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Robin Smeyers

Publications and source records attributed to Robin Smeyers.

6 recordsLinked to original sources

Bandwidth-Limited Critical Currents in Electrically Tunable Moir\'e Bands

Moir\'e superlattices host narrow minibands whose bandwidth governs correlated and topological phases. Here, we demonstrate that the bandwidth also sets the critical current for the onset of out-of-equilibrium transport. In bilayer graphene aligned to hexagonal boron nitride, we explore the high-current transport regime as we continuously flatten the valence miniband using an out-of-plane displacement field. We observe a significant reduction in the critical current, which is captured by a minimal analytical model and corresponds to the calculated narrowing of the miniband. Moreover, by comparing distinct moir\'e platforms, we show that the scaling between critical current and bandwidth is a universal feature of graphene superlattices. Our results reveal a direct link between miniband dispersion and high-current transport, and establish this regime as a fast and accessible electrical probe of bandwidth evolution.

cond-mat.mes-hall

Evolution of the Berry curvature dipole in uniaxially strained bilayer graphene

While in pristine bilayer graphene the Berry curvature dipole (BCD), a necessary ingredient for the nonlinear anomalous Hall effect, is zero, uniaxial strain can give rise to finite BCD. We investigate this by using a tight-binding (TB) approach build on the Slater-Koster parameterization to capture lattice deformation effects often missed by continuum models. We demonstrate that the BCD's evolution with strain and doping is highly sensitive to the choice in parameterization, particularly when including the longer range interlayer skew hoppings. Additionally, out-of-plane compression enhances the response by broadening the Dirac cones. These findings benchmark low-energy continuum models and highlight the necessity of realistic tight-binding models for accurately predicting strain-engineered Hall effects in bilayer graphene.

cond-mat.mes-hall

Single-photon detection enabled by negative differential conductivity in moir\'e superlattices

Detecting individual light quanta is essential for quantum information, space exploration, advanced machine vision, and fundamental science. Here, we introduce a novel single photon detection mechanism using highly photosensitive non-equilibrium electron phases in moir\'e materials. Using tunable bands in bilayer graphene/hexagonal-boron nitride superlattices, we engineer negative differential conductance and a sensitive bistable state capable of detecting single photons. Operating in this regime, we demonstrate single-photon counting at mid-infrared (11.3 microns) and visible wavelengths (675 nanometres) and temperatures up to 25 K. This detector offers new prospects for broadband, high-temperature quantum technologies with CMOS compatibility and seamless integration into photonic integrated circuits (PICs). Our analysis suggests the mechanism underlying our device operation originates from negative differential velocity, and represents an important milestone in the field of high-bias transport in two-dimensional moir\'e quantum materials.

cond-mat.mes-hall

Machine-Learning Interatomic Potential for Twisted Hexagonal Boron Nitride: Accurate Structural Relaxation and Emergent Polarization

The emerging ferroelectric properties of two-dimensional (2D) heterostructures are at the forefront of science and prospective technology. In moir\'e bilayers, twisting or heterostructuring causes local atomic reconstruction, which even at picometer scale, can lead to pronounced ferroelectric polarization. Accurately determining this reconstruction utilizing ab initio methods is unfeasible for the relevant system sizes, but modern machine-learning interatomic potentials offer a viable solution. Here, we present the Gaussian Approximation Potential for twisted hexagonal boron nitride (hBN) layers validated against ab initio datasets. This approach enables the precise analysis of their structural properties, which is particularly relevant at small twist angles. We couple the structural information to a tight-binding model based on accurate interatomic positioning, and determine the twist-dependent polarization, yielding results that closely align with previous experimental findings - even at room temperature. This methodology enables further studies that are unattainable otherwise and is transferable to other 2D materials of interest.

cond-mat.mtrl-sci

Elastic Screening of Pseudogauge Fields in Graphene

Lattice deformations in graphene couple to the low-energy electronic degrees of freedom as effective scalar and gauge fields. Using molecular dynamics simulations, we show that the optical component of the displacement field, i.e., the relative motion of different sublattices, contributes at equal order as the acoustic component and effectively screens the pseudogauge fields. In particular, we consider twisted bilayer graphene and corrugated monolayer graphene. In both cases, optical lattice displacements significantly reduce the overall magnitude of the pseudomagnetic fields. For corrugated graphene, optical contributions also reshape the pseudomagnetic field and significantly modify the electronic bands near charge neutrality. Previous studies based on continuum elasticity, which ignores this effect, have therefore systematically overestimated the strength of the strain-induced pseudomagnetic field. Our results have important consequences for the interpretation of experiments and design of straintronic applications.

cond-mat.mes-hall

Strong gate-tunability of flat bands in bilayer graphene due to moiré encapsulation between hBN monolayers

When using hexagonal boron-nitride (hBN) as a substrate for graphene, the resulting moiré pattern creates secondary Dirac points. By encapsulating a multilayer graphene within aligned hBN sheets the controlled moiré stacking may offer even richer benefits. Using advanced tight-binding simulations on atomistically-relaxed heterostructures, here we show that the gap at the secondary Dirac point can be opened in selected moiré-stacking configurations, and is independent of any additional vertical gating of the heterostructure. On the other hand, gating can broadly tune the gap at the principal Dirac point, and may thereby strongly compress the first moiré mini-band in width against the moiré-induced gap at the secondary Dirac point. We reveal that in hBN-encapsulated bilayer graphene this novel mechanism can lead to isolated bands flatter than 10~meV under moderate gating, hence presenting a convenient pathway towards electronically-controlled strongly-correlated states on demand.

cond-mat.mes-hall