arXiv subjects

Robert-Jan Slager

Publications and source records attributed to Robert-Jan Slager.

At least 73 records · Page 4Linked to original sources

arXiv2022

Floquet multi-gap topology: Non-Abelian braiding and anomalous Dirac string phase

Topological phases of matter span a wide area of research shaping fundamental pursuits and offering promise for future applications. While a significant fraction of topological materials has been characterized using symmetry requirements of wave functions, the past two years have witnessed the rise of novel multi-gap dependent topological states, the properties of which go beyond these approaches and are yet to be fully explored. Thriving upon these insights, we report on uncharted anomalous phases and properties that can only arise in out-of-equilibrium Floquet settings. In particular, we identify Floquet-induced non-Abelian braiding mechanisms, which in turn lead to a phase characterized by an anomalous Euler class, the prime example of a multi-gap topological invariant. Most strikingly, we also retrieve the first example of an `anomalous Dirac string phase'. This gapped out-of-equilibrium phase features an unconventional Dirac string configuration that physically manifests itself via anomalous edge states on the boundary. Our results therefore not only provide a stepping stone for the exploration of intrinsically dynamical and experimentally viable multi-gap topological phases, but also demonstrate a powerful way to observe these non-Abelian processes notably in quantum simulators.

cond-mat.mes-hall↗

arXiv2022

Rare-earth monopnoctides -- family of antiferromagnets hosting magnetic Fermi arcs

Since the discovery of topological insulators a lot of research effort has been devoted to magnetic topological materials, in which non-trivial spin properties can be controlled by magnetic fields, culminating in a wealth of fundamental phenomena and possible applications. The main focus was on ferromagnetic materials that can host Weyl fermions and therefore spin textured Fermi arcs. The recent discovery of Fermi arcs and new magnetic bands splitting in antiferromagnet (AFM) NdBi has opened up new avenues for exploration. Here we show that these uncharted effects are not restricted to this specific compound, but rather emerge in CeBi, NdBi, and NdSb when they undergo paramagnetic to AFM transition. Our data show that the Fermi arcs in NdSb have 2-fold symmetry, leading to strong anisotropy that may enhance effects of spin textures on transport properties. Our findings thus demonstrate that the RBi and RSb series are materials that host magnetic Fermi arcs and may be a potential platform for modern spintronics.

cond-mat.other↗

arXiv2022

Multi-gap topological conversion of Euler class via band-node braiding: minimal models, $PT$-linked nodal rings, and chiral heirs

The past few years have seen rapid progress in characterizing topological band structures using symmetry eigenvalue indicated methods. Recently, however, there has been increasing theoretical and experimental interest in multi-gap dependent topological phases that cannot be captured by this paradigm. These topologies arise by braiding band degeneracies that reside between different bands and carry non-Abelian charges due to the presence of either $C_2T$ or $PT$ symmetry, culminating in different invariants such as $\mathbb{Z}$-valued Euler class. Here, we present a universal formulation for Euler phases motivated by their homotopy classification that is related to the Skyrmion-profile of a single unit-vector in three-level systems, and that of two unit-vectors in four-level systems. In addition, upon employing the strategy of systematically building 3D models from a pair of sub-dimensional Euler phases, we show that phase transitions between any two inequivalent Euler phases are mediated by the presence of adjacent (in-gap) nodal rings linked with sub-gap nodal lines, forming trajectories corresponding to the braiding or debraiding of nodal points. The stability of the linked adjacent nodal rings is furthermore demonstrated to be indicated by an Euler class monopole charge matching with its $\mathbb{Z}$-valued linking numbers. We finally also systematically address the conversion of Euler phases into descendant Chern phases upon breaking the $C_2T$ or $PT$ symmetry. All the topological phases discussed in this work are corroborated with explicit minimal lattice models. These models can themselves directly serve as an extra impetus for experimental searches or be employed for theoretical studies, thereby underpinning the upcoming of this nascent pursuit.

