arXiv subjects

Robert Keil

Publications and source records attributed to Robert Keil.

At least 19 recordsLinked to original sources

arXiv2026

Franson-Interferometric Bounds on Entangled Two-Photon Absorption

Entangled photons offer quantum correlations with no classical analogue. In entangled pair two-photon absorption (ETPA), absorption rate is predicted to scale linearly rather than quadratically with photon flux, promising molecular excitation at fluxes far below the classical threshold. Reported ETPA cross sections nevertheless vary widely across experiments, largely since the observable, the differential of the transmitted flux or weak fluorescence, is difficult to separate from scattering and linear losses. We present a method which uses Franson interference to study entangled two-photon absorption through delay-dependent coincidence measurements on dye molecules. Applying the method to Rhodamine 6G, we observe a small asymmetry in the Franson interference envelope and obtain a model-derived effective cross section of approximately 2.1 E(-21) centimeter squared for Rhodamine 6G. However, the estimated systematic uncertainty does not allow a definitive ETPA assignment. Instead, the experiment establishes a quantitative bound on the ETPA response and provides a background-free benchmark for future measurements.

physics.chem-ph↗

arXiv2026

Photonic hyperentanglement in polarisation and frequency via joint spectrum shaping

Hyperentanglement offers enhanced capacity for quantum information processing and communication protocols, especially in combination with robust high-dimensional degrees of freedom such as frequency-bin encoding. Here, we present a single-pass, unfiltered, down-conversion source of hyperentangled photon pairs in polarisation and frequency-bin degrees of freedom with dynamically tunable state dimension and composition at telecom wavelengths. We achieve this by optimal tailoring of the photons' joint spectral amplitude via pump and nonlinearity shaping. Using polarisation-resolved time-of-flight spectrometry and Hong-Ou-Mandel interference, we characterise the hyperentangled states and demonstrate for the polarisation component fidelities exceeding 99% averaged over frequency bins and concurrences above 98%. The degree of spectral entanglement, quantified by the Hong-Ou-Mandel visibility, is measured as 90%, well in line with numerical simulations. This approach provides a scalable route toward high-dimensional quantum states for quantum communication and computing applications.

quant-ph↗

arXiv2025

Optimised spectral purity of unfiltered photons via pump and nonlinearity shaping

Photonic quantum technologies rely on the efficient generation and interference of indistinguishable photons. Exceptional achievements in this respect have been obtained by domain engineering of quasi-phase-matched parametric down-conversion sources, demonstrating high two-photon interference visibility using only moderate bandpass spectral filtering. Here, we optimised the spectral purity and indistinguishability of photons from telecom-wavelength sources by combining Gaussian quasi-phase-matching with Gaussian pump spectral shaping. Without spectral filtering, we used time-of-flight spectrometry to estimate an upper bound spectral purity of 99.9272(6)%, and achieved visibilities of up to 98.5(8)% in two-photon interference experiments with independent sources.

quant-ph↗

arXiv2024

Nonlinear response of telecom-wavelength superconducting single-photon detectors

We measure the nonlinearity of a telecom-wavelength superconducting nanowire single-photon detector via incoherent beam combination. At typical photon count rates and detector bias current, the observed relative deviation from a perfectly linear response is in the order of 0.1% when the flux is doubled. This arises from a balance between the counteracting nonlinearities of deadtime-induced detector saturation and of multi-photon detections. The observed behaviour is modelled empirically, which suffices for a correction of measured data. In addition, statistical simulations, taking into account the measured recovery of the detection efficiency, provide insight into possible mechanisms of multi-photon detection.

quant-ph↗

arXiv2024

Photoneutralization of charges in GaAs quantum dot based entangled photon emitters

