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Rinaldo Trotta

Publications and source records attributed to Rinaldo Trotta.

At least 19 recordsLinked to original sources

Picosecond-resolved entanglement distribution over an urban free-space channel

Time-evolving entangled states describe quantum particles whose correlations evolve in time according to a well-defined dynamics. Such states can be generated in a variety of physical systems and are promising resources for several quantum technologies, ranging from quantum clock synchronization to quantum communication. However, their full potential is currently limited by the fact that the entanglement dynamics often occur on timescales comparable to the achievable synchronization precision, especially in experiments aimed at distributing entanglement through noisy urban channels. In this context, accurate timing is not merely a technical detail, but a fundamental requirement for faithfully observing and exploiting the underlying quantum correlations. Here, we demonstrate the faithful distribution of a fast-evolving entangled state over a 270 m free-space channel connecting two buildings in the center of Rome. The developed system incorporates a synchronization device capable of achieving sub-50 ps timing accuracy between the two ends of the link while simultaneously supporting channel stabilization. Our results demonstrate that time-evolving entanglement can be reliably transmitted through a noisy urban free-space channel, representing an important benchmark toward long-distance free-space quantum communication and the future implementation of time-correlated entangled states in demanding scenarios such as satellite-based quantum networks.

quant-ph

A diode nanocavity for fast, efficient and tunable emission of highly entangled photon pairs and Fourier-transform-limited single photons

Deterministic sources of entangled photon pairs and indistinguishable photons are expected to play a key role in photonic quantum technologies. Semiconductor quantum dots are promising candidates due to their on-demand emission and compatibility with nanophotonic structures. However, current implementations face trade-offs between extraction efficiency, Purcell enhancement, as well as charge noise that causes blinking and degrades indistinguishability. Here we demonstrate a tunable nano-optoelectronic device based on a quantum dot embedded in a p-i-n diode circular-Bragg-grating-resonator and featuring extraction efficiencies up to 0.55(6) and Purcell-factor of $\sim$8. The device generates wavelength-tunable entangled photon pairs with suppressed blinking and raw (corrected) concurrence > 0.89 (0.91) over a range of 1.6 nm. The very same source also emits single, nearly Fourier-limited and highly indistinguishable photons with raw (corrected) $\mathcal{V}_{\text{HOM}}$ = 0.951(4) (0.988(6)). These results demonstrate a viable platform for semiconductor quantum photonics.

quant-ph

Industry-ready spin-photon interfaces for hybrid photonic quantum computing

Hybrid photonic quantum computers, combining stationary matter qubits and flying photonic qubits, offer an intrinsically networked and resource-efficient route to large-scale, error-corrected quantum computation. Their core components are cavity-coupled matter qubits that act as light--matter interfaces, enabling: high-efficiency on-demand single-photon generation, stable near-unity photon indistinguishability and spin--multi-photon entanglement. Semiconductor quantum dots in microcavities are a leading platform for realizing such devices. Yet reaching the performance, reproducibility and spin-coherence thresholds for large-scale error correction remains a major challenge requiring industrial fabrication and control. Here we report thousands of monolithic semiconductor quantum-dot devices fabricated using a III--V pilot production-line process compatible with large-scale deployment. Systematic control of source parameters yields state-of-the-art efficiency and supports a path to optical losses below fault-tolerance thresholds. Using field-quadrature state reconstruction as a stringent joint test of efficiency and indistinguishability, we observe near-unity photon quantum purity stable over tens of minutes and a record single-photon Wigner-function negativity. We further demonstrate seven-partite spin--multi-photon entanglement and spin coherence extendable to microsecond timescales in the low-magnetic-field regime. Finally, photons from distant sources are as indistinguishable as photons emitted successively by a single source. These results establish foundry-compatible III--V quantum dots as a scalable platform for hybrid photonic quantum computing.

quant-ph

Cascaded Metasurface Interferometer for Multipath Interference with Classical and Quantum Light

Beamsplitters represent fundamental components in both classical and quantum optical systems, enabling the distribution of light, as well as the generation of interference, superposition and entanglement. However, optical networks constructed from conventional bulk 2x2-beamsplitters encounter inherent scalability issues, as the number of required beamsplitters scales quadratically with the number of optical modes for a fully connected network. Metasurfaces offer a promising route to overcome these constraints. By manipulating light at the wavelength scale compact optical components with advanced functionalities can be constructed, which address several modes simultaneously. In this work, we design and experimentally utilize a metasurface as a multiport beamsplitter. Furthermore, we realize a multimode interferometer composed of two cascaded metasurfaces. We characterize the individual and cascaded metasurfaces using classical light, showing controllable splitting ratios through tunable phase relations. We then expand the approach to quantum light, employing single photons to demonstrate second- and third-order photon correlations, as well as single photon interference across multiple spatial paths. These results establish metasurface-based multiport beamsplitters as a scalable and reconfigurable platform bridging classical and quantum photonics.