cond-mat.mes-hall↗

arXiv2022

Phase transitions of non-Abelian charged nodal links in a spring-mass system

Although a large class of topological materials have uniformly been identified using symmetry properties of wave functions, the past two years have seen the rise of multi-gap topologies beyond this paradigm. Given recent reports of unexplored features of such phases, platforms that are readily implementable to realize them are therefore desirable. Here, we demonstrate that multi-gap topological phase transitions of non-Abelian charged nodal lines arise in classical phonon waves. By adopting a simple spring-mass system, we construct nodal lines of a three-band system. The braiding process of the nodal lines is readily performed by adjusting the spring constants. The generation and annihilation of the nodal lines are then analyzed using Euler class. Finally, we retrieve topological transitions from trivial nodal lines to a nodal link. Our work provides a simple platform that can offer diverse insights to not only theoretical but also experimental studies on multi-gap topology.

cond-mat.soft↗

arXiv2022

Emergence of Fermi arcs and novel magnetic splitting in an antiferromagnet

The Fermi arcs are signatures of exotic states in solids because they defy conventional concept of Fermi surfaces as closed contours in momentum space. Fermi arcs were first discovered in cuprates, and caused by the pseudogap. Weyl semimetals provided another way to generate Fermi arcs by breaking either the time reversal symmetry (TRS) or inversion symmetry of a 3D Dirac semimetal, which can result in a Weyl semimetal with pairs of Weyl nodes that have opposite chirality. The bulk-boundary correspondence associated with the Chern number leads to the emergence of Fermi arcs on the boundary. Here, we present experimental evidence that pairs of magnetically split hole- and electron-like Fermi arcs emerge below the Neel temperature, in the antiferromagnetic (AFM) state of cubic NdBi due to a novel band splitting effect. Whereas TRS is broken by the AFM order, both inversion and nonsymmorphic TRS are preserved in the bulk, precluding the possibility of a Weyl semimetal. The observed magnetic splitting is highly unusual, as it creates bands of opposing curvature, that changes with temperature and follows the antiferromagnetic order parameter. This is completely different from previously reported cases of magnetic splittings such as traditional Zeeman and Rashba, where the curvature of the bands is preserved. Therefore, our finding represents a new Fermionic state created by new type of magnetic band splitting in the presence of a long-range AFM order that are not readily explained by existing theoretical ideas.

cond-mat.str-el↗

arXiv2021

Phonons as a platform for non-Abelian braiding and its manifestation in layered silicates

Topological phases of matter have revolutionised the fundamental understanding of band theory and hold great promise for next-generation technologies such as low-power electronics or quantum computers. Single-gap topologies have been extensively explored, and a large number of materials have been theoretically proposed and experimentally observed. These ideas have recently been extended to multi-gap topologies with band nodes that carry non-Abelian charges, characterised by invariants that arise by the momentum space braiding of such nodes. However, the constraints placed by the Fermi-Dirac distribution to electronic systems have so far prevented the experimental observation of multi-gap topologies in real materials. Here, we show that multi-gap topologies and the accompanying phase transitions driven by braiding processes can be readily observed in the bosonic phonon spectra of known monolayer silicates. The associated braiding process can be controlled by means of an electric field and epitaxial strain, and involves, for the first time, more than three bands. Finally, we propose that the band inversion processes at the $Γ$ point can be tracked by following the evolution of the Raman spectrum, providing a clear signature for the experimental verification of the band inversion accompanied by the braiding process.

cond-mat.mes-hall↗

arXiv2021

Chirality flip of Weyl nodes and its manifestation in strained MoTe$_2$

Due to their topological charge, or chirality, the Weyl cones present in topological semimetals are considered robust against arbitrary perturbations. One well-understood exception to this robustness is the pairwise creation or annihilation of Weyl cones, which involves the overlap of two oppositely charged nodes in energy and momentum. Here we show that their topological charge can in fact change sign, in a process that involves the merging of not two, but three Weyl nodes. This is facilitated by the presence of rotation and time-reversal symmetries, which constrain the relative positions of Weyl cones in momentum space. We analyze the chirality flip process, showing that transport properties distinguish it from the conventional, double Weyl merging. Moreover, we predict that the chirality flip occurs in MoTe$_2$, where experimentally accessible strain leads to the merging of three Weyl cones close to the Fermi level. Our work sets the stage to further investigate and observe such chirality flipping processes in different topological materials.

