arXiv subjects

Rogério de Sousa

Publications and source records attributed to Rogério de Sousa.

16 recordsLinked to original sources

arXiv2026

Scattering-Induced Loss in Ferroelectric Photonic Devices

Ferroelectric materials have colossal optical nonlinearities, but their integration into quantum photonic chips is made challenging by the additional loss mechanisms that they introduce. Here we present a perturbative theory that expresses non-absorptive (elastic) photon scattering-induced loss as a functional of a general spectral density for spatial fluctuations of electric permittivity. We apply the theory to calculations of attenuation coefficients $α$ in slab waveguides in order to compare two distinct loss mechanisms: Interface roughness and ferroelectric domain disorder. Our theory can account for realistic roughness without special symmetry considerations, and it demonstrates how to use electron microscopy images of ferroelectric domains to obtain explicit numerical predictions for $α$. Loss is maximum when the mean domain length is comparable to the wavelength of light (Mie regime), indicating that, for telecom wavelengths, sub-micron domains (Rayleigh regime) or single domain waveguides provide equivalent strategies for reducing loss.

physics.optics↗

arXiv2026

Anisotropic magnon transport in an antiferromagnetic trilayer heterostructure: is BiFeO$_3$ an altermagnet?

Magnons provide a route to ultra-fast transport and non-destructive readout of spin-based information transfer. Here, we report magnon transport and its emergent anisotropic nature in BiFeO$_3$ layers confined between ultrathin layers of the antiferromagnet LaFeO$_3$. Due to the confined state, BiFeO$_3$ serves as an efficient magnon transmission channel as well as a magnetoelectric knob by which to control the stack by means of an electric field. We discuss the mechanism of the anisotropic spin transport based on the interaction between the antiferromagnetic order and the electric field. This allows us to manipulate and amplify the spin transport in such a confined geometry. Furthermore, lower crystal symmetric and suppression of the spin cycloid in ultrathin BiFeO$_3$ stabilizes a non-trivial antiferromagnetic state exhibiting symmetry-protected spin-split bands that provide the non-trivial sign inversion of the spin current, which is a characteristic of an altermagnet. This work provides an understanding of the anisotropic spin transport in complex antiferromagnetic heterostructures where ferroelectricity and altermagnetism coexist, paving the way for a new route to realize electric-field control of a novel state of magnetism.

cond-mat.mes-hall↗

arXiv2025

Nonequilibrium Quasiparticles in Superconducting Circuits: Energy Relaxation, Charge and Flux Noise

The quasiparticle density observed in low-temperature superconducting circuits is several orders of magnitude larger than the value expected at thermal equilibrium. The tunneling of this excess of quasiparticles across Josephson junctions is recognized as one of the main loss and decoherence mechanisms in superconducting qubits. Here, we present a unified impedance theory that accounts for quasiparticle energy loss in circuit regions both far and near (across) junctions. Our theory leverages the recent experimental demonstration that the excess quasiparticles are in \emph{quasiequilibrium} [T. Connolly et al., Phys. Rev. Lett. $\textbf{132}$, 217001 (2024)] and uses a generalized fluctuation-dissipation theorem to predict the amount of charge and flux noise generated by them. We compute the resulting energy relaxation time $T_1$ in transmon qubits with and without junction asymmetric gap engineering, and show that quasiparticles residing away from junctions can play a dominant role in the former case. They also may provide an upper limit for resonator quality factors if the density of amorphous two-level systems is reduced. In addition, we show that charge noise from quasiparticles leads to flux noise that is logarithmic-in-frequency, giving rise to a ``nearly white" contribution that is comparable to the flux noise observed in flux qubits. This contrasts with amorphous two-level systems, whose associated flux noise is shown to be superOhmic. We discuss how this quasiparticle flux noise can limit $T_2^{*}$ coherence times in flux-tunable qubits. The conclusion is that asymmetric gap engineering can greatly reduce noise and increase coherence times in superconducting qubits.

