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Richard Spieker

Publications and source records attributed to Richard Spieker.

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Piezomagnetism in a model cubic noncollinear altermagnet

Altermagnets constitute a distinct class of magnetic materials that combine compensated magnetic order with spin-polarized electronic bands, hence carrying characteristics of both antiferromagnets and ferromagnets. Piezomagnetism - the linear relationship between lattice strain and a net magnetic moment - has emerged as smoking-gun evidence of altermagnetism that distinguishes it from antiferromagnetism. Here, we uncover a large piezomagnetic response in MnTe2, a cubic altermagnet with a noncollinear spin arrangement and weak spin-orbit coupling. We combine dilatometry with nuclear magnetic resonance, a bulk local probe, to observe signatures of both direct and inverse piezomagnetism consistent with symmetry considerations and first-principles calculations. The dilatometry measurements reveal a shear deformation proportional to an applied magnetic field, while magnetic resonance detects a ferromagnetic moment induced by shear strain. The respective results for the piezomagnetic coupling strength are in good agreement, and they are captured by first-principles results. These findings for simple binary MnTe2 position this material as a model altermagnet, demonstrate the utility of nuclear magnetic resonance in investigations of piezomagnetism, and open new avenues for multimodal strain and magnetic-field control in spintronic and memory applications.

cond-mat.mtrl-sci

Structural Properties of Plastically Deformed SrTiO3 and KTaO3

Dislocation engineering has the potential to open new avenues toward the exploration and modification of the properties of quantum materials. Strontium titanate (SrTiO3, STO) and potassium tantalate (KTaO3, KTO) are incipient ferroelectrics that show metallization and superconductivity at extremely low charge carrier concentrations, and have been the subject of resurgent interest. These materials also exhibit remarkable ambient-temperature ductility, and thus represent exceptional platforms for studies of the effects of deformation-induced dislocation structures on electronic properties. Recent work on plastically deformed STO revealed an enhancement of the superconducting transition temperature and the emergence of local ferroelectricity and magnetism near self-organized dislocation walls. Here we present a comprehensive structural analysis of plastically deformed STO and KTO, employing specially designed strain cells, diffuse neutron and x-ray scattering, Raman scattering, and nuclear magnetic resonance (NMR). Diffuse scattering and NMR provide insight into the dislocation configurations and densities and their dependence on strain. As in the prior work on STO, Raman scattering reveals evidence for local ferroelectric order near dislocation walls in plastically deformed KTO. Our findings provide valuable information about the self-organized defect structures in both materials, and they position KTO as a second model system with which to explore the associated emergent physics.

cond-mat.mtrl-sci