arXiv subjects

Roland Wiesendanger

Publications and source records attributed to Roland Wiesendanger.

At least 19 recordsLinked to original sources

arXiv2026

Exchange-induced suppression of superconductivity in a nano-skyrmion lattice - superconductor hybrid

Engineered magnet-superconductor hybrids have recently been identified as promising platforms for the investigation of topological superconductivity. Beyond ferro- and antiferromagnetic structures, coupling non-collinear spin textures, such as skyrmion lattices, to superconductors offers an exciting route for creating and manipulating unconventional superconducting states. In this work, by preparing monolayer Fe on Ir(111) thin films grown epitaxially on a Nb(110) surface, we realize a hybrid system of a nano-skyrmion lattice proximitized to a superconducting substrate. Scanning tunneling spectroscopy shows that superconductivity becomes suppressed by the Fe nano-skyrmion lattice, with both the superconducting gap and coherence peaks disappearing. Tight-binding calculations reveal that with increasing exchange coupling, the gap is progressively filled up and eventually superconductivity gets quenched. These results reveal microscopic constraints for designing topologically non-trivial states based on magnet-superconducting heterostructures.

cond-mat.supr-con↗

arXiv2026

Distinguishing Majorana zero modes from trivial defect states in an iron-based superconductor

Majorana zero modes, which obey non-Abelian exchange statistics, are promising candidates for topological quantum computation due to their robustness against environmental perturbations. The iron-based superconductor Fe(Te,Se) has been identified as an intrinsic topological superconductor, possibly hosting Majorana zero modes. In this paper, we report the observation of near-zero-energy localized states at multiple structural defects on the Fe(Te,Se) surface, which could be misidentified as Majorana zero modes without additional verification. By using spin-polarized scanning tunneling spectroscopy, we demonstrate that the near-zero-energy localized states on step edges and line defects originate from topologically trivial Yu-Shiba-Rusinov states. In addition, zero-energy bound states are also observed for regions without surface defects. A combined spatial and magnetic field dependent analysis of the spin-resolved tunneling spectra in these regions reveals that this type of zero-energy states cannot be attributed to the presence of Majorana bound states. These findings emphasize the importance of spin-dependent studies of low-energy states for pursuing Majorana zero modes.

cond-mat.supr-con↗

arXiv2026

Creation and motion of antiferromagnetic skyrmions by edge manipulation

Magnetic racetrack architectures that use topological magnetic particles to store information are one of the most promising concepts for future storage applications. Antiferromagnetic racetracks are particularly appealing as they are not susceptible to external magnetic fields. State-of-the-art racetracks use magnetic fields, spin-transfer and spin-orbit torques caused by electric currents to move the bits across the entire circuit. However, the application of currents in many antiferromagnetic racetracks is limited because many of them are insulating. Recently, however, a concept for ferromagnetic racetrack memories that are free of global driving forces has been proposed. It has been demonstrated that various topological entities can be generated and transported over long distances solely through local magnetization rotation at the sample boundaries, independent of global driving forces. Here, we demonstrate that the local rotation of magnetization at the boundary of an antiferromagnetic sample can be exploited in racetracks to efficiently generate and transmit antiferromagnetic skyrmions. Additionally, we demonstrate that local switching of staggered magnetization at the edge of an antiferromagnetic racetrack can be even more successful than the rotational procedure. A comparison of ferromagnetic and antiferromagnetic processing of skyrmionic bits, together with energy considerations, shows that this procedure is fairly efficient in antiferromagnets.

cond-mat.mes-hall↗

arXiv2026

Effects of interlayer Dzyaloshinskii-Moriya interaction on the shape and dynamics of magnetic twin-skyrmions

Magnetic skyrmions have been proposed as promising candidates for storing information due to their high stability and easy manipulation by spin-polarized currents. Here, we study how these properties are influenced by the interlayer Dzyaloshinskii--Moriya interaction (IL-DMI), which stabilizes twin-skyrmions in magnetic bilayers. We find that the spin configuration of the twin-skyrmion adapts to the direction of the IL-DMI by elongating or changing the helicities in the two layers. Driving the skyrmions by spin-polarized currents in the current-perpendicular-to-plane configuration, we observe significant changes either in the skyrmion velocity or in the skyrmion Hall angle depending on the current polarization. These findings unravel further prospects for skyrmion manipulation enabled by the IL-DMI.

cond-mat.mes-hall↗

arXiv2026

In-plane ferromagnetism-driven topological nodal-point superconductivity with tilted Weyl cones

