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Ritam Banerjee

Publications and source records attributed to Ritam Banerjee.

3 recordsLinked to original sources

Magnetoconductance evolution across the topological-trivial phase transition in ${In_{x}}({Bi_{0.3}}{Sb_{0.7}})_{2-x}{Te_3}$ thin films

We investigate the evolution of electronic transport across the topological-trivial phase transition in ${\rm In}_{x}({\rm Bi}_{0.3}{\rm Sb}_{0.7})_{2-x}{\rm Te}_3$ thin films by systematically tuning the indium concentration $x$. Increasing $x$ reduces the effective spin-orbit coupling, driving a topological quantum phase transition near $x \approx 7\%$, and at higher disorder a crossover from diffusive to strongly localized transport around $x \approx 15\%$. In the diffusive regime, the magnetoconductance is well described by the Hikami-Larkin-Nagaoka formalism, with the evolution of the WAL prefactor $\alpha$ correlating with the band-inversion transition. Beyond the diffusive limit, transport crosses into variable-range hopping, accompanied by a striking reversal of magnetoconductance from negative to positive. The observed positive low-field magnetoconductance, its pronounced anisotropy, and its temperature evolution point to an orbital origin of the response. These features are naturally captured by incorporating the incoherent hopping mechanism of Raikh \textit{et al.} together with wavefunction shrinkage, rather than by conventional quantum-correction frameworks. Our results provide a unified picture of how topology, spin-orbit coupling, and disorder collectively determine the full field-temperature magnetotransport landscape in this material class, establishing a clear experimental link between the topological phase transition and the onset of incoherent hopping-dominated conduction.

cond-mat.mtrl-sci

Optimizing defect states in $(Bi_{0.3}Sb_{0.7})_{2}Te_{3}$ ternary topological insulators using indium doping

This study investigates the influence of indium doping on the defect states in (Bi0.3Sb0.7)2Te3 (BST) ternary topological insulators. Thin (10 nm) and thick (60 nm) films of pristine BST and indium-doped BST (In0.14(Bi0.3Sb0.7)1.86Te3) were synthesized using pulsed laser deposition. The electronic properties were characterized through low-frequency noise spectroscopy and temperature-dependent resistance (R-T) measurements. For the 10 nm films, R-T analysis revealed that indium doping shifts the thermal activation energy by approximately 100 meV. This doping also suppresses a shallow impurity band at 72 meV, a finding corroborated by 1/f noise measurements. In the 60 nm films, noise spectroscopy was used to probe deep defect states, where indium doping was found to increase the activation energy from 292.3 meV to 392 meV -- a consistent shift of 100 meV. These findings demonstrate that indium doping is an effective method for systematically modifying both shallow and deep defect states, enhancing the insulating properties and offering a mechanism to engineer the electronic behavior of topological insulators for advanced electronic applications where noise reduction is crucial.

cond-mat.mtrl-sci

Tensor Factorized Hamiltonian Downfolding To Optimize The Scaling Complexity Of The Electronic Correlations Problem on Classical and Quantum Computers

Achieving chemical accuracy for strongly correlated molecules is a defining milestone for first-generation, fault-tolerant quantum computers, yet the factorial growth of three, four, and six-index tensor contractions in coupled-cluster CCSD(T), full configuration interaction (FCI), and multireference CI (MRCI) makes current classical and quantum approaches prohibitive. We introduce tensor-factorized Hamiltonian downfolding (TFHD) and its quantum analogue, qubitized downfolding (QD)- a hybrid classical-quantum framework that collapses every high-rank object to rank-2 networks executed in depth-optimal, block-encoded circuits. The complexity of these operations scales exponentially with the system size. We aim to find properties of chemical systems by optimizing this scaling through mathematical transformations on the Hamiltonian and the state space. By defining a bi-partition of the many-body Hilbert space into electronoccupied and electron-unoccupied blocks for a given orbital, we perform a downfolding transformation that decouples the electron-occupied block from its complement. We factorize high-rank electronic integrals and cluster amplitude tensors into low-rank tensor factors of a downfolding transformation, mapping the full many-body Hamiltonian into a smaller dimensional block-Hamiltonians. This reduces the computational complexity of solving the residual equations for Hamiltonian downfolding from O(N7) for CCSD(T) and O(N9) - O(N10) for CI and MRCI to O(N3). This operations can be implemented as a family of tensor networks solely made from two-rank tensors. Additionally, we create block-encoding quantum circuits of the tensor networks, generating circuits of O(N2) depth with O(logN) qubits. We demonstrate super-quadratic speedups of expensive quantum chemistry algorithms on both classical and quantum computers.

quant-ph