arXiv subjects

Robert J. Schoelkopf

Publications and source records attributed to Robert J. Schoelkopf.

At least 37 records · Page 2Linked to original sources

arXiv2023

Surpassing millisecond coherence times in on-chip superconducting quantum memories by optimizing materials, processes, and circuit design

The performance of superconducting quantum circuits for quantum computing has advanced tremendously in recent decades; however, a comprehensive understanding of relaxation mechanisms does not yet exist. In this work, we utilize a multimode approach to characterizing energy losses in superconducting quantum circuits, with the goals of predicting device performance and improving coherence through materials, process, and circuit design optimization. Using this approach, we measure significant reductions in surface and bulk dielectric losses by employing a tantalum-based materials platform and annealed sapphire substrates. With this knowledge we predict and experimentally verify the relaxation times of aluminum- and tantalum-based transmon qubits. We additionally optimize device geometry to maximize coherence within a coaxial tunnel architecture, and realize on-chip quantum memories with single-photon Ramsey times of 2.0$-$2.7 ms, limited by their energy relaxation times of 1.0$-$1.4 ms. To our knowledge this is the highest coherence achieved in an on-chip quantum memory, and demonstrates an advancement towards a more modular and compact coaxial circuit architecture for bosonic qubits with reproducibly high coherence.

quant-ph↗

arXiv2023

Microwave loss characterization using multi-mode superconducting resonators

Measuring the losses arising from different materials and interfaces is crucial to improving the coherence of superconducting quantum circuits. Although this has been of interest for a long time, current studies can either only provide bounds to those losses, or require several devices for a complete characterization. In this work, we introduce a method to measure the microwave losses of materials and interfaces with a single multi-mode superconducting resonator. We demonstrate a formalism for analyzing the loss sensitivity of multi-mode systems and discuss the design strategies of multi-mode resonators for material loss studies. We present two types of multi-mode superconducting resonators for the study of bulk superconductors: the forky whispering-gallery-mode resonator (FWGMR) and the ellipsoidal cavity. We use these resonators to measure the surface dielectric, conductor, and seam losses of high-purity (5N5) aluminum and aluminum alloy (6061), as well as how they are affected by chemical etching, diamond turning, and thin-film coating. We find that chemical etching and diamond turning reduce both the surface dielectric and conductive losses of high-purity aluminum, but provide no appreciable improvement to the seam. Coating the surfaces of diamond-turned aluminum alloys with e-beam evaporated or sputtered aluminum thin-films significantly reduces all three losses under study. In addition, we study the effect of chemical etching on the surface of high-purity aluminum using transmission electron microscopy (TEM) and find that the chemical etching process creates a thinner and more uniform oxide layer, consistent with the observed improvement in the surface dielectric loss.

quant-ph↗

arXiv2023

Precision measurement of the microwave dielectric loss of sapphire in the quantum regime with parts-per-billion sensitivity

Dielectric loss is known to limit state-of-the-art superconducting qubit lifetimes. Recent experiments imply upper bounds on bulk dielectric loss tangents on the order of $100$ parts-per-billion, but because these inferences are drawn from fully fabricated devices with many loss channels, they do not definitively implicate or exonerate the dielectric. To resolve this ambiguity, we have devised a measurement method capable of separating and resolving bulk dielectric loss with a sensitivity at the level of $5$ parts per billion. The method, which we call the dielectric dipper, involves the in-situ insertion of a dielectric sample into a high-quality microwave cavity mode. Smoothly varying the sample's participation in the cavity mode enables a differential measurement of the sample's dielectric loss tangent. The dielectric dipper can probe the low-power behavior of dielectrics at cryogenic temperatures, and does so without the need for any lithographic process, enabling controlled comparisons of substrate materials and processing techniques. We demonstrate the method with measurements of EFG sapphire, from which we infer a bulk loss tangent of $62(7) \times 10^{-9}$ and a substrate-air interface loss tangent of $12(2) \times 10^{-4}$. For a typical transmon, this bulk loss tangent would limit device quality factors to less than $20$ million, suggesting that bulk loss is likely the dominant loss mechanism in the longest-lived transmons on sapphire. We also demonstrate this method on HEMEX sapphire and bound its bulk loss tangent to be less than $15(5) \times 10^{-9}$. As this bound is about 3 times smaller than the bulk loss tangent of EFG sapphire, use of HEMEX sapphire as a substrate would lift the bulk dielectric coherence limit of a typical transmon qubit to several milliseconds.

