arXiv subjects

Rodrigo A. Muniz

Publications and source records attributed to Rodrigo A. Muniz.

At least 19 recordsLinked to original sources

arXiv2019

Quantum Interference Control of Localized Carrier Distributions in the Brillouin Zone

Using transition-metal dichalcogenides as an example, we show that the quantum interference arising in two- and three-photon absorption processes can lead to controllable, highly localized carrier distributions in the Brillouin zone. We contrast this with the previously studied one- and two-photon absorption, and find qualitatively different features, including changes in the relevance of interband and intraband processes according to the excitation energy. Thus, the distribution of excitations arising under certain circumstances in two- and three-photon absorption can facilitate the study of far-from-equilibrium states that are initially well localized in crystal momentum space.

cond-mat.mes-hall↗

arXiv2019

Microscopic polarization and magnetization fields in extended systems

We introduce microscopic polarization and magnetization fields at each site of an extended system, as well as free charge and current density fields associated with charge movement from site to site, by employing a lattice gauge approach based on a set of orthogonal orbitals associated with each site. These microscopic fields are defined using a single-particle electron Green function, and the equations governing its evolution under excitation by an electromagnetic field at arbitrary frequency involve the electric and magnetic fields rather than the scalar and vector potentials. If the sites are taken to be far from each other, we recover the limit of isolated atoms. For an infinite crystal we choose the orbitals to be maximally-localized Wannier functions, and in the long wavelength limit we recover the expected linear response of an insulator, including the zero frequency transverse conductivity of a topologically nontrivial insulator. For a topologically trivial insulator we recover the expected expressions for the macroscopic polarization and magnetization in the ground state, and find that the linear response to excitation at arbitrary frequency is described solely by the microscopic polarization and magnetization fields. For very general optical response calculations the microscopic fields necessarily satisfy charge conservation, even under basis truncation, and do not suffer from the false divergences at zero frequency that can plague response calculations using other approaches.

cond-mat.mes-hall↗

arXiv2019

Quantum Interference Control of Carriers and Currents in Zincblende Semiconductors based on Nonlinear Absorption Processes

Quantum interference between optical absorption processes can excite carriers with a polarized distribution in the Brillouin zone depending on properties of the incident optical fields. The polarized distribution of carriers introduces a current that can be controlled by the phases and polarizations of the incident optical fields. Here we study the quantum interference of 2- and 3-photon absorption processes in AlGaAs. We present theoretical predictions for carrier and current injection rates considering different frequencies, phases, and polarizations of the incident fields. We also discuss the important features that result from only nonlinear optical processes being involved, which leads for instance to a sharper distribution of carriers in the Brillouin zone.

cond-mat.mtrl-sci↗

arXiv2019

Quantum Interference Control of Photocurrents in Semiconductors by Nonlinear Optical Absorption Processes

We report experiments demonstrating Quantum Interference Control (QuIC) based on two nonlinear optical absorption processes in semiconductors. We use two optical beams of frequencies $ω$ and $3ω/2$ incident on AlGaAs and measure the injection current due to the interference between 2- and 3-photon absorption processes. We analyze the dependence of the injection current on the intensities and phases of the incident fields.

cond-mat.mes-hall↗

arXiv2018

Jerk current: A novel bulk photovoltaic effect

We investigate a physical divergence of the third order polarization susceptibility representing a photoinduced current in biased crystalline insulators. This current grows quadratically with illumination time in the absence of momentum relaxation and saturation; we refer to it as the \textit{jerk current}. Two contributions to the current are identified. The first is a hydrodynamic acceleration of optically injected carriers by the static electric field, and the second is the change in the carrier injection rate in the presence of the static electric field. The jerk current can have a component perpendicular to the static field, a feature not captured by standard hydrodynamic descriptions of carriers in electric fields. We suggest an experiment to detect the jerk current and some of its interesting features.

cond-mat.mes-hall↗

arXiv2018

The optical properties of dibenzoterrylene

Dibenzoterrylene (DBT) has garnered interest as a potential single photon source (SPS). To have a better grasp of any possible limitations of using DBT for this application, a better understanding of its optical properties is needed. We use a configuration interaction (CI) strategy to calculate the many body wavefunctions of DBT, and we use these wavefunctions to calculate its optical properties. We calculate the linear absorption spectrum and the spatial distributions of electrons involved in several bright transitions. We also calculate the two-photon absorption spectrum of DBT and show that there are several excited states that are bright due to two-photon absorption. Except at high photon energies, we predict that there are no competing optical processes regarding the use of DBT as a SPS. Our calculations provide details of the optical properties of DBT that are interesting in general, and useful for considering optical applications of DBT.

