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Rishi Acharya

Publications and source records attributed to Rishi Acharya.

3 recordsLinked to original sources

Plasmon-driven electron-hole pair formation in a non-equilibrium Fermi liquid

Collective modes in Fermi liquids are usually regarded as dissipation channels that relax electronic excitations through Landau damping. Whether such modes can instead mediate the formation of correlated electronic states under non-equilibrium conditions remains an open question. Here, we show that under optical photo-doping, a bulk plasmon can drive correlated inter-band transfer within a transient electronic continuum. Using time- and angle-resolved photoemission spectroscopy (Tr-ARPES) on EuCd$_2$As$_2$ supported by electronic structure calculations, we observe that at high excitation density, plasmons transfer energy from a weakly dispersing bulk band into unoccupied surface states. This bulk-to-surface redistribution stabilizes a long-lived, energy-localized spectral feature consistent with a Mahan exciton. Our results reveal a non-equilibrium regime of Fermi-liquid physics in which collective modes do not merely dissipate energy, but also stabilize correlated bound states.

cond-mat.mes-hall

Visualizing Berry curvature in a Floquet-Chern insulator

Circularly polarized light can open a topological gap in a gapless Dirac system, creating a Floquet-Chern insulator. However, its Berry curvature has not been directly resolved. Here we use circular-dichroism time- and angle-resolved photoemission spectroscopy (Tr-ARPES) to map the light-induced Berry curvature of Floquet-Bloch states on the surface of Bi$_2$Se$_3$. By comparing spectra for opposite helicities of the mid-infrared pump, we isolate the induced geometric response. We observe alternating-sign Berry-curvature features at Floquet gaps that repeat at intervals set by the pump photon energy and redistribute with pump field strength in agreement with calculations for a periodically driven Dirac Hamiltonian. Both the induced Berry-curvature and the Floquet Dirac gap decay faster than the replica intensity, showing that spectral replicas can persist even after coherent Floquet hybridization weakens. These results establish momentum-resolved Berry-curvature mapping as a direct probe of light-induced topology and coherent Floquet band formation.

cond-mat.mes-hall

Evidence for bootstrap percolation dynamics in a photo-induced phase transition

Upon intense femtosecond photo-excitation, a many-body system can undergo a phase transition through a non-equilibrium route, but understanding these pathways remains an outstanding challenge. Here, we use time-resolved second harmonic generation to investigate a photo-induced phase transition in Ca$_3$Ru$_2$O$_7$ and show that mesoscale inhomogeneity profoundly influences the transition dynamics. We observe a marked slowing down of the characteristic time, $τ$, that quantifies the transition between two structures. $τ$ evolves non-monotonically as a function of photo-excitation fluence, rising from below 200~fs to $\sim$1.4~ps, then falling again to below 200~fs. To account for the observed behavior, we perform a bootstrap percolation simulation that demonstrates how local structural interactions govern the transition kinetics. Our work highlights the importance of percolating mesoscale inhomogeneity in the dynamics of photo-induced phase transitions and provides a model that may be useful for understanding such transitions more broadly.

cond-mat.str-el