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Rene Gerritsma

Publications and source records attributed to Rene Gerritsma.

At least 19 recordsLinked to original sources

Precision spectroscopy of a trapped $^{173}$Yb$^+$ ion using a bath of ultracold atoms

We demonstrate precision laser spectroscopy of a trapped $^{173}$Yb$^+$ ion that is not directly laser cooled by coupling it to ultracold atoms. The atomic bath continuously cools the internal degrees of freedom of the ion to its hyperfine ground state via spin-exchange collisions. Successful laser excitation is detected via state-selective charge transfer and subsequent ion loss. We probe the $6^2S_{1/2}\rightarrow 6^2P_{3/2}$ transition at 329 nm and measure the magnetic and electric hyperfine interaction constants for the $6^2P_{3/2}$ state to be $A=-241(1)$ MHz and $B=1460(8)$ MHz, respectively. Our results are in agreement with a previous measurement obtained in a hollow-cathode discharge experiment but are a factor of 6-9 more precise. The techniques demonstrated in this work may be extended to perform precision spectroscopy on other ions with complex level structures.

physics.atom-ph

Direct observation of the optical Magnus effect with a trapped ion

We directly observe and spatially map an optical analog of the Magnus effect, where intrinsic spin-orbit-like coupling of light generates a spin-dependent transverse displacement of the atom-light interaction profile for a $^{40}$Ca$^+$ ion. Probed on a quadrupole transition using a tightly focused beam, we observe displacements of the maximum in the profile of the effective interaction by several 100 nm originating from intrinsic longitudinal electric field components beyond the paraxial approximation. The tight focus of the beam induces additional transverse polarization gradients, which we characterize through a phase-sensitive measurement and spatial maps for different beam configurations. The results establish the physical basis of polarization-gradient interactions relevant to optical tweezer-based quantum control.

physics.atom-ph

Global Variational Quantum Circuits for Arbitrary Symmetric State Preparation

Quantum states that are symmetric under particle exchange play a crucial role in fields such as quantum metrology and quantum error correction. We use a variational circuit composed of global one-axis twisting and global rotations to efficiently prepare arbitrary symmetric states, i.e. any superposition of Dicke states. The circuit does not require local addressability or ancilla qubits and thus can be readily implemented in a variety of experimental platforms including trapped-ion quantum simulators and cavity QED systems. We provide analytic and numerical evidence that any $N$-qubit symmetric state can be prepared in $2N/3$ steps. We demonstrate the utility of our protocol by preparing (i) metrologically useful $N$-qubit Dicke states of up to $N = 300$ qubits in $\mathcal{O}(1)$ gate steps with theoretical infidelities $1-\mathcal{F} < 10^{-3}$, (ii) the $N = 9$ Ruskai codewords in $P = 4$ gate steps with $1-\mathcal{F} < 10^{-4}$, and (iii) the $N = 13$ Gross codewords in $P = 7$ gate steps with $1-\mathcal{F} < 10^{-4}$. Focusing on trapped-ion platforms, for the $N = 9$ Ruskai and $N = 13$ Gross codewords we estimate that the protocol achieves fidelities $\gtrsim 95\%$ in the presence of typical experimental noise levels, thus providing a pathway to the preparation of a wide range of useful highly-entangled quantum states.

quant-ph

Ultracold collisions of a neutral atom with a trapped ion in 1D

We present a fully quantum mechanical description of a free $^6$Li atom scattering from a trapped $^{171}$Yb$^+$ ion in one dimension. By reformulating the system in polar coordinates and employing the adiabatic representation, we extract a set of coupled adiabatic potentials representing the atom interacting with the ion in different trap states. In an approach similar to quantum defect theory (QDT), we leverage the vast difference in energy scale between the interaction, the trap, and the scattering energy to encapsulate the short-range atom-ion scattering behavior in a single phase parameter. The presence of trapped $({}^{171}\text{Yb}^6\text{Li})^+$ molecular-ion states leads to a series of roughly evenly spaced resonances in the scattering cross section. The predicted distribution of resonances at low collision energies is at odds with the expectation of quantum chaos and the Bohigas-Giannoni-Schmit (BGS) conjecture.

