arXiv subjects

Rodolfo A. Jalabert

Publications and source records attributed to Rodolfo A. Jalabert.

At least 19 recordsLinked to original sources

arXiv2026

Non-local effects in charge and energy transport with dissipative electrodes

Recent advances in nano-thermometry motivate the extension of the Landauer-Büttiker scattering theory as to include the non-local dissipation associated with charge transport. Such a program is implemented by describing the inelastic scattering in the connecting electrodes within an electrostatically self-consistent scheme. The restriction to quasi-one-dimensional geometries, weak excitation and low temperature allows to obtain general expressions of the current density and the dissipated power, valid in different regimes, for the cases of an energy-independent mean-free-path or an energy-independent relaxation-rate. In particular, the dissipation asymmetry at both sides of a nano-device and the conditions for observing heating spots with a local maximum of the dissipated power are formulated in terms of the key parameters that define the nano-device and its environment.

cond-mat.mes-hall↗

arXiv2024

Going beyond Landauer scattering theory to describe spatially-resolved non-local heating and cooling in quantum thermoelectrics

Spatially-resolved heating and cooling in nanostructures is nowadays measured with various nanoscale thermometry techniques, including scanning thermometry. Yet the most commonly used theory of nanoscale heating and thermoelectricity -- Landauer scattering theory -- is not appropriate to model such measurements. Hence, we analyze a minimal model of spatially-resolved heat transfer between electrons and phonons in simple thermoelectric nanostructures. This combines Landauer scattering formalism with a Boltzmann equation for transport, revealing the non-locality of Joule heating and Peltier cooling induced by a scatterer in a nanowire. The corresponding heating or cooling of the phonons is caused by the voltage drop at the scatterer, but is often maximal at a certain distance from the scatterer. This distance is of the order of the electron-phonon scattering length. Scanning thermal microscopy, such as SQUID-on-tip thermometers, should detect this non-locality as phonon hot spots and cold spots, spatially separated from the scatterer. We provide physical arguments explaining the thermoelectric response of the combined system of wire and scatterer, and in particular, why the resulting heating and cooling is sometimes the opposite to that predicted by the standard Landauer scattering theory.

cond-mat.mes-hall↗

arXiv2023

Scanning gate microscopy in graphene nanostructures

The conductance of graphene nanoribbons and nanoconstrictions under the effect of a scanning gate microscopy tip is systematically studied. Using a scattering approach for noninvasive probes, the first- and second-order conductance corrections caused by the tip potential disturbance are expressed explicitly in terms of the scattering states of the unperturbed structure. Numerical calculations confirm the perturbative results, showing that the second-order term prevails in the conductance plateaus, exhibiting a universal scaling law for armchair graphene strips. For stronger tips, at specific probe potential widths and strengths beyond the perturbative regime, the conductance corrections reveal the appearance of resonances originated from states trapped below the tip. The zero-transverse-energy mode of an armchair metallic strip is shown to be insensitive to the long-range electrostatic potential of the probe. For nanoconstrictions defined on a strip, scanning gate microscopy allows to get insight into the breakdown of conductance quantization. The first-order correction generically dominates at low tip strength, while for Fermi energies associated with faint conductance plateaus, the second-order correction becomes dominant for relatively small potential tip strengths. In accordance with the spatial dependence of the partial local density of states, the largest tip effect occurs in the central part of the constriction, close to the edges. Nanoribbons and nanoconstrictions with zigzag edges exhibit a similar response as in the case of armchair nanostructures, except when the intervalley coupling induced by the tip potential destroys the chiral edge states.

cond-mat.mes-hall↗

arXiv2022

Out-of-time-order correlators and quantum chaos

Quantum Chaos has originally emerged as the field which studies how the properties of classical chaotic systems arise in their quantum counterparts. The growing interest in quantum many-body systems, with no obvious classical meaning has led to consider time-dependent quantities that can help to characterize and redefine Quantum Chaos. This article reviews the prominent role that the out of time ordered correlator (OTOC) plays to achieve such goal.

