SearcharxivSearch

arXiv subjects

Reza Rouzegar

Publications and source records attributed to Reza Rouzegar.

13 recordsLinked to original sources

Terahertz switching of antiferromagnetic order by Néel spin-orbit torques

Ultrafast electric manipulation of magnetic order in solids is critical for the development of future terahertz data processing. A fascinating concept for such high-speed operation is offered in metallic antiferromagnets by Néel spin-orbit torque. It should allow one to coherently rotate the ordered spins by simply applying an electric current of suitable amplitude and polarity. However, such switching has been severely hampered by competing heat-induced effects, and it has not yet been achieved on the intrinsically ultrafast time scales of antiferromagnets. Here, we report robust, direction-controlled and non-thermal rotation of the Néel vector $\mathbf{L}$ by $\pm$90° at room temperature in the antiferromagnet Mn$_2$Au driven by phase-locked terahertz current pulses. All observed features are consistent with ultrafast Néel spin-orbit torque: First, nonlinear optical imaging reveals that the terahertz current direction sets the final orientation of $\mathbf{L}$ in the absence of any bias field for at least two months. Second, transient optical birefringence shows that the switching proceeds ultrafast in less than 15 picoseconds. Finally, atomistic spin-dynamics simulations reproduce the observed dynamics and confirm the minor role of thermal effects. While the switching is already one order of magnitude faster than in ferromagnets at comparable dissipated energy, our simulations predict routes toward switching times and energies which are another order of magnitude lower. Our approach can be transferred to electric-field-driven switching in many more antiferromagnets, including magnetoelectric insulators. The engineering of spin torques, resonance frequencies and read-out mechanisms provides an exciting pathway toward on-chip applications of terahertz antiferromagnetic spin-orbitronics.

cond-mat.mes-hall

Femtosecond signatures of optically induced magnons before ultrafast demagnetization

Optically induced demagnetization of 3d metallic ferromagnets proceeds as fast as ~100 fs and is a crucial prerequisite for spintronic applications, such as ultrafast magnetization switching and spin transport. On the 100 fs time scale, the magnetization dynamics is widely understood in the context of temperature models considering energy transfers between conduction electrons, magnons and crystal lattice. However, on even faster time scales, the flow of both angular momentum and energy between these subsystems has so far not been studied. Here, we measure ultrafast demagnetization by ultrabroadband THz-emission spectroscopy. We find that the rate of change of the magnetization does not rise instantaneously, but on a time scale as short as 10 fs. This rise is a signature that a transfer of angular momentum from the magnons to conduction electrons proceeds in less than 10 fs, before substantial demagnetization has happened. We further conclude that most of the spin dissipated by the lattice is transferred via magnon-lattice rather than electron-lattice interaction. These results show that the limiting speed of magnetization dynamics is not demagnetization, as generally believed, and harnessing the earliest magnon dynamics could be a new route towards an even faster spintronics.

cond-mat.mes-hall

Femtosecond photocurrents by the Dresselhaus bulk spin-galvanic effect in an inversion-asymmetric ferromagnet

We study ultrafast photocurrents in thin films of a model ferromagnetic metal with broken bulk inversion symmetry, the half-metallic Heusler compound NiMnSb, following excitation with an optical pump pulse with photon energy 1.55 eV. Remarkably, in terms of the direction of the sample magnetization M, all photocurrents are found to be a superposition of a component with Rashba- and Dresselhaus-type symmetry. We explain the Dresselhaus bulk photocurrent as follows: Pump-induced electron heating induces an excess of spin μ_s||M, which transfers spin angular momentum into states with Dresselhaus-type spin-momentum locking. The resulting charge current relaxes on a time scale of 10 fs by momentum relaxation and, thus, follows μ_s quasi-instantaneously. The relaxation of μ_s is governed by the cooling of the electrons and not by the significantly slower spin-lattice relaxation of half-metals. Our findings add the Dresselhaus spin-galvanic effect (SGE) to the set of ultrafast spin-charge-conversion phenomena. They indicate a route to more efficient spintronic terahertz emitters and detectors based on the volume scaling of the bulk SGE.

cond-mat.mtrl-sci

Ultrafast electron heating as the dominant driving force of photoinduced terahertz spin currents

Ultrafast spintronics strongly relies on the generation, transport, manipulation and detection of terahertz spin currents (TSCs). In F|HM stacks consisting of a ferromagnetic layer F and a heavy-metal layer HM, ultrafast spin currents are typically triggered by femtosecond optical laser pulses. A key open question is whether the initial step, optical excitation and injection of spin currents, can be controlled by tuning the photon energy of the femtosecond pulse. While many theoretical works suggest a marked impact of photon-energy and of highly excited non-thermal electrons, profound experimental evidence is lacking. Here, we use terahertz-emission spectroscopy to study TSCs triggered with two different photon energies of 1.5 eV and 3 eV. We study a wide range of magnetic systems covering metallic ferromagnets, ferrimagnetic insulators, half-metals, as well as systems including tunneling barriers, and rare-earth metallic alloys. We find that variation of the exciting photon energy does not change the dynamics and only slightly the amplitude of the induced TSC in all sample systems. Our results reveal that the ultrafast pump-induced heating of electrons is a highly efficient process for generating TSCs, whereas highly excited primary photoelectrons are of minor importance.

