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Reza Loloee

Publications and source records attributed to Reza Loloee.

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Rapid supercurrent decay in Mn$_5$Si$_3$ Josephson junctions

Theoretical work predicts that Josephson junctions containing metallic altermagnetic barriers should display $0$-$\pi$ transitions of the critical current as a function of both barrier thickness and temperature, with the decay and oscillation period of the supercurrent depending on the orientation of the crystal axes relative to the transport direction. Motivated by these predictions, and by reports of a compensated magnetic phase attributed to altermagnetism in epitaxial Mn$_5$Si$_3$ thin films, we fabricate and measure Nb/Pt/Mn$_5$Si$_3$/Pt/Nb Josephson junctions varying the thickness of the Mn$_5$Si$_3$ barrier. The critical current decays as a single exponential over more than four orders of magnitude with decay length $\xi_{\text{Mn}_5\text{Si}_3} = 0.31 \pm 0.03$ nm, shorter than reported for Josephson junctions containing the metallic antiferromagnets FeMn, Cr, and NiMn. The Mn$_5$Si$_3$ barrier has an estimated current-perpendicular-to-plane resistivity of $320 \pm 10 \mu\Omega\,$cm. No $0$-$\pi$ transition is resolved at the sampled barrier thicknesses, and the temperature dependence of the critical current of a junction with a 1 nm barrier is smooth and monotonic. We discuss the absence of resolvable transitions in terms of the microstructure of the barrier, its uncertain magnetic phase, and the narrow thickness window imposed by the rapid decay, and identify barriers with well-defined crystalline orientation as the key requirement for future tests of altermagnetic Josephson physics.

cond-mat.supr-con

Large critical current density Josephson $\pi$ junctions with PdNi barriers

We report large $\pi$-state critical current densities, $J_c(\pi)$, in Nb/Pd$_{89}$Ni$_{11}$/Nb Josephson junctions at Pd$_{89}$Ni$_{11}$ thicknesses near the first $\pi$-state. We observe oscillations in the critical current with ferromagnetic barrier thickness consistent with a $0$-$\pi$ transition. For a junction with a 9.4~nm Pd$_{89}$Ni$_{11}$ barrier, we obtain $J_c(\pi) = 410~\mathrm{kA/cm^{2}}$ at 4.2~K, exceeding values reported in prior PdNi-based studies. Magnetization measurements on continuous films, together with coercivity tests on patterned arrays, confirm that Pd$_{89}$Ni$_{11}$ exhibits perpendicular magnetic anisotropy, enabling zero-field operation without magnetic initialization. The combination of large $J_c(\pi)$ and intrinsic anisotropy establishes Pd$_{89}$Ni$_{11}$ as a promising barrier material for passive $\pi$-shifters in superconducting digital logic and qubit architectures.

cond-mat.supr-con

Upper critical fields in normal metal-superconductor-normal metal trilayers

The role of spin orbit interaction in superconducting proximity effect is an area of intense research effort. Recent theoretical and experimental works investigate the possible role of spin-orbit interaction in generating spin-triplet pair correlations. In this work, we present an experimental survey of thin normal metal-superconductor-normal metal trilayers with Nb superconductor and Al, Ti, Cu, Pt, Ta, and Au normal metals, along with single layers of Nb as reference. We aim to probe the role of spin-orbit interaction and resistivity on the normal metal proximity effect through measurements of the upper critical field. We find that the upper critical fields of the trilayers are lower than that of a single layer Nb reference sample, and that the trilayers with higher resistivity metals, Ti, Pt, and Ta, behave as 2-dimensional superconductors. At low applied in-plane magnetic fields and temperatures close to the zero field transition temperature, we find a possible deviation from 2-dimensional to 3-dimensional behavior in the Ti and Pt trilayers. We also find that compared to single layer Nb films, all of our trilayers show a greater suppression of critical temperature during rotation from an in-plane to an out-of-plane applied magnetic field, with the greatest suppression observed in trilayers with Au or Al. This suppression of the critical temperature under field rotation might appear analogous to the colossal spin valve effect that can be achieved in systems with ferromagnetic materials; however, in our trilayers, only conventional orbital screening contributions to the suppression are present and the additional suppression is not present in the absence of applied magnetic field.