quant-ph↗

arXiv2022

Asymmetric power dissipation in electronic transport through a quantum point contact

We investigate the power dissipated by an electronic current flowing through a quantum point contact in a two-dimensional electron gas. Based on the Landauer-Büttiker approach to quantum transport, we evaluate the power that is dissipated on the two sides of the constriction as a function of the Fermi energy, temperature, and applied voltage. We demonstrate that an asymmetry appears in the dissipation, which is most pronounced when the quantum point contact is tuned to a conductance step where the transmission strongly depends on energy. At low temperatures, the asymmetry is enhanced when the temperature increases. An estimation for the position of the maximum dissipation is provided.

cond-mat.mes-hall↗

arXiv2022

Spontaneous orbital magnetization of mesoscopic dipole dimers

Ensembles of gold nanoparticles present a magnetic behavior which is at odds with the weakly diamagnetic response of bulk gold. In particular, an unusual ferromagnetic order has been unveiled by several experiments. Here we investigate if the combined effect of orbital magnetism of conduction electrons and interparticle dipolar interaction can lead to magnetic ordering. Using different model systems of interacting mesoscopic magnetic dipoles, together with a microscopic description of the electron dynamics within the nanoparticles, we find that a spontaneous magnetic moment may arise in dimers of metallic nanoparticles when the latter are characterized by a large orbital paramagnetic susceptibility.

cond-mat.mes-hall↗

arXiv2022

Magnetic response of metallic nanoparticles: Geometric and weakly relativistic effects

While the large paramagnetic response measured in certain ensembles of metallic nanoparticles has been assigned to orbital effects of conduction electrons, the spin-orbit coupling has been pointed out as a possible origin of the anomalously large diamagnetic response observed in other cases. Such a relativistic effect, arising from the inhomogeneous electrostatic potential seen by the conduction electrons, might originate from the host ionic lattice, impurities, or the self-consistent confining potential. Here we theoretically investigate the effect of the spin-orbit coupling arising from the confining potential, quantifying its contribution to the zero-field magnetic susceptibility and gauging it against the ones generated by other weakly-relativistic corrections. Two ideal geometries are considered in detail, the sphere and the half-sphere, focusing on the expected increased role of the spin-orbit coupling upon a symmetry reduction, and the application of these results to actual metallic nanoparticles is discussed. The matrix elements of the different weakly-relativistic corrections are obtained and incorporated in a perturbative treatment of the magnetic field, leading to tractable semi-analytical and semiclassical expressions for the case of the sphere, while a numerical treatment becomes necessary for the half-sphere. The correction to the zero-field susceptibility arising from the spin-orbit coupling in a single sphere is quite small, and it is dominated by the weakly-relativistic kinetic energy correction, which in turn remains considerably smaller than the typical values of the nonrelativistic zero-field susceptibility. Moreover, the spin-orbit contribution to the average response for ensembles of nanoparticles with a large size dispersion is shown to vanish. The symmetry reduction in going from the single sphere to the half-sphere does not translate into a significant (...)

cond-mat.mes-hall↗

arXiv2021

Signatures of folded branches in the scanning gate microscopy of ballistic electronic cavities

We demonstrate the emergence of classical features in electronic quantum transport for the scanning gate microscopy response in a cavity defined by a quantum point contact and a micron-sized circular reflector. The branches in electronic flow characteristic of a quantum point contact opening on a two-dimensional electron gas with weak disorder are folded by the reflector, yielding a complex spatial pattern. Considering the deflection of classical trajectories by the scanning gate tip allows to establish simple relationships of the scanning pattern, which are in agreement with recent experimental findings.