physics.optics

A complete fs-laser-ablation route to miniaturized single-crystal PMN-PT piezoelectric actuators

This article presents a novel fabrication route for miniaturized piezoelectric actuators that relies exclusively on processes based on femtosecond (fs) laser ablation. Previous work has already demonstrated that fs-lasers are uniquely suited for the fabrication of piezoelectric actuators based on PMN-PT, which are required for multiaxial strain-tuning of quantum dots (QDs) to enable, e.g. the generation of highly entangled photon pairs. Building on these foundations, the present work advances actuator performance and capabilities by introducing a local thinning strategy. This approach allows the realization of smaller devices, which in turn enables lower operating voltages, while simultaneously offering the possibility of integrating multiple quantum light sources on a single chip. The article provides a detailed description of the full fabrication chain, entirely based on fs-laser processing steps, from substrate thinning to metal layer structuring and final device definition. A particular focus is placed on the final cutting process, where the implementation of a third-harmonic ultraviolet (UV) fs-laser wavelength significantly improves edge quality and shape definition compared to the second harmonic (SH) wavelength used in previous work. The device fabricated through the combination of local thinning and UV-based cutting promises not only to enhance the efficiency of strain transfer but also to ensure the mechanical stability required for practical applications. These results establish fs-laser-based fabrication as a versatile and scalable method for next-generation piezoelectric actuators, paving the way for advanced strain-engineering approaches in semiconductor quantum optics and integrated quantum photonics.

physics.app-ph

All-photonic entanglement swapping with remote quantum dots

Entanglement swapping is a protocol that details how to create entanglement between previously uncorrelated particles. Its all-photonic version - mediated by the interference of photon pairs generated by separate quantum systems-finds disparate applications in quantum networks. So far, all-photonic entanglement swapping between remote systems has been implemented only using sources that operate probabilistically. However, the scaling up of quantum networks requires deterministic quantum emitters that do not suffer from a trade-off between degree of entanglement and photonpair generation rate. Here, we demonstrate all-photonic entanglement swapping using photon-pairs generated by two separate GaAs quantum dots. The emitters are deterministically embedded in hybrid semiconductor-piezoelectric devices that make the entangled-photons from two dissimilar quantum dots nearly identical. Entanglement swapping is demonstrated with a fidelity as high as 0.71(2), more than 10 standard deviations above the classical limit. The experimental data are quantitatively explained by a theoretical model that also suggests how to boost the protocol performances. Our work opens the path to the exploitation of quantum dot entangled-photon sources in quantum repeater networks.

quant-ph

Ability of entanglement and purity to help to detect systematic experimental errors

Measurements are central in all quantitative sciences, and a fundamental challenge is to make observations without systematic measurement errors. This holds in particular for quantum information processing, where other error sources, such as noise and decoherence, are unavoidable. Consequently, methods for detecting systematic errors have been developed, but the required quantum state properties are yet unexplored. We theoretically develop a direct and efficient method to detect systematic errors in quantum experiments and demonstrate it experimentally using quantum state tomography of photon pairs emitted from a semiconductor quantum dot. Our method can be scaled to multi-qubit systems, and we find that entanglement and quantum states with high purity can help identify systematic errors.

quant-ph

Quantum teleportation with dissimilar quantum dots over a hybrid quantum network

Photonic quantum information processing in metropolitan quantum networks lays the foundation for cloud quantum computing [1, 2], secure communication [3, 4], and the realization of a global quantum internet [5, 6]. This paradigm shift requires on-demand and high-rate generation of flying qubits and their quantum state teleportation over long distances [7]. Despite the last decade has witnessed an impressive progress in the performances of deterministic photon sources [8-11], the exploitation of distinct quantum emitters to implement all-photonic quantum teleportation among distant parties has remained elusive. Here, we overcome this challenge by using dissimilar quantum dots whose electronic and optical properties are engineered by light-matter interaction [12], multi-axial strain [13] and magnetic fields [14] so as to make them suitable for the teleportation of polarization qubits. This is demonstrated in a hybrid quantum network harnessing both fiber connections and 270 m free-space optical link connecting two buildings of the University campus in the center of Rome. The protocol exploits GPS-assisted synchronization, ultra-fast single photon detectors as well as stabilization systems that compensate for atmospheric turbulence. The achieved teleportation state fidelity reaches up to 82+-1%, above the classical limit by more than 10 standard deviations. Our field demonstration of all-photonic quantum teleportation opens a new route to implement solid-state based quantum relays and builds the foundation for practical quantum networks.