cond-mat.mtrl-sci↗

arXiv2017

The role of impurities on the optical properties of rectangular graphene flakes

We study rectangular graphene flakes using mean field states as the basis for a configuration interaction calculation, which allows us to analyze the low lying electronic excited states including electron correlations beyond the mean field level. We find that the lowest energy transition is polarized along the long axis of the flake, but the charge distributions involved in these transitions are invariably localized on the zigzag edges. We also investigate the impact of both short and long range impurity potentials on the optical properties of these systems. We predict that even a weak impurity localized at a zigzag edge of the flake can have a significant -- and often dramatic -- effect on its optical properties. This is in contrast to impurities localized at armchair edges or central regions of the flake, for which we predict almost no change to the optical properties of the flake even with strong impurity potentials.

cond-mat.mtrl-sci↗

arXiv2017

An effective model for the electronic and optical properties of stanene

The existence of several 2D materials with heavy atoms in their composition has been recently demonstrated. The electronic and optical properties of these materials can be accurately computed with numerically intensive density functional theory methods. However, it is desirable to have simple effective models that can accurately describe these properties at low energies. Here we present an effective model for stanene that is reliable for electronic and optical properties for photon energies up to 1.1 eV. For this material, we find that a quadratic model with respect to the lattice momentum is the best suited for calculations based on the bandstructure, even with respect to band warping. We also find that splitting the two spin-z subsectors is a good approximation, which indicates that the lattice buckling can be neglected in calculations based on the bandstructure. We illustrate the applicability of the model by computing the linear optical injection rates of carrier and spin densities in stanene. Our calculations indicate that an incident circularly polarized optical field only excites electrons with spin that matches its helicity.

cond-mat.mtrl-sci↗

arXiv2017

A Green function method to study thin diffraction gratings

The anomalous features in diffraction patterns first observed by Wood over a century ago have been the subject of many investigations, both experimental and theoretical. The sharp, narrow structures - and the large resonances with which they are sometimes associated - arise in numerous studies in optics and photonics. In this paper we present an analytical method to study diffracted fields of optically thin gratings that highlights the nonanalyticities associated with the anomalies. Using this approach we can immediately derive diffracted fields for any polarization in a compact notation. While our equations are approximate, they fully respect energy conservation in the electromagnetic field, and describe the large exchanges of energy between incident and diffracted fields that can arise even for thin gratings.

physics.optics↗

arXiv2016

Strong and Anisotropic Third Harmonic Generation in Monolayer and Multilayer ReS$_2$

We report observation of strong and anisotropic third harmonic generation (THG) in monolayer and multilayer ReS$_2$. The third-order nonlinear optical susceptibility of monolayer ReS$_2$, $\left| χ^{(3)} \right|$ is on the order of $10^{-18} $ m$^2$/V$^2$, which is about one order of magnitude higher than reported results for hexagonal-lattice transition metal dichalcogenides such as MoS$_2$. A similar magnitude for the third-order nonlinear optical susceptibility was also obtained for a multilayer sample. The intensity of the THG field was found to be dependent on the direction of the incident light polarization for both monolayer and multilayer samples. A point group symmetry analysis shows that such anisotropy is not expected from a perfect $1T$ lattice, and must arise from the distortions in the ReS$_2$ lattice. Our results show that THG measurements can be used to characterize lattice distortions of two-dimensional materials, and that lattice distortions are important for the nonlinear optical properties of such materials.

cond-mat.mtrl-sci↗

arXiv2016

Photocurrents in Bi2Se3: bulk versus surface, and injection versus shift currents

Optical injection and detection of charge currents can complement conventional transport and photoemission measurements without the necessity of invasive contact that may disturb the system being examined. This is a particular concern for the surface states of a topological insulator. In this work one- and two-color sources of photocurrents are examined in epitaxial, thin films of Bi2Se3. We demonstrate that optical excitation and terahertz detection simultaneously captures one- and two- color photocurrent contributions, as previously not required in other material systems. A method is devised to isolate the two components, and in doing so each can be related to surface or bulk excitations through symmetry. This strategy allows surface states to be examined in a model system, where they have independently been verified with angle-resolved photoemission spectroscopy.

physics.optics↗

arXiv2014

All-optical injection of charge, spin and valley currents in monolayer transition metal dichalcogenides

Monolayer transition metal dichalcogenides have recently become a playground for spin- and valleytronics research. Their low energy spectrum can be described by Dirac cones on the corners of Brillouin zone, but the physical properties are richer than those of graphene since the spin degeneracy is lifted and the optical selection rules are valley dependent. This has been exploited for the optical injection of spin and valley polarized currents by the application of static electric fields. In this paper we consider an all-optical method for the injection of charge, spin and valley polarized currents. The presence of both a fundamental optical field and its second harmonic can lead to the injection of currents due to a nonlinear effect involving the quantum interference between one- and two-photon absorption processes. We analyze how the injected quantities can be controlled through the parameters of the incident light fields, allowing capabilities of control beyond those achieved with static fields, and discuss the conditions for experimental verification of our results.

cond-mat.mes-hall↗

arXiv2014

Coherent control of optical injection of spin and currents in topological insulators