cond-mat.mes-hall↗

arXiv2021

Multi-gap topology and non-Abelian braiding of phonons from first principles

Non-Abelian states of matter, in which the final state depends on the order of the interchanges of two quasiparticles, can encode information immune from environmental noise with the potential to provide a robust platform for topological quantum computation. We demonstrate that phonons can carry non-Abelian frame charges at the band crossing points of their frequency spectrum, and that external stimuli can drive their braiding. We present a general framework to understand the topological configurations of phonons from first principles calculations using a topological invariant called Euler class, and provide a complete analysis of phonon braiding by combining different topological configurations. Taking a well-known dielectric material, Al$_2$O$_3$, as a representative example, we demonstrate that electrostatic doping gives rise to phonon band inversions that can induce redistribution of the frame charges, leading to non-Abelian braiding of phonons. Our work provides a new quasiparticle platform for realizable non-Abelian braiding in reciprocal space, and expands the toolset for studying braiding processes.

cond-mat.mes-hall↗

arXiv2021

Localization via Quasi-Periodic Bulk-Bulk Correspondence

We report on a direct connection between quasi-periodic topology and the Almost Mathieu (Andre-Aubry) metal insulator transition (MIT). By constructing quasi-periodic transfer matrix equations from the limit of rational approximate projected Green's functions, we relate results from $\text{SL}(2,\mathbb{R})$ co-cycle theory (transfer matrix eigenvalue scaling) to consequences of rational band theory. This reduction links the eigenfunction localization of the MIT to the chiral edge modes of the Hofstadter Hamiltonian, implying the localized phase roots in a topological "bulk-bulk" correspondence, a bulk-boundary correspondence between the 1D AAH system (boundary) and its 2D parent Hamiltonian (bulk). This differentiates quasi-periodic localization from Anderson localization in disordered systems. Our results are widely applicable to systems beyond this paradigmatic model.

cond-mat.mes-hall↗

arXiv2021

Optical $N$-insulators: topological obstructions in the atomistic susceptibility tensor

A powerful result of topological band theory is that nontrivial phases manifest obstructions to constructing localized Wannier functions. In Chern insulators, it is impossible to construct Wannier functions that respect translational symmetry in both directions. Similarly, Wannier functions that respect time-reversal symmetry cannot be formed in quantum spin Hall insulators. This molecular orbital interpretation of topology has been enlightening and was recently extended to topological crystalline insulators which include obstructions tied to space group symmetries. In this article, we introduce a new class of two-dimensional topological materials known as optical $N$-insulators that possess obstructions to constructing localized molecular polarizabilities. The optical $N$-invariant $N\in\mathbb{Z}$ is the winding number of the atomistic susceptibility tensor $χ$ and counts the number of singularities in the electromagnetic linear response theory. We decipher these singularities by analyzing the optical band structure of the material -- the eigenvectors of the susceptibility tensor -- which constitutes the collection of optical Bloch functions. The localized basis of these eigenvectors are optical Wannier functions which represent the molecular polarizabilities at different lattice sites. We prove that in a nontrivial optical phase $N\neq 0$, such a localized polarization basis is impossible to construct. Utilizing the mathematical machinery of $K$-theory, these optical $N$-phases are refined further to account for the underlying crystalline symmetries of the material, generating a classification of the topological electromagnetic phase of matter.

cond-mat.mes-hall↗

arXiv2021

Rational Approximations of Quasi-Periodic Problems via Projected Green's Functions

