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Robert Schmidt

Publications and source records attributed to Robert Schmidt.

At least 19 recordsLinked to original sources

Strain engineering of transient exciton diffusion in WSe2 monolayers at cryogenic temperatures

Tungsten-based transition metal dichalcogenides exhibit dark excitons as the energetically lowest states. These are crucial for exciton thermalization and propagation and they dominate low-temperature photoluminescence via the emergence of pronounced phonon sidebands. After a resonant excitation, highly mobile hot dark excitons are formed, which quickly thermalize into an equilibrium distribution. The application of strain modifies the exciton energy landscape and, in particular, the relative energy separation between bright and dark exciton states. The impact of strain on the transient photoluminescence and diffusion of non-equilibrium excitons has remained largely unexplored so far. In this work, we investigate the spatiotemporal exciton dynamics in strained hBN-encapsulated WSe2 monolayers at cryogenic temperatures. We demonstrate that tensile strain abruptly increases the excess energy of hot excitons, thereby accelerating their transient diffusion. We trace this back to suppressed phonon-mediated scattering from bright to dark excitons. Furthermore, we predict a periodic modulation of the transient exciton diffusion in the presence of a compressive strain resulting from strain-driven emission of M phonons. The gained microscopic insights illustrate how strain can be used to engineer transient photoluminescence and exciton diffusion in technologically promising 2D semiconductors.

cond-mat.mes-hall

An O-RAN Framework for AI/ML-Based Localization with OpenAirInterface and FlexRIC

Localization is increasingly becoming an integral component of wireless cellular networks. The advent of artificial intelligence (AI) and machine learning (ML) based localization algorithms presents potential for enhancing localization accuracy. Nevertheless, current standardization efforts in the third generation partnership project (3GPP) and the O-RAN Alliance do not support AI/ML-based localization. In order to close this standardization gap, this paper describes an O-RAN framework that enables the integration of AI/ML-based localization algorithms for real-time deployments and testing. Specifically, our framework includes an O-RAN E2 Service Model (E2SM) and the corresponding radio access network (RAN) function, which exposes the Uplink Sounding Reference Signal (UL-SRS) channel estimates from the E2 agent to the Near real-time RAN Intelligent Controller (Near-RT RIC). Moreover, our framework includes, as an example, a real-time localization external application (xApp), which leverages the custom E2SM-SRS in order to execute continuous inference on a trained Channel Charting (CC) model, which is an emerging self-supervised method for radio-based localization. Our framework is implemented with OpenAirInterface (OAI) and FlexRIC, democratizing access to AI-driven positioning research and fostering collaboration. Furthermore, we validate our approach with the CC xApp in real-world conditions using an O-RAN based localization testbed at EURECOM. The results demonstrate the feasibility of our framework in enabling real-time AI/ML localization and show the potential of O-RAN in empowering positioning use cases for next-generation AI-native networks.

cs.NI

Theory of In-Plane-Magnetic-Field-Dependent Excitonic Spectra in Atomically Thin Semiconductors

The linear absorption spectrum of excitons in TMDC monolayers under the influence of an in-plane magnetic field is theoretically studied. We demonstrate that in-plane magnetic fields induce a hybridization between spin-bright and spin-dark exciton transitions, resulting in a brightening of spin-dark excitons. We analytically investigate spectral features including resonance energy shifts, broadening and amplitudes ratios. In particular, for a MoSe$_2$ monolayer with radiatively-limited linewidth, we find a complex interplay of dark-bright splitting and linewidth difference of both involved spin-bright and spin-dark excitons.

cond-mat.mes-hall

AraRACH: Enhancing NextG Random Access Reliability in Programmable Wireless Living Labs

