arXiv subjects

Rianne S. Lous

Publications and source records attributed to Rianne S. Lous.

10 recordsLinked to original sources

arXiv2026

Quantum Chemistry in a Novel Hybrid Dipolar Atom-Ion Mixture

Merging trapped ions with cold atomic clouds offers intriguing prospects for quantum chemistry and many-body quantum simulations. Especially when going beyond the standard alkali atomic baths by using lanthanide atoms, opportunities arise to study the interplay between the intermediate-range atom-ion interaction and the tunable long-range dipolar atom-atom interactions. However, the high total angular momentum of the ground-state of open-shell lanthanides, e.g. $^{5}I_{8}$ for dysprosium, affects the atom-ion potential. Here, we discuss the implications for long- and short-range atom-ion interactions and present a novel apparatus which combines an ytterbium ion (Yb$^{+}$) with dipolar dysprosium (Dy) atoms. We highlight the consequences of this novel Dy-Yb$^{+}$ mixture for observing buffer gas cooling, (non-) radiative charge transfer, and three-body recombination. While the energy-averaged rates are dominated by radiative charge transfer, particularly radiative association, we find that three-body recombination can compete with molecular-ion formation at Dy densities $n\gtrsim 10^{12}$ cm$^{-3}$. This competition is further enhanced by the expected non-thermal distribution of ion energies. These processes could be experimentally characterised through controlled variation of the atom-ion interaction parameters, providing a direct test of our theoretical predictions.

physics.atom-ph↗

arXiv2026

General circuit mapping algorithm for neutral atom quantum computers

Neutral atom quantum computers (NAQC) are emerging as a promising, scalable quantum computing platform because of their long qubit coherence, flexible qubit arrangement, and multiqubit gate capabilities. However, circuit execution often requires physically moving qubits, making compilation a critical optimization challenge. We propose a circuit independent mathematical framework built on graph-theoretic combinatorial optimization that determines the minimal number of required qubit transfers. This model captures spatial constraints specific to NAQC platforms with zone-limited gate operations and multi-qubit gates. From this framework, we encode the qubit mapping problem as a nonlinear integer program and solve it using a genetic algorithm, enabling trade-offs between minimizing the total traveled distance and the number of parallel transfer operations. Compared to the state-of-the-art scalable compiler for zoned architectures, our approach consistently finds fewer transfers. Depending on the optimization focus, our method produces shorter traveled distances or fewer parallel transfer operations. This work provides both theoretical guaranties and a practical tool for efficient, architecture-aware quantum circuit compilation. As a result, practitioners can generate hardware-aware mappings that reduce movement-induced errors and better exploit atom transfer parallelism, directly improving execution efficiency on NAQC devices.

quant-ph↗

arXiv2022

Ultracold ion-atom experiments: cooling, chemistry, and quantum effects

Experimental setups that study laser-cooled ions immersed in baths of ultracold atoms merge the two exciting and well-established fields of quantum gases and trapped ions. These experiments benefit both from the exquisite read-out and control of the few-body ion systems as well as the many-body aspects, tunable interactions, and ultracold temperatures of the atoms. However, combining the two leads to challenges both in the experimental design and the physics that can be studied. Nevertheless, these systems have provided insights into ion-atom collisions, buffer gas cooling of ions and quantum effects in the ion-atom interaction. This makes them promising candidates for ultracold quantum chemistry studies, creation of cold molecular ions for spectroscopy and precision measurements, and as test beds for quantum simulation of charged impurity physics. In this review we aim to provide an experimental account of recent progress and introduce the experimental setup and techniques that enabled the observation of quantum effects.

physics.atom-ph↗

arXiv2020

Controlling the nature of a charged impurity in a bath of Feshbach dimers

We theoretically study the dynamics of a trapped ion that is immersed in an ultracold gas of weakly bound atomic dimers created by a Feshbach resonance. Using quasi-classical simulations, we find a crossover from dimer dissociation to molecular ion formation depending on the binding energy of the dimers. The location of the crossover strongly depends on the collision energy and the time-dependent fields of the Paul trap. Deeply bound dimers lead to fast molecular ion formation, with rates approaching the Langevin collision rate $Γ'_\text{L}\approx4.8\times10^{-9}\,$cm$^3$s$^{-1}$. The kinetic energies of the created molecular ions have a median below $1\,$mK, such that they will stay confined in the ion trap. We conclude that interacting ions and Feshbach molecules may provide a novel approach towards the creation of ultracold molecular ions with applications in precision spectroscopy and quantum chemistry.

