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Robert-Jan Slager

Publications and source records attributed to Robert-Jan Slager.

At least 19 recordsLinked to original sources

Geometric Ginzburg-Landau theory of charge ordering and commensurability

The concept of quantum geometry has recently led to reinvigorated insights in a wide range of fields including physical responses, superconductivity, and optical transitions, with effects most pronounced in systems with nearly flat dispersion. Here, we show that it plays an essential role in charge density wave formation (CDW) -- an important physical phenomenon that is responsible for driving various sharp changes in material transport properties including metal-insulator transitions. We derive an effective Ginzburg-Landau theory including uncharted contributions and, as a highlight, discover a general criterion for both CDW formation and commensurability transitions where underlying electron-phonon interactions manifest purely as electronic quantum geometric enhancements/suppressions. We benchmark our framework in a class of transition-metal dichalcogenides and resolve a longstanding puzzle where well-established purely kinetic CDW criteria fail in describing the correct ordering wavevector. Besides rendering robust criteria and fundamental insights that are immediately relevant to several experimental charge ordering systems, our theory can also be applied directly to other phonon-mediated phases such as superconductivity, and can be used as an important tool to explore the interplay between various such states. More generally, our framework provides a recipe for investigating the role of quantum geometry in phase transitions.

cond-mat.str-el

Magnetononlinear Hall effect from multigap topology in metal-organic frameworks

We unveil that non-Abelian multigap band topology characterized by nontrivial Euler class invariants induces observable magnetononlinear Hall transport phenomena. We demonstrate these effects in a highly-tunable class of recently synthesized two-dimensional kagome N-heterocyclic carbene (NHC) metal-organic frameworks. We showcase the controllability of the nonlinear effect upon applying external voltage, changing temperature, and chemical substitutions that preserve the bulk topology and associated edge states. Our findings therefore reveal an uncharted presence of Euler class topology in metal-organic materials that can be experimentally deduced through measurable magnetotransport.

cond-mat.mes-hall

Operator Space Transport and the Emergence of Boundary Time Crystals

Boundary time crystals (BTCs) are prominent examples of continuous time crystals in collective spin systems governed by Lindbladian evolution. To date, their analysis has mostly relied on semiclassical and numerical approaches. Here, we develop a fully quantum-compatible framework to classify collective spin dynamics and show that BTC behavior emerges from the absence of non-trivial weak symmetries of the Liouvillian. To this end, we introduce an irreducible tensor representation of operator space, in which the Lindbladian dynamics maps onto a non-Hermitian hopping problem. Within this picture, the dynamics corresponds to the transport of operator weight across tensor sectors. This mapping allows an identification of distinct dynamical regimes, including collective precession, pure relaxation, and the BTC phase, within a single unified framework. We show that BTCs arise from non-reciprocal transport in operator space, which delocalizes Liouvillian eigenmodes across multiple tensor sectors. This non-reciprocal transport provides a microscopic mechanism for the insensitivity to initial conditions of BTC oscillations. More broadly, our results establish operator space transport as a perspective for understanding dissipative many-body dynamics and highlights connections to non-Hermitian phenomena.

quant-ph

Topological Optical Chirality Dichroism

We report on a universal topological dichroism of chiral three-dimensional systems in response to the chirality of light. We show that chiral topological invariants result in integer-quantized dichroic excitation rate differences. Moreover, we demonstrate that such topological effects arise more generally from coupling optical chirality to higher tensor Berry curvatures and Dixmier-Douady invariants of quantum states, including Hopf indices. We finally propose an experimental setup that leverages superchiral light as a smoking-gun probe of chiral band topologies in three-dimensional materials. Our findings establish an optical route for probing to date unobserved chiral electronic band topologies.

cond-mat.mes-hall

Realizing anomalous Floquet non-Abelian band topology in photonic scattering networks