quant-ph↗

arXiv2024

Resonant squeezed light from photonic Cooper pairs

Raman scattering of photons into phonons gives rise to entangled photon pairs when the phonon emitted in a Stokes process is coherently absorbed in antiStokes scattering, forming the photonic analog of Cooper pairs. We present a nonperturbative theory for the time evolution of photonic Cooper pairs that treats interacting photons and phonons as a hybrid excitation, the Ramaniton. As the Ramaniton propagates in a wave guide it displays quantum oscillations between photon and phonon occupation, leading to resonant squeezed Stokes-antiStokes light when the phonon occupation becomes equal to zero without recurring back to the photon vacuum. This phenomenon is predicted to generate up to 28 dB of squeezed light even in standard silicon on insulator waveguides.

quant-ph↗

arXiv2023

Model for 1/f Flux noise in Superconducting Aluminum Devices: Impact of External Magnetic Fields

Superconducting quantum interference devices (SQUIDs) and related circuits made of aluminum are known to display $1/ω$ flux noise, where $ω$ is frequency. A recent experiment showed that the application of an external magnetic field in the $10-100$~G range changed the noise to a single Lorentzian peaked at $ω=0$. Here it is shown that a model based on independent impurity spin flips with coexisting cross and direct mechanisms of spin relaxation may explain these experiments. The model shows that application of an external magnetic field can be used to reduce the impact of flux noise in qubits.

quant-ph↗

arXiv2023

Fast quantum gate design with deep reinforcement learning using real-time feedback on readout signals

The design of high-fidelity quantum gates is difficult because it requires the optimization of two competing effects, namely maximizing gate speed and minimizing leakage out of the qubit subspace. We propose a deep reinforcement learning algorithm that uses two agents to address the speed and leakage challenges simultaneously. The first agent constructs the qubit in-phase control pulse using a policy learned from rewards that compensate short gate times. The rewards are obtained at intermediate time steps throughout the construction of a full-length pulse, allowing the agent to explore the landscape of shorter pulses. The second agent determines an out-of-phase pulse to target leakage. Both agents are trained on real-time data from noisy hardware, thus providing model-free gate design that adapts to unpredictable hardware noise. To reduce the effect of measurement classification errors, the agents are trained directly on the readout signal from probing the qubit. We present proof-of-concept experiments by designing X and square root of X gates of various durations on IBM hardware. After just 200 training iterations, our algorithm is able to construct novel control pulses up to two times faster than the default IBM gates, while matching their performance in terms of state fidelity and leakage rate. As the length of our custom control pulses increases, they begin to outperform the default gates. Improvements to the speed and fidelity of gate operations open the way for higher circuit depth in quantum simulation, quantum chemistry and other algorithms on near-term and future quantum devices.

quant-ph↗

arXiv2022

Flux noise in disordered spin systems

Impurity spins randomly distributed at the surfaces and interfaces of superconducting wires are known to cause flux noise in Superconducting Quantum Interference Devices, providing a mechanism for decoherence in superconducting qubits. While flux noise is well characterised experimentally, the microscopic model underlying spin dynamics remains unknown. First-principles theories are too computationally expensive to capture spin diffusion over large length scales, third-principles approaches lump spin dynamics into a single phenomenological spin-diffusion operator that is not able to describe the quantum noise regime and connect to microscopic models and disorder scenarios. Here we propose an intermediate "second principles" method to describe general spin dissipation and flux noise in the quantum regime. It leads to the interpretation that flux noise arises from the density of paramagnon excitations at the edge of the wire, with paramagnon-paramagnon interactions leading to spin diffusion, and interactions between paramagnons and other degrees of freedom leading to spin energy relaxation. At high frequency we obtain an upper bound for flux noise, showing that the (super)Ohmic noise observed in experiments does not originate from interacting spin impurities. We apply the method to Heisenberg models in two dimensional square lattices with random distribution of vacancies and nearest-neighbour spins coupled by constant exchange. Numerical calculations of flux noise show that it follows the observed power law $A/ω^α$, with amplitude $A$ and exponent $α$ depending on temperature and inhomogeneities. These results are compared to experiments in niobium and aluminium devices. The method establishes a connection between flux noise experiments and microscopic Hamiltonians identifying relevant microscopic mechanisms and guiding strategies for reducing flux noise.