cond-mat.supr-con

Comparison of NiFeCr and NiFe in ferromagnetic Josephson junctions

Josephson junctions containing ferromagnetic materials are under consideration for applications in digital superconducting logic and memory. Some memory applications rely on the ability to reverse the magnetization direction of a "soft" magnetic layer within the junction using a small local magnetic field generated on the chip. It is crucial, therefore, to find a suitable soft magnetic material with a low switching field and low switching energy. A popular magnetic material for such applications is Ni$_{80}$Fe$_{20}$, also known as Permalloy, however Permalloy has a rather large magnetization, leading to large magnetic switching energies. In this work we explore Cr-doped Permalloy, specifically Ni$_{73}$Fe$_{18}$Cr$_{9}$, which has a saturation magnetization just under two-thirds that of Permalloy. Josephson junctions containing this NiFeCr alloy undergo a 0-$\pi$ transition at a NiFeCr thickness of 2.3 nm, and the critical supercurrent decays in the alloy over a short characteristic length of 0.36 nm. Switching fields of a few millitesla are promising, but the short decay length and overall small values of the critical current in the Josephson junctions may preclude the use of NiFeCr in current cryogenic memory technologies.

cond-mat.supr-con

Demonstration of 0-pi transition in Josephson junctions containing unbalanced synthetic antiferromagnets

Josephson junctions containing ferromagnetic (F) materials have been the subject of intense study over the past two decades. The ground state of such junctions oscillates between 0 and pi as the thickness of the ferromagnetic layer increases. For some applications, it might be beneficial to replace a very thin F layer with an unbalanced synthetic antiferromagnet (SAF) consisting of two F layers of different thicknesses whose magnetizations are coupled antiparallel to each other. According to theory, such a system should behave similarly to a single F layer whose thickness is equal to the difference of the two F-layer thicknesses in the SAF. We test that theoretical prediction with Josephson junctions containing unbalanced Ni/Ru/Ni SAFs, keeping the thickness of one layer fixed at 2.0 nm and varying the thickness of the other layer between 2.0 and 5.0 nm. We observe the first 0-pi transition at a thickness difference of 0.86 nm, which closely matches the position of the transition observed previously using single Ni layers.

cond-mat.supr-con

Effect of interfaces on supercurrent through ferromagnetic materials

Ferromagnetic Josephson junctions exhibit fascinating physics and the potential for applications in superconducting logic and memory. The junctions in a demonstrated superconducting memory prototype contain a magnetic spin-valve structure with Ni as the fixed layer and NiFe (Permalloy) as the free layer. However, NiFe exhibits poor supercurrent transmission, which limits the efficiency of the Josephson junction. We have previously shown that the supercurrent transmission through a Cu/NiFe/Cu trilayer can be improved by adding thin layers of Ni between the Cu and NiFe -- possibly due to the advantageous spin-dependent transport properties of the Cu/Ni interfaces. In this work we explore this idea further by replacing the Cu/NiFe interfaces with Pd/NiFe, which also have more desirable transport properties. Compared to the reference junctions containing Cu/NiFe interfaces, the new junctions exhibit an increase in the $\pi$-state supercurrent by a factor of 2 along with a change in the position of the first $0-\pi$ transition.

cond-mat.supr-con

Enhancement of supercurrent through ferromagnetic materials by interface engineering

