Searcharxiv⌕ Search

arXiv subjects

Rodrigo Soto

Publications and source records attributed to Rodrigo Soto.

At least 55 records · Page 3Linked to original sources
arXiv2018

Universality of active wetting transitions

Four on-lattice and six off-lattice models for active matter are studied numerically, showing that in contact with a wall, they display universal wetting transitions between three distinctive phases. The particles, which interact via exclusion volume only, move persistently and, depending on the model, change their direction either via tumble processes or rotational diffusion. When increasing the turning rate $ν_T$, the systems transit from total wetting, to partial wetting and dewetted phases. In the first phase, a wetting film covers the wall, with increasing heights while decreasing $ν_T$. The second phase is characterized by wetting droplets on the walls. And, finally, the walls dries with few particles in contact with it. These phases present two continuous non-equilibrium transitions. For the first transition, from partial to total wetting, the fraction of dry sites vanishes continuously when decreasing $ν_T$, with a power law of exponent 1. And, for the second transition, an order parameter proportional to the excess mass in droplets decreases continuously with a power law of exponent 3 when approaching a critical value of $ν_T$. The critical exponents are the same for all the models studied.

cond-mat.stat-mech↗
arXiv2018

Effective two-dimensional model for granular matter with phase separation

Granular systems confined in vertically vibrated shallow horizontal boxes (quasi two-dimensional geometry) present a liquid to solid phase transition when the frequency of the periodic forcing is increased. An effective model, where grains move and collide in two-dimensions is presented, which reproduces the aforementioned phase transition. The key element is that besides the two-dimensional degrees of freedom, each grain has an additional variable $ε$ that accounts for the kinetic energy stored in the vertical motion in the real quasi two-dimensional motion. This energy grows monotonically during free flight, mimicking the energy gain by collisions with the vibrating walls and, at collisions, this energy is instantaneously transferred to the horizontal degrees of freedom. As a result, the average values of $ε$ and the kinetic temperature are decreasing functions of the local density, giving rise to an effective pressure that can present van der Waals loops. A kinetic theory approach predicts the conditions that must satisfy the energy grow function to obtain the phase separation, which are verified with molecular dynamics simulations. Notably, the effective equation of state and the critical points computed considering the velocity--time-of-flight correlations differ only slightly from those obtained by simple kinetic theory calculations that neglect those correlations.

cond-mat.stat-mech↗
arXiv2018

Critical Phenomena in Quasi-Two-Dimensional Vibrated Granular Systems

The critical phenomena associated to the liquid to solid transition of quasi-two-dimensional vibrated granular systems is studied using molecular dynamics simulations of the inelastic hard sphere model. The critical properties are associated to the fourfold bond-orientational order parameter $χ_4$, which measures the level of square crystallization of the system. Previous experimental results have shown that the transition of $χ_4$, when varying the vibration amplitude, can be either discontinuous or continuous, for two different values of the height of the box. Exploring the amplitude-height phase space, a transition line is found, which can be either discontinuous or continuous, merging at a tricritical point and the continuous branch ends in an upper critical point. In the continuous transition branch, the critical properties are studied. The exponent associated to the amplitude of the order parameter is $β=1/2$, for various system sizes, in complete agreement with the experimental results. However, the fluctuations of $χ_4$ do not show any critical behavior, probably due to crossover effects by the close presence of the tricritical point. Finally, in quasi-one-dimensional systems, the transition is only discontinuous, limited by one critical point, indicating that two is the lower dimension for having a tricritical point.

cond-mat.soft↗
arXiv2017

Wetting Transitions Displayed by Persistent Active Particles

A lattice model for active matter is studied numerically, showing that it displays wettings transitions between three distinctive phases when in contact with an impenetrable wall. The particles in the model move persistently, tumbling with a small rate $α$, and interact via exclusion volume only. When increasing the tumbling rates $α$, the system transits from total wetting to partial wetting and unwetting phases. In the first phase, a wetting film covers the wall, with increasing heights when $α$ is reduced. The second phase is characterized by wetting droplets on the wall with a periodic spacing between them. Finally, the wall dries with few particles in contact with it. These phases present nonequilibrium transitions. The first transition, from partial to total wetting, is continuous and the fraction of dry sites vanishes continuously when decreasing the tumbling rate $α$. For the second transition, from partial wetting to dry, the mean droplet distance diverges logarithmically when approaching the critical tumbling rate, with saturation due to finite-size effects.