quant-ph↗

arXiv2022

Error-detectable bosonic entangling gates with a noisy ancilla

Bosonic quantum error correction has proven to be a successful approach for extending the coherence of quantum memories, but to execute deep quantum circuits, high-fidelity gates between encoded qubits are needed. To that end, we present a family of error-detectable two-qubit gates for a variety of bosonic encodings. From a new geometric framework based on a "Bloch sphere" of bosonic operators, we construct $ZZ_L(θ)$ and $\text{eSWAP}(θ)$ gates for the binomial, 4-legged cat, dual-rail and several other bosonic codes. The gate Hamiltonian is simple to engineer, requiring only a programmable beamsplitter between two bosonic qubits and an ancilla dispersively coupled to one qubit. This Hamiltonian can be realized in circuit QED hardware with ancilla transmons and microwave cavities. The proposed theoretical framework was developed for circuit QED but is generalizable to any platform that can effectively generate this Hamiltonian. Crucially, one can also detect first-order errors in the ancilla and the bosonic qubits during the gates. We show that this allows one to reach error-detected gate fidelities at the $10^{-4}$ level with today's hardware, limited only by second-order hardware errors.

quant-ph↗

arXiv2022

Architectures for Multinode Superconducting Quantum Computers

Many proposals to scale quantum technology rely on modular or distributed designs where individual quantum processors, called nodes, are linked together to form one large multinode quantum computer (MNQC). One scalable method to construct an MNQC is using superconducting quantum systems with optical interconnects. However, a limiting factor of these machines will be internode gates, which may be two to three orders of magnitude noisier and slower than local operations. Surmounting the limitations of internode gates will require a range of techniques, including improvements in entanglement generation, the use of entanglement distillation, and optimized software and compilers, and it remains unclear how improvements to these components interact to affect overall system performance, what performance from each is required, or even how to quantify the performance of each. In this paper, we employ a `co-design' inspired approach to quantify overall MNQC performance in terms of hardware models of internode links, entanglement distillation, and local architecture. In the case of superconducting MNQCs with microwave-to-optical links, we uncover a tradeoff between entanglement generation and distillation that threatens to degrade performance. We show how to navigate this tradeoff, lay out how compilers should optimize between local and internode gates, and discuss when noisy quantum links have an advantage over purely classical links. Using these results, we introduce a roadmap for the realization of early MNQCs which illustrates potential improvements to the hardware and software of MNQCs and outlines criteria for evaluating the landscape, from progress in entanglement generation and quantum memory to dedicated algorithms such as distributed quantum phase estimation. While we focus on superconducting devices with optical interconnects, our approach is general across MNQC implementations.

quant-ph↗

arXiv2022

Acoustic radiation from a superconducting qubit: From spontaneous emission to Rabi oscillations

Acoustic spontaneous emission into bulk dielectrics can be a strong source of decoherence in quantum devices, especially when a qubit is in the presence of piezoelectric materials. We study the dynamics of a qubit coupled to an acoustic resonator by a piezoelectric film. By varying the surface topography of the resonator from rough to polished to shaped, we explore the crossover from fast decay of an excited qubit to quantum-coherent coupling between the qubit and an isolated phonon mode. Our experimental approach may be used for precision measurements of crystalline vibrations, the design of quantum memories, and the study of electro-mechanical contributions to dielectric loss.

quant-ph↗

arXiv2022

The squeezed Kerr oscillator: spectral kissing and phase-flip robustness

By applying a microwave drive to a specially designed Josephson circuit, we have realized an elementary quantum optics model, the squeezed Kerr oscillator. This model displays, as the squeezing amplitude is increased, a cross-over from a single ground state regime to a doubly-degenerate ground state regime. In the latter case, the ground state manifold is spanned by Schrödinger-cat states, i.e. quantum superpositions of coherent states with opposite phases. For the first time, having resolved up to the tenth excited state in a spectroscopic experiment, we confirm that the proposed emergent static effective Hamiltonian correctly describes the system, despite its driven character. We also find that the lifetime of the coherent state components of the cat states increases in steps as a function of the squeezing amplitude. We interpret the staircase pattern as resulting from pairwise level kissing in the excited state spectrum. Considering the Kerr-cat qubit encoded in this ground state manifold, we achieve for the first time quantum nondemolition readout fidelities greater than 99%, and enhancement of the phase-flip lifetime by more than two orders of magnitude, while retaining universal quantum control. Our experiment illustrates the crucial role of parametric drive Hamiltonian engineering for hardware-efficient quantum computation.