Josephson junctions containing ferromagnetic materials exhibit interesting physics and show promise as circuit elements for superconducting logic and memory. For memory applications, the properties of the junction should be controllable by changing the magnetic configuration inside the junction. To achieve good magnetic switching properties, one should choose a soft magnetic material such as NiFe (permalloy); however, NiFe exhibits poor supercurrent transmission in Josephson junctions. In this work we put thin layers of Ni on either side of the NiFe and characterize the magnetic behavior and supercurrent transmission properties of the Ni/NiFe/Ni trilayers as a function of Ni and NiFe thicknesses. Using a Ni thickness of 0.4 nm, we find that the magnetic switching behavior of the trilayers is not severely degraded relative to plain NiFe, while the maximum supercurrent in the $\pi$-state of the trilayer Josephson junctions is increased by a factor of four relative to that of NiFe junctions. We speculate that the supercurrent enhancement is due to the different spin-dependent transport properties of the Cu/Ni and Cu/NiFe interfaces.

cond-mat.supr-con

Supercurrent transmission through Ni/Ru/Ni synthetic antiferromagnets

Josephson junctions containing ferromagnetic materials are generating interest for use in superconducting electronics and cryogenic memory. Optimizing the performance of such junctions is an ongoing effort, requiring exploration of a broad range of magnetic systems. Here we study supercurrent transmission through Ni/Ru/Ni synthetic antiferromagnets, with the idea that their magnetic properties may be superior to those of isolated Ni layers. We find that the decay of the supercurrent as a function of Ni thickness is very slow, with a decay length of 7.5 $\pm$ 0.8 nm. We also characterize the magnetic properties of the synthetic antiferromagnets as a function of Ni and Ru thicknesses.

cond-mat.supr-con

Spin-polarized triplet supercurrent in Josephson junctions with perpendicular ferromagnetic layers

Josephson junctions containing three ferromagnetic layers with non-collinear magnetizations between adjacent layers carry spin-triplet supercurrent under certain conditions. The signature of the spin-triplet supercurrent is a relatively slow decay of the maximum supercurrent as a function of the thickness of the middle ferromagnetic layer. In this work we focus on junctions where the middle magnetic layer is a [Co/Pd]$_N$ multilayer with perpendicular magnetic anisotropy (PMA), while the outer two layers have in-plane anisotropy. We compare junctions where the middle PMA layer is or is not configured as a synthetic antiferromagnet (PMA-SAF). We find that the supercurrent decays much more rapidly with increasing the number $N$ of [Co/Pd] bilayers in the PMA-SAF junctions compared to the PMA junctions. Similar behavior is observed in junctions containing [Co/Ni]$_N$ PMA multilayers. We model that behavior by assuming that each Co/Pd or Co/Ni interface acts as a partial spin filter, so that the spin-triplet supercurrent in the PMA junctions becomes more strongly spin-polarized as $N$ increases while the supercurrent in the PMA-SAF junctions is suppressed with increasing $N$. We also address a question raised in a previous work regarding how much spin-singlet supercurrent is transmitted through our nominally spin-triplet junctions. We do that by comparing spin-triplet junctions with similar junctions where the order of the magnetic layers has been shuffled. The results of this work are expected to be helpful in designing spin-triplet Josephson junctions for use in cryogenic memory.

cond-mat.supr-con

Dirac surface states in superconductors: a dual topological proximity effect

In this paper we present scanning tunneling microscopy of Bi$_2$Se$_3$ with superconducting Nb deposited on the surface. We find that the topologically protected surface states of the Bi$_2$Se$_3$ leak into the superconducting over-layer, suggesting a dual topological proximity effect. Coupling between theses states and the Nb states leads to an effective pairing mechanism for the surface states, leading to a modified model for a topological superconductor in these systems. This model is consistent with fits between the experimental data and the theory.

cond-mat.supr-con

Distortions to the penetration depth and coherence length of superconductor/normal-metal superlattices