cond-mat.soft↗
arXiv2017

GPU parallel simulation algorithm of Brownian particles with excluded volume using Delaunay triangulations

A novel parallel simulation algorithm on the GPU, implemented in CUDA and C++, is presented for the simulation of Brownian particles that display excluded volume repulsion and interact with long and short range forces. When an explicit Euler-Maruyama integration step is performed to take into account the pairwise forces and Brownian motion, particle overlaps can appear. The excluded volume property brings up the need for correcting these overlaps as they happen, since predicting them is not feasible due to the random displacement of Brownian particles. The proposed solution handles, at each time step, a Delaunay triangulation of the particle positions because it allows us to efficiently solve overlaps between particles by checking just their neighborhood. The algorithm starts by generating a Delaunay triangulation of the particle initial positions on CPU, but after that the triangulation is always kept on GPU memory. We used a parallel edge-flip implementation to keep the triangulation updated during each time step, checking previously that the triangulation was not rendered invalid due to the particle displacements. The algorithm is validated with two models of active colloidal particles. Upon testing the parallel implementation of a long range forces simulation, the results show a performance improvement of up to two orders of magnitude when compared to the previously existing sequential solution.

cs.DC↗
arXiv2016

Coarsening and clustering in run-and-tumble dynamics with short-range exclusion

The emergence of clustering and coarsening in crowded ensembles of self-propelled agents is studied using a lattice model in one-dimension. The persistent exclusion process, where particles move at directions that change randomly at a low tumble rate $α$, is extended allowing sites to be occupied by more than one particle, with a maximum $n_\text{max}$ per site. Three phases are distinguished. For $n_\text{max}=1$ a gas of clusters form, with sizes distributed exponentially and no coarsening takes place. For $n_\text{max}\geq 3$ and small values of $α$, coarsening takes place and few large clusters appear, with a large fraction of the total number of particles in them. In the same range of $n_\text{max}$ but for larger values of $α$, a gas phase where a negligible fraction of particles takes part of clusters. Finally, $n_\text{max}=2$ corresponds to a crossover phase. The character of the transitions between phases is studied extending the model to allow $n_\text{max}$ to take real values and jumps to an occupied site are probabilistic. The transition from the gas of clusters to the coarsening phase is continuous and the mass of the large clusters grows continuously when varying the maximum occupancy, and the crossover found corresponds to values close to the transition. The second transition, from the coarsening to the gaseous phase can be either continuous or discontinuous depending on the parameters, with a critical point separating both cases.

cond-mat.stat-mech↗
arXiv2016

Effect of the vibration profile on shallow granular systems

We describe the collective behavior of a system of many inelastic spherical particles inside a box which is being periodically vibrated. The box is shallow, with large horizontal dimensions, while the height is less than two particle diameters. The vibrations are not symmetric: the time the box is moving up is, in general, different to the time it is moving down. The limit cycles of isolated grains are largely affected by the asymmetry of the vibration mode, increasing the size in phase space of the chaotic regions. When many grains are placed in the box, the phase separation between dense, solid-like regions, coexisting with fluid-like regions takes place at smaller global densities for asymmetric vibration profiles. Besides, the order parameter of the transition takes larger values when asymmetric forcing is used.

cond-mat.soft↗
arXiv2016

Dynamics of noncohesive confined granular media

Despite the ubiquitousness and technological and scientific importance of granular matter, our understanding is still very poor compared to molecular fluids and solids. Until today, there is no unified description, which indeed seems unreachable. However, it has been proposed that important advances could be attained for noncohesive, hard-sphere like systems, by combining fluid dynamics with phase-field modeling through an appropriate order parameter (Aranson and Tsimring, 2006). Here, we present a review of the dynamics of confined granular matter, for which this systematic approach has proven its value. Motivated by the pioneering work of Olafsen and Urbach (1998), many experimental, theoretical and numerical studies of model confined granular systems have been realized, which have unveiled a very large variety of fundamental phenomena. In this review, we focus on few of these fundamental aspects, namely phase coexistence, effective surface tension, and a detailed description of the liquid state.

