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Roderich Moessner

Publications and source records attributed to Roderich Moessner.

At least 145 records · Page 8Linked to original sources

Suppression of inter-band heating for random driving

Heating to high-lying states strongly limits the experimental observation of driving induced non-equilibrium phenomena, particularly when the drive has a broad spectrum. Here we show that, for entire families of structured random drives known as random multipolar drives, particle excitation to higher bands can be well controlled even away from a high-frequency driving regime. This opens a window for observing drive-induced phenomena in a long-lived prethermal regime in the lowest band.

cond-mat.quant-gas

Dirac magnons, nodal lines, and nodal plane in elemental gadolinium

We investigate the magnetic excitations of elemental gadolinium (Gd) using inelastic neutron scattering, showing that Gd is a Dirac magnon material with nodal lines at $K$ and nodal planes at half integer $\ell$. We find an anisotropic intensity winding around the $K$-point Dirac magnon cone, which is interpreted to indicate Berry phase physics. Using linear spin wave theory calculations, we show the nodal lines have non-trivial Berry phases, and topological surface modes. We also discuss the origin of the nodal plane in terms of a screw-axis symmetry, and introduce a topological invariant characterizing its presence and effect on the scattering intensity. Together, these results indicate a highly nontrivial topology, which is generic to hexagonal close packed ferromagnets. We discuss potential implications for other such systems.

cond-mat.str-el

Spin exchange Hamiltonian and topological degeneracies in elemental gadolinium

We present a comprehensive study of the magnetic exchange Hamiltonian of elemental Gadolinium. We use neutron scattering to measure the magnon spectrum over the entire Brillouin zone, and fit the excitations to a spin wave model to extract the first 26 nearest neighbor magnetic exchange interactions with rigorously defined uncertainty. We find these exchange interactions to follow RKKY behavior, oscillating from ferromagnetic to antiferromagnetic as a function of distance. Finally, we discuss the topological features and degeneracies in Gd, and HCP ferromagnets in general. We show theoretically how, with asymmetric exchange, topological properties could be tuned with a magnetic field.

cond-mat.str-el

Order by disorder in classical kagome antiferromagnets with chiral interactions

The Heisenberg antiferromagnet on the kagome lattice is an archetypal instance of how large ground state degeneracies arise, and how they may get resolved by thermal and quantum fluctuations. Augmenting the Heisenberg model by chiral spin interactions has proved to be of particular interest in the discovery of certain chiral quantum spin liquids. Here we consider the classical variant of this chiral kagome model and find that it exhibits, similar to the classical Heisenberg antiferromagnet, a remarkably large and structured ground-state manifold, which combines continuous and discrete degrees of freedom. This allows for a rich set of order-by-disorder phenomena. Degeneracy lifting occurs in a highly selective way, choosing already at the harmonic level specific triaxial states which however retain an emergent $Z_2$ degree of freedom (absent in the conventional Heisenberg model). We also study the competition of entropic and energetic ground state selection as the model interpolates between the purely chiral and Heisenberg cases. For this mixed model, we find a "proximate ordered-by-disorder" finite-temperature regime where fluctuations overcome the energetic ground state preference of the perturbation. Finally, a semiclassical route to a spin liquid is provided by quantum order by disorder in the purely chiral models, where the aforementioned $Z_2$ degrees of freedom are elevated to the role of an emergent gauge field.

cond-mat.str-el

Rabi Regime of Current Rectification in Solids

We investigate rectified currents in response to oscillating electric fields in systems lacking inversion and time-reversal symmetries. These currents, in second-order perturbation theory, are inversely proportional to the relaxation rate, and, therefore, naively diverge in the ideal clean limit. Employing a combination of the non-equilibrium Green function technique and Floquet theory, we show that this is an artifact of perturbation theory, and that there is a well-defined periodic steady-state akin to Rabi oscillations leading to finite rectified currents in the limit of weak coupling to a thermal bath. In this Rabi regime the rectified current scales as the square root of the radiation intensity, in contrast with the linear scaling of the perturbative regime, allowing to readily diagnose it in experiments. More generally, our description provides a smooth interpolation from the ideal Periodic Gibbs Ensemble describing the Rabi oscillations of a closed system to the perturbative regime of rapid relaxation due to strong coupling to a thermal bath.