physics.atom-ph

Vibrationally coupled Rydberg atom-ion molecules

We study the occurrence of Rydberg atom-ion molecules (RAIMs) in a hybrid atom-ion system with an ion crystal trapped in a Paul trap coupled to Rydberg atoms on its either ends. To assess the feasibility of such a system, we perform a detailed Floquet analysis of the effect of the Paul trap's rf potential on the RAIMs and provide a qualitative analysis of the survival probability based on scaling laws. We conclude that the RAIM survives for sufficiently weak and low frequency traps. We then use this hybrid system and propose a scheme to utilise the common motional modes of the ion crystal to suppress (blockade) or enhance (anti-blockade) the probability of forming two RAIMs at the ends of the chain, replacing the typical blockade radius by the length of the ion crystal.

quant-ph

Phonon-mediated quantum gates in trapped ions coupled to an ultracold atomic gas

We study the dynamics of phonon-mediated qubit-qubit interactions between trapped ions in the presence of an ultracold atomic gas. By deriving and solving a master equation to describe the combined system, we show that the presence of the atoms causes the quantum gate quality to reduce because of motional decoherence. On the other hand, we calculate that the gas may be used to keep the ion crystal cold in the presence of external heating due to electric field noise. We show that tuning the atom-ion scattering length allows one to tune the cooling rate of the ions and would make it possible to temporarily reduce the effects of the gas during a quantum gate while keeping the ions cold over long timescales. In this way, the trapped ion quantum computer may be buffer gas cooled. The system may also be used for quantum-enhanced measurements of the atom-ion interactions or properties of the atomic bath.

quant-ph

Ultracold ion-atom experiments: cooling, chemistry, and quantum effects

Experimental setups that study laser-cooled ions immersed in baths of ultracold atoms merge the two exciting and well-established fields of quantum gases and trapped ions. These experiments benefit both from the exquisite read-out and control of the few-body ion systems as well as the many-body aspects, tunable interactions, and ultracold temperatures of the atoms. However, combining the two leads to challenges both in the experimental design and the physics that can be studied. Nevertheless, these systems have provided insights into ion-atom collisions, buffer gas cooling of ions and quantum effects in the ion-atom interaction. This makes them promising candidates for ultracold quantum chemistry studies, creation of cold molecular ions for spectroscopy and precision measurements, and as test beds for quantum simulation of charged impurity physics. In this review we aim to provide an experimental account of recent progress and introduce the experimental setup and techniques that enabled the observation of quantum effects.

physics.atom-ph

The Effect of Micromotion and Local Stress in Quantum simulation with Trapped Ions in Optical Tweezers

The ability to program and control interactions provides the key to implementing large-scale quantum simulation and computation in trapped ion systems. Adding optical tweezers, which can tune the phonon spectrum and thus modify the phonon-mediated spin-spin interaction, was recently proposed as a way of programming quantum simulators for a broader range of spin models [Arias Espinoza et al., Phys. Rev. A {\bf 103}, 052437]. In this work we study the robustness of our findings in the presence of experimental imperfections: micromotion, local stress, and intensity noise. We show that the effects of micromotion can be easily circumvented when designing and optimizing tweezer patterns to generate a target interaction. Furthermore, while local stress, whereby the tweezers apply small forces on individual ions, may appear to enable further tuning of the spin-spin interactions, any additional flexibility is negligible. We conclude that optical tweezers are a useful method for controlling interactions in trapped ion quantum simulators in the presence of micromotion and imperfections in the tweezer alignment, but require intensity stabilization on the sub-percent level.

quant-ph

Dynamics of a trapped ion in a quantum gas: effects of particle statistics

We study the quantum dynamics of an ion confined in a radiofrequency trap in interaction with either a Bose or spin-polarized Fermi gas. To this end, we derive quantum optical master equations in the limit of weak coupling and the Lamb-Dicke approximations. For the bosonic bath, we also include the so-called "Lamb-shift" correction to the ion trap due to the coupling to the quantum gas as well as the extended Fröhlich interaction within the Bogolyubov approximation that have been not considered in previous studies. We calculate the ion kinetic energy for various atom-ion scattering lengths as well as gas temperatures by considering the intrinsic micromotion and we analyse the damping of the ion motion in the gas as a function of the gas temperature. We find that the ion's dynamics depends on the quantum statistics of the gas and that a fermionic bath enables to attain lower ionic energies.

cond-mat.quant-gas

Engineering spin-spin interactions with optical tweezers in trapped ions

We propose a new method for generating programmable interactions in one- and two-dimensional trapped-ion quantum simulators. Here we consider the use of optical tweezers to engineer the sound-wave spectrum of trapped ion crystals. We show that this approach allows us to tune the interactions and connectivity of the ion qubits beyond the power-law interactions accessible in current setups. We demonstrate the experimental feasibility of our proposal using realistic tweezer settings and experimentally relevant trap parameters to generate the optimal tweezer patterns to create target spin-spin interaction patterns in both one- and two-dimensional crystals. Our approach will advance quantum simulation in trapped-ion platforms as it allows them to realize a broader family of quantum spin Hamiltonians.