Topological insulators have surface states with a remarkable helical spin structure, with promising prospects for applications in spintronics. Strategies for generating spin polarized currents, such as the use of magnetic contacts and photoinjection, have been the focus of extensive research. While several optical methods for injecting currents have been explored, they have all focused on one-photon absorption. Here we consider the use of both a fundamental optical field and its second harmonic, which allows the injection of spin polarized carriers and current by a nonlinear process involving quantum interference between one- and two-photon absorption. General expressions are derived for the injection rates in a generic two-band system, including those for one- and two-photon absorption processes as well as their interference. Results are given for carrier, spin density and current injection rates on the surface of topological insulators, for both linearly and circularly polarized light. We identify the conditions that would be necessary for experimentally verifying these predictions.

cond-mat.mes-hall↗

arXiv2013

Low-energy theory of a two-dimensional itinerant chiral magnet

Effective actions, such as nonlinear sigma models, are important tools in studying low-energy fluctuations of magnetically ordered states. Here we derive an effective action for the smooth order-parameter distortions of noncoplanar magnetic textures [with an SO(3) order parameter, as opposed to the SO(3)/SO(2)=S^2 of collinear magnets] coupled to itinerant electrons. Noncoplanar magnetic textures commonly arise in the presence of electron-mediated long-range spin exchange interactions, giving rise to the emergence of rich electronic phenomena such as anomalous quantum Hall effect. We parameterize the smooth order-parameter distortions of such a magnetic texture by certain non-Abelian fields, and derive the action in terms of these fields by integrating out the itinerant electrons. As a concrete example, we perform explicit calculations for a triangular-lattice model with tetrahedral magnetic ordering. The action encodes the charge and spin quantum-Hall responses as well as the energetics of twisting the magnetic texture.

cond-mat.str-el↗

arXiv2013

Generalized spin-wave theory: application to the bilinear-biquadratic model

We present a generalized spin-wave theory (GSWT) for treating spin Hamiltonians of arbitrary spin $S$. The generalization consists of an extension of the traditional spin-wave theory from SU(2) to SU($N$). Low energy excitations are waves of the local order parameter that fluctuates in the SU($N$) space of unitary transformations of the local spin states, instead of the SU(2) space of local spin rotations. Since the generators of the SU($N$) group can be represented as bilinear forms in $N$-flavored bosons, the low-energy modes of the GSWT are described with $N-1$ different bosons. The generalization allows treating quantum spin systems whose ground state exhibit multipolar ordering as well as detecting instabilities of magnetically ordered states (dipolar ordering) towards higher multipolar orderings. We illustrate these advantages by applying the GSWT to a bilinear-biquadratic model of arbitrary spin $S$ on hypercubic lattices.

cond-mat.str-el↗

arXiv2013

Anyons in integer quantum Hall magnets

Strongly correlated fractional quantum Hall liquids support fractional excitations, which can be understood in terms of adiabatic flux insertion arguments. A second route to fractionalization is through the coupling of weakly interacting electrons to topologically nontrivial backgrounds such as in polyacetylene. Here we demonstrate that electronic fractionalization combining features of both these mechanisms occurs in noncoplanar itinerant magnetic systems, where integer quantum Hall physics arises from the coupling of electrons to the magnetic background. The topologically stable magnetic vortices in such systems carry fractional (in general irrational) electronic quantum numbers and exhibit Abelian anyonic statistics. We analyze the properties of these topological defects by mapping the distortions of the magnetic texture onto effective non-Abelian vector potentials. We support our analytical results with extensive numerical calculations.

cond-mat.str-el↗

arXiv2012

Fractionalization in spontaneous integer quantum Hall systems

It is widely believed that integer quantum Hall systems do not have fractional excitations. Here we show the converse to be true for a class of systems where integer quantum Hall effect emerges spontaneously due to the interplay of itinerant electrons and noncoplanar magnetic ordering. We show that magnetic $Z_2$ vortices in such systems, whose topological stability is guaranteed by the structure of the order parameter, indeed carry fractional charge.

cond-mat.str-el↗

arXiv2011

Visualization of nano-plasmons in graphene

We study localized plasmons at the nanoscale (nano-plasmons) in graphene. The collective excitations of induced charge density modulations in graphene are drastically changed in the vicinity of a single impurity compared to graphene's bulk behavior. The dispersion of nano-plasmons depends on the number of electrons and the sign, strength and size of the impurity potential. Due to this rich parameter space the calculated dispersions are intrinsically multidimensional requiring an advanced visualization tool for their efficient analysis, which can be achieved with parallel rendering. To overcome the problem of analyzing thousands of very complex spatial patterns of nano-plasmonic modes, we take a combined visual and quantitative approach to investigate the excitations on the two-dimensional graphene lattice. Our visual and quantitative analysis shows that impurities trigger the formation of localized plasmonic excitations of various symmetries. We visually identify dipolar, quadrupolar and radial modes, and quantify the spatial distributions of induced charges.

cond-mat.mtrl-sci↗