arXiv subjects

Rik Broekhoven

Publications and source records attributed to Rik Broekhoven.

5 recordsLinked to original sources

arXiv2025

Single-shot readout of the nuclear spin of an on-surface atom

Nuclear spins owe their long-lived magnetic states to their excellent isolation from the environment. At the same time, a finite degree of interaction with their surroundings is necessary for reading and writing the spin state. Therefore, detailed knowledge of and control over the atomic environment of a nuclear spin is key to optimizing conditions for quantum information applications. While various platforms enabled single-shot readout of nuclear spins, their direct environments were either unknown or impossible to controllably modify on the atomic scale. Scanning tunnelling microscopy (STM), combined with electron spin resonance (ESR), provides atomic-scale information of individual nuclear spins via the hyperfine interaction. Here, we demonstrate single-shot readout of an individual $^{\text{49}}$Ti nuclear spin with an STM. Employing a pulsed measurement scheme, we find its lifetime to be in the order of seconds. Furthermore, we shed light on the pumping and relaxation mechanisms of the nuclear spin by investigating its response to both ESR driving and tunnelling current, which is supported by model calculations. These findings give an atomic-scale insight into the nature of nuclear spin relaxation and are relevant for the development of atomically assembled qubit platforms.

cond-mat.mes-hall↗

arXiv2024

Protocol for certifying entanglement in surface spin systems using a scanning tunneling microscope

Certifying quantum entanglement is a critical step towards realizing quantum-coherent applications of surface spin systems. In this work, we show that entanglement can be unambiguously shown in a scanning tunneling microscope (STM) with electron spin resonance by exploiting the fact that entangled states undergo a free time evolution with a distinct characteristic time constant that clearly distinguishes it from any other time evolution in the system. By implementing a suitable phase control scheme, the phase of this time evolution can be mapped back onto the population of one entangled spin in a pair, which can then be read out reliably using a weakly coupled sensor spin in the junction of the scanning tunneling microscope. We demonstrate through open quantum system simulations with realistic spin systems, which are currently available with spin coherence times of $T_2\approx$ 300 ns, that a signal directly correlated with the degree of entanglement can be measured at a temperature range of 100$-$400 mK accessible in sub-Kelvin cryogenic STM systems.

cond-mat.mes-hall↗

arXiv2023

Coherent spin dynamics between electron and nucleus within a single atom

The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom. These qualities have been demonstrated in a variety of nuclear spin qubit architectures, albeit with limited control over the direct environment of the nuclei. As a contrasting approach, the combination of electron spin resonance (ESR) and scanning tunnelling microscopy (STM) provides a bottom-up platform to study the fundamental properties of nuclear spins of single atoms on a surface. However, access to the time evolution of these nuclear spins, as was recently demonstrated for electron spins, remained a challenge. Here, we present an experiment resolving the nanosecond coherent dynamics of a hyperfine-driven flip-flop interaction between the spin of an individual nucleus and that of an orbiting electron. We use the unique local controllability of the magnetic field emanating from the STM probe tip to bring the electron and nuclear spins in tune, as evidenced by a set of avoided level crossings in ESR-STM. Subsequently, we polarize both spins through scattering of tunnelling electrons and measure the resulting free evolution of the coupled spin system using a DC pump-probe scheme. The latter reveals a complex pattern of multiple interfering coherent oscillations, providing unique insight into the atom's hyperfine physics. The ability to trace the coherent hyperfine dynamics with atomic-scale structural control adds a new dimension to the study of on-surface spins, offering a pathway towards dynamic quantum simulation of low-dimensional magnonics.

cond-mat.mes-hall↗

arXiv2022

Confined vacuum resonances as artificial atoms with tunable lifetime

Atomically engineered artificial lattices are a useful tool for simulating complex quantum phenomena, but have so far been limited to the study of Hamiltonians where electron-electron interactions do not play a role -- but it's precisely the regime in which these interactions do matter where computational times lend simulations a critical advantage over numerical methods. Here, we propose a new platform for constructing artificial matter that relies on the confinement of field-emission resonances, a class of vacuum-localized discretized electronic states. We use atom manipulation of surface vacancies in a chlorine-terminated Cu(100) surface to reveal square patches of the underlying metal, thereby creating atomically-precise potential wells that host particle-in-a-box modes. By adjusting the shape and size of the confining potential, we can access states with different quantum numbers, making these patches attractive candidates as quantum dots or artificial atoms. We demonstrate that the lifetime of electrons in these engineered states can be extended and tuned through modification of the confining potential, either via atomic assembly or by changing the tip-sample distance. We also demonstrate control over a finite range of state-filling, a parameter which plays a key role in the evolution of quantum many-body states. We model the transport through the localized state to disentangle and quantify the lifetime-limiting processes, illustrating the critical dependency of the electron lifetime on the properties of the underlying bulk band structure. The interplay with the bulk bands also gives rise to negative differential resistance, opening possible avenues for engineering custom atomic-scale resonant tunnelling diodes, which exhibit similar current-voltage characteristics.

cond-mat.mes-hall↗

arXiv2021

Free coherent evolution of a coupled atomic spin system initialized by electron scattering

Full insight into the dynamics of a coupled quantum system depends on the ability to follow the effect of a local excitation in real-time. Here, we trace the coherent evolution of a pair of coupled atomic spins by means of scanning tunneling microscopy. We use a pump-probe scheme to detect the local magnetization following a current-induced excitation performed on one of the spins. Making use of magnetic interaction with the probe tip, we are able to tune the relative precession of the spins. We show that only if their Larmor frequencies match, the two spins can entangle, causing the excitation to be swapped back and forth. These results provide insight into the locality of electron-spin scattering, and set the stage for controlled migration of a quantum state through an extended spin lattice.

cond-mat.mes-hall↗