arXiv subjects

Roland Wiesendanger

Publications and source records attributed to Roland Wiesendanger.

At least 73 records · Page 4Linked to original sources

arXiv2020

Domain Walls in a Row-Wise Antiferromagnetic Mn Monolayer

We investigate magnetic domain walls in a single fcc Mn layer on Re(0001) employing spin-polarized STM, atom manipulation, and spin dynamics simulations. The low symmetry of the row-wise antiferromagnetic (1Q) state leads to a new type of domain wall which connects rotational 1Q domains by a transient 2Q state with characteristic 90$^\circ$ angles between neighboring magnetic moments. The domain wall properties depend on their orientation and their width of about 2 nm essentially results from a balance of Heisenberg and higher-order exchange interactions. Atom manipulation allows domain wall imaging with atomic spin-resolution, as well as domain wall positioning, and we demonstrate that the force to move an atom is anisotropic on the 1Q domain.

cond-mat.mes-hall↗

arXiv2020

Spin-polarized Yu-Shiba-Rusinov states in an iron based superconductor

Yu-Shiba-Rusinov (YSR) bound states appear when a magnetic atom interacts with a superconductor. Here, we report on spin-resolved spectroscopic studies of YSR states related with Fe atoms deposited on the surface of the topological superconductor FeTe0.55Se0.45 using a spin-polarized scanning tunneling microscope. We clearly identify the spin signature of pairs of YSR bound states at finite energies within the superconducting gap having opposite spin polarization as theoretically predicted. In addition, we also observe zero-energy bound states for some of the adsorbed Fe atoms. In this case, a spin signature is found to be absent indicating the absence of Majorana bound states associated with Fe adatoms on FeTe0.55Se0.45.

cond-mat.supr-con↗

arXiv2020

Spin-orbit coupling induced splitting of Yu-Shiba-Rusinov states in antiferromagnetic dimers

Magnetic atoms coupled to the Cooper pairs of a superconductor induce Yu-Shiba-Rusinov states (in short Shiba states). In the presence of sufficiently strong spin-orbit coupling, the bands formed by hybridization of the Shiba states in ensembles of such atoms can support low-dimensional topological superconductivity with Majorana bound states localized on the ensembles' edges. Yet, the role of spin-orbit coupling for the hybridization of Shiba states in dimers of magnetic atoms, the building blocks for such systems, is largely unexplored. Here, we reveal the evolution of hybridized multi-orbital Shiba states from a single Mn adatom to artificially constructed ferromagnetically and antiferromagnetically coupled Mn dimers placed on a Nb(110) surface. Upon dimer formation, the atomic Shiba orbitals split for both types of magnetic alignment. Our theoretical calculations attribute the unexpected splitting in antiferromagnetic dimers to spin-orbit coupling and broken inversion symmetry at the surface. Our observations