cond-mat.mes-hall↗

arXiv2020

Signatures of quantum chaos transition in short spin chains

The non-integrability of quantum systems, often associated with chaotic behavior, is a concept typically applied to cases with a high-dimensional Hilbert space Among different indicators signaling this behavior, the study of the long-time oscillations of the out-of-time-ordered correlator (OTOC) appears as a versatile tool, that can be adapted to the case of systems with a small number of degrees of freedom. Using such an approach, we consider the oscillations observed after the scrambling time in the measurement of OTOCs of local operators for an Ising spin chain on a nuclear magnetic resonance quantum simulator [J. Li,et al, Phys. Rev. X 7, 031011 (2017)]. We show that the systematic of the OTOC oscillations describes qualitatively well, in a chain with only 4 spins, the integrability-to-chaos transition inherited from the infinite chain.

quant-ph↗

arXiv2019

Energy Stability of Branching in the Scanning Gate Response of Two-Dimensional Electron Gases with Smooth Disorder

The branched pattern typically observed through the scanning gate microscopy (SGM) of two dimensional electron gases in the presence of weak, smooth disorder has recently been found to be robust against a very large shift in the Fermi energy of the electron gas. We propose a toy model, where the potential landscape reduces to a single localized feature, that makes it possible to recast the understanding of branch formation through the effect of caustics in an appropriate set of classical trajectories, and it is simple enough to allow for a quantitative analysis of the energy and spatial dependence of the branches. We find the energy stability to be extremely generic, as it rests only upon the assumptions of weak disorder, weak scattering, and the proportionality of the SGM response to the density of classical electron trajectories. Therefore, the robustness against changes of the electron's Fermi energy remains when adopting progressively realistic models of smooth disorder.

cond-mat.mes-hall↗

arXiv2019

Gauging classical and quantum integrability through out-of-time ordered correlators

Out-of-time-order correlators (OTOCs) have been proposed as a probe of chaos in quantum mechanics, on the basis of their short-time exponential growth found in some particular set-ups. However, it has been seen that this behavior is not universal. Therefore, we query other quantum chaos manifestations arising from the OTOCs and we thus study their long-time behavior in systems of completely different nature: quantum maps, which are the simplest chaotic one-body system and spin chains, which are many-body systems without a classical limit. It is shown that studying the long-time regime of the OTOCs it is possible to detect and gauge the transition between integrability and chaos, and we benchmark the transition with other indicators of quantum chaos based on the spectra and the eigenstates of the systems considered. For systems with classical analogue, we show that the proposed OTOC indicators have a very high accuracy that allow to detect subtle features along the integrability-to-chaos transition.

quant-ph↗

arXiv2019

Semiclassical theory of out-of-time-order correlators for low-dimensional classically chaotic systems

The out-of-time-order correlator (OTOC), recently analyzed in several physical contexts, is studied for low-dimensional chaotic systems through semiclassical expansions and numerical simulations. The semiclassical expansion for the OTOC yields a leading-order contribution in $\hbar^2$ that is exponentially increasing with time within an intermediate, temperature-dependent, time-window. The growth-rate in such a regime is governed by the Lyapunov exponent of the underlying classical system and scales with the square-root of the temperature.

quant-ph↗

arXiv2018

Chaos signatures in the short and long time behavior of the out-of-time ordered correlator

Two properties are needed for a classical system to be chaotic: exponential stretching and mixing. Recently, out-of-time order correlators were proposed as a measure of chaos in a wide range of physical systems. While most of the attention has previously been devoted to the short time stretching aspect of chaos, characterized by the Lyapunov exponent, we show for quantum maps that the out-of-time correlator approaches its stationary value exponentially with a rate determined by the Ruelle-Pollicot resonances. This property constitutes clear evidence of the dual role of the underlying classical chaos dictating the behavior of the correlator at different timescales.