The concept of multi-gap topology has recently been shown to give rise to uncharted phases beyond conventional single-gap classifications. These phases relate to band nodes with non-Abelian quaternion charges and momentum-space braiding processes characterized by new invariants such as paradigmatic Euler class, phenomena that intrinsically require at least two spatial dimensions. Extending such phases into the non-equilibrium regime is predicted to unlock even richer multi-gap topologies beyond static settings, yet their experimental realization has remained elusive due to the stringent requirements on dimensionality, symmetry, and dynamical control. Here, we theoretically demonstrate and, for the first time, experimentally realize two-dimensional (2D) Floquet non-Abelian band topology in photonic scattering networks. Within this platform, we uncover a sequence of topological phenomena unique to 2D multi-gap systems far from equilibrium, including anomalous multi-gap phases interconnected by band nodes, Floquet Euler transfer, gapped phases with anomalous Dirac string configurations, and Floquet-induced non-Abelian braiding of band nodes. In addition, we observe Floquet-periodic anomalous edge states across multiple gaps, providing experimental signatures of these sought-after 2D multi-gap Floquet topological phases. Our results establish photonic scattering networks as a practical and versatile route to non-Abelian Floquet systems, opening avenues for dynamical topological physics with braiding capability and robust photonic functionalities.

physics.optics

Topological Boundary Time Crystal Oscillations

Boundary time crystals (BTCs) break time-translation symmetry and exhibit long-lived, robust oscillations insensitive to initial conditions. We show that collective spin BTCs can admit emergent topological winding numbers in operator space. Expanding the density operator in a spherical tensor basis, we map the Lindblad dynamics onto an effective local hopping problem, where collective degrees of freedom label sites of an emergent two-dimensional operator space lattice and identify topological obstructions that enforce the delocalization of operator modes on the lattice. The resulting spectral delocalization provides a natural explanation for the robust oscillatory dynamics observed in BTCs. When combined with non-reciprocal transport of operator weight across operator space, this mechanism moreover also leads to the universality of long-time dynamics across a broad class of initial states. Our results frame BTC dynamics as a form of topologically constrained operator space transport and suggest a close connection to non-Hermitian skin-effects.

quant-ph

Topological Acoustic Diode

We show that certain three-dimensional topological phases can act as acoustic diodes realizing nonlinear odd acoustoelastic effects. Beyond uncovering topologically-induced anomalous acoustic second-harmonic generation and rectification, we demonstrate how such nonlinear responses are uniquely captured by the momentum-space nonmetricity tensor in the quantum state Hilbert-space geometry. In addition to completing the classification of quantum geometric observables in the quadratic response regime, our findings reveal unexplored avenues for experimental realizations of acoustic diodes using effective $\theta$ vacua of axion insulators adaptable for topological engineering applications.

cond-mat.mes-hall

Orbital magnetization reveals multiband topology

We demonstrate that nontrivial multiband topological invariants of electronic wavefunctions can be revealed through orbital magnetization responses to external magnetic fields. We find that decomposing orbital magnetization into energetic and quantum-geometric contributions allows one to deduce nontrivial multiband topology, provided knowledge of the energy spectrum. We showcase our findings in general effective models with multiband Euler topology. We moreover identify such multiband topological invariants in effective models of strontium ruthenate ($\text{Sr}_2 \text{Ru} \text{O}_4$), which may in principle be verified in the state-of-the-art doping-dependent magnetization measurements. Our reconstruction scheme for multiband invariants sheds a topological perspective on the multiorbital effects in materials realizing unconventional phenomenologies of orbital currents or multiband superconductivity.

cond-mat.mes-hall

Nonlinear Odd Viscoelastic Effect

We uncover a class of nonlinear odd viscoelastic effects in three spatial dimensions. We show that these dissipationless effects arise upon combining geometric distortions in two orthogonal directions, yielding momentum flow in the third direction. We demonstrate that the effect arises from nontrivial geometric tensors in quantum states, and can be scaled up with integer topological invariants. We further show that the effect fingerprints the multiband Hilbert-space geometry of the underlying quantum states, as encoded in the nonmetricity and three-state quantum geometric tensors. Our findings unravel the role of multistate geometry in viscoelastic phenomena, paving a path for experimental observation of uncharted nonlinear odd viscoelastic responses in quantum systems.

cond-mat.mes-hall

Measuring non-Abelian quantum geometry and topology in a multi-gap photonic lattice

