Rodolfo Gallardo | Searcharxiv

arXiv2026

Chiral molecule-induced contributions to ferromagnetic resonance

Despite extensive research on chirality-driven spin selectivity, most studies have focused on static magnetic properties, while the influence of chirality on the dynamic magnetic response remains largely unexplored. Here, we investigate how chiral molecular interfaces affect magnetization dynamics in thin Co/Ni multilayers with perpendicular magnetic anisotropy using broadband ferromagnetic resonance spectroscopy. A comparison between bare (reference) films and molecule-functionalized (hybrid) samples reveals no measurable changes in either the resonance field or the linewidth that could be attributed to the presence of the chiral environment. Motivated by our findings we develop a macrospin description that distinguishes equilibrium modifications of the magnetic free-energy landscape (MIPAC-type effects) from non-equilibrium, CISS-induced spin torques. Our analysis shows that equilibrium modifications primarily shift the resonance condition via changes to the free energy landscape and thereby the effective field, whereas damping-like non-equilibrium torques provide a distinct channel for varying the effective damping rate. This approach establishes clear criteria for disentangling chiral-interface-induced energy modifications from torque-driven dynamical effects in ferromagnetic resonance experiments.

cond-mat.mtrl-sci↗

arXiv2022

Finite-element dynamic-matrix approach for propagating spin waves: Extension to mono- and multilayers of arbitrary spacing and thickness

In our recent work [AIP Adv. 11, 095006], we presented an efficient numerical method to compute dispersions and spatial mode profiles of spin waves propagating in waveguides with translationally invariant equilibrium magnetization. Using a finite-element method (FEM) allowed to model two-dimensional waveguide cross sections of arbitrary shape but only finite size. Here, we extend our FEM propagating-wave dynamic-matrix approach from finite waveguides to the important practical cases of infinitely-extended mono- and multilayers of arbitrary spacing and thickness. To obtain the mode profiles and frequencies, the linearized equation of motion of magnetization is solved as an eigenvalue problem only on a one-dimensional line-trace mesh, defined along the normal direction of the layers. Being an important contribution in multilayer systems, we introduce interlayer-exchange interaction into our FEM approach. With the calculation of dynamic dipolar fields being the main focus of this paper, we also extend the previously presented plane-wave Fredkin-Koehler method to calculate the dipolar potential of spin waves in infinite layers. The major benefit of this method is that it avoids the discretization of any non-magnetic material, such as non-magnetic spacers in multilayers. Therefore, the computational effort becomes completely independent on the spacer thicknesses. Furthermore, it keeps the resulting discretized eigenvalue problem sparse, which therefore, inherits a comparably low arithmetic complexity. As a validation of our method (implemented into the open-source finite-element micromagnetic package TetraX), we present results for various systems and compare them with theoretical predictions as well as with established finite-difference numerical methods. We believe this method offers an efficient and versatile tool to calculate spin-wave dispersions in layered magnetic systems.

cond-mat.mes-hall↗