quant-ph

A high-fidelity method for a single-step $N$-bit Toffoli gate in trapped ions

Conditional multi-qubit gates are a key component for elaborate quantum algorithms. In a recent work, Rasmussen et al. (Phys. Rev. A 101, 022308) proposed an efficient single-step method for a prototypical multi-qubit gate, a Toffoli gate, based on a combination of Ising interactions between control qubits and an appropriate driving field on a target qubit. Trapped ions are a natural platform to implement this method, since Ising interactions mediated by phonons have been demonstrated in increasingly large ion crystals. However, the simultaneous application of these interactions and the driving field required for the gate results in undesired entanglement between the qubits and the motion of the ions, reducing the gate fidelity. In this work, we propose a solution based on adiabatic switching of these phonon mediated Ising interactions. We study the effects of imperfect ground state cooling, and use spin-echo techniques to undo unwanted phase accumulation in the achievable fidelities. For gates coupling to all axial modes of a linear crystal, we calculate high fidelities ($>$ 99%) $N$-qubit rotations with $N=$ 3-7 ions cooled to their ground state of motion and a gate time below 1~ms. The high fidelities obtained also for large crystals could make the gate competitive with gate-decomposed, multi-step variants of the $N$-qubit Toffoli gate, at the expense of requiring ground state cooling of the ion crystal.

quant-ph

Controlling the nature of a charged impurity in a bath of Feshbach dimers

We theoretically study the dynamics of a trapped ion that is immersed in an ultracold gas of weakly bound atomic dimers created by a Feshbach resonance. Using quasi-classical simulations, we find a crossover from dimer dissociation to molecular ion formation depending on the binding energy of the dimers. The location of the crossover strongly depends on the collision energy and the time-dependent fields of the Paul trap. Deeply bound dimers lead to fast molecular ion formation, with rates approaching the Langevin collision rate $Γ'_\text{L}\approx4.8\times10^{-9}\,$cm$^3$s$^{-1}$. The kinetic energies of the created molecular ions have a median below $1\,$mK, such that they will stay confined in the ion trap. We conclude that interacting ions and Feshbach molecules may provide a novel approach towards the creation of ultracold molecular ions with applications in precision spectroscopy and quantum chemistry.

physics.atom-ph

Signal processing techniques for efficient compilation of controlled rotations in trapped ions

Quantum logic gates with many control qubits are essential in many quantum algorithms, but remain challenging to perform in current experiments. Trapped ion quantum computers natively feature a different type of entangling operation, namely the Molmer-Sorensen (MS) gate which effectively applies an Ising interaction to all qubits at the same time. We consider a sequence of equal all-to-all MS operations, interleaved with single qubit gates that act only on one special qubit. Using a connection with quantum signal processing techniques, we find that it is possible to perform an arbitray SU(2) rotation on the special qubit if and only if all other qubits are in the state |1>. Such controlled rotation gates with N-1 control qubits require 2N applications of the MS gate, and can be mapped to a conventional Toffoli gate by demoting a single qubit to ancilla.

quant-ph

Cold hybrid ion-atom systems

Hybrid systems of laser-cooled trapped ions and ultracold atoms combined in a single experimental setup have recently emerged as a new platform for fundamental research in quantum physics. This paper reviews the theoretical and experimental progress in research on cold hybrid ion-atom systems which aim to combine the best features of the two well-established fields. We provide a broad overview of the theoretical description of ion-atom mixtures and their applications, and report on advances in experiments with ions trapped in Paul or dipole traps overlapped with a cloud of cold atoms, and with ions directly produced in a Bose-Einstein condensate. We start with microscopic models describing the electronic structure, interactions, and collisional physics of ion-atom systems at low and ultralow temperatures, including radiative and non-radiative charge transfer processes and their control with magnetically tunable Feshbach resonances. Then we describe the relevant experimental techniques and the intrinsic properties of hybrid systems. In particular, we discuss the impact of the micromotion of ions in Paul traps on ion-atom hybrid systems. Next, we review recent proposals for using ions immersed in ultracold gases for studying cold collisions, chemistry, many-body physics, quantum simulation, and quantum computation and their experimental realizations. In the last part we focus on the formation of molecular ions via spontaneous radiative association, photoassociation, magnetoassociation, and sympathetic cooling. We discuss applications and prospects of cold molecular ions for cold controlled chemistry and precision spectroscopy.