cond-mat.mes-hall

Terahertz time-domain signatures of the inverse Edelstein effect in topological-insulator|ferromagnet heterostructures

Three-dimensional topological insulators possess topologically protected surface states with spin-momentum locking, which enable spin-charge-current interconversion (SCI) by the inverse Edelstein effect (IEE). However, it remains experimentally challenging to separate the surface-related IEE from the bulk-type inverse spin Hall effect (ISHE). Here, we search for distinct time-domain signatures of the two SCI phenomena in a $\mathcal{F}$|TI model stack of a ferromagnetic-metal layer $\mathcal{F}$ (Co and Fe) and a topological-insulator layer TI (Bi$_2$Te$_3$, SnBi$_2$Te$_4$ and Bi$_{1-x}$Sb$_x$ with $x$ = 0.15 and 0.3), where the focus is on Bi$_2$Te$_3$. A femtosecond laser pulse serves to induce a transient spin voltage $μ_s^{\mathcal{F}}$ in $\mathcal{F}$ and, thus, drive an ultrafast spin current out of $\mathcal{F}$. SCI results in a transverse charge current with a sheet density $I_c$ that is detected by sampling the emitted terahertz electric field. Analysis of the dynamics of $I_c(t)$ vs time $t$ relative to $μ_s^{\mathcal{F}}(t)$ reveals two components with distinct time scales: (i) a quasi-instantaneous response and (ii) a longer-lived response with a relaxation time of 270 fs, which is independent of the chosen $\mathcal{F}$ material. Component (i) is consistently ascribed to the ISHE. In contrast, we interpret component (ii) as a signature of interfacial spin accumulation and the IEE at the $\mathcal{F}$/Bi$_2$Te$_3$ interface, with a fraction of $< 10^{-2}$ of the incident spins participating. This assignment is fully consistent with respect to its dynamics and magnitude. We rate other possible signal contributions, such as spin trapping in intermediate states, as less likely. Our results show that the femtosecond dynamics of photocurrents provide important insights into the mechanisms of spin transport and SCI in $\mathcal{F}$|TI stacks.

cond-mat.mes-hall

Hallmarks of terahertz magnon currents in an antiferromagnetic insulator

The efficient transport of spin angular momentum is expected to play a crucial role in future spintronic devices, which potentially operate at frequencies reaching the terahertz range. Antiferromagnetic insulators exhibit significant potential for facilitating ultrafast pure spin currents by terahertz magnons. Consequently, we here use femtosecond laser pulses to trigger ultrafast spin currents across antiferromagnetic NiO thin films in Py|NiO|Pt stacks, where permalloy (Py) and Pt serve as spin-current source and detector respectively. We find that the spin current pulses traversing NiO reach a velocity up to 40 nm/ps and experience increasing delay and broadening as the NiO thickness is increased. We can consistently explain our observations by ballistic transport of incoherent magnon. Our approach has high potential to characterize terahertz magnon transport in magnetic insulators with any kind of magnetic order.

cond-mat.mes-hall

Magnon-mediated terahertz spin transport in metallic Gd|Pt stacks

We study femtosecond spin transport in a Gd|Pt stack induced by a laser pulse. Remarkably, the dynamics of the spin current from Gd to Pt suggests that its dominant driving force is the ultrafast spin Seebeck effect. As the contribution of a transient spin voltage in the metal Gd is minor, Gd acts akin a magnetic insulator here. This view is supported by time- and spin-resolved photoemission, which indicates that a buildup of spin voltage is suppressed by exchange scattering, leading to similar amplitudes and relaxation rates of hot majority- and minority-spin electron populations.

cond-mat.mes-hall

Accessing ultrafast spin-transport dynamics in copper using broadband terahertz spectroscopy

We study the spatiotemporal dynamics of ultrafast electron spin transport across nanometer-thick copper layers using broadband terahertz spectroscopy. Our analysis of temporal delays, broadening and attenuation of the spin-current pulse revealed ballistic-like propagation of the pulse peak, approaching the Fermi velocity, and diffusive features including a significant velocity dispersion. A comparison to the frequency-dependent Ficks law identified the diffusion-dominated transport regime for distances larger than 2 nm. The findings lie the groundwork for designing future broadband spintronic devices.

cond-mat.mes-hall

Shaping THz emission spectra by using sub-wavelength nanopatterned spintronic THz emitters