cond-mat.mes-hall

Many-body physics in the NISQ era: quantum programming a discrete time crystal

Recent progress in the realm of noisy, intermediate scale quantum (NISQ) devices represents an exciting opportunity for many-body physics, by introducing new laboratory platforms with unprecedented control and measurement capabilities. We explore the implications of NISQ platforms for many-body physics in a practical sense: we ask which {\it physical phenomena}, in the domain of quantum statistical mechanics, they may realize more readily than traditional experimental platforms. As a particularly well-suited target, we identify discrete time crystals (DTCs), novel non-equilibrium states of matter that break time translation symmetry. These can only be realized in the intrinsically out-of-equilibrium setting of periodically driven quantum systems stabilized by disorder induced many-body localization. While precursors of the DTC have been observed across a variety of experimental platforms - ranging from trapped ions to nitrogen vacancy centers to NMR crystals - none have \emph{all} the necessary ingredients for realizing a fully-fledged incarnation of this phase, and for detecting its signature long-range \emph{spatiotemporal order}. We show that a new generation of quantum simulators can be programmed to realize the DTC phase and to experimentally detect its dynamical properties, a task requiring extensive capabilities for programmability, initialization and read-out. Specifically, the architecture of Google's Sycamore processor is a remarkably close match for the task at hand. We also discuss the effects of environmental decoherence, and how they can be distinguished from `internal' decoherence coming from closed-system thermalization dynamics. Already with existing technology and noise levels, we find that DTC spatiotemporal order would be observable over hundreds of periods, with parametric improvements to come as the hardware advances.

cond-mat.dis-nn

Quantum percolation of monopole paths and the response of quantum spin ice

We consider quantum spin ice in a temperature regime in which its response is dominated by the coherent motion of a dilute gas of monopoles. The hopping amplitude of a monopole is sensitive to the configuration of its surrounding spins, taken to be quasi-static on the relevant timescales. This leads to well-known blocked directions in the monopole motion; we find that these are sufficient to reduce the coherent propagation of monopoles to quantum diffusion. This result is robust against disorder, as a direct consequence of the ground-state degeneracy, which disrupts the quantum interference processes needed for weak localization. Moreover, recent work [Tomasello et al., Phys. Rev. Lett. 123, 067204 (2019)] has shown that the monopole hopping amplitudes are roughly bimodal: for $\approx 1/3$ of the flippable spins surrounding a monopole, these amplitudes are extremely small. We exploit this structure to construct a theory of quantum monopole motion in spin ice. In the limit where the slow hopping terms are set to zero, the monopole wavefunctions appear to be fractal; we explain this observation via a mapping to quantum percolation on trees. The fractal, non-ergodic nature of monopole wavefunctions manifests itself in the low-frequency behavior of monopole spectral functions, and is consistent with experimental observations.

cond-mat.stat-mech

Topological Route to New and Unusual Coulomb Spin Liquids

Coulomb spin liquids are topological magnetic states obeying an emergent Gauss' law. Little distinction has been made between different kinds of Coulomb liquids. Here we show how a series of distinct Coulomb liquids can be generated straightforwardly by varying the constraints on a classical spin system. This leads to pair creation, and coalescence, of topological defects of an underlying vector field. The latter makes higher-rank spin liquids, of recent interest in the context of fracton theories, with attendant multi-fold pinch points in the structure factor, appear naturally. New Coulomb liquids with an abundance of pinch points also arise. We thus establish a new and general route to uncovering exotic Coulomb liquids, via the manipulation of topological defects in momentum space.