quant-ph↗

arXiv2021

Confined Magnons

Magnetic structures are known to possess magnon excitations confined to their surfaces and interfaces, but these spatially localized modes are often not resolved in spectroscopy experiments. We develop a theory to calculate the confined magnon spectra and its associated spin scattering function, which is the physical observable in neutron and electron scattering, and a proxy for photon spectroscopy based on X-ray, Raman and THz sources. We show that extra anisotropy at the surface or interface plays a key role in magnon confinement. We obtain analytical expressions for the confinement length scale, and show that it is qualitatively similar for ferromagnets and antiferromagnets in dimension d>=2. For d=1 we find remarkable differences between ferromagnetic and antiferromagnetic models. The theory indicates the presence of several confined magnon resonances in addition to the usual magnons thought to explain the excitations of magnetic nanostructures. Detecting these modes may elucidate the impact of the interface on spin anisotropy and magnetic order.

cond-mat.mtrl-sci↗

arXiv2021

Benchmarking Hamiltonian Noise in the D-Wave Quantum Annealer

Various sources of noise limit the performance of quantum computers by altering qubit states in an uncontrolled manner throughout computations and reducing their coherence time. In quantum annealers, this noise introduces additional fluctuations to the parameters defining the original problem Hamiltonian, such that they find the ground states of problems perturbed from those originally programmed. Here we describe a method to benchmark the amount of noise affecting the programmed Hamiltonian of a quantum annealer. We show that a sequence of degenerate runs with the coefficients of the programmed Hamiltonian set to zero leads to an estimate of the noise spectral density affecting Hamiltonian parameters "in situ" during the quantum annealing protocol. The method is demonstrated in D-Wave's lower noise 2000 qubit device (DW_2000Q_6) and in its recently released 5000 qubit device (Advantage_system1.1). Our benchmarking of DW_2000Q_6 shows Hamiltonian noise dominated by the $1/f^{0.7}$ frequency dependence characteristic of flux noise intrinsic to the materials forming flux qubits. In contrast, Advantage_system1.1 is found to be affected by additional noise sources for low annealing times, with underlying intrinsic flux noise amplitudes $2-3$ times higher than in DW_2000Q_6 for all annealing times.

quant-ph↗

arXiv2020

Intrinsic Photon Loss at the Interface of Superconducting Devices

We present a quantum theory of dielectric energy loss arising from the piezoelectric coupling between photons and phonons in superconducting devices. Photon loss is shown to occur predominantly at the interface, where the piezoelectric effect is non-zero even when the materials are perfectly crystalline (epitaxial) and free of two-level system defects. We present explicit numerical calculations for the value of the intrinsic loss tangent at several interfaces to conclude that the $T_1$ of superconducting qubits may reach $10^{4}$ $μ$s if the device is made with defect-free interfaces.

quant-ph↗

arXiv2020

Noise Mitigation with Delay Pulses in the IBM Quantum Experience

One of the greatest challenges for current quantum computing hardware is how to obtain reliable results from noisy devices. A recent paper [A. Kandala et al., Nature 567, 491 (2019)] described a method for injecting noise by stretching gate times, enabling the calculation of quantum expectation values as a function of the amount of noise in the IBM-Q devices. Extrapolating to zero noise led to excellent agreement with exact results. Here an alternative scheme is described that employs the intentional addition of identity pulses, pausing the device periodically in order to gradually subject the quantum computation to increased levels of noise. The scheme is implemented in a one qubit circuit on an IBM-Q device. It is determined that this is an effective method for controlled addition of noise, and further, that using noisy results to perform extrapolation can lead to improvements in the final output, provided careful attention is paid to how the extrapolation is carried out.

quant-ph↗

arXiv2020

Impact of the surface phase transition on magnon and phonon excitations in BiFeO3 nanoparticles

We have performed Raman scattering measurements on BiFeO3 nanoparticles and studied both magnetic and lattice modes. We reveal strong anomalies between 140 K and 200 K in the frequency of magnon and E(LO1), E(TO1) and A1(LO1) phonon modes. These anomalies are related to a surface expansion and are enhanced for nanoparticle sizes approaching the spin cycloidal length. These observations point out the strong interplay between the surface, the lattice, and the magnetism for sizes of BiFeO3 nanoparticles close to the cycloid periodicity.