physics.atom-ph

Operation of a Microfabricated Planar Ion-Trap for Studies of a Yb$^+$-Rb Hybrid Quantum System

In order to study interactions of atomic ions with ultracold neutral atoms, it is important to have sub-$μ$m control over positioning ion crystals. Serving for this purpose, we introduce a microfabricated planar ion trap featuring 21 DC electrodes. The ion trap is controlled by a home-made FPGA voltage source providing independently variable voltages to each of the DC electrodes. To assure stable positioning of ion crystals with respect to trapped neutral atoms, we integrate into the overall design a compact mirror magneto optical chip trap (mMOT) for cooling and confining neutral $^{87}$Rb atoms. The trapped atoms will be transferred into an also integrated chipbased Ioffe-Pritchard trap potential formed by a Z-shaped wire and an external bias magnetic field.We introduce the hybrid atom-ion chip, the microfabricated planar ion trap and use trapped ion crystals to determine ion lifetimes, trap frequencies, positioning ions and the accuracy of the compensation of micromotion.

physics.atom-ph

Dynamics of a single ion spin impurity in a spin-polarized atomic bath

We report on observations of spin dynamics in single Yb$^+$ ions immersed in a cold cloud of spin-polarized $^6$Li atoms. This species combination has been proposed to be the most suitable system to reach the quantum regime in atom-ion experiments. For $^{174}$Yb$^+$, we find that the atomic bath polarizes the spin of the ion by 93(4)\,\% after a few Langevin collisions, pointing to strong spin-exchange rates. For the hyperfine ground states of $^{171}$Yb$^+$, we also find strong rates towards spin polarization. However, relaxation towards the $F=0$ ground state occurs after 7.7(1.5) Langevin collisions. We investigate spin impurity atoms as possible source of apparent spin-relaxation leading us to interpret the observed spin-relaxation rates as an upper limit. Using ab initio electronic structure and quantum scattering calculations, we explain the observed rates and analyze their implications for the possible observation of Feshbach resonances between atoms and ions once the quantum regime is reached.

physics.atom-ph

Spectroscopy of the $^2S_{1/2} \rightarrow\,^2P_{3/2}$ transition in Yb II: Isotope shifts, hyperfine splitting and branching ratios

We report on spectroscopic results on the $^2S_{1/2} \rightarrow\,^2P_{3/2}$ transition in single trapped Yb$^+$ ions. We measure the isotope shifts for all stable Yb$^+$ isotopes except $^{173}$Yb$^+$, as well as the hyperfine splitting of the $^2P_{3/2}$ state in $^{171}$Yb$^+$. Our results are in agreement with previous measurements but are a factor of 5-9 more precise. For the hyperfine constant $A\left(^2P_{3/2}\right) = 875.4(10)$ MHz our results also agree with previous measurements but deviate significantly from theoretical predictions. We present experimental results on the branching ratios for the decay of the $^2P_{3/2}$ state. We find branching fractions for the decay to the $^2D_{3/2}$ state and $^2D_{5/2}$ state of 0.17(1)% and 1.08(5)%, respectively, in rough agreement with theoretical predictions. Furthermore, we measured the isotope shifts of the $^2F_{7/2} \rightarrow\,^1D\left[5/2\right]_{5/2}$ transition and determine the hyperfine structure constant for the $^1D\left[5/2\right]_{5/2}$ state in $^{171}$Yb$^+$ to be $A\left(^1D\left[5/2\right]_{5/2}\right) = -107(6)$ MHz.

physics.atom-ph

Controlled long-range interactions between Rydberg atoms and ions

We theoretically investigate trapped ions interacting with atoms that are coupled to Rydberg states. The strong polarizabilities of the Rydberg levels increases the interaction strength between atoms and ions by many orders of magnitude, as compared to the case of ground state atoms, and may be mediated over micrometers. We calculate that such interactions can be used to generate entanglement between an atom and the motion or internal state of an ion. Furthermore, the ion could be used as a bus for mediating spin-spin interactions between atomic spins in analogy to much employed techniques in ion trap quantum simulation. The proposed scheme comes with attractive features as it maps the benefits of the trapped ion quantum system onto the atomic one without obviously impeding its intrinsic scalability. No ground state cooling of the ion or atom is required and the setup allows for full dynamical control. Moreover, the scheme is to a large extent immune to the micromotion of the ion. Our findings are of interest for developing hybrid quantum information platforms and for implementing quantum simulations of solid state physics.

quant-ph