quant-ph↗

arXiv2018

Orbital magnetism in ensembles of gold nanoparticles

The last two decades have witnessed various experiments reporting very unusual magnetic properties of ensembles of gold nanoparticles surrounded by organic ligands, including ferromagnetic, paramagnetic, or (large) diamagnetic responses. These behaviors are at odds with the small diamagnetic response of macroscopic gold samples. Here we theoretically investigate the possibility that the observed unusual magnetism in capped gold nanoparticles is of orbital origin. Employing semiclassical techniques, we calculate the orbital component to the zero-field susceptibility of individual as well as ensembles of metallic nanoparticles. While the result for the orbital response of individual nanoparticles can exceed by orders of magnitude the bulk Landau susceptibility in absolute value, and can be either diamagnetic or paramagnetic depending on nanoparticle size, we show that the magnetic susceptibility of a noninteracting ensemble of nanoparticles with a smooth size distribution is always paramagnetic at low magnetic fields. In particular, we predict that the zero-field susceptibility follows a Curie-type law for small nanoparticle sizes and/or low temperatures. The calculated field-dependent magnetization of an ensemble of diluted nanoparticles is shown to be in good agreement with existing experiments that yielded a large paramagnetic response. The width of the size distribution of the nanoparticles is identified as a key element for the quantitative determination of the orbital response.

cond-mat.mes-hall↗

arXiv2017

Partial local density of states from scanning gate microscopy

Scanning gate microscopy images from measurements made in the vicinity of quantum point contacts were originally interpreted in terms of current flow. Some recent work has analytically connected the local density of states to conductance changes in cases of perfect transmission, and at least qualitatively for a broader range of circumstances. In the present paper, we show analytically that in any time-reversal invariant system there are important deviations that are highly sensitive to imperfect transmission. Nevertheless, the unperturbed partial local density of states can be extracted from a weakly invasive scanning gate microscopy experiment, provided the quantum point contact is tuned anywhere on a conductance plateau. A perturbative treatment in the reflection coefficient shows just how sensitive this correspondence is to the departure from the quantized conductance value and reveals the necessity of local averaging over the tip position. It is also shown that the quality of the extracted partial local density of states decreases with increasing tip radius.

cond-mat.mes-hall↗

arXiv2017

Correlation between peak-height modulation and phase-lapses in transport through quantum dots

We show that two intriguing features of mesoscopic transport, namely the modulation of Coulomb blockade peak-heights and the transmission phase-lapses occurring between subsequent peaks, are closely related. Our analytic arguments are corroborated by numerical simulations for chaotic ballistic quantum dots. The correlations between the two properties are experimentally testable. The statistical distribution of the partial-width amplitude, at the heart of the previous relationship, is determined, and its characteristic parameters are estimated from simple models.

cond-mat.mes-hall↗

arXiv2017

Spin-relaxation time in the impurity band of wurtzite semiconductors

The spin-relaxation time for electrons in the impurity band of semiconductors with wurtzite crystal structure is determined. The effective Dresselhaus spin-orbit interaction Hamiltonian is taken as the source of the spin relaxation at low temperature and for doping densities corresponding to the metallic side of the metal-insulator transition. The spin-flip hopping matrix elements between impurity states are calculated and used to set up a tight-binding Hamiltonian that incorporates the symmetries of wurtzite semiconductors. The spin-relaxation time is obtained from a semiclassical model of spin diffusion, as well as from a microscopic self-consistent diagrammatic theory of spin and charge diffusion in doped semiconductors. Estimates are provided for particularly important materials. The theoretical spin-relaxation times compare favorably with the corresponding low-temperature measurements in GaN and ZnO. For InN and AlN, we predict that tuning of the spin-orbit coupling constant induced by an external potential leads to a potentially dramatic increase of the spin-relaxation time related to the mechanism under study.

cond-mat.mes-hall↗

arXiv2017

Classical origin of conductance oscillations in an integrable cavity

Scanning gate microscopy measurements in a circular ballistic cavity with a tip placed near its center yield a non-monotonic dependence of the conductance on the tip voltage. Detailed numerical quantum calculations reproduce these conductance oscillations, and a classical scheme leads to its physical understanding. The large-amplitude conductance oscillations are shown to be of classical origin, and well described by the effect of a particular class of short trajectories.

cond-mat.mes-hall↗