quant-ph↗

arXiv2022

Fast Universal Control of an Oscillator with Weak Dispersive Coupling to a Qubit

A controlled evolution generated by nonlinear interactions is required to perform full manipulation of a quantum system, and such control is only coherent when the rate of nonlinearity is large compared to the rate of decoherence. As a result, engineered quantum systems typically rely on a bare nonlinearity much stronger than all decoherence rates, and this hierarchy is usually assumed to be necessary. In this work, we challenge this assumption by demonstrating the universal control of a quantum system where the relevant rate of bare nonlinear interaction is comparable to the fastest rate of decoherence. We do this by introducing a novel noise-resilient protocol for the universal quantum control of a nearly-harmonic oscillator that takes advantage of an in-situ enhanced nonlinearity instead of harnessing a bare nonlinearity. Our experiment consists of a high quality-factor microwave cavity with weak-dispersive coupling to a much lower quality superconducting qubit. By using strong drives to temporarily excite the oscillator, we realize an amplified three-wave-mixing interaction, achieving typical operation speeds over an order of magnitude faster than expected from the bare dispersive coupling. Our demonstrations include preparation of a single-photon state with $98\pm 1(\%)$ fidelity and preparation of squeezed vacuum with a squeezing level of $11.1$ dB, the largest intracavity squeezing reported in the microwave regime. Finally, we also demonstrate fast measurement-free preparation of logical states for the binomial and Gottesman-Kitaev-Preskill (GKP) quantum error-correcting codes.

quant-ph↗

arXiv2022

Observation of wave-packet branching through an engineered conical intersection

In chemical reactions, the interplay between coherent evolution and dissipation is central to determining key properties such as the rate and yield. Of particular interest are cases where two potential energy surfaces cross at features known as conical intersections (CIs), resulting in nonadiabatic dynamics that may promote ultrafast and highly efficient reactions when rovibrational damping is present. A prominent chemical reaction that involves a CI is the cis-trans isomerization reaction in rhodopsin, which is crucial to vision. CIs in real molecular systems are typically investigated via optical pump-probe spectroscopy, which has demanding spectral bandwidth and temporal resolution requirements, and where precise control of the environment is challenging. A complementary approach for understanding chemical reactions is to use quantum simulators that can provide access to a wider range of observables, though thus far combining strongly interacting linear (rovibrational) and nonlinear (electronic) degrees of freedom with engineered dissipation has yet to be demonstrated. Here, we create a tunable CI in a hybrid qubit-oscillator circuit QED processor and simultaneously track both a reactive wave-packet and electronic qubit in the time-domain. We identify dephasing of the electronic qubit as the mechanism that drives wave-packet branching along the reactive coordinate in our model. Furthermore, we directly observe enhanced branching when the wave-packet passes through the CI. Thus, the forces that influence a chemical reaction can be viewed as an effective measurement induced dephasing rate that depends on the position of the wave-packet relative to the CI. Our results set the groundwork for more complex simulations of chemical dynamics, offering deeper insight into the role of dissipation in determining macroscopic quantities of interest such as the quantum yield of a chemical reaction.

quant-ph↗

arXiv2021

Quantum control of bosonic modes with superconducting circuits

Bosonic modes have wide applications in various quantum technologies, such as optical photons for quantum communication, magnons in spin ensembles for quantum information storage and mechanical modes for reversible microwave-to-optical quantum transduction. There is emerging interest in utilizing bosonic modes for quantum information processing, with circuit quantum electrodynamics (circuit QED) as one of the leading architectures. Quantum information can be encoded into subspaces of a bosonic superconducting cavity mode with long coherence time. However, standard Gaussian operations (e.g., beam splitting and two-mode squeezing) are insufficient for universal quantum computing. The major challenge is to introduce additional nonlinear control beyond Gaussian operations without adding significant bosonic loss or decoherence. Here we review recent advances in universal control of a single bosonic code with superconducting circuits, including unitary control, quantum feedback control, driven-dissipative control and holonomic dissipative control. Various approaches to entangling different bosonic modes are also discussed.