Recent discoveries in semi-metallic multi-gap systems featuring band singularities have galvanized enormous interest in particular due to the emergence of non-Abelian braiding properties of band nodes. This previously uncharted set of topological phases necessitates novel approaches to probe them in laboratories, a pursuit that intricately relates to evaluating non-Abelian generalizations of the Abelian quantum geometric tensor (QGT) that characterizes geometric responses. Here, we pioneer the direct measurement of the non-Abelian QGT. We achieve this by implementing a novel orbital-resolved polarimetry technique to probe the full Bloch Hamiltonian of a six-band two-dimensional (2D) synthetic lattice, which grants direct experimental access to non-Abelian quaternion charges, the Euler curvature, and the non-Abelian quantum metric associated with all bands. Quantum geometry has been highlighted to play a key role on macroscopic phenomena ranging from superconductivity in flat-bands, to optical responses, transport, metrology, and quantum Hall physics. Therefore, our work unlocks the experimental probing of a wide phenomenology of multi-gap systems, at the confluence of topology, geometry and non-Abelian physics.

cond-mat.mes-hall

Topological non-Abelian gauge structures in Cayley-Schreier lattices

Crystalline constructions known as Cayley-Schreier lattices have been suggested as a platform for realizing arbitrary gauge fields in synthetic crystals with real hopping amplitudes. Here, we reveal that Cayley-Schreier lattices can naturally give rise to implementable lattice systems that incorporate non-Abelian gauge structures transforming into a space-group symmetry. We show that their symmetry sectors can be interpreted as blocks of pseudospin models---some of which correspond to true spinors---that can realize a wealth of different topological invariants in a single setup. We underpin these general results with concrete models and illustrate how they can be implemented in technologically available experimental platforms. Our work sets the stage for a systematic investigation of topological insulators and metals with non-Abelian gauge structures.

cond-mat.mes-hall

Gapped spinful phases obtained via Gutzwiller projections of Euler states

Gutzwiller projections of non-interacting chiral topological phases are known to give rise to fractional, topologically ordered chiral phases. Here, we carry out a similar construction using two copies of non-interacting Euler insulators to produce a class of spinful interacting Euler models. To that end, we take advantage of the recently discovered exact representation of certain Euler insulators by a projected entangled pair state (PEPS) of bond dimension $D = 2$. The Gutzwiller projection can be implemented within the tensor network formalism, giving rise to a new PEPS of bond dimension $D = 4$. We, moreover, apply very recent state-of-the-art tensor network tools to evaluate these phases. In particular, we analyze its entanglement entropy scaling and find no topological correction to the area law, indicating that the state is not intrinsically topologically ordered. Its entanglement spectrum shows a clear cusp at momentum zero, similar to non-interacting Euler insulators, and the spectrum of the transfer operator indicates that the state is gapped, which could imply non-intrinsic topological features. Finally, the static structure factor displays Bragg peaks, indicating the simultaneous presence of local order.

cond-mat.str-el

Quantum Geometry of Altermagnetic Magnons Probed by Light

Magnons with momentum-dependent chirality are a key signature of altermagnets. We identify bicircular light as a smoking-gun optical probe for chiral altermagnetic magnons, selectively targeting their quantum geometry induced by an alternation of magnonic chirality. We show that in $d$-wave altermagnets, under a canting magnetic field, the altermagnetic magnons realize a nontrivial quantum geometry, resulting in an enhancement of the nonlinear second-order light-magnon interactions. We find that the scattering of bicircular pulses probes the present magnonic quantum geometry, even if the magnonic topology is trivial. Hence, our findings establish bicircular Raman response as an optical effect of choice to identify altermagnetic magnons. As such, we propose a universal experimental protocol to distinguish altermagnets from antiferromagnets by detecting their magnon chirality patterns with light, independently of the underlying magnon topology.

cond-mat.mes-hall

Non-periodic Boundary Conditions for Euler Class and Dynamical Signatures of Obstruction

While the landscape of free-fermion phases has drastically been expanded in the last decades, recently novel multi-gap topological phases were proposed where groups of bands can acquire new invariants such as Euler class. As in conventional single-gap topologies, obstruction plays an inherent role that so far has only been incidentally addressed. We here systematically investigate the nuances of the relation between the non-Bravais lattice configurations and the Brillouin zone boundary conditions (BZBCs) for any number of dimensions. Clarifying the nomenclature, we provide a general periodictization recipe to obtain a gauge with an almost Brillouin-zone-periodic Bloch Hamiltonian both generally and upon imposing a reality condition on Hamiltonians for Euler class. Focusing on three-band $\mathcal{C}_2$ symmetric Euler systems in two dimensions as a guiding example, we present a procedure to enumerate the possible lattice configurations, and thus the unique BZBCs possibilities. We establish a comprehensive classification for the identified BZBC patterns according to the parity constraints they impose on the Euler invariant, highlighting how it extends to more bands and higher dimensions. Moreover, by building upon previous work utilizing Hopf maps, we illustrate physical consequences of non-trivial BZBCs in the quench dynamics of non-Bravais lattice Euler systems, reflecting the parity of the Euler invariant. We numerically confirm our results and corresponding observable signatures, and discuss possible experimental implementations. Our work presents a general framework to study the role of non-trivial boundary conditions and obstructions on multi-gap topology that can be employed for arbitrary number bands or in higher dimensions.