cond-mat.soft↗
arXiv2015

Self-assembly of Active Colloidal Molecules with Dynamic Function

Catalytically active colloids maintain non-equilibrium conditions in which they produce and deplete chemicals and hence effectively act as sources and sinks of molecules. While individual colloids that are symmetrically coated do not exhibit any form of dynamical activity, the concentration fields resulting from their chemical activity decay as $1/r$ and produce gradients that attract or repel other colloids depending on their surface chemistry and ambient variables. This results in a non-equilibrium analogue of ionic systems, but with the remarkable novel feature of action-reaction symmetry breaking. We study solutions of such chemically active colloids in dilute conditions when they join up to form molecules via generalized ionic bonds, and discuss how we can achieve structures with time dependent functionality. In particular, we study a molecule that adopts a spontaneous oscillatory pattern of conformations, and another that exhibits a run-and-tumble dynamics similar to bacteria. Our study shows that catalytically active colloids could be used for designing self-assembled structures that posses dynamical functionalities that are determined by their prescribed 3D structures, a strategy that follows the design principle of proteins.

cond-mat.soft↗
arXiv2015

Universality and criticality of a second-order granular solid-liquid-like phase transition

We experimentally study the critical properties of the non-equilibrium solid-liquid-like transition that takes place in vibrated granular matter. The critical dynamics is characterized by the coupling of the density field with the bond-orientational order parameter $Q_4$, which measures the degree of local crystallization. Two setups are compared, which present the transition at different critical accelerations as a a result of modifying the energy dissipation parameters. In both setups five independent critical exponents are measured, associated to different properties of $Q_4$: the correlation length, relaxation time, vanishing wavenumber limit (static susceptibility), the hydrodynamic regime of the pair correlation function, and the amplitude of the order parameter. The respective critical exponents agree in both setups and are given by $ν_{\perp} = 1$, $ν_{\parallel} = 2$, $γ= 1$, $η\approx 0.6 - 0.67$, and $β=1/2$, whereas the dynamical critical exponent is $z = ν_{\parallel}/ν_{\perp} = 2$. The agreement on five exponents is an exigent test for the universality of the transition. Thus, while dissipation is strictly necessary to form the crystal, the path the system undergoes towards the phase separation is part of a well defined universality class. In fact, the local order shows critical properties while density does not. Being the later conserved, the appropriate model that couples both is model C in the Hohenberg and Halperin classification. The measured exponents are in accord with the non-equilibrium extension to model C if we assume that $α$, the exponent associated in equilibrium to the specific heat divergence but with no counterpart in this non-equilibrium experiment, vanishes.

cond-mat.stat-mech↗
arXiv2014

Shear viscosity of a model for confined granular media

The shear viscosity in the dilute regime of a model for confined granular matter is studied by simulations and kinetic theory. The model consists on projecting into two dimensions the motion of vibrofluidized granular matter in shallow boxes by modifying the collision rule: besides the restitution coefficient that accounts for the energy dissipation, there is a separation velocity that is added in each collision in the normal direction. The two mechanisms balance on average, producing stationary homogeneous states. Molecular dynamics simulations show that in the steady state the distribution function departs from a Maxwellian, with cumulants that remain small in the whole range of inelasticities. The shear viscosity normalized with stationary temperature presents a clear dependence with the inelasticity, taking smaller values compared to the elastic case. A Boltzmann-like equation is built and analyzed using linear response theory. It is found that the predictions show an excellent agreement with the simulations when the correct stationary distribution is used but a Maxwellian approximation fails in predicting the inelasticity dependence of the viscosity. These results confirm that transport coefficients depend strongly on the mechanisms that drive them to stationary states.

cond-mat.stat-mech↗
arXiv2014

Dynamics of a first order transition to an absorbing state

A granular system confined in a quasi two-dimensional box that is vertically vibrated can transit to an absorbing state in which all particles bounce vertically in phase with the box, with no horizontal motion. In principle, this state can be reached for any density lower than the one corresponding to one complete monolayer, which is then the critical density. Below this critical value, the transition to the absorbing state is of first order, with long metastable periods, followed by rapid transitions driven by homogeneous nucleation. Molecular dynamics simulations and experiments show that there is a dramatic increase on the metastable times far below the critical density; in practice, it is impossible to observe spontaneous transitions close to the critical density. This peculiar feature is a consequence of the non-equilibrium nature of this first order transition to the absorbing state. A Ginzburg-Landau model, with multiplicative noise, describes qualitatively the observed phenomena and explains the macroscopic size of the critical nuclei. The nuclei become of small size only close to a second critical point where the active phase becomes unstable via a saddle node bifurcation. It is only close to this second critical point that experiments and simulations can evidence spontaneous transitions to the absorbing state while the metastable times grow dramatically moving away from it.

cond-mat.stat-mech↗
arXiv2014

Self-assembly of catalytically active colloidal molecules: Tailoring activity through surface chemistry