quant-ph↗

arXiv2021

Single-shot number-resolved detection of microwave photons with error mitigation

Single-photon detectors are ubiquitous and integral components of photonic quantum cryptography, communication, and computation. Many applications, however, require not only detecting the presence of any photons, but distinguishing the number present with a single shot. Here, we implement a single-shot, high-fidelity photon number-resolving detector of up to 15 microwave photons in a cavity-qubit circuit QED platform. This detector functions by measuring a series of generalized parity operators which make up the bits in the binary decomposition of the photon number. Our protocol consists of successive, independent measurements of each bit by entangling the ancilla with the cavity, then reading out and resetting the ancilla. Photon loss and ancilla readout errors can flip one or more bits, causing nontrivial errors in the outcome, but these errors have a traceable form which can be captured in a simple hidden Markov model. Relying on the independence of each bit measurement, we mitigate biases in ensembles of measurements, showing good agreement with the predictions of the model. The mitigation improves the average total variation distance error of Fock states from $13.5\%$ to $1.1\%$. We also show that the mitigation is efficiently scalable to an $M$-mode system provided that the errors are independent and sufficiently small. Our work motivates the development of new algorithms that utilize single-shot, high-fidelity PNR detectors.

quant-ph↗

arXiv2020

Path-Independent Quantum Gates with Noisy Ancilla

Ancilla systems are often indispensable to universal control of a nearly isolated quantum system. However, ancilla systems are typically more vulnerable to environmental noise, which limits the performance of such ancilla-assisted quantum control. To address this challenge of ancilla-induced decoherence, we propose a general framework that integrates quantum control and quantum error correction, so that we can achieve robust quantum gates resilient to ancilla noise. We introduce the path independence criterion for fault-tolerant quantum gates against ancilla errors. As an example, a path-independent gate is provided for superconducting circuits with a hardware-efficient design.

quant-ph↗

arXiv2020

High coherence superconducting microwave cavities with indium bump bonding

Low-loss cavities are important in building high-coherence superconducting quantum computers. Generating high quality joints between parts is crucial to the realization of a scalable quantum computer using the circuit quantum electrodynamics (cQED) framework. In this paper, we adapt the technique of indium bump bonding to the cQED architecture to realize high quality superconducting microwave joints between chips. We use this technique to fabricate compact superconducting cavities in the multilayer microwave integrated quantum circuits (MMIQC) architecture and achieve single photon quality factor over 300 million or single-photon lifetimes approaching 5 ms. To quantify the performance of the resulting seam, we fabricate microwave stripline resonators in multiple sections connected by different numbers of bonds, resulting in a wide range of seam admittances. The measured quality factors combined with the designed seam admittances allow us to bound the conductance of the seam at $g_\text{seam} \ge 2\times 10^{10} /(Ω\text{m})$. Such a conductance should enable construction of micromachined superconducting cavities with quality factor of at least a billion. These results demonstrate the capability to construct very high quality microwave structures within the MMIQC architecture.

physics.app-ph↗

arXiv2020

Hardware-efficient quantum random access memory with hybrid quantum acoustic systems

Hybrid quantum systems in which acoustic resonators couple to superconducting qubits are promising quantum information platforms. High quality factors and small mode volumes make acoustic modes ideal quantum memories, while the qubit-phonon coupling enables the initialization and manipulation of quantum states. We present a scheme for quantum computing with multimode quantum acoustic systems, and based on this scheme, propose a hardware-efficient implementation of a quantum random access memory (QRAM). Quantum information is stored in high-Q phonon modes, and couplings between modes are engineered by applying off-resonant drives to a transmon qubit. In comparison to existing proposals that involve directly exciting the qubit, this scheme can offer a substantial improvement in gate fidelity for long-lived acoustic modes. We show how these engineered phonon-phonon couplings can be used to access data in superposition according to the state of designated address modes--implementing a QRAM on a single chip.

quant-ph↗

arXiv2019

Efficient multiphoton sampling of molecular vibronic spectra on a superconducting bosonic processor

The efficient simulation of quantum systems is a primary motivating factor for developing controllable quantum machines. For addressing systems with underlying bosonic structure, it is advantageous to utilize a naturally bosonic platform. Optical photons passing through linear networks may be configured to perform quantum simulation tasks, but the efficient preparation and detection of multiphoton quantum states of light in linear optical systems are challenging. Here, we experimentally implement a boson sampling protocol for simulating molecular vibronic spectra [Nature Photonics $\textbf{9}$, 615 (2015)] in a two-mode superconducting device. In addition to enacting the requisite set of Gaussian operations across both modes, we fulfill the scalability requirement by demonstrating, for the first time in any platform, a high-fidelity single-shot photon number resolving detection scheme capable of resolving up to 15 photons per mode. Furthermore, we exercise the capability of synthesizing non-Gaussian input states to simulate spectra of molecular ensembles in vibrational excited states. We show the re-programmability of our implementation by extracting the spectra of photoelectron processes in H$_2$O, O$_3$, NO$_2$, and SO$_2$. The capabilities highlighted in this work establish the superconducting architecture as a promising platform for bosonic simulations, and by combining them with tools such as Kerr interactions and engineered dissipation, enable the simulation of a wider class of bosonic systems.