quant-ph

Wavevector-resolved polarization entanglement from radiative cascades

The generation of entangled photons from radiative cascades has enabled milestone experiments in quantum information science with several applications in photonic quantum technologies. Significant efforts are being devoted to pushing the performances of near-deterministic entangled-photon sources based on single quantum emitters often embedded in photonic cavities, so to boost the flux of photon pairs. The general postulate is that the emitter generates photons in a nearly maximally entangled state of polarization, ready for application purposes. Here, we demonstrate that this assumption is unjustified. We show that in radiative cascades there exists an interplay between photon polarization and emission wavevector, strongly affecting quantum correlations when emitters are embedded in micro-cavities. We discuss how the polarization entanglement of photon pairs from a biexciton-exciton cascade in quantum dots strongly depends on their propagation wavevector, and it can even vanish for large emission angles. Our experimental results, backed by theoretical modelling, yield a brand-new understanding of cascaded emission for various quantum emitters. In addition, our model provides quantitative guidelines for designing optical microcavities that retain both a high degree of entanglement and collection efficiency, moving the community one step further towards an ideal source of entangled photons for quantum technologies.

quant-ph

A source of entangled photons based on a cavity-enhanced and strain-tuned GaAs quantum dot

A quantum-light source that delivers photons with a high brightness and a high degree of entanglement is fundamental for the development of efficient entanglement-based quantum-key distribution systems. Among all possible candidates, epitaxial quantum dots are currently emerging as one of the brightest sources of highly entangled photons. However, the optimization of both brightness and entanglement currently requires different technologies that are difficult to combine in a scalable manner. In this work, we overcome this challenge by developing a novel device consisting of a quantum dot embedded in a circular Bragg resonator, in turn, integrated onto a micromachined piezoelectric actuator. The resonator engineers the light-matter interaction to empower extraction efficiencies up to 0.69(4). Simultaneously, the actuator manipulates strain fields that tune the quantum dot for the generation of entangled photons with corrected fidelities to a maximally entangled state up to 0.96(1). This hybrid technology has the potential to overcome the limitations of the key rates that plague QD-based entangled sources for entanglement-based quantum key distribution and entanglement-based quantum networks.

quant-ph

Polarized and Un-Polarized Emission from a Single Emitter in a Bullseye Resonator

We present polarized |S|=0.99$\pm$0.01, and unpolarized |S|=0.03$\pm$0.01 emission from a single emitter embedded in a single, cylindrically symmetric device design. We show that the polarization stems from a position offset of the single emitter with respect to the cavity center, which breaks the cylindrical symmetry, and a position-dependent coupling to the frequency degenerate eigenmodes of the resonator structure. The experimental results are interpreted by using numerical simulations and by experimental mapping of the polarization-resolved far-field emission patterns. Our findings can be generalized to any nanophotonic structure where two orthogonal eigenmodes are not fully spatially overlapping.

physics.optics

Post-fabrication tuning of circular Bragg resonators for enhanced emitter-cavity coupling

Solid-state quantum emitters embedded in circular Bragg resonators are attractive due to their ability to emit quantum states of light with high brightness and low multi-photon probability. As for any emitter-microcavity system, fabrication imperfections limit the spatial and spectral overlap of the emitter with the cavity mode, thus limiting their coupling strength. Here, we show that an initial spectral mismatch can be corrected after device fabrication by repeated wet chemical etching steps. We demonstrate ~16 nm wavelength tuning for optical modes in AlGaAs resonators on oxide, leading to a 4-fold Purcell enhancement of the emission of single embedded GaAs quantum dots. Numerical calculations reproduce the observations and suggest that the achievable performance of the resonator is only marginally affected in the explored tuning range. We expect the method to be applicable also to circular Bragg resonators based on other material platforms, thus increasing the device yield of cavity-enhanced solid-state quantum emitters.

quant-ph

Signatures of the Optical Stark Effect on Entangled Photon Pairs from Resonantly-Pumped Quantum Dots