The potential application of topological superconductivity in quantum transport and quantum information has fueled an intense investigation of hybrid materials with emergent electronic properties, including magnet-superconductor heterostructures. Here, we report evidence of a topological nodal-point superconducting phase in a one-atom-thick in-plane ferromagnet in direct proximity to a conventional $s$-wave superconductor. Low-temperature scanning tunneling spectroscopy data reveal the presence of a double-peak low-energy feature in the local density of states of the hybrid system, which is rationalized via model calculations to be an emergent topological nodal-point superconducting phase with tilted Weyl cones. Our results further establish the combination of in-plane ferromagnetism and conventional superconductivity as a route to design two-dimensional topological quantum phases.

cond-mat.supr-con↗

arXiv2025

Topological spin textures in an antiferromagnetic monolayer

Topological spin structures such as magnetic skyrmions are of fundamental interest and promising for various types of applications in spintronics. Skyrmions have been predicted to emerge also in antiferromagnetic materials where they exhibit superior transport properties. They were experimentally revealed in synthetic antiferromagnets, however, still remain elusive in intrinsic antiferromagnets. Here, we demonstrate the stabilization of topological spin structures in an antiferromagnetic monolayer. Using spin-polarized scanning tunneling microscopy, we observe an antiferromagnetic spin spiral in the Mn monolayer and a collinear antiferromagnetic state in the Mn double-layer on Ta(110). Near the boundary to the double-layer half-skyrmions form in the monolayer as revealed in combination with first-principles calculations and micromagnetic simulations. Our work shows how the topological state in antiferromagnetic material systems can be controlled by the configuration within a lateral heterostructure, resulting in trivial non-coplanar states or antiferromagnetic skyrmions.

cond-mat.mtrl-sci↗

arXiv2025

Reciprocity of Magnetism and Nanostructure Growth

The growth of thin films and nanostructures is a fundamental process for constructing both model-type systems and nanoscale devices, where performance and functionalities can be controlled by the choice of parameters. For magnetic systems the crystal structure, material composition, size, and shape determine already most of the magnetism-related properties. Here, we investigate the reciprocal route, which is controlling nanostructure growth via magnetism. To this end we deposit Co on a uniaxial antiferromagnetic surface above and below its Néel temperature. Growth above the Néel temperature results in the formation of roughly hexagonal islands, reflecting the surface symmetry. For growth below the Néel temperature we find quasi-one-dimensional Co nanostructures along distinct crystallographic directions, which signal the local antiferromagnetic domain orientation. Our findings demonstrate the feasibility of controlling growth via magnetism and the necessity to take magnetism-related effects into account for growth on magnetic surfaces.

cond-mat.mtrl-sci↗

arXiv2025

Spin-polarized edge modes between different magnet-superconductor-hybrids

The interplay of magnetism and superconductivity can lead to intriguing emergent phenomena. Here we combine two different two-dimensional antiferromagnetic magnet-superconductor hybrids (MSH) and study their properties using spin-polarized scanning tunneling microscopy. Both MSHs show the characteristics of a topological nodal point superconducting phase with edge modes to the trivial substrate superconductor. At the boundary between the two MSHs we find low-energy modes which are spin-polarized. Based on a tight-binding model we can explain the experimental observations by considering two different topological nodal point superconductors. This gives rise to spin-polarized chiral edge modes that connect topological nodal points of the two different MSH. We demonstrate via the complex band structure that due to an asymmetric lateral decay these edge modes are spin-polarized, regardless of the details of the spin structure at the boundary. The presence of spin-polarized edge states between different topological superconductors enables advanced functional design for the exploitation of MSHs as a platform for topology-based applications.

cond-mat.supr-con↗

arXiv2025

Robustness of Majorana modes to potential disorder in Fe chains on a superconducting Rashba alloy

Majorana modes offer great potential for fault-tolerant quantum computation due to their topological protection. However, for superconductor-semiconductor nanowire hybrids, intrinsic disorder makes the unambiguous detection of Majorana modes difficult. Here, we construct 1D spin chains from individual Fe atoms on the Rashba surface alloy BiAg2/Ag(111) with proximity-induced superconductivity from a Nb(110) substrate. While the Fe chains exhibit perfect crystalline order, we observe nano-scale potential disorder of the BiAg2/Ag(111)/Nb(110) heterostructure by scanning tunneling microscopy. However, this does not prevent the emergence of zero-energy modes at both ends of the Fe chains, in agreement with tight-binding calculations showing that they are only found in the topologically non-trivial regime of the phase diagram. These Majorana modes are indeed robust against potential disorder.

cond-mat.supr-con↗

arXiv2025

Effect of substrate spin-orbit coupling on the topological gap size of Shiba chains

