arXiv subjects

Robert H. Hadfield

Publications and source records attributed to Robert H. Hadfield.

At least 19 recordsLinked to original sources

arXiv2026

Reaching the intrinsic performance limits of superconducting nanowire single-photon detectors up to 0.1 mm wide

Superconducting nanowire single-photon detectors (SNSPDs) combine high detection efficiency, low noise, and excellent timing resolution, making them a leading platform for photon-counting applications. However, despite decades of materials and fabrication research, detector performance has never been shown to match theoretical performance expectations. Here, we demonstrate for the first time in situ tuning of a detector from its typical, suboptimal operation, to a regime limited only by material quality, allowing the device to reach its intrinsic performance limit. Our approach is based on current-biased superconducting "rails" placed on either side of the detector that redistribute current across its width to achieve its peak performance. This technique reduces the dark count rate by ten orders of magnitude. Further, we show operation at this intrinsic performance limit for devices up to 0.1 mm wide, and also demonstrate near-unity internal detection efficiency (IDE) at a wavelength of 4um for a 20um-wide detector--a factor of 20 wider than the current state of the art. This work enables future detectors to overcome the Pearl limit for device width, paving the way for arbitrarily large detectors.

cond-mat.supr-con↗

arXiv2026

Tungsten Germanide Superconducting Nanowire Single-Photon Detectors with Saturated Internal Detection Efficiency at Wavelengths up to 29 μm

Superconducting nanowire single-photon detectors (SNSPDs) are among the most sensitive single-photon detectors available and have the potential to transform fields ranging from infrared astrophysics to molecular spectroscopy. However, extending their performance into the mid-infrared spectral region - crucial for applications such as exoplanet transit spectroscopy and vibrational fingerprinting of molecules - has remained a major challenge, primarily due to material limitations and scalability constraints. Here, we report on the development of SNSPDs based on tungsten germanide, a novel material system that combines high mid-infrared sensitivity with compatibility for large-scale fabrication. Our detectors exhibit saturated internal detection efficiency at wavelengths up to 29 μm, while using 2.7x thicker films (8 nm vs 3 nm) and up to 4.5x wider nanowires (360 nm vs 80 nm) compared to mid-infrared-optimized SNSPDs fabricated from tungsten silicide. This advance will enable scalable, high-performance single-photon detection in a spectral region that was previously inaccessible, opening new frontiers in remote sensing, thermal imaging, environmental monitoring, molecular physics, and astronomy.

physics.ins-det↗

arXiv2026

Review of germanium-silicon single-photon avalanche diodes

While it took about a decade for a germanium (Ge) thin film grown on a silicon (Si) substrate to be successfully applied as a detector material for high-speed optical fiber communication application, it took about another decade to further expand its usage as a sensor material for active optical sensing and imaging applications. In this paper, we shall review the progress of a shortwave infrared (SWIR) single-photon detection (SPD) with germanium-silicon (GeSi) single-photon avalanche diode (SPAD), ranging from the first demonstration at cryogenic temperature (Z. Lu et al., 2011) to the recent demonstration at room temperature (N. Na et al, 2024). Potential new applications will also be discussed.

physics.ins-det↗

arXiv2025

Quasiparticle Dynamics in NbN Superconducting Microwave Resonators at Single Photon Regime

Exchanging energy below the superconducting gap introduces quasiparticle energy distributions in superconducting quantum circuits, which will be responsible for their decoherence. This study examines the impact of quasiparticle energy on the performance of NbN superconducting microwave coplanar waveguide resonators on silicon chips. We measured the resonance frequency and internal quality factor in response to temperature sweeps to evaluate the effect of quasiparticle dynamics. Moreover, by calculating the complex conductivity of the NbN film, we identified the contribution of quasiparticle density to the experimental results.

quant-ph↗

arXiv2024

Engineering high-Q superconducting tantalum microwave coplanar waveguide resonators for compact coherent quantum circuits