cond-mat.str-el

A comment on "Discrete time crystals: rigidity, criticality, and realizations"

The Letter by N. Y. Yao et. al. [1,2] presents three models for realizing a many-body localized discrete time-crystal (MBL DTC): a short-ranged model [1], its revised version [2], as well as a long-range model of a trapped ion experiment [1,3]. We show that none of these realize an MBL DTC for the parameter ranges quoted in Refs. [1,2]. The central phase diagrams in [1] therefore cannot be reproduced. The models show rapid decay of oscillations from generic initial states, in sharp contrast to the robust period doubling dynamics characteristic of an MBL DTC. Long-lived oscillations from special initial states (such as polarized states) can be understood from the familiar low-temperature physics of a static transverse field Ising model, rather than the nonequilibrium physics of an eigenstate-ordered MBL DTC. Our results on the long-range model also demonstrate, by extension, the absence of an MBL DTC in the trapped ion experiment of Ref. [3].

cond-mat.dis-nn

The Emergent Fine Structure Constant of Quantum Spin Ice Is Large

Condensed matter systems provide alternative `vacua' exhibiting emergent low-energy properties drastically different from those of the standard model. A case in point is the emergent quantum electrodynamics (QED) in the fractionalized topological magnet known as quantum spin ice, whose magnetic monopoles set it apart from the familiar QED of the world we live in. Here, we show that the two greatly differ in their fine-structure constant $α$, which parametrizes how strongly matter couples to light: $α_{\mathrm{QSI}}$ is more than an order of magnitude greater than $α_{\mathrm{QED}} \approx 1/137$. Furthermore, $α_{\mathrm{QSI}}$, the emergent speed of light, and all other parameters of the emergent QED, are tunable by engineering the microscopic Hamiltonian. We find that $α_{\mathrm{QSI}}$ can be tuned all the way from zero up to what is believed to be the \textit{strongest possible} coupling beyond which QED confines. In view of the small size of its constrained Hilbert space, this marks out quantum spin ice as an ideal platform for studying exotic quantum field theories and a target for quantum simulation. The large $α_{\mathrm{QSI}}$ implies that experiments probing candidate condensed-matter realizations of quantum spin ice should expect to observe phenomena arising due to strong interactions.

cond-mat.str-el

Sleuthing out exotic quantum spin liquidity in the pyrochlore magnet Ce$_2$Zr$_2$O$_7$

The search for quantum spin liquids (QSL) -- topological magnets with fractionalized excitations -- has been a central theme in condensed matter and materials physics. While theories are no longer in short supply, tracking down materials has turned out to be remarkably tricky, in large part because of the difficulty to diagnose experimentally a state with only topological, rather than conventional, forms of order. Pyrochlore systems have proven particularly promising, hosting a classical Coulomb phase in the spin ices Dy/Ho$_2$Ti$_2$O$_7$, with subsequent proposals of candidate QSLs in other pyrochlores. Connecting experiment with detailed theory exhibiting a robust QSL has remained a central challenge. Here, focusing on the strongly spin-orbit coupled effective $S=1/2$ pyrochlore Ce$_2$Zr$_2$O$_7$, we analyse recent thermodynamic and neutron scattering experiments, to identify a microscopic effective Hamiltonian through a combination of finite temperature Lanczos, Monte Carlo and analytical spin dynamics calculations. Its parameter values suggest a previously unobserved exotic phase, a $π$-flux U(1) QSL. Intriguingly, the octupolar nature of the moments makes them less prone to be affected by crystal imperfections or magnetic impurities, while also hiding some otherwise characteristic signatures from neutrons, making this QSL arguably more stable than its more conventional counterparts.