We show in theory and experiment that in periodically patterned spintronic THz emitters (STE), charge dynamics can modify the emission spectrum in a well-controlled way. Characterization of sub-wavelength patterned STE at frequencies up to 30 THz shows that the STE's emission spectrum systematically changes with emitter size. The spectral intensity exhibits significant reductions at frequencies below 4 THz, accompanied by pronounced dips at around 15 THz and 24 THz. While reducing the STE size enhances the modulation of all features, it does not alter the dip frequencies. The effect originates from the charging of the structure's edges by THz currents, causing a backflow that interferes with the primary current pulse. An analytical model quantitatively reproduces these results and agrees well with control experiments. Our findings enable a detailed investigation of the charge dynamics in STE and provide additional means for controlled shaping of STE emission spectra by nano patterning.

physics.app-ph

Time-domain observation of ballistic orbital-angular-momentum currents with giant relaxation length in tungsten

The emerging field of orbitronics exploits the electron orbital momentum $\textit{L}$. Compared to spin-polarized electrons, $\textit{L}$ may allow magnetic-information transfera with significantly higher density over longer distances in more materials. However, direct experimental observation of $\textit{L}$ currents, their extended propagation lengths and their conversion into charge currents has remained challenging. Here, we optically trigger ultrafast angular-momentum transport in Ni|W|SiO$_2$ thin-film stacks. The resulting terahertz charge-current bursts exhibit a marked delay and width that grow linearly with W thickness. We consistently ascribe these observations to a ballistic $\textit{L}$ current from Ni through W with giant decay length (~80 nm) and low velocity (~0.1 nm/fs). At the W/SiO$_2$ interface, the $\textit{L}$ flow is efficiently converted into a charge current by the inverse orbital Rashba-Edelstein effect, consistent with ab-initio calculations. Our findings establish orbitronic materials with long-distance ballistic $\textit{L}$ transport as possible candidates for future ultrafast devices and an approach to discriminate Hall- and Rashba-Edelstein-like conversion processes.

physics.app-ph

Spin-voltage-driven efficient terahertz spin currents from the magnetic Weyl semimetals Co$_2$MnGa and Co$_2$MnAl

Magnetic Weyl semimetals are an emerging material class that combines magnetic order and a topologically non-trivial band structure. Here, we study ultrafast optically driven spin injection from thin films of the magnetic Weyl semimetals Co$_2$MnGa and Co$_2$MnAl into an adjacent Pt layer by means of terahertz emission spectroscopy. We find that (i) Co$_2$MnGa and Co$_2$MnAl are efficient terahertz spin-current generators reaching efficiencies of typical 3d-transition-metal ferromagnets such as Fe. (ii) The relaxation of the spin current provides an estimate of the electron-spin relaxation time of Co$_2$MnGa (165 fs) and Co$_2$MnAl (102 fs), which is comparable to Fe (92 fs). Both observations are consistent with a simple analytical model and highlight the large potential of magnetic Weyl semimetals as spin-current sources in terahertz spintronic devices. Finally, our results provide a strategy to identify magnetic materials that provide maximum spin current amplitudes for a given deposited optical energy density.

cond-mat.mes-hall

Transition of laser-induced terahertz spin currents from torque- to conduction-electron-mediated transport

Spin transport is crucial for future spintronic devices operating at bandwidths up to the terahertz (THz) range. In F|N thin-film stacks made of a ferro/ferrimagnetic layer F and a normal-metal layer N, spin transport is mediated by (1) spin-polarized conduction electrons and/or (2) torque between electron spins. To identify a cross-over from (1) to (2), we study laser-driven spin currents in F|Pt stacks where F consists of model materials with different degrees of electrical conductivity. For the magnetic insulators YIG, GIG and maghemite, identical dynamics is observed. It arises from the THz interfacial spin Seebeck effect (SSE), is fully determined by the relaxation of the electrons in the metal layer and provides an estimate of the spin-mixing conductance of the GIG/Pt interface. Remarkably, in the half-metallic ferrimagnet Fe3O4 (magnetite), our measurements reveal two spin-current components with opposite direction. The slower, positive component exhibits SSE dynamics and is assigned to torque-type magnon excitation of the A- and B-spin sublattices of Fe3O4. The faster, negative component arises from the pyro-spintronic effect and can consistently be assigned to ultrafast demagnetization of e-sublattice minority-spin hopping electrons. This observation supports the magneto-electronic model of Fe3O4. In general, our results provide a new route to the contact-free separation of torque- and conduction-electron-mediated spin currents.

cond-mat.mes-hall

Atomic scale control of spin current transmission at interfaces

Spin transmission at ferromagnet/heavy metal interfaces is of vital importance for many spintronic devices. Usually the spin current transmission is limited by the spin mixing conductance and loss mechanisms such as spin memory loss. In order to understand these effects, we study the interface transmission when an insulating interlayer is inserted between the ferromagnet and the heavy metal. For this we measure the inverse spin Hall voltage generated from optically injected spin current pulses as well as the magnitude of the spin pumping using ferromagnetic resonance. From our results we conclude that significant spin memory loss only occurs for 5d metals with less than half filled d-shell.

cond-mat.mes-hall