Two-photon resonant excitation of the biexciton-exciton cascade in a quantum dot generates highly polarization-entangled photon pairs in a near-deterministic way. However, the ultimate level of achievable entanglement is still debated. Here, we observe the impact of the laser-induced AC-Stark effect on the quantum dot emission spectra and on entanglement. For increasing pulse-duration/lifetime ratios and pump powers, decreasing values of concurrence are recorded. Nonetheless, additional contributions are still required to fully account for the observed below-unity concurrence.

quant-ph

Hyperfine-interaction limits polarization entanglement of photons from semiconductor quantum dots

Excitons in quantum dots are excellent sources of polarization-entangled photon pairs, but a quantitative understanding of their interaction with the nuclear spin bath is still missing. Here we investigate the role of hyperfine energy shifts using experimentally accessible parameters and derive an upper limit to the achievable entanglement fidelity. Our results are consistent with all available literature, indicate that spin-noise is often the dominant process limiting the entanglement in InGaAs quantum dots, and suggest routes to alleviate its effect.

quant-ph

Coherent Quantum Interconnection between On-Demand Quantum Dot Single Photons and a Resonant Atomic Quantum Memory

Long-range quantum communication requires the development of in-out light-matter interfaces to achieve a quantum advantage in entanglement distribution. Ideally, these quantum interconnections should be as fast as possible to achieve high-rate entangled qubits distribution. Here, we demonstrate the coherent quanta exchange between single photons generated on-demand from a GaAs quantum dot and atomic ensemble in a $^{87}$Rb vapor quantum memory. Through an open quantum system analysis, we demonstrate the mapping between the quantized electric field of photons and the coherence of the atomic ensemble. Our results play a pivotal role in understanding quantum light-matter interactions at the short time scales required to build fast hybrid quantum networks.

quant-ph

Strain-induced dynamic control over the population of quantum emitters in two-dimensional materials

The discovery of quantum emitters (QEs) in two-dimensional materials (2D) has triggered a surge of research to assess their suitability for quantum photonics. While their microscopic origin is still the subject of intense studies, position-controlled QEs are routinely fabricated using static strain gradients, which are used to drive excitons towards localized regions of the crystal where quantum light emission takes place. However, the use of strain in a dynamic fashion to control the brightness of single-photon sources in 2D materials has not been explored so far. In this work, we address this challenge by introducing a novel hybrid semiconductorpiezoelectric device in which WSe2 monolayers are integrated onto piezoelectric pillars that provide both static and dynamic strains. The static strains are first used to induce the formation of QEs, whose emission shows photon anti-bunching. Their energy and brightness are then controlled via the application of voltages to the piezoelectric pillars. Numerical simulations combined with drift-diffusion equations show that these effects are due to a strain-induced modification of the confining-potential landscape, which in turn leads to a net redistribution of excitons among the different QEs. Our work provides a method to dynamically control the brightness of single photon sources based on 2D materials.

cond-mat.mtrl-sci

Experimental Multi-state Quantum Discrimination in the Frequency Domain with Quantum Dot Light

The quest for the realization of effective quantum state discrimination strategies is of great interest for quantum information technology, as well as for fundamental studies. Therefore, it is crucial to develop new and more efficient methods to implement discrimination protocols for quantum states. Among the others, single photon implementations are more advisable, because of their inherent security advantage in quantum communication scenarios. In this work, we present the experimental realization of a protocol employing a time-multiplexing strategy to optimally discriminate among eight non-orthogonal states, encoded in the four-dimensional Hilbert space spanning both the polarization degree of freedom and photon energy. The experiment, built on a custom-designed bulk optics analyser setup and single photons generated by a nearly deterministic solid-state source, represents a benchmarking example of minimum error discrimination with actual quantum states, requiring only linear optics and two photodetectors to be realized. Our work paves the way for more complex applications and delivers a novel approach towards high-dimensional quantum encoding and decoding operations.

quant-ph

Daylight entanglement-based quantum key distribution with a quantum dot source

Entanglement-based quantum key distribution can enable secure communication in trusted node-free networks and over long distances. Although implementations exist both in fiber and in free space, the latter approach is often considered challenging due to environmental factors. Here, we implement a quantum communication protocol during daytime for the first time using a quantum dot source. This technology presents advantages in terms of narrower spectral bandwidth -- beneficial for filtering out sunlight -- and negligible multiphoton emission at peak brightness. We demonstrate continuous operation over the course of three and a half days, across an urban 270-m-long free-space optical link, under different light and weather conditions.

quant-ph