Semiconductor-based emitters of pairwise photonic entanglement are a promising constituent of photonic quantum technologies. They are known for the ability to generate discrete photonic states on-demand with low multiphoton emission, near-unity entanglement fidelity, and high single photon indistinguishability. However, quantum dots typically suffer from luminescence blinking, lowering the efficiency of the source and hampering their scalable application in quantum networks. In this paper, we investigate and adjust the intermittence of the neutral exciton emission in a GaAs/AlGaAs quantum dot under two-photon resonant excitation of the neutral biexciton. We investigate the spectral and quantum optical response of the quantum dot emission to an additional wavelength tunable gate laser, revealing blinking caused by the intrinsic Coulomb blockade due to charge capture processes. Our finding demonstrates that the emission quenching can be actively suppressed by controlling the balance of free electrons and holes in the vicinity of the quantum dot and thereby significantly increasing the quantum efficiency by 30%.

quant-ph↗

arXiv2023

Entanglement-induced collective many-body interference

Entanglement and interference are both hallmark effects of quantum physics. Particularly rich dynamics arise when multiple (at least partially) indistinguishable particles are subjected to either of these phenomena. By combining both entanglement and many-particle interference, we propose an interferometric setting through which N-particle interference can be observed, while any interference of lower orders is strictly suppressed. We experimentally demonstrate this effect in a four-photon interferometer, where the interference is nonlocal, in principle, as only pairs of photons interfere at two separate and independent beam splitters. A joint detection of all four photons identifies a high-visibility interference pattern varying as a function of their collective four-particle phase, a genuine four-body property.

quant-ph↗

arXiv2023

Surface quantum dots with pure, coherent, and blinking-free single photon emission

The surface of semiconductor nanostructures has a major impact on their electronic and optical properties. Disorder and defects in the surface layer typically cause degradation of charge carrier transport and radiative recombination dynamics. However, surface vicinity is inevitable for many scalable nano-optical applications. Epitaxially grown quantum dots are the best candidate for high-performance single photon emission and show great potential for quantum technologies. Yet, these emitters only reveal their excellent properties if they are deeply embedded in a semiconductor host. Until today, quantum dots close to surfaces yield weak, broad, and unstable emissions. Here, we show the complete restoration of optical properties from quantum dots grown directly on a semiconductor surface. The vanishing luminescence from the as-grown sample turns into bright, ultra-stable, coherent and blinking-free single photon emission after sulphur passivation. Under quasi-resonant excitation, single photons are generated with 98.8% purity, 77% indistinguishability, linewidths down to 4 $μ$eV and 99.69% persistency across 11 orders of magnitude in time. The emission is stable even after two years and when being subjected to nanomanufacturing processes. Some long-standing stumbling blocks for surface-dominated quantum dots are thereby removed, unveiling new possibilities for hybrid nano-devices and applications in quantum communication or sensing.

cond-mat.mes-hall↗

arXiv2022

Statistical limits for quantum networks with semiconductor entangled photon sources

Semiconductor quantum dots are promising building blocks for quantum communication applications. Although deterministic, efficient, and coherent emission of entangled photons has been realized, implementing a practical quantum repeater remains outstanding. Here we explore the statistical limits for entanglement swapping with sources of polarization-entangled photons from the commonly used biexciton-exciton cascade. We stress the necessity of tuning the exciton fine structure, and explain why the often observed time evolution of photonic entanglement in quantum dots is not applicable for large quantum networks. We identify the critical, statistically distributed device parameters for entanglement swapping based on two sources. A numerical model for benchmarking the consequences of device fabrication, dynamic tuning techniques, and statistical effects is developed, in order to bring the realization of semiconductor-based quantum networks one step closer to reality.

quant-ph↗

arXiv2022

Fast and efficient demultiplexing of single photons from a quantum dot with resonantly enhanced electro-optic modulators