Realizing Majorana bound states in chains of magnetic impurities on $s$-wave superconducting substrates relies on a fine tuning of the energy and hybridization of the single magnetic impurity bound states and of the spin-orbit coupling (SOC). While recent experiments investigate the influence of the former two parameters, the effect of SOC remained experimentally largely unexplored. Here, we present a scanning tunneling spectroscopy study of close-packed Mn chains along the [001]-direction on Ta(110) which has almost identical atomic and surface electronic structure compared to the previously studied Nb(110) system, but a three times larger SOC. The dominant Shiba band has a very similar dispersion, but its minigap, taken relative to $\varDelta$, is increased by a factor of 1.9 with respect to the Nb case, which can be ascribed to the stronger SOC.

cond-mat.supr-con↗

arXiv2025

Coexistence of topologically trivial and non-trivial Yu-Shiba-Rusinov bands in magnetic atomic chains on a superconductor

Majorana zero modes (MZMs) have been proposed as a promising basis for Majorana qubits offering great potential for topological quantum computation. Such modes may form at the ends of a magnetic atomic chain on a superconductor. Typically only a single MZM may be present at one end of the chain, but symmetry may protect multiple MZMs at the same end. Here, we study the topological properties of Yu-Shiba-Rusinov (YSR) bands of excitations in Mn chains constructed on a Nb(110) and on a Ta(110) substrate using first-principles calculations and scanning tunneling microscopy and spectroscopy experiments. We demonstrate that even and odd YSR states with respect to mirroring on the symmetry plane containing the chain have different dispersions, and both of them may give rise to MZMs separately. Although the spin-orbit coupling leads to a hybridization between the bands, multiple MZMs may still exist due to the mirror symmetry. These findings highlight the influence of symmetries on interpreting the spectroscopic signatures of candidates for MZMs.

cond-mat.supr-con↗

arXiv2025

Majorana quasiparticles in atomic spin chains on superconductors

For the past decade, Majorana quasiparticles have become one of the hot topics in condensed matter research. Besides the fundamental interest in the realization of particles being their own antiparticles, going back to basic concepts of elementary particle physics, Majorana quasiparticles in condensed matter systems offer exciting potential applications in topological quantum computation due to their non-Abelian quantum exchange statistics. Motivated by theoretical predictions about possible realizations of Majorana quasiparticles as zero-energy modes at boundaries of topological superconductors, experimental efforts have focussed in particular on quasi-one-dimensional semiconductor-superconductor and magnet-superconductor hybrid systems. However, an unambiguous proof of the existence of Majorana quasiparticles is still challenging and requires considerable improvements in materials science, atomic-scale characterization and control of interface quality, as well as complementary approaches of detecting various facets of Majorana quasiparticles. Bottom-up atom-by-atom fabrication of disorder-free atomic spin chains on atomically clean superconducting substrates has recently allowed deep insight into the emergence of topological sub-gap Shiba bands and associated Majorana states from the level of individual atoms up to extended chains, thereby offering the possibility for critical tests of Majorana physics in disorder-free model-type 1D hybrid systems.

cond-mat.mes-hall↗

arXiv2025

Preparation and readout of Majorana qubits in magnet-superconductor hybrid systems

Initializing the ground state of a quantum bit (qubit) based on Majorana zero modes is one of the most pressing issues for future topological quantum computers. We explore a protocol for initializing such topological qubits based on magnet-superconductor hybrid networks by coupling magnetic chains to a single molecule magnet. The parity of the Majorana state is converted to the presence or absence of a Yu-Shiba-Rusinov state at the molecule. The coupling can be activated by switching the spin state of the molecule, allowing the ground-state parity of the chain to be controlled. We demonstrate that initialization with either parity for a Majorana qubit can be achieved. We then introduce the augmented Majorana qubit, which includes the state of the molecule in the definition of the logical qubit. Using this definition we can initialize a qubit without high-precision timing.

cond-mat.supr-con↗

arXiv2024

Topological meron-antimeron domain walls and skyrmions in a low-symmetry system

The generation of topologically non-trivial magnetic configurations has been a pivotal topic in both basic and applied nanomagnetism research. Localized non-coplanar magnetic defects such as skyrmions or merons were found to interact strongly with currents, making them interesting candidates for future spintronics applications. Here, we study a low-symmetry bcc(110) system by spin-polarized scanning tunneling microscopy and an atomistic spin model using parameters obtained from first-principles calculations. We demonstrate how a delicate balance between energy terms generates both topologically trivial and non-trivial domain walls, depending on their crystallographic direction. The topological walls consist of merons and antimerons and the topological charge amounts to about 0.2/nm wall length. The incorporation of holes in the films facilitates the transition from an in-plane ferromagnetic ground state to a spin-spiral state. Both domain walls and spirals transition into isolated elongated magnetic skyrmions in applied magnetic fields, establishing low-symmetry systems as a versatile platform for spin-texture engineering.