Superconducting ($S$) thin film superlattices composed of Nb and a normal metal spacer ($N$) have been extensively utilized in Josephson junctions given their favorable surface roughness compared to Nb films of comparable thickness. In this work, we characterize the London penetration depth and Ginzburg-Landau coherence lengths of $S/N$ superlattices using polarized neutron reflectometry and electrical transport. Despite the normal metal spacer layers being only approximately 8% of the total superlattice thickness, we surprisingly find that the introduction of these thin $N$ spacers between $S$ layers leads to a dramatic increase in the measured London penetration depth compared to that of a single Nb film of comparable thickness. Using the measured values for the effective in- and out-of-plane coherence lengths, we quantify the induced anisotropy of the superlattice samples and compare to a single Nb film sample. From these results, we find that that the superlattices behave similarly to layered 2D superconductors.

cond-mat.supr-con

Supercurrent in ferromagnetic Josephson junctions with heavy metal interlayers. II. Canted magnetization

It has been suggested by theoretical works that equal spin-triplet Cooper pairs can be generated in Josephson junctions containing both a ferromagnet and a source of spin-orbit coupling. Our recent experimental work suggested that spin-triplet Cooper pairs were not generated by a Pt spin-orbit coupling layer when the ferromagnetic weak link had entirely in-plane anisotropy (N. Satchell and N.O. Birge, Phys. Rev. B 97, 214509 (2018)). Here, we revisit the experiment using Pt again as a source for spin-orbit coupling and a [Co(0.4 nm)/Ni(0.4 nm)]$_{\times8}$/Co(0.4 nm) ferromagnetic weak link with both in-plane and out-of-plane magnetization components (canted magnetization). The canted magnetization more closely matches theoretical predictions than our previous experimental work. Our results suggest that there is no supercurrent contribution in our junctions from equal spin-triplets. In addition, this work includes the first systematic study of supercurrent dependence on Cu interlayer thickness, a common additional layer used to buffer the growth of the ferromagnet and which for Co may significantly improve the growth morphology. We report that the supercurrent in the [Co(0.4 nm)/Ni(0.4 nm)]$_{\times8}$/Co(0.4 nm) ferromagnetic weak links can be enhanced by over two orders of magnitude by tuning the Cu interlayer thickness. This result has important application in superconducting spintronics, where large critical currents are desirable for devices.

cond-mat.supr-con

Phase Controllable Josephson Junctions for Cryogenic Memory

Josephson junctions containing ferromagnetic layers have generated interest for application in cryogenic memory. In a junction containing both a magnetically hard fixed layer and soft free layer with carefully chosen thicknesses, the ground-state phase difference of the junction can be controllably switched between 0 and π by changing the relative orientation of the two ferromagnetic layers from antiparallel to parallel. This phase switching has been observed in junctions using Ni fixed layers and NiFe free layers. We present phase-sensitive measurements of such junctions in low-inductance symmetric SQUID loops which simplify analysis relative to our previous work. We confirm controllable 0 - π switching in junctions with 2.0 nm Ni fixed layers and 1.25 nm NiFe free layers across multiple devices and using two SQUID designs, expanding the phase diagram of known thicknesses that permit phase control.

cond-mat.supr-con

Phase Control in a Spin-Triplet SQUID

It is now well established that a Josephson junction made from conventional spin-singlet superconductors containing ferromagnetic layers can carry spin-triplet supercurrent under certain conditions. The first experimental signature of that fact is the propagation of such supercurrent over long distances through strong ferromagnetic materials. Surprisingly, one of the most salient predictions of the theory has yet to be verified experimentally -- namely that a Josephson junction containing three magnetic layers with coplanar magnetizations should exhibit a ground-state phase shift of either zero or pi depending on the relative orientations of those magnetizations. Here we demonstrate this property using Josephson junctions containing three different types of magnetic layers, chosen so that the magnetization of one layer can be switched by 180 degrees without disturbing the other two. Phase-sensitive detection is accomplished using a superconducting quantum interference device, or SQUID. Such a phase-controllable junction could be used as the memory element in a fully-superconducting computer.

cond-mat.supr-con

Spin-triplet supercurrent in Josephson junctions containing a synthetic antiferromagnet with perpendicular magnetic anisotropy