We introduce the projected Green's function technique to study quasi-periodic systems such as the Andre-Aubry-Harper (AAH) model and beyond. In particular, we use projected Green's functions to construct a "rational approximate" sequence of transfer matrix equations consistent with quasi-periodic topology, where convergence of these sequences corresponds to the existence of extended eigenfunctions. We motivate this framework by applying it to a few well studied cases such as the almost-Mathieu operator (AAH model), as well as more generic non-dual models that challenge standard routines. The technique is flexible and can be used to extract both analytic and numerical results, e.g. we analytically extract a modified phase diagram for Liouville irrationals. As a numerical tool, it does not require the fixing of boundary conditions and circumvents a primary failing of numerical techniques in quasi-periodic systems, extrapolation from finite size. Instead, it uses finite size scaling to define convergence bounds on the full irrational limit.

cond-mat.mes-hall↗

arXiv2021

Topological continuum charges of acoustic phonons in 2D

We analyze the band topology of acoustic phonons in 2D materials by considering the interplay of spatial and internal symmetries with additional constraints that arise from the physical context. These supplemental constraints trace back to the Nambu-Goldstone theorem and the requirements of structural stability. We show that this interplay can give rise to previously unaddressed non-trivial nodal charges that are associated with the crossing of the acoustic phonon branches at the center ($Γ$-point) of the phononic Brillouin zone. We moreover apply our perspective to the concrete context of graphene, where we demonstrate that the phonon spectrum harbors these kinds of non-trivial nodal charges. Apart from its fundamental appeal, this analysis is physically consequential and dictates how the phonon dispersion is affected when graphene is grown on a substrate. Given the generality of our framework, we anticipate that our strategy that thrives on combining physical context with insights from topology should be widely applicable in characterizing systems beyond electronic band theory.

cond-mat.mes-hall↗

arXiv2021

Manipulation and braiding of Weyl nodes using symmetry-constrained phase transitions

Weyl semimetals are arguably the most paradigmatic form of a gapless topological phase. While the stability of Weyl nodes, as quantified by their topological charge, has been extensively investigated, recent interest has shifted to the manipulation of the location of these Weyl nodes for non-Abelian braiding. To accomplish this braiding it is necessary to drive significant Weyl node motion using realistic experimental parameter changes. We show that a family of phase transitions characterized by certain symmetry constraints impose that the Weyl nodes have to reorganise by a large amount, shifting from one high symmetry plane to another. Additionally, for a subset of pairs of nodes with nontrivial Euler class topology, this reorganization can only occur through a braiding process with adjacent nodes. As a result, the Weyl nodes are forced to move a large distance across the Brillouin zone and to braid, all driven by small temperature changes, a process we illustrate with Cd$_2$Re$_2$O$_7$. Our work opens up routes to readily manipulate Weyl nodes using only slight external parameter changes, paving the way for the practical realization of reciprocal space braiding.

cond-mat.mes-hall↗

arXiv2021

Topological correspondence between magnetic space group representations

The past years have seen rapid progress in the classification of topological materials. These diagnostical methods are increasingly getting explored in the pertinent context of magnetic structures. We report on a general class of electronic configurations within a set of anti-ferromagnetic-compatible space groups that are necessarily topological. Interestingly, we find a systematic correspondence between these anti-ferromagnetic phases to necessarily nontrivial topological ferro/ferrimagnetic counterparts that are readily obtained through physically motivated perturbations. Addressing the exhaustive list of magnetic space groups in which this mechanism occurs, we also verify its presence on planes in 3D systems that were deemed trivial in existing classification schemes. This leads to the formulation of the concept of subdimensional topologies, featuring non-triviality within part of the system that coexists with stable Weyl points away from these planes, thereby uncovering novel topological materials in the full 3D sense that have readily observable features in their bulk and surface spectrum.

cond-mat.mes-hall↗

arXiv2021

Bicircular light tuning of magnetic symmetry and topology in Dirac semimetal Cd$_3$As$_2$