cond-mat.str-el

Dynamics and correlations at a quantum phase transition beyond Kibble-Zurek

Kibble-Zurek theory (KZ) stands out as the most robust theory of defect generation in the dynamics of phase transitions. KZ utilizes the structure of equilibrium states away from the transition point to estimate the excitations due to the transition using adiabatic and impulse approximations. Here we show, the actual nonequilibrium dynamics lead to a qualitatively different scenario from KZ, as far correlations between the defects (rather than their densities) are concerned. For a quantum Ising chain, we show, this gives rise to a Gaussian spatial decay in the domain wall (kinks) correlations, while KZ would predict an exponential fall. We propose a simple but general framework on top of KZ, based on the "quantum coarsening" dynamics of local correlators in the supposed impulse regime. We outline how our picture extends to generic interacting situations.

cond-mat.str-el

Anomalous magnetic noise in imperfect flat bands in the topological magnet Dy2Ti2O7

The spin ice compound Dy_2Ti_2O_7 stands out as the first topological magnet in three dimensions, with its tell-tale emergent fractionalized magnetic monopole excitations. Its real-time dynamical properties have been an enigma from the very beginning. Using ultrasensitive, non-invasive SQUID measurements, we show that Dy_2Ti_2O_7 exhibits a highly anomalous noise spectrum, in three qualitatively different regimes: equilibrium spin ice, a `frozen' regime extending to ultra-low temperatures, as well as a high-temperature `anomalous' paramagnet. We show that in the simplest model of spin ice, the dynamics is not anomalous, and we present several distinct mechanisms which give rise to a coloured noise spectrum. In addition, we identify the structure of the single-ion dynamics as a crucial ingredient for any modelling. Thus, the dynamics of spin ice Dy_2Ti_2O_7 reflects the interplay of local dynamics with emergent topological degrees of freedom and a frustration-generated imperfectly flat energy landscape, and as such should be relevant for a broad class of magnetic materials.

cond-mat.str-el

From hard spheres to hard-core spins

A system of hard spheres exhibits physics that is controlled only by their density. This comes about because the interaction energy is either infinite or zero, so all allowed configurations have exactly the same energy. The low density phase is liquid, while the high density phase is crystalline, an example of "order by disorder" as it is driven purely by entropic considerations. Here we study a family of hard spin models, which we call hardcore spin models, where we replace the translational degrees of freedom of hard spheres with the orientational degrees of freedom of lattice spins. Their hardcore interaction serves analogously to divide configurations of the many spin system into allowed and disallowed sectors. We present detailed results on the square lattice in $d=2$ for a set of models with $\mathbb{Z}_n$ symmetry, which generalize Potts models, and their $U(1)$ limits, for ferromagnetic and antiferromagnetic senses of the interaction, which we refer to as exclusion and inclusion models. As the exclusion/inclusion angles are varied, we find a Kosterlitz-Thouless phase transition between a disordered phase and an ordered phase with quasi-long-ranged order, which is the form order by disorder takes in these systems. These results follow from a set of height representations, an ergodic cluster algorithm, and transfer matrix calculations.

cond-mat.stat-mech

Fractonic plaquette-dimer liquid beyond renormalization

We consider close-packed tiling models of geometric objects -- a mixture of hardcore dimers and plaquettes -- as a generalisation of the familiar dimer models. Specifically, on an anisotropic cubic lattice, we demand that each site be covered by either a dimer on a z-link or a plaquette in the x-y plane. The space of such fully packed tilings has an extensive degeneracy. This maps onto a fracton-type `higher-rank electrostatics', which can exhibit a plaquette-dimer liquid and an ordered phase. We analyse this theory in detail, using height representations and T-duality to demonstrate that the concomitant phase transition occurs due to the proliferation of dipoles formed by defect pairs. The resultant critical theory can be considered as a fracton version of the Kosterlitz-Thouless transition. A significant new element is its UV-IR mixing, where the low energy behavior of the liquid phase and the transition out of it is dominated by local (short-wavelength) fluctuations, rendering the critical phenomenon beyond the renormalization group paradigm.