physics.atom-ph↗

arXiv2018

Breathing Mode of a BEC Repulsively Interacting with a Fermionic Reservoir

We investigate the fundamental breathing mode of a small-sized elongated Bose-Einstein condensate coupled to a large Fermi sea of atoms. Our observations show a dramatic shift of the breathing frequency when the mixture undergoes phase separation at strong interspecies repulsion. We find that the maximum frequency shift in the full phase-separation limit depends essentially on the atom number ratio of the components. We interpret the experimental observations within a model that assumes an adiabatic response of the Fermi sea, or within another model that considers single fermion trajectories for a fully phase-separated mixture. These two complementary models capture the observed features over the full range of interest.

cond-mat.quant-gas↗

arXiv2018

Probing the Interface of a Phase-Separated State in a Repulsive Bose-Fermi Mixture

We probe the interface between a phase-separated Bose-Fermi mixture consisting of a small BEC of $^{41}$K residing in a large Fermi sea of $^6$Li. We quantify the residual spatial overlap between the two components by measuring three-body recombination losses for variable strength of the interspecies repulsion. A comparison with a numerical mean-field model highlights the importance of the kinetic energy term for the condensed bosons in maintaining the thin interface far into the phase-separated regime. Our results demonstrate a corresponding smoothing of the phase transition in a system of finite size.

quant-ph↗

arXiv2017

Thermometry of a deeply degenerate Fermi gas with a Bose-Einstein condensate

We measure the temperature of a deeply degenerate Fermi gas, by using a weakly interacting sample of heavier bosonic atoms as a probe. This thermometry method relies on the thermalization between the two species and on the determination of the condensate fraction of the bosons. In our experimental implementation, a small sample of 41K atoms serves as the thermometer for a 6Li Fermi sea. We investigate the evaporative cooling of a 6Li spin mixture in a single-beam optical dipole trap and observe how the condensate fraction of the thermometry atoms depends on the final trap depth. From the condensate fraction, the temperature can be readily extracted. We show that the lowest temperature of 6.3(5)% of the Fermi temperature is obtained, when the decreasing trap depth closely approaches the Fermi energy. To understand the systematic effects that may in uence the results, we carefully investigate the role of the number of bosons and the thermalization dynamics between the two species. Our thermometry approach provides a conceptually simple, accurate, and general way to measure the temperature of deeply degenerate Fermi gases. Since the method is independent of the specific interaction conditions within the Fermi gas, it applies to both weakly and strongly interacting Fermi gases.

cond-mat.quant-gas↗

arXiv2017

Lifetime of Feshbach dimers in a Fermi-Fermi mixture of $^6$Li and $^{40}$K

We present a joint experimental and theoretical investigation of the lifetime of weakly bound dimers formed near narrow interspecies Feshbach resonances in mass-imbalanced Fermi-Fermi systems, considering the specific example of a mixture of $^6$Li and $^{40}$K atoms. Our work addresses the central question of the increase in the stability of the dimers resulting from Pauli suppression of collisional losses, which is a well-known effect in mass-balanced fermionic systems near broad resonances. We present measurements of the spontaneous dissociation of dimers in dilute samples, and of the collisional losses in dense samples arising from both dimer-dimer processes and from atom-dimer processes. We find that all loss processes are suppressed close to the Feshbach resonance. Our general theoretical approach for fermionic mixtures near narrow Feshbach resonances provides predictions for the suppression of collisional decay as a function of the detuning from resonance, and we find excellent agreement with the experimental benchmarks provided by our $^6$Li-$^{40}$K system. We finally present model calculations for other Feshbach-resonant Fermi-Fermi systems, which are of interest for experiments in the near future.

cond-mat.quant-gas↗

arXiv2015

Decoherence of Impurities in a Fermi Sea of Ultracold Atoms

We investigate the decoherence of $^{40}$K impurities interacting with a three-dimensional Fermi sea of $^{6}$Li across an interspecies Feshbach resonance. The decoherence is measured as a function of the interaction strength and temperature using a spin-echo atom interferometry method. For weak to moderate interaction strengths, we interpret our measurements in terms of scattering of K quasiparticles by the Fermi sea and find very good agreement with a Fermi liquid calculation. For strong interactions, we observe significant enhancement of the decoherence rate, which is largely independent of temperature, pointing to behavior that is beyond the Fermi liquid picture.

cond-mat.quant-gas↗

arXiv2014

Observation of a Strong Atom-Dimer Attraction in a Mass-Imbalanced Fermi-Fermi Mixture

We investigate a mixture of ultracold fermionic $^{40}$K atoms and weakly bound $^{6}$Li$^{40}$K dimers on the repulsive side of a heteronuclear atomic Feshbach resonance. By radio-frequency spectroscopy we demonstrate that the normally repulsive atom-dimer interaction is turned into a strong attraction. The phenomenon can be understood as a three-body effect in which two heavy $^{40}$K fermions exchange the light $^{6}$Li atom, leading to attraction in odd partial-wave channels (mainly p-wave). Our observations show that mass imbalance in a fermionic system can profoundly change the character of interactions as compared to the well-established mass-balanced case.

cond-mat.quant-gas↗