuum Rabi oscillations and bound polariton states.

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