The rapid evolution of wireless technologies has intensified interest in open and fully programmable radio access networks for whole-stack research, innovation, and evaluation of emerging solutions. Large-scale wireless living labs, such as ARA, equipped with real-world infrastructure play a vital role in this evolution by enabling researchers to prototype and evaluate advanced algorithms for next-generation wireless systems in outdoor and over-the-air environments benefiting from real-world fidelity and end-to-end programmability. However, at the core of this innovation is the performance in terms of coverage and reliability of these wireless living labs. For instance, interfacing power amplifiers and low noise amplifiers with software-defined radios (SDRs) for experimenting outdoors introduces issues in random access procedure-a process crucial in establishing connectivity between user equipment (UE) and the core network in 5G and 6G systems. Therefore, to ensure seamless connectivity and reliable communications in open-source 5G software stacks such as OpenAirInterface (OAI), we propose a slot-based approach to the 5G random access procedure leveraging full downlink (DL) and uplink (UL) slots instead of using special or mixed slots. We highlight how this approach achieves reliable 5G connectivity over 1 mile-the longest communication range that has been achieved so far in real-world settings using open-source 5G software stacks and the Universal Software Radio Peripheral (USRP) SDRs. We also demonstrate that, in a highly obstructed environment such as an industrial setting, we can increase the probability of a successful random access procedure to 90%-100% when we use at least 9 OFDM symbols to transmit msg2 and msg3.

cs.NI

Nanoscale resolved mapping of the dipole emission of hBN color centers with a scattering-type scanning near-field optical microscope

Color centers in hexagonal boron nitride (hBN) are promising candidates as quantum light sources for future technologies. In this work, we utilize a scattering-type near-field optical microscope (s-SNOM) to study the photoluminescence (PL) emission characteristics of such quantum emitters in metalorganic vapor phase epitaxy grown hBN. On the one hand, we demonstrate direct near-field optical excitation and emission through interaction with the nanofocus of the tip resulting in a sub-diffraction limited tip-enhanced PL hotspot. On the other hand, we show that indirect excitation and emission via scattering from the tip significantly increases the recorded PL intensity. This demonstrates that the tip-assisted PL (TAPL) process efficiently guides the generated light to the detector. We apply the TAPL method to map the in-plane dipole orientations of the hBN color centers on the nanoscale. This work promotes the widely available s-SNOM approach to applications in the quantum domain including characterization and optical control.

cond-mat.mes-hall

Driving Innovation in 6G Wireless Technologies: The OpenAirInterface Approach

The development of 6G wireless technologies is rapidly advancing, with the 3rd Generation Partnership Project (3GPP) entering the pre-standardization phase and aiming to deliver the first specifications by 2028. This paper explores the OpenAirInterface (OAI) project, an open-source initiative that plays a crucial role in the evolution of 5G and future 6G networks. OAI provides a comprehensive implementation of 3GPP and O-RAN compliant networks, including Radio Access Network (RAN), Core Network (CN), and software-defined User Equipment (UE) components. This paper details the history and evolution of OAI, its licensing model, and the various projects under its umbrella, such as RAN, the CN, and the Operations, Administration and Maintenance (OAM) projects. It also highlights the development methodology, Continuous Integration/Continuous Delivery (CI/CD) processes, and end-to-end systems powered by OAI. Furthermore, the paper discusses the potential of OAI for 6G research, focusing on spectrum, reflective intelligent surfaces, and Artificial Intelligence (AI)/Machine Learning (ML) integration. The open-source approach of OAI is emphasized as essential for tackling the challenges of 6G, fostering community collaboration, and driving innovation in next-generation wireless technologies.

cs.NI

Pressure dependence of intra- and interlayer excitons in 2H-MoS$_2$ bilayers

The optical and electronic properties of multilayer transition metal dichalcogenides differ significantly from their monolayer counterparts due to interlayer interactions. The separation of individual layers can be tuned in a controlled way by applying pressure. Here, we use a diamond anvil cell to compress bilayers of 2H-MoS$_2$ in the gigapascal range. By measuring optical transmission spectra, we find that increasing pressure leads to a decrease in the energy splitting between the A and interlayer exciton. Comparing our experimental findings with ab initio calculations, we conclude that the observed changes are not due to the commonly assumed hydrostatic compression. This effect is attributed to the MoS$_2$ bilayer adhering to the diamond, which reduces in-plane compression. Moreover, we demonstrate that the distinct real-space distributions and resulting contributions from the valence band account for the different pressure dependencies of the inter- and intralayer excitons in compressed MoS$_2$ bilayers.