We show that Floquet engineering using bicircular light (BCL) is a versatile way to control magnetic symmetries and topology in materials. The electric field of BCL, which is a superposition of two circularly polarized light waves with frequencies that are integer multiples of each other, traces out a rose pattern in the polarization plane that can be chosen to break selective symmetries, including spatial inversion. Using a realistic low-energy model, we theoretically demonstrate that the three-dimensional Dirac semimetal Cd$_3$As$_2$ is a promising platform for BCL Floquet engineering. Without strain, BCL irradiation induces a transition to a non-centrosymmetric magnetic Weyl semimetal phase with tunable energy separation between the Weyl nodes. In the presence of strain, we predict the emergence of a magnetic topological crystalline insulator with exotic unpinned surface Dirac states that are protected by a combination of twofold rotation and time-reversal $(2')$ and can be controlled by light.

cond-mat.mes-hall↗

arXiv2021

Observation of non-Abelian topological semimetals and their phase transitions

Topological phases of matter lie at the heart of physics, connecting elegant mathematical principles to real materials that are believed to shape future electronic and quantum computing technologies. To date, studies in this discipline have almost exclusively been restricted to single-gap band topology because of the Fermi-Dirac filling effect. Here, we theoretically analyze and experimentally confirm a novel class of multi-gap topological phases, which we will refer to as non-Abelian topological semimetals, on kagome geometries. These unprecedented forms of matter depend on the notion of Euler class and frame charges which arise due to non-Abelian charge conversion processes when band nodes of different gaps are braided along each other in momentum space. We identify such exotic phenomena in acoustic metamaterials and uncover a rich topological phase diagram induced by the creation, braiding and recombination of band nodes. Using pump-probe measurements, we verify the non-Abelian charge conversion processes where topological charges of nodes are transferred from one gap to another. Moreover, in such processes, we discover symmetry-enforced intermediate phases featuring triply-degenerate band nodes with unique dispersions that are directly linked to the multi-gap topological invariants. Furthermore, we confirm that edge states can faithfully characterize the multi-gap topological phase diagram. Our study unveils a new regime of topological phases where multi-gap topology and non-Abelian charges of band nodes play a crucial role in understanding semimetals with inter-connected multiple bands.

cond-mat.mes-hall↗

arXiv2021

Topological Descendants of Multicritical EuTl2

The past decades have witnessed a transformation in characterizing condensed matter systems with topology. Aided by a refined understanding of topological band structures with crystalline symmetries that has emerged recently, many electronic phases have been identified and a plethora of materials have been predicted to host novel properties and functionalities. A key underlying question, also with respect to future application, is to what extent the related physical features can be manipulated, especially in the context of magnetic order. Here we describe a paradigmatic semimetal that simultaneously incorporates multiple, and sometimes conflicting topology which guarantees gaplessness and leads to an exceptionally rich family of descendent phases on lowering symmetry. We predict that this multicritical phase is realized in EuTl2. Starting from the parent semimetallic state, which already separates two topological insulating regimes, the interplay of inherent magnetism and strain allows for an exceptionally rich phase diagram of topological descendant states.

cond-mat.mtrl-sci↗

arXiv2021

Non-Abelian reciprocal braiding of Weyl points and its manifestation in $\textrm{ZrTe}$

Weyl semimetals in three-dimensional crystals provide the paradigm example of topologically protected band nodes. It is usually taken for granted that a pair of colliding Weyl points annihilate whenever they carry opposite chiral charge. In a stark contrast, here we report that Weyl points in systems symmetric under the composition of time-reversal with a $π$-rotation are characterized by a non-Abelian topological invariant. The topological charges of the Weyl points are transformed via braid phase factors which arise upon exchange inside symmetric planes of the reciprocal momentum space. We elucidate this process with an elementary two-dimensional tight-binding model implementable in cold-atoms setups and in photonic systems. In three dimensions, interplay of the non-Abelian topology with point-group symmetry is shown to enable topological phase transitions in which pairs of Weyl points may scatter or convert into nodal-line rings. By combining our theoretical arguments with first-principles calculations, we predict that Weyl points occurring near the Fermi level of zirconium telluride ($\textrm{ZrTe}$) carry non-trivial values of the non-Abelian charge, and that uniaxial compression strain drives a non-trivial conversion of the Weyl points into nodal lines.

cond-mat.mes-hall↗