cond-mat.mes-hall↗

arXiv2024

Magnet-superconductor hybrid quantum systems: a materials platform for topological superconductivity

Magnet-superconductor hybrid (MSH) systems have recently emerged as one of the most significant developments in condensed matter physics. This has generated, in the last decade, a steadily rising interest in the understanding of their unique properties. They have been proposed as one of the most promising platforms for the establishment of topological superconductivity, which holds high potential for application in future quantum information technologies. Scanning tunneling microscopy (STM) and spectroscopy (STS) plays a crucial role in the race to unveil the fundamental origin of the unique properties of MSH systems, with the aim to discover new hybrid quantum materials capable of hosting topologically non-trivial unconventional superconducting phases. In particular, the combination of STM studies with tight-binding model calculations have represented, so far, the most successful approach to unveil and explain the emergent electronic properties of MSHs. The scope of this review is to offer a broad perspective on the field of MSHs from an atomic-level investigation point-of-view. The focus is on discussing the link between the magnetic ground state hosted by the hybrid system and the corresponding emergent superconducting phase. This is done for MSHs with both one-dimensional (atomic chains) and two-dimensional (atomic lattices and thin films) magnetic systems proximitized to conventional s-wave superconductors. We present a systematic categorization of the experimentally investigated systems with respect to defined experimentally accessible criteria to verify or falsify the presence of topological superconductivity and Majorana edge modes. Given the vast number of publications on the topic, we limit ourselves to discuss works which are most relevant to the search for topological superconductivity.

cond-mat.supr-con↗

arXiv2024

Non-local detection of coherent Yu-Shiba-Rusinov quantum projections

Probing spatially confined quantum states from afar - a long-sought goal to minimize external interference - has been proposed to be achievable in condensed matter systems via coherent projection. The latter can be tailored by sculpturing the eigenstates of the electron sea that surrounds the quantum state using atom-by-atom built cages, so-called quantum corrals. However, assuring the coherent nature of the projection, and manipulating its quantum composition, has remained an elusive goal. Here, we experimentally realize the coherent projection of a magnetic impurity-induced, Yu-Shiba-Rusinov quantum state using the eigenmodes of corrals on the surface of a superconductor, which enables us to manipulate the particle-hole composition of the projected state by tuning corral eigenmodes through the Fermi energy. Our results demonstrate a controlled non-local method for the detection of magnet superconductor hybrid quantum states.

cond-mat.supr-con↗

arXiv2024

Interlayer and interfacial Dzyaloshinskii-Moriya interaction in magnetic trilayers: first-principles calculations

We determine the Dzyaloshinskii-Moriya interaction within and between two magnetic cobalt layers separated by a non-magnetic spacer through ab initio calculations. We investigate different materials for the non-magnetic layer, focusing on the experimentally realized Co/Ag/Co system. We laterally shift the atoms in the non-magnetic layer to achieve the symmetry breaking required for the interlayer Dzyaloshinskii-Moriya interaction. We compare the resulting interactions with the Lévy-Fert model and observe a good overall agreement between the model and the ab initio calculations for the dependence on the atomic positions. Additionally, we derive a formula for the strength of the interlayer isotropic exchange interaction depending on the position of the atoms in the non-magnetic layer and compare it to the first-principles results. We investigate the limitations of the Lévy-Fert model by turning off the spin-orbit coupling separately on the non-magnetic and magnetic atoms and by studying the effect of band filling. Our work advances the understanding of the microscopic mechanisms of the interlayer Dzyaloshinskii-Moriya interaction and gives insight into possible new material combinations with strong interlayer Dzyaloshinskii-Moriya interaction.

cond-mat.mtrl-sci↗

arXiv2024

Large diversity of magnetic phases in two-dimensional magnets with spin-orbit coupling and superconductivity

We classify the magnetic ground states of a 2D lattice of localized magnetic moments which are coupled to a superconducting substrate with Rashba-spin-orbit coupling. We discover a rich magnetic phase diagram with surprisingly complex structures including 2q-spin-spirals, a 2x2-periodic pattern, and skyrmion lattices, self-consistently, using an effective classical spin Hamiltonian and show that the system hosts non-zero 4-spin interactions. Our in-depth analysis of about ten thousand magnetic configurations becomes feasible using contrastive clustering, a recent advanced unsupervised machine learning technique. This work proposes simple few-band systems for non-collinear magnetic states and stimulates further research on topological effects in their self-consistent electronic structure.

cond-mat.supr-con↗