cond-mat.mes-hall

Nanoimprint strain-engineering of 2D semiconductors

Mechanical strain is a powerful tool to tune the optical and optoelectronic properties of atomically thin semiconductors. Inhomogeneous strain plays an important role in exciton funneling and the activation of single-photon emitters in 2D materials. Here, we create an inhomogeneous strain profile in a 2D semiconductor on a micrometer scale by a nanoimprint process. We present a nanoimprint setup, where a mold is used to apply pressure in a controlled way to a WS2 monolayer on a heated polymer layer. After printing, the strain created in the 2D semiconductor is verified by hyperspectral optical imaging. The developed nanoimprint technique is scalable and could be transferred to commercial nanoimprint machines.

physics.app-ph

Resonant and phonon-assisted ultrafast coherent control of a single hBN color center

Single-photon emitters in solid-state systems are important building blocks for scalable quantum technologies. Recently, quantum light emitters have been discovered in the wide-gap van der Waals insulator hBN. These color centers have attracted considerable attention due to their quantum performance at elevated temperatures and wide range of transition energies. Here, we demonstrate coherent state manipulation of a single hBN color center with ultrafast laser pulses and investigate in our joint experiment-theory study the coupling between the electronic system and phonons. We demonstrate that coherent control can not only be performed resonantly on the optical transition giving access to the decoherence but also phonon-assisted, which reveals the internal phonon quantum dynamics. In the case of optical phonons we measure their decoherence, stemming in part from their anharmonic decay. Dephasing induced by the creation of acoustic phonons manifests as a rapid decrease of the coherent control signal when traveling phonon wave packets are emitted. Furthermore, we demonstrate that the quantum superposition between a phonon-assisted process and the resonant excitation causes ultrafast oscillations of the coherent control signal. Our results pave the way for ultrafast phonon quantum state control on the nanoscale and open up a new promising perspective for hybrid quantum technologies.

cond-mat.mes-hall

High-performance broadband Faraday rotation spectroscopy of 2D materials and thin magnetic films

We present a Faraday rotation spectroscopy (FRS) technique for measurements on the micron scale. Spectral acquisition speeds of many orders of magnitude faster than state-of-the-art modulation spectroscopy setups are demonstrated. The experimental method is based on charge-coupled-device detection, avoiding speed-limiting components, such as polarization modulators with lock-in amplifiers. At the same time, FRS spectra are obtained with a sensitivity of 20 $\mu$rad (0.001$^\circ$) over a broad spectral range (525 nm - 800 nm), which is on par with state-of-the-art polarization-modulation techniques. The new measurement technique also automatically cancels unwanted Faraday rotation backgrounds. Using the setup, we perform Faraday rotation spectroscopy of excitons in a hBN-encapsulated atomically thin semiconductor WS$_2$ under magnetic fields of up to 1.4 T at room temperature and liquid helium temperature. We determine the A exciton g-factor of -4.4 $\pm$ 0.3 at room temperature, and -4.2 $\pm$ 0.2 at liquid helium temperature. In addition, we perform FRS and hysteresis loop measurements on a 20 nm thick film of an amorphous magnetic Tb$_{0.2}$Fe$_{0.8}$ alloy.

cond-mat.mes-hall

Full-sky photon simulation of clusters and active galactic nuclei in the soft X-rays for eROSITA