cond-mat.quant-gas

Probing Tensor Monopoles and Gerbe Invariants in Three-Dimensional Topological Matter

We show that momentum-space tensor monopoles corresponding to nontrivial vector bundle generalizations, known as bundle gerbes, can be realized in bands of three-dimensional topological matter with nontrivial Hopf invariants. We provide a universal construction of tensor Berry connections in these topological phases, demonstrating how obstructions therein lead to $\mathbb{Z}$-quantized bulk magnetoelectric and nonlinear optical phenomena. We then pinpoint that these quantum effects are supported by intraband and interband torsion leading to nontrivial Dixmier-Douady classes in most known Hopf phases and in more general topological insulators realizing gerbe invariants falling beyond the tenfold classification of topological phases of matter. We furthermore provide an interacting generalization upon introducing many-body gerbe invariants by employing twisted boundary conditions. This opens an avenue to study gerbe invariants realized through higher-dimensional charge fractionalizations that can be electromagnetically probed.

cond-mat.mes-hall

Euler topology in classical spin liquids

Classical spin liquids have recently been analyzed in view of the single-gap homotopy classification of their dispersive eigenvectors. We show that the recent progress in defining multi-gap topologies, notably exemplified by the Euler class, can be naturally included in these homotopy-based classification schemes and present phases that change topology by band node braiding. This process alters the topology of the pinch points in the spin structure factor and consequently their stability. Furthermore, we discuss how these notions also pertain to models discussed previously in the literature and have a broader range of application beyond our specific results. Our work thus opens up an uncharted avenue in the understanding of spin liquids.

cond-mat.str-el

Coexisting Euler and Stiefel-Whitney Topological Phases in Elastic Metamaterials

The study of topological band theory in classical structures has led to the development of novel topological metamaterials with intriguing properties. While single-gap topologies are well understood, recent novel multi-gap phases have garnished increasing interest. These novel phases are characterized by invariants, such as the Euler and second Stiefel-Whitney classes, which involve Bloch eigen-subspaces of multiple bands and can change by braiding in momentum space non-Abelian charged band degeneracies belonging to adjacent energy gaps. Here, we theoretically predict and experimentally demonstrate that two of such topological phases can coexist within a single system using vectorial elastic waves. The inherent coupling between different polarization modes enables non-Abelian braiding of nodal points of multiple energy band gaps and results in coexisting Euler and Stiefel-Whitney topological insulator phases. We furthermore unveil the central role played by the topologically stable Goldstone modes' degeneracy. Our findings represent the first realization of hybrid phases in vectorial fields exhibiting topologically nontrivial Goldstone modes, paving the way for bifunctional applications that leverage the coexistence of topological edge and corner states.

cond-mat.mtrl-sci

Field-driven band asymmetry and non-reciprocal transport in a helimagnet

Helimagnets exhibit noncollinear spin arrangements characterized by a periodic helical modulation, giving rise to emergent chiral properties. These materials have attracted significant interest due to their potential applications in spintronics, particularly for robust information storage and the realization of topological spin textures such as skyrmions. In this work, we focus on Yoshimori-type helimagnets, where competing exchange interactions mediated by conduction electrons stabilize helical spin structures without requiring Dzyaloshinskii-Moriya interaction. We introduce a minimal model describing the electronic structure of a one-dimensional helimagnet in the presence of an external magnetic field and investigate its impact on non-reciprocal transport. We demonstrate how band asymmetry emerges in the conical phase induced by the external field, leading to a nonzero second-order electronic conductivity and injection photoconductivity. Our results provide insight into the interplay between the real space magnetic texture and electronic properties, paving the way for future studies on chirality-driven transport phenomena in centrosymmetric helimagnets.

cond-mat.mes-hall