cond-mat.str-el↗

arXiv2019

Size-dependent bistability in multiferroic nanoparticles

Most multiferroic materials with coexisting ferroelectric and magnetic order exhibit cycloidal antiferromagnetism with wavelength of several nanometers. The prototypical example is bismuth ferrite (BiFeO$_3$ or BFO), a room-temperature multiferroic considered for a number of technological applications. While most applications require small sizes such as nanoparticles, little is known about the state of these materials when their sizes are comparable to the cycloid wavelength. This work describes a microscopic theory of cycloidal magnetism in nanoparticles based on Hamiltonian calculations. It is demonstrated that magnetic anisotropy close to the surface has a huge impact on the multiferroic ground state. For certain nanoparticle sizes the modulus of the ferromagnetic and ferroelectric moments are bistable, an effect that may be used in the design of ideal memory bits that can be switched electrically and read out magnetically.

cond-mat.mtrl-sci↗

arXiv2019

Impact of nonlocal electrodynamics on flux noise and inductance of superconducting wires

We present exact numerical calculations of supercurrent density, inductance, and impurity-induced flux noise of cylindrical superconducting wires in the nonlocal Pippard regime, which occurs when the Pippard coherence length is larger than the London penetration depth. In this regime the supercurrent density displays a peak away from the surface, and changes sign inside the superconductor, signalling a breakdown of the usual approximation of local London electrodynamics with a renormalized penetration depth. Our calculations show that the internal inductance and the bulk flux noise power is enhanced in nonlocal superconductors. In contrast, the kinetic inductance is reduced and the surface flux noise remains the same. As a result, impurity spins in the bulk may dominate the flux noise in superconducting qubits in the Pippard regime, such as the ones using aluminum superconductors with large electron mean free path.

cond-mat.supr-con↗

arXiv2018

Quantum theory of an atom in proximity to a superconductor

The impact of superconducting correlations on localized electronic states is important for a wide range of experiments in fundamental and applied superconductivity (SC). This includes scanning tunneling microscopy of atomic impurities at the surface of superconductors, as well as superconducting-ion-chip spectroscopy of neutral ions and Rydberg states. Moreover, atom-like centers close to the surface are currently believed to be the main source of noise and decoherence in qubits based on superconducting devices. The proximity effect is known to dress atomic orbitals in Cooper-pair-like states known as Yu-Shiba-Rusinov states (YSR), but the impact of SC on the measured orbital splittings and optical/noise transitions is not known. Here we study the interplay between orbital degenerescence and particle number admixture in atomic states, beyond the usual classical spin approximation. We model the atom as a generalized Anderson model interacting with a conventional $s$-wave superconductor. In the limit of zero on-site Coulomb repulsion ($U=0$), we obtain YSR subgap energy levels that are identical to the ones obtained from the classical spin model. When $Δ$ is large and $U>0$, the YSR spectra is no longer quasiparticle-like, and the highly degenerate orbital subspaces are split according to their spin, orbital, and number-parity symmetry. We show that $U>0$ activates additional poles in the atomic Green's function, suggesting an alternative explanation for the peak splittings recently observed in scanning tunneling microscopy of orbitally-degenerate impurities in superconductors. We describe optical excitation and absorption of photons by YSR states, showing that many additional optical channels open up in comparison to the non-superconducting case. Conversely, the additional dissipation channels imply increased electromagnetic noise due to impurities in superconducting devices.

cond-mat.supr-con↗

arXiv2011

Sinusoidal electromagnon in RMnO3: Indication of anomalous magnetoelectric coupling

The optical spectra in the family of multiferroic manganites RMnO3 is a great puzzle. Current models can not explain the fact that two strong electromagnons are present in the non-collinear spin cycloidal phase, with only one electromagnon surviving the transition into the collinear spin sinusoidal phase. We show that this is a signature of the presence of anomalous magnetoelectric coupling that breaks rotational invariance in spin space and generates oscillatory polarization in the ground state.

cond-mat.str-el↗