The eROSITA X-ray telescope on board the Spectrum-Roentgen-Gamma (SRG) mission will measure the position and properties of about 100,000 clusters of galaxies and 3 million active galactic nuclei over the full sky. To study the statistical properties of this ongoing survey, it is key to estimate the selection function accurately. We create a set of full sky light-cones using the MultiDark and UNIT dark matter only N-body simulations. We present a novel method to predict the X-ray emission of galaxy clusters. Given a set of dark matter halo properties (mass, redshift, ellipticity, offset parameter), we construct an X-ray emissivity profile and image for each halo in the light-cone. We follow the eROSITA scanning strategy to produce a list of X-ray photons on the full sky. We predict scaling relations for the model clusters, which are in good agreement with the literature. The predicted number density of clusters as a function of flux also agrees with previous measurements. Finally, we obtain a scatter of 0.21 (0.07, 0.25) for the X-ray luminosity -- mass (temperature -- mass, luminosity -- temperature) model scaling relations. We provide catalogues with the model photons emitted by clusters and active galactic nuclei. These catalogues will aid the eROSITA end to end simulation flow analysis and in particular the source detection process and cataloguing methods.

astro-ph.CO

Theory of the Coherent Response of Magneto-Excitons and Magneto-Biexcitons in Monolayer Transition Metal Dichalcogenides

The recent accessibility of high quality, charge neutral monolayer transition metal dichalcogenides with narrow exciton linewidths at the homogeneous limit provides an ideal platform to study excitonic many-body interactions. In particular, the possibility to manipulate coherent exciton-exciton interactions, which govern the ultrafast nonlinear optical response, by applying an external magnetic field has not been considered so far. We address this discrepancy by presenting a nonlinear microscopic theory in the coherent limit for optical excitations in the presence of out-of-plane, in-plane, and tilted magnetic fields. Specifically, we explore the magnetic-field-induced exciton and biexciton fine structure and calculate their oscillator strengths based on a Heisenberg equations of motion formalism. Our microscopic evaluations of pump-probe spectra allow to interpret and predict coherent signatures in future wave-mixing experiments.

cond-mat.mes-hall

Strain-dependent exciton diffusion in transition metal dichalcogenides

Monolayers of transition metal dichalcogenides (TMDs) have a remarkable excitonic landscape with deeply bound bright and dark exciton states. Their properties are strongly affected by lattice distortions that can be created in a controlled way via strain. Here, we perform a joint theory-experiment study investigating exciton diffusion in strained tungsten disulfide (WS$_2$) monolayers. We reveal a non-trivial and non-monotonic influence of strain. Lattice deformations give rise to different energy shifts for bright and dark excitons changing the excitonic landscape, the efficiency of intervalley scattering channels, and the weight of single exciton species to the overall exciton diffusion. We predict a minimal diffusion coefficient in unstrained WS$_2$ followed by a steep speed-up by a factor of 3 for tensile biaxial strain at about 0.6\% strain - in excellent agreement with our experiments. The obtained microscopic insights on the impact of strain on exciton diffusion are applicable to a broad class of multi-valley 2D materials.

cond-mat.mes-hall

Ultrafast dynamics in monolayer TMDCs: the interplay of dark excitons, phonons and intervalley Coulomb exchange

Understanding the ultrafast coupling and relaxation mechanisms between valleys in transition metal dichalcogenide semiconductors is of crucial interest for future valleytronic devices. Recent ultrafast pump-probe experiments showed an unintuitive significant bleaching at the excitonic $B$ transition after optical excitation of the energetically lower excitonic $A$ transition. Here, we present a possible microscopic explanation for this surprising effect. It is based on the joint action of exchange coupling and phonon-mediated thermalization into dark exciton states and does not involve a population of the B exciton. Our work demonstrates how intra- and intervalley coupling on a femtosecond timescale governs the optical valley response of 2D semiconductors.

cond-mat.mes-hall

Thickness determination of MoS2, MoSe2, WS2 and WSe2 on transparent stamps used for deterministic transfer of 2D materials

Here, we propose a method to determine the thickness of the most common transition metal dichalcogenides (TMDCs) placed on the surface of transparent stamps, used for the deterministic placement of two-dimensional materials, by analyzing the red, green and blue channels of transmission-mode optical microscopy images of the samples. In particular, the blue channel transmittance shows a large and monotonic thickness dependence, making it a very convenient probe of the flake thickness. The method proved to be robust given the small flake-to-flake variation and the insensitivity to doping changes of MoS2. We also tested the method for MoSe2, WS2 and WSe2. These results provide a reference guide to identify the number of layers of this family of materials on transparent substrates only using optical microscopy.