quant-ph↗

arXiv2019

High-fidelity measurement of qubits encoded in multilevel superconducting circuits

Qubit measurements are central to quantum information processing. In the field of superconducting qubits, standard readout techniques are not only limited by the signal-to-noise ratio, but also by state relaxation during the measurement. In this work, we demonstrate that the limitation due to relaxation can be suppressed by using the many-level Hilbert space of superconducting circuits: in a multilevel encoding, the measurement is only corrupted when multiple errors occur. Employing this technique, we show that we can directly resolve transmon gate errors at the level of one part in $10^3.$ Extending this idea, we apply the same principles to the measurement of a logical qubit encoded in a bosonic mode and detected with a transmon ancilla, implementing a proposal by Hann et al. [Phys. Rev. A \textbf{98} 022305 (2018)]. Qubit state assignments are made based on a sequence of repeated readouts, further reducing the overall infidelity. This approach is quite general and several encodings are studied; the codewords are more distinguishable when the distance between them is increased with respect to photon loss. The tradeoff between multiple readouts and state relaxation is explored and shown to be consistent with the photon-loss model. We report a logical assignment infidelity of $5.8\times 10^{-5}$ for a Fock-based encoding and $4.2\times 10^{-3}$ for a QEC code (the $S=2,N=1$ binomial code). Our results will not only improve the fidelity of quantum information applications, but also enable more precise characterization of process or gate errors.

quant-ph↗

arXiv2019

Error-corrected gates on an encoded qubit

To solve classically hard problems, quantum computers need to be resilient to the influence of noise and decoherence. In such a fault-tolerant quantum computer, noise-induced errors must be detected and corrected in real-time to prevent them from propagating between components. This requirement is especially pertinent while applying quantum gates, when the interaction between components can cause errors to quickly spread throughout the system. However, the large overhead involved in most fault-tolerant architectures makes implementing these systems a daunting task, which motivates the search for hardware-efficient alternatives. Here, we present a gate enacted by a multilevel ancilla transmon on a cavity-encoded logical qubit that is fault-tolerant with respect to decoherence in both the ancilla and the encoded qubit. We maintain the purity of the encoded qubit in the presence of ancilla errors by detecting those errors in real-time, and applying the appropriate corrections. We show a reduction of the logical gate error by a factor of two in the presence of naturally occurring decoherence, and demonstrate resilience against ancilla bit-flips and phase-flips by observing a sixfold suppression of the gate error with increased energy relaxation, and a fourfold suppression with increased dephasing noise. The results demonstrate that bosonic logical qubits can be controlled by error-prone ancilla qubits without inheriting the ancilla's inferior performance. As such, error-corrected ancilla-enabled gates are an important step towards fully fault-tolerant processing of bosonic qubits.

quant-ph↗

arXiv2018

Creation and control of multi-phonon Fock states in a bulk acoustic wave resonator

Quantum states of mechanical motion can be important resources for quantum information, metrology, and studies of fundamental physics. Recent demonstrations of superconducting qubits coupled to acoustic resonators have opened up the possibility of performing quantum operations on macroscopic motional modes, which can act as long-lived quantum memories or transducers. In addition, they can potentially be used to test for novel decoherence mechanisms in macroscopic objects and other modifications to standard quantum theory. Many of these applications call for the ability to create and characterize complex quantum states, putting demanding requirements on the speed of quantum operations and the coherence of the mechanical mode. In this work, we demonstrate the controlled generation of multi-phonon Fock states in a macroscopic bulk-acoustic wave resonator. We also perform Wigner tomography and state reconstruction to highlight the quantum nature of the prepared states. These demonstrations are made possible by the long coherence times of our acoustic resonator and our ability to selectively couple to individual phonon modes. Our work shows that circuit quantum acousto-dynamics (circuit QAD) enables sophisticated quantum control of macroscopic mechanical objects and opens the door to using acoustic modes as novel quantum resources.

quant-ph↗