A heterogeneous and dilute suspension of catalytically active colloids is studied as a non-equilibrium analogue of ionic systems, which has the remarkable feature of action-reaction symmetry breaking. Symmetrically coated colloids are found to join up to form self-assembled molecules that could be inert or have spontaneous activity in the form of net translational velocity and spin depending on their symmetry properties and their constituents. The type of activity can be adjusted by changing the surface chemistry and ambient variables that control the surface reactions and the phoretic drift.

cond-mat.soft↗
arXiv2013

Run-and-tumble in a crowded environment: persistent exclusion process for swimmers

The effect of crowding on the run-and-tumble dynamics of swimmers such as bacteria is studied using a discrete lattice model of mutually excluding particles that move with constant velocity along a direction that is randomized at a rate $α$. In stationary state, the system is found to break into dense clusters in which particles are trapped or stopped from moving. The characteristic size of these clusters predominantly scales as $α^{-0.5}$ both in 1D and 2D. For a range of densities, due to cooperative effects, the stopping time scales as ${\cal T}_{1d}^{0.85}$ and as ${\cal T}_{2d}^{0.8}$, where ${\cal T}_d$ is the diffusive time associated with the motion of cluster boundaries. Our findings might be helpful in understanding the early stages of biofilm formation.

cond-mat.soft↗
arXiv2013

Capillary-like Fluctuations of a Solid-Liquid Interface in a Non-Cohesive Granular System

One of the most noticeable collective motion of non-cohesive granular matter is clustering under certain conditions. In particular, when a quasi-two-dimensional monolayer of mono-disperse non-cohesive particles is vertically vibrated, a solid-liquid-like transition occurs when the driving amplitude exceeds a critical value. Here, the physical mechanism underlying particle clustering relies on the strong interactions mediated by grain collisions, rather than on grain-grain cohesive forces. In average, the solid cluster resembles a drop, with a striking circular shape. We experimentally investigate the coarse-grained solid-liquid interface fluctuations, which are characterized through the static and dynamic correlation functions in the Fourier space. These fluctuations turn out to be well described by the capillary wave theory, which allows us to measure the solid-liquid interface surface tension and mobility once the granular "thermal" kinetic energy is determined. Despite the system is strongly out of equilibrium and that the granular temperature is not uniform, there is energy equipartition at the solid-liquid interface, for a relatively large range of angular wave-numbers. Furthermore, both surface tension and mobility are consistent with a simple order of magnitude estimation considering the characteristic energy, length and time scales, which is very similar to what can be done for atomic systems. Please find the supplementary material of this article here: arXiv:1304.2646

cond-mat.soft↗
arXiv2013

Hydrodynamic modes in a confined granular fluid

Confined granular fluids, placed in a shallow box that is vibrated vertically, can achieve homogeneous stationary states thanks to energy injection mechanisms that take place throughout the system. These states can be stable even at high densities and inelasticities allowing for a detailed analysis of the hydrodynamic modes that govern the dynamics of granular fluids. Analyzing the decay of the time correlation functions it is shown that there is a crossover between a quasielastic regime in which energy evolves as a slow mode, to a inelastic regime, with energy slaved to the other conserved fields. The two regimes have well differentiated transport properties and, in the inelastic regime, the dynamics can be described by a reduced hydrodynamics with modified longitudinal viscosity and sound speed. The crossover between the two regimes takes place at a wavevector that is proportional to the inelasticity. A two dimensional granular model, with collisions that mimic the energy transfers that take place in a confined system is studied by means of microscopic simulations. The results show excellent agreement with the theoretical framework and allows the validation of hydrodynamic-like models.

cond-mat.soft↗
arXiv2012

Stochastic resonance on the transverse displacement of swimmers in an oscillatory shear flow

Self-propelled microorganisms, such as unicellular algae or bacteria, swim along their director relative to the fluid velocity. Under a steady shear flow the director rotates in close orbit, a periodic structure that is preserved under an oscillatory shear flow. If the shear flow is subjected to small fluctuations produced by small irregularities in the microchannel or by other swimmers nearby, the director dynamics becomes stochastic. Numerical integration of the swimmer motion shows that there is stochastic resonance: The displacement in the vorticity direction is maximized for a finite noise intensity. This transverse displacement resonance is observed when the displacement is coarse grained over several periods, although the director is preferentially oriented along the flow. The resonant noise intensity is proportional to the oscillation frequency and independent of the shear rate. The enhanced displacement can have effects on the transverse diffusion of swimmers and the rheology of the suspension.

cond-mat.soft↗