physics.app-ph

Simulation Environment for Link Energy Estimation in Networks-on-Chip with Virtual Channels

Network-on-chip (NoC) is the most promising design paradigm for the interconnect architecture of a multiprocessor system-on-chip (MPSoC). On the downside, a NoC has a significant impact on the overall energy consumption of the system. NoC simulators are highly relevant for design space exploration even at an early stage. Since links in NoC consume up to 50% of the energy, a realistic energy consumption of links in NoC simulators is important. This work presents a simulation environment which implements a technique to precisely estimate the data dependent link energy consumption in NoCs with virtual channels for the first time. Our model works at a high level of abstraction, making it feasible to estimate the energy requirements at an early design stage. Additionally, it enables the fast evaluation and early exploration of low-power coding techniques. The presented model is applicable for 2D and 3D NoCs. A case study for an image processing application shows that the current link model leads to an underestimate of the link energy consumption by up to a factor of four. In contrast, the technique presented in this paper estimates the energy quantities precisely with an error below 1% compared to results obtained by precise, but computational extensive, bit-level simulation.

eess.SP

Phonon-assisted emission and absorption of individual color centers in hexagonal boron nitride

Defect centers in hexagonal boron nitride represent room-temperature single-photon sources in a layered van der Waals material. These light emitters appear with a wide range of transition energies ranging over the entire visible spectrum, which renders the identification of the underlying atomic structure challenging. In addition to their eminent properties as quantum light emitters, the coupling to phonons is remarkable. Their photoluminescence exhibits significant side band emission well separated from the zero phonon line (ZPL) and an asymmetric broadening of the ZPL itself. In this combined theoretical and experimental study we show that the phonon side bands can be well described in terms of the coupling to bulk longitudinal optical (LO) phonons. To describe the ZPL asymmetry we show that in addition to the coupling to longitudinal acoustic (LA) phonons also the coupling to local mode oscillations of the defect center with respect to the entire host crystal has to be considered. By studying the influence of the emitter's wave function dimensions on the phonon side bands we find reasonable values for size of the wave function and the deformation potentials. We perform photoluminescence excitation measurements to demonstrate that the excitation of the emitters is most efficient by LO-phonon assisted absorption.

cond-mat.mes-hall

Zeeman spectroscopy of excitons and hybridization of electronic states in few-layer WSe$_2$, MoSe$_2$ and MoTe$_2$

Monolayers and multilayers of semiconducting transition metal dichalcogenides (TMDCs) offer an ideal platform to explore valley-selective physics with promising applications in valleytronics and information processing. Here we manipulate the energetic degeneracy of the $\mathrm{K}^+$ and $\mathrm{K}^-$ valleys in few-layer TMDCs. We perform high-field magneto-reflectance spectroscopy on WSe$_2$, MoSe$_2$, and MoTe$_2$ crystals of thickness from monolayer to the bulk limit under magnetic fields up to 30 T applied perpendicular to the sample plane. Because of a strong spin-layer locking, the ground state A excitons exhibit a monolayer-like valley Zeeman splitting with a negative $g$-factor, whose magnitude increases monotonically when thinning the crystal down from bulk to a monolayer. Using the $\mathbf{k\cdot p}$ calculation, we demonstrate that the observed evolution of $g$-factors for different materials is well accounted for by hybridization of electronic states in the $\mathrm{K}^+$ and $\mathrm{K}^-$ valleys. The mixing of the valence and conduction band states induced by the interlayer interaction decreases the $g$-factor magnitude with an increasing layer number. The effect is the largest for MoTe$_2$, followed by MoSe$_2$, and smallest for WSe$_2$. Keywords: MoSe$_2$, WSe$_2$, MoTe$_2$, valley Zeeman splitting, transition metal dichalcogenides, excitons, magneto optics.

cond-mat.mes-hall