cond-mat.str-el

Interacting spin-3/2 fermions in a Luttinger semimetal: Competing phases and their selection in the global phase diagram

We compute the effects of electronic interactions on gapless spin-3/2 excitations that in a noninteracting system emerge at a bi-quadratic touching of Kramers degenerate valence and conduction bands, known as Luttinger semimetal. This model can describe the low-energy physics of HgTe, gray-Sn, 227 pyrochlore iridates and half-Heuslers. For the sake of concreteness we only consider the short-range components of the Coulomb interaction. By combining mean-field analysis with a renormalization group (RG) calculation, we construct multiple cuts of the global phase diagram of interacting spin-3/2 fermions at zero and finite temperature and chemical doping. Such phase diagrams display a rich confluence of competing orders, among which rotational symmetry breaking nematic insulators and time reversal symmetry breaking magnetic orders are the prominent excitonic phases. We also show that even repulsive interactions can be conducive for both s-wave and d-wave pairings. The reconstructed band structure inside the ordered phases allows us to organize them according to the energy (entropy) gain in the following (reverse) order: s-wave pairing, nematic phases, magnetic orders and d-wave pairings, at zero chemical doping. But, the paired states are always energetically superior over the excitonic ones for finite doping. The phase diagrams obtained from the RG analysis show that an ordered phase with higher energy (entropy) gain is realized at low (high) temperature. In addition, we establish a "selection rule" between the interaction channels and the resulting ordered phases, suggesting that repulsive interactions in the magnetic (nematic) channels are conducive for the nucleation of d-wave (s-wave) pairing. The proposed methodology can shed light on the global phase diagram of other strongly interacting multi-band systems, such as doped Dirac semimetal, topological insulators and the like.

cond-mat.str-el

Super-resonant transport of topological surface states subjected to in-plane magnetic fields

Magnetic oscillations of Dirac surface states of topological insulators are expected to be associated with the formation of Landau levels or the Aharonov-Bohm effect. We instead study the conductance of Dirac surface states subjected to an in-plane magnetic field in presence of a barrier potential. Strikingly, we find that, in the case of large barrier potentials, the surface states exhibit pronounced oscillations in the conductance when varying the magnetic field, in the \textit{absence} of Landau levels or the Aharonov-Bohm effect. These novel magnetic oscillations are attributed to the emergence of \textit{super-resonant regimes} by tuning the magnetic field, in which almost all propagating electrons cross the barrier with perfect transmission. In the case of small and moderate barrier potentials, we also identify a positive magnetoconductance which is due to the increase of the Fermi surface by tilting the surface Dirac cone. Moreover, we show that for weak magnetic fields, the conductance displays a shifted sinusoidal dependence on the field direction with period $π$ and phase shift determined by the tilting direction with respect to the field direction. Our predictions can be applied to many topological insulators, such as HgTe and Bi$_{2}$Se$_{3}$, and provide important insights into exploring and understanding exotic magnetotransport properties of topological surface states.

cond-mat.mes-hall

Possible inversion symmetry breaking in the $S=1/2$ pyrochlore Heisenberg magnet

We address the ground-state properties of the long-standing and much-studied three-dimensional quantum spin liquid candidate, the $S=\frac 1 2$ pyrochlore Heisenberg antiferromagnet. By using $SU(2)$ density-matrix renormalization group (DMRG), we are able to access cluster sizes of up to 128 spins. Our most striking finding is a robust spontaneous inversion symmetry breaking, reflected in an energy density difference between the two sublattices of tetrahedra, familiar as a starting point of earlier perturbative treatments. We also determine the ground-state energy, $E_0/N_\text{sites} = -0.490(6) J$, by combining extrapolations of DMRG with those of a numerical linked cluster expansion. These findings suggest a scenario in which a finite-temperature spin liquid regime gives way to a symmetry-broken state at low temperatures.

cond-mat.str-el