We present measurements of Josephson junctions containing three magnetic layers with noncolinear magnetizations. The junctions are of the form $S/F^{\prime}/N/F/N/F^{\prime \prime}/S$, where $S$ is superconducting Nb, $F^\prime$ is either a thin Ni or Permalloy layer with in-plane magnetization, $N$ is the normal metal Cu, $F$ is a synthetic antiferromagnet (SAF) with magnetization perpendicular to the plane, composed of Pd/Co multilayers on either side of a thin Ru spacer, and $F^{\prime \prime}$ is a thin Ni layer with in-plane magnetization. The supercurrent in these junctions decays more slowly as a function of the $F$-layer thickness than for similar spin-singlet junctions not containing the $F^\prime$ and $F^{\prime \prime}$ layers. The slower decay is the prime signature that the supercurrent in the central part of these junctions is carried by spin-triplet pairs. The junctions containing $F^{\prime}=$ Permalloy are suitable for future experiments where either the amplitude of the critical current or the ground-state phase difference across the junction is controlled by changing the relative orientations of the magnetizations of the $F^{\prime}$ and $F^{\prime \prime}$ layers.

cond-mat.supr-con

Critical Current Oscillations of Elliptical Josephson Junctions with Single-Domain Ferromagnetic Layers

Josephson junctions containing ferromagnetic layers are of considerable interest for the development of practical cryogenic memory and superconducting qubits. Such junctions exhibit a phase shift of $π$ for certain ranges of ferromagnetic layer thickness. We present studies of Nb based micron-scale elliptically-shaped Josephson junctions containing ferromagnetic barriers of Ni$_{81}$Fe$_{19}$ or Ni$_{65}$Co$_{20}$Fe$_{15}$. By applying an external magnetic field, the critical current of the junctions are found to follow characteristic Fraunhofer patterns, and display sharp switching behavior suggestive of single-domain magnets. The high quality of the Fraunhofer patterns enables us to extract the maximum value of the critical current even when the peak is shifted significantly outside the range of the data due to the magnetic moment of the ferromagnetic layer. The maximum value of the critical current oscillates as a function of the ferromagnetic barrier thickness, indicating transitions in the phase difference across the junction between values of zero and $π$. We compare the data to previous work and to models of the 0-$π$ transitions based on existing theories.

cond-mat.supr-con

Critical Current Oscillations of Josephson Junctions Containing PdFe Nanomagnets

Josephson junctions with ferromagnetic layers are vital elements in a new class of cryogenic memory devices. One style of memory device contains a spin valve with one "hard" magnetic layer and one "soft" layer. To achieve low switching fields, it is advantageous for the soft layer to have low magnetization and low magnetocrystalline anisotropy. A candidate class of materials that fulfills these criteria is the Pd$_{1-x}$Fe$_{x}$ alloy system with low Fe concentrations. We present studies of micron-scale elliptically-shaped Josephson junctions containing Pd$_{97}$Fe$_{3}$ layers of varying thickness. By applying an external magnetic field, the critical current of the junctions are found to follow characteristic Fraunhofer patterns. The maximum value of the critical current, extracted from the Fraunhofer patterns, oscillates as a function of the ferromagnetic barrier thickness, indicating transitions in the phase difference across the junction between values of zero and $π$.

cond-mat.supr-con

Scanning tunneling microscopy of superconducting topological surface states in Bi$_2$Se$_3$

In this paper we present scanning tunneling microscopy of a large $\textrm{Bi}_2\textrm{Se}_3$ crystal with superconducting PbBi islands deposited on the surface. Local density of states measurements are consistent with induced superconductivity in the topological surface state with a coherence length of order 540 nm. At energies above the gap the density of states exhibits oscillations due to scattering caused by a nonuniform order parameter. Strikingly, the spectra taken on islands also display similar oscillations along with traces of the Dirac cone, suggesting an inverse topological proximity effect.

cond-mat.supr-con