We report on a multi-photon source based on active demultiplexing of single photons emitted from a resonantly excited GaAs quantum dot. Active temporal-to-spatial mode demultipexing is implemented via resonantly enhanced free-space electro-optic modulators, making it possible to route individual photons at high switching rates of 38 MHz. We demonstrate routing into four spatial modes with a high end-to-end efficiency of 79% and measure a four-photon coincidence rate of 0.17 Hz mostly limited by the single-photon source brightness and not by the efficiency of the demultiplexer itself. We use the demultiplexer to characterize the pairwise indistinguishability of consecutively emitted photons from the quantum dot with variable delay time.

quant-ph↗

arXiv2021

Towards probing for hypercomplex quantum mechanics in a waveguide interferometer

We experimentally investigate the suitability of a multi-path waveguide interferometer with mechanical shutters for performing a test for hypercomplex quantum mechanics. Probing the interferometer with coherent light we systematically analyse the influence of experimental imperfections that could lead to a false-positive test result. In particular, we analyse the effects of detector nonlinearity, input-power and phase fluctuations on different timescales, closed-state transmissivity of shutters and crosstalk between different interferometer paths. In our experiment, a seemingly small shutter transmissivity in the order of about $2 \times 10^{-4}$ is the main source of systematic error, which suggests that this is a key imperfection to monitor and mitigate in future experiments.

quant-ph↗

arXiv2021

Symmetry allows for distinguishability in totally destructive many-particle interference

We investigate, in a four photon interference experiment in a laser-written waveguide structure, how symmetries control the suppression of many-body output events of a $J_x$ unitary. We show that totally destructive interference does not require mutual indistinguishability between all, but only between symmetrically paired particles, in agreement with recent theoretical predictions. The outcome of the experiment is well described by a quantitative simulation which accounts for higher order emission of the photon source, imbalances in the scattering network, partial distinguishability, and photon loss.

quant-ph↗

arXiv2021

Approaching the Tsirelson bound with a Sagnac source of polarization-entangled photons

High-fidelity polarization-entangled photons are a powerful resource for quantum communication, distributing entanglement and quantum teleportation. The Bell-CHSH inequality $S\leq2$ is violated by bipartite entanglement and only maximally entangled states can achieve $S=2\sqrt{2}$, the Tsirelson bound. Spontaneous parametric down-conversion sources can produce entangled photons with correlations close to the Tsirelson bound. Sagnac configurations offer intrinsic stability, compact footprint and high collection efficiency, however, there is often a trade off between source brightness and entanglement visibility. Here, we present a Sagnac polarization-entangled source with $2\sqrt{2}-S=(5.65\pm0.57)\times10^{-3}$, on-par with the highest values recorded, while generating and detecting $(4660\pm70)$ pairs/s/mW, which is a substantially higher brightness than previously reported for Sagnac sources and around two orders of magnitude brighter than for traditional cone sources with the highest $S$ parameter. Our source records $0.9953\pm0.0003$ concurrence and $0.99743\pm0.00014$ fidelity to an ideal Bell state. By studying systematic errors in Sagnac sources, we identify that the precision of the collection focal point inside the crystal plays the largest role in reducing the $S$ parameter in our experiment. We provide a pathway that could enable the highest $S$ parameter recorded with a Sagnac source to-date while maintaining very high brightness.

quant-ph↗

arXiv2020

Deterministic preparation of spin qubits in droplet etched GaAs quantum dots using quasi-resonant excitation

We present a first comprehensive study on deterministic spin preparation employing excited state resonances of droplet etched GaAs quantum dots. This achievement facilitates future investigations of spin qubit based quantum memories using the GaAs quantum dot material platform. By observation of excitation spectra for a range of fundamental excitonic transitions the properties of different quantum dot energy levels, i.e. shells, are revealed. The innovative use of polarization resolved excitation and detection in quasi-resonant excitation spectroscopy facilitates determination of $85$ $\%$ maximum spin preparation fidelity - irrespective of the relative orientations of lab and quantum dot polarization eigenbases. Additionally, the characteristic non-radiative decay time is investigated as a function of ground state, excitation resonance and excitation power level, yielding decay times as low as $29$ ps for s-p-shell exited state transitions. Finally, by time resolved correlation spectroscopy it is demonstrated that the employed excitation scheme has a significant impact on the electronic environment of quantum dot transitions thereby influencing its charge and coherence.

