arXiv subjects

Roberto De Renzi

Publications and source records attributed to Roberto De Renzi.

25 records · Page 2Linked to original sources

arXiv2016

Ferromagnetic Quantum Critical Point Avoided by the Appearance of Another Magnetic Phase in LaCrGe$_3$ under Pressure

The temperature-pressure phase diagram of the ferromagnet LaCrGe$_3$ is determined for the first time from a combination of magnetization, muon-spin-rotation and electrical resistivity measurements. The ferromagnetic phase is suppressed near $2.1$~GPa, but quantum criticality is avoided by the appearance of a magnetic phase, likely modulated, AFM$_Q$. Our density functional theory total energy calculations suggest a near degeneracy of antiferromagnetic states with small magnetic wave vectors $Q$ allowing for the potential of an ordering wave vector evolving from $Q=0$ to finite $Q$, as expected from the most recent theories on ferromagnetic quantum criticality. Our findings show that LaCrGe$_3$ is a very simple example to study this scenario of avoided ferromagnetic quantum criticality and will inspire further study on this material and other itinerant ferromagnets.

cond-mat.str-el↗

arXiv2016

Toward the computational prediction of muon sites and interaction parameters

The rapid developments of computational quantum chemistry methods and supercomputing facilities motivate the renewed interest in the analysis of the muon/electron interactions in $μ$SR experiments with \emph{ab initio} approaches. Modern simulation methods seem to be able to provide the answers to the frequently asked questions of many $μ$SR experiments: where is the muon? Is it a passive probe? What are the interaction parameters governing the muon-sample interaction? In this review we describe some of the approaches used to provide quantitative estimations of the aforementioned quantities and we provide the reader with a short discussion on the current developments in this field.

cond-mat.mtrl-sci↗

arXiv2016

First-principles investigation of MnP magnetic states precursors of superconductivity under high pressure

The discovery of a superconducting dome in the proximity of the magnetic to paramagnetic transition in the electronic phase diagram of MnP as a function of hydrostatic pressure has renewed the interest in the magnetic properties of this binary pnictide. Here we present an ab initio study obtained with Density Functional Theory (DFT) simulations as a function of pressure. We show that the itinerant-electron magnetism of MnP is well characterized by the mean-field Kohn-Sham method which correctly describes the ambient pressure magnetic states, the anomalous trend of the lattice parameters as a function of pressure and the critical pressure for the disappearance of the magnetic order. We are finally able to confirm the nature of the new helical structure observed at high pressure.

cond-mat.supr-con↗

arXiv2014

Tuning the magnetic and structural phase transitions of PrFeAsO via Fe/Ru spin dilution

Neutron diffraction and muon spin relaxation measurements are used to obtain a detailed phase diagram of Pr(Fe,Ru)AsO. The isoelectronic substitution of Ru for Fe acts effectively as spin dilution, suppressing both the structural and magnetic phase transitions. The temperature of the tetragonal-orthorhombic structural phase transition decreases gradually as a function of x. Slightly below the transition temperature coherent precessions of the muon spin are observed corresponding to static magnetism, possibly reflecting a significant magneto-elastic coupling in the FeAs layers. Short range order in both the Fe and Pr moments persists for higher levels of x. The static magnetic moments disappear at a concentration coincident with that expected for percolation of the J1-J2 square lattice model.

cond-mat.supr-con↗

arXiv2014

A numerical method to calculate the muon relaxation function in the presence of diffusion

We present an accurate and efficient method to calculate the effect of random fluctuations of the local field at the muon, for instance in the case muon diffusion, within the framework of the strong collision approximation. The method is based on a reformulation of the Markovian process over a discretized time base, leading to a summation equation for the muon polarization function which is solved by discrete Fourier transform. The latter is formally analogous, though not identical, to the integral equation of the original continuous-time model, solved by Laplace transform. With real-case parameter values, the solution of the discrete-time strong collision model is found to approximate the continuous-time solution with excellent accuracy even with a coarse-grained time sampling. Its calculation by the fast Fourier transform algorithm is very efficient and suitable for real time fitting of experimental data even on a slow computer.

cond-mat.other↗

arXiv2012

Effect of external pressure on the magnetic properties of LnFeAsO (Ln = La, Ce, Pr, Sm)

We investigate the effect of external pressure on magnetic order in undoped LnFeAsO (Ln = La, Ce, Pr, La) by using muon-spin relaxation measurements and ab-initio calculations. Both magnetic transition temperature $T_m$ and Fe magnetic moment decrease with external pressure. The effect is observed to be lanthanide dependent with the strongest response for Ln = La and the weakest for Ln = Sm. The trend is qualitatively in agreement with our DFT calculations. The same calculations allow us to assign a value of 0.68(2) $μ_B$ to the Fe moment, obtained from an accurate determination of the muon sites. Our data further show that the magnetic lanthanide order transitions do not follow the simple trend of Fe, possibly as a consequence of the different $f$-electron overlap.

cond-mat.supr-con↗

arXiv2011

Magnetic properties of spin diluted iron pnictides from muSR and NMR in LaFe1-xRuxAsO

The effect of isoelectronic substitutions on the microscopic properties of LaFe1-xRuxAsO, for 0< x< 0.8, has been investigated by means of muSR and 139La NMR. It was found that Ru substitution causes a progressive reduction of the Nèel temperature (T_N) and of the magnetic order parameter without leading to the onset of superconductivity. The temperature dependence of 139La nuclear spin-lattice relaxation rate 1/T_1 can be suitably described within a two-band model. One band giving rise to the spin density wave ground-state, while the other one is characterized by weakly correlated electrons. Fe for Ru substitution yields to a progressive decrease of the density of states at the Fermi level close to the one derived from band structure calculations. The reduction of T_N with doping follows the predictions of the J_1-J_2 model on a square lattice, which appears to be an effective framework to describe the magnetic properties of the spin density wave ground-state.

cond-mat.str-el↗