Tantalum (Ta) has recently received considerable attention in manufacturing robust superconducting quantum circuits. Ta offers low microwave loss, high kinetic inductance compared to aluminium (Al) and niobium (Nb), and good compatibility with complementary metal-oxide-semiconductor (CMOS) technology, which is essential for quantum computing applications. Here, we demonstrate the fabrication engineering of thickness-dependent high quality factor (high-Q_i) Ta superconducting microwave coplanar waveguide resonators. All films are deposited on high-resistivity silicon substrates at room temperature without additional substrate heating. Before Ta deposition, a niobium (Nb) seed layer is used to ensure a body-centred cubic lattice (α-Ta) formation. We further engineer the kinetic inductance (L_K) resonators by varying Ta film thicknesses. High L_K is a key advantage for applications because it facilitates the realisation of high-impedance, compact quantum circuits with enhanced coupling to qubits. The maximum internal quality factor Q_i of ~ 3.6 * 10^6 is achieved at the high power regime for 100 nm Ta, while the highest kinetic inductance is obtained to be 0.6 pH/sq for the thinnest film, which is 40 nm. This combination of high Q_i and high L_K highlights the potential of Ta microwave circuits for high-fidelity operations of compact quantum circuits.

quant-ph↗

arXiv2024

Mid-infrared characterization of NbTiN superconducting nanowire single-photon detectors on silicon-on-insulator

Superconducting nanowire single-photon detectors are widely used for detecting individual photons across various wavelengths from ultraviolet to near-infrared range. Recently, there has been increasing interest in enhancing their sensitivity to single photons in the mid-infrared spectrum, driven by applications in quantum communication, spectroscopy and astrophysics. Here, we present our efforts to expand the spectral detection capabilities of U-shaped NbTiN-based superconducting nanowire single-photon detectors, fabricated in a 2-wire configuration on a silicon-on-insulator substrate, into the mid-infrared range. We demonstrate saturated internal detection efficiency extending up to a wavelength of 3.5 μm for a 5 nm thick and 50 nm wide NbTiN nanowire with a dark count rate less than 10 counts per second at 0.9 K and a rapid recovery time of 4.3 ns. The detectors are engineered for integration on waveguides in a silicon-on-insulator platform for compact, multi-channel device applications.

quant-ph↗

arXiv2023

Characterizing Niobium Nitride Superconducting Microwave Coplanar Waveguide Resonator Array for Circuit Quantum Electrodynamics in Extreme Conditions

The high critical magnetic field and relatively high critical temperature of niobium nitride (NbN) make it a promising material candidate for applications in superconducting quantum technology. However, NbN-based devices and circuits are sensitive to decoherence sources such as two-level system (TLS) defects. Here, we numerically and experimentally investigate NbN superconducting microwave coplanar waveguide resonator arrays, with a 100 nm thickness, capacitively coupled to a common coplanar waveguide on a silicon chip. We observe that the resonators' internal quality factor (Qi) decreases from Qi ~ 1.07*10^6 in a high power regime (< nph > = 27000) to Qi ~ 1.36 *10^5 in single photon regime at temperature T = 100 mK. Data from this study is consistent with the TLS theory, which describes the TLS interactions in resonator substrates and interfaces. Moreover, we study the temperature dependence internal quality factor and frequency tuning of the coplanar waveguide resonators to characterise the quasiparticle density of NbN. We observe that the increase in kinetic inductance at higher temperatures is the main reason for the frequency shift. Finally, we measure the resonators' resonance frequency and internal quality factor at single photon regime in response to in-plane magnetic fields B||. We verify that Qi stays well above 10^4 up to B|| = 240 mT in the photon number < nph > = 1.8 at T = 100 mK. Our results may pave the way for realising robust microwave superconducting circuits for circuit quantum electrodynamics (cQED) at high magnetic fields necessary for fault-tolerant quantum computing, and ultrasensitive quantum sensing.

quant-ph↗

arXiv2022

Two-dimensional cuprate nanodetector with single photon sensitivity at T = 20 K

Detecting light at the single-photon level is one of the pillars of emergent photonic technologies. This is realized through state-of-the-art superconducting detectors that offer efficient, broadband and fast response. However, the use of superconducting thin films with low TC limits their operation temperature below 4K. In this work, we demonstrate proof-of-concept nanodetectors based on exfoliated, two-dimensional cuprate superconductor Bi2Sr2CaCu2O8-δ (BSCCO) that exhibit single-photon sensitivity at telecom wavelength at a record temperature of T = 20K. These non-optimized devices exhibit a slow (ms) reset time and a low detection efficiency (10^(-4)). We realize the elusive prospect of single-photon sensitivity on a high-TC nanodetector thanks to a novel approach, combining van der Waals fabrication techniques and a non-invasive nanopatterning based on light ion irradiation. This result paves the way for broader application of single-photon technologies, relaxing the cryogenic constraints for single-photon detection at telecom wavelength.

cond-mat.supr-con↗

arXiv2022

Materials and devices for fundamental quantum science and quantum technologies

Technologies operating on the basis of quantum mechanical laws and resources such as phase coherence and entanglement are expected to revolutionize our future. Quantum technologies are often divided into four main pillars: computing, simulation, communication, and sensing & metrology. Moreover, a great deal of interest is currently also nucleating around energy-related quantum technologies. In this Perspective, we focus on advanced superconducting materials, van der Waals materials, and moiré quantum matter, summarizing recent exciting developments and highlighting a wealth of potential applications, ranging from high-energy experimental and theoretical physics to quantum materials science and energy storage.

quant-ph↗

arXiv2021

Near-maximal two-photon entanglement for quantum communications at 2.1 $μ$m

Owing to a reduced solar background and low propagation losses in the atmosphere, the 2- to 2.5-$μ$m waveband is a promising candidate for daylight quantum communication. This spectral region also offers low losses and low dispersion in hollow-core fibers and in silicon waveguides. We demonstrate for the first time near-maximally entangled photon pairs at 2.1 $μ$m that could support device independent quantum key distribution (DIQKD) assuming sufficiently high channel efficiencies. The state corresponds to a positive secure-key rate (0.254 bits/pair, with a quantum bit error rate of 3.8%) based on measurements in a laboratory setting with minimal channel loss and transmission distance. This is promising for the future implementation of DIQKD at 2.1 $μ$m.

quant-ph↗

arXiv2021

Strong magnon-photon coupling with chip-integrated YIG in the zero-temperature limit

The cross-integration of spin-wave and superconducting technologies is a promising method for creating novel hybrid devices for future information processing technologies to store, manipulate, or convert data in both classical and quantum regimes. Hybrid magnon-polariton systems have been widely studied using bulk Yttrium Iron Garnet (Y$_{3}$Fe$_{5}$O$_{12}$, YIG) and three-dimensional microwave photon cavities. However, limitations in YIG growth have thus far prevented its incorporation into CMOS compatible technology such as high quality factor superconducting quantum technology. To overcome this impediment, we have used Plasma Focused Ion Beam (PFIB) technology -- taking advantage of precision placement down to the micron-scale -- to integrate YIG with superconducting microwave devices. Ferromagnetic resonance has been measured at millikelvin temperatures on PFIB-processed YIG samples using planar microwave circuits. Furthermore, we demonstrate strong coupling between superconducting resonator and YIG ferromagnetic resonance modes by maintaining reasonably low loss while reducing the system down to the micron scale. This achievement of strong coupling on-chip is a crucial step toward fabrication of functional hybrid quantum devices that advantage from spin-wave and superconducting components.

cond-mat.mes-hall↗

arXiv2020

Two-photon Quantum Interference and Entanglement at 2 μm

Quantum-enhanced optical systems operating within the 2- to 2.5-$μ$m spectral region have the potential to revolutionize emerging applications in communications, sensing, and metrology. However, to date, sources of entangled photons have been realized mainly in the near-infrared 700- to 1550-nm spectral window. Here, using custom-designed lithium niobate crystals for spontaneous parametric down-conversion and tailored superconducting nanowire single-photon detectors, we demonstrate two-photon interference and polarization-entangled photon pairs at 2090 nm. These results open the 2- to 2.5-$μ$m mid-infrared window for the development of optical quantum technologies such as quantum key distribution in next-generation mid-infrared fiber communication systems and future Earth-to-satellite communications.

quant-ph↗

arXiv2019

Niobium diselenide superconducting photodetectors

We report the photoresponse of niobium diselenide (NbSe$_2$), a transition metal dichalcogenide (TMD) which exhibits superconducting properties down to a single layer. Devices are built by using micro-mechanically cleaved 2 to 10 layers and tested under current bias using nano-optical mapping in the 350mK-5K range, where they are found to be superconducting. The superconducting state can be broken by absorption of light, resulting in a voltage signal when the devices are current biased. The response found to be energy dependent making the devices useful for applications requiring energy resolution, such as bolometry, spectroscopy and infrared imaging.