cond-mat.mes-hall↗

arXiv2020

Exploring complex graphs using three-dimensional quantum walks of correlated photons

Graph representations are a powerful concept for solving complex problems across natural science, as patterns of connectivity can give rise to a multitude of emergent phenomena. Graph-based approaches have proven particularly fruitful in quantum communication and quantum search algorithms in highly branched quantum networks. Here we introduce a new paradigm for the direct experimental realization of excitation dynamics associated with three-dimensional networks by exploiting the hybrid action of spatial and polarization degrees of freedom of photon pairs in complex waveguide circuits with tailored birefringence. This novel testbed for the experimental exploration of multi-particle quantum walks on complex, highly connected graphs paves the way towards exploiting the applicative potential of fermionic dynamics in integrated quantum photonics.

physics.optics↗

arXiv2019

Entanglement Swapping with Semiconductor-generated Photons

Transferring entangled states between photon pairs is essential for quantum communication technologies. Semiconductor quantum dots are the most promising candidate for generating polarization-entangled photons deterministically. Recent improvements in photonic quality and brightness now make them suited for complex quantum optical purposes in practical devices. Here we demonstrate for the first time swapping of entangled states between two pairs of photons emitted by a single quantum dot. A joint Bell measurement heralds the successful generation of the Bell state $Ψ^+$ with a fidelity of up to $0.81 \pm 0.04$. The state's nonlocal nature is confirmed by violating the CHSH-Bell inequality. Our photon source is compatible with atom-based quantum memories, enabling implementation of hybrid quantum repeaters. This experiment thus is a major step forward for semiconductor based quantum communication technologies.

quant-ph↗

arXiv2018

Totally Destructive Interference for Permutation-Symmetric Many-Particle States

Several distinct classes of unitary mode transformations have been known to exhibit the strict suppression of a large set of transmission events, as a consequence of totally destructive many-particle interference. In another work [Dittel et al., Phys. Rev. Lett. 120, 240404 (2018)] we unite these cases by identifying a general class of unitary matrices which exhibit such interferences. Here, we provide a detailed theoretical analysis that substantially expands on all aspects of this generalisation: We prove the suppression laws put forward in our other paper, establish how they interrelate with forbidden single-particle transitions, show how all suppression laws hitherto known can be retrieved from our general formalism, and discuss striking differences between bosons and fermions. Furthermore, beyond many-particle Fock states on input, we consider arbitrary pure initial states and derive suppression laws which stem from the wave function's permutation symmetry alone. Finally, we identify conditions for totally destructive interference to persist when the involved particles become partially distinguishable.

quant-ph↗

arXiv2018

Totally Destructive Many-Particle Interference

In a general, multi-mode scattering setup, we show how the permutation symmetry of a many-particle input state determines those scattering unitaries which exhibit strictly suppressed many-particle transition events. We formulate purely algebraic suppression laws that identify these events and show that the many-particle interference at their origin is robust under weak disorder and imperfect indistinguishability of the interfering particles. Finally, we demonstrate that all suppression laws so far described in the literature are embedded in the general framework that we here introduce.

quant-ph↗

arXiv2018

Many-particle interference in a two-component bosonic Josephson junction: an all-optical simulation

We conceive an all-optical representation of the dynamics of two distinct types of interacting bosons in a double well by an array of evanescently coupled photonic waveguides. Many-particle interference effects are probed for various interaction strengths by changing the relative abundance of the particle species and can be readily identified by monitoring the propagation of the light intensity across the waveguide array. In particular, we show that finite inter-particle interaction strengths reduce the many-particle interference contrast by dephasing. A general description of the many-particle dynamics for arbitrary initial states is given in terms of two coupled spins by generalising the Schwinger representation to two particle species.

quant-ph↗