cond-mat.supr-con↗

arXiv2018

Space QUEST mission proposal: Experimentally testing decoherence due to gravity

Models of quantum systems on curved space-times lack sufficient experimental verification. Some speculative theories suggest that quantum properties, such as entanglement, may exhibit entirely different behavior to purely classical systems. By measuring this effect or lack thereof, we can test the hypotheses behind several such models. For instance, as predicted by Ralph and coworkers [T C Ralph, G J Milburn, and T Downes, Phys. Rev. A, 79(2):22121, 2009, T C Ralph and J Pienaar, New Journal of Physics, 16(8):85008, 2014], a bipartite entangled system could decohere if each particle traversed through a different gravitational field gradient. We propose to study this effect in a ground to space uplink scenario. We extend the above theoretical predictions of Ralph and coworkers and discuss the scientific consequences of detecting/failing to detect the predicted gravitational decoherence. We present a detailed mission design of the European Space Agency's (ESA) Space QUEST (Space - Quantum Entanglement Space Test) mission, and study the feasibility of the mission schema.

quant-ph↗

arXiv2015

Quantum Photonic Interconnect

Integrated photonics has enabled much progress towards quantum technologies. Many applications, including quantum communication, sensing, and distributed and cloud quantum computing, will require coherent photonic interconnection between separate chip-based sub-systems. Large-scale quantum computing systems and architectures may ultimately require quantum interconnects to enable scaling beyond the limits of a single wafer and towards "multi-chip" systems. However, coherently interconnecting separate chips is challenging due to the fragility of these quantum states and the demanding challenges of transmitting photons in at least two media within a single coherent system. Distribution and manipulation of qubit entanglement between multiple devices is one of the most stringent requirements of the interconnected system. Here, we report a quantum photonic interconnect demonstrating high-fidelity entanglement distribution and manipulation between two separate chips, implemented using state-of-the-art silicon photonics. Path-entangled states are generated and manipulated on-chip, and distributed between the chips by interconverting between path-encoding and polarisation-encoding. We use integrated state analysers to confirm a Bell-type violation of $S$=2.638+-0.039 between two chips. With improvements in loss, this quantum interconnect will provide new levels of flexible systems and architectures for quantum technologies.

quant-ph↗

arXiv2015

Chip-based Quantum Key Distribution

Improvement in secure transmission of information is an urgent practical need for governments, corporations and individuals. Quantum key distribution (QKD) promises security based on the laws of physics and has rapidly grown from proof-of-concept to robust demonstrations and even deployment of commercial systems. Despite these advances, QKD has not been widely adopted, and practical large-scale deployment will likely require integrated chip-based devices for improved performance, miniaturisation and enhanced functionality, fully integrated into classical communication networks. Here we report low error rate, GHz clocked QKD operation of an InP transmitter chip and a SiO$_x$N$_y$ receiver chip --- monolithically integrated devices that use state-of-the-art components and manufacturing processes from the telecom industry. We use the reconfigurability of these devices to demonstrate three important QKD protocols --- BB84, Coherent One Way (COW) and Differential Phase Shift (DPS) --- with performance comparable to state-of-the-art. These devices, when combined with integrated single photon detectors, satisfy the requirements at each of the levels of future QKD networks --- from point-of-use through to backbone --- and open the way to operation in existing and emerging classical communication networks.

quant-ph↗

arXiv2015

Nanoantenna enhancement for telecom-wavelength superconducting single photon detectors

Superconducting nanowire single photon detectors are rapidly emerging as a key infrared photon-counting technology. Two front-side-coupled silver dipole nanoantennas, simulated to have resonances at 1480 nm and 1525 nm, were fabricated in a two-step process. An enhancement of 50% to 130% in the system detection efficiency was observed when illuminating the antennas. This offers a pathway to increasing absorption into superconducting nanowires, creating larger active areas, and achieving more efficient detection at longer wavelengths.

physics.optics↗

arXiv2014

On-chip quantum interference between silicon photon-pair sources

Large-scale integrated quantum photonic technologies will require the on-chip integration of identical photon sources with reconfigurable waveguide circuits. Relatively complex quantum circuits have already been demonstrated, but few studies acknowledge the pressing need to integrate photon sources and waveguide circuits together on-chip. A key step towards such large-scale quantum technologies is the integration of just two individual photon sources within a waveguide circuit, and the demonstration of high-visibility quantum interference between them. Here, we report a silicon-on-insulator device combining two four-wave mixing sources, in an interferometer with a reconfigurable phase shifter. We configure the device to create and manipulate two-colour (non-degenerate) or same-colour (degenerate), path-entangled or path-unentangled photon pairs. We observe up to 100.0+/-0.4% visibility quantum interference on-chip, and up to 95+/-4% off-chip. Our device removes the need for external photon sources, provides a path to increasing the complexity of quantum photonic circuits, and is a first step towards fully-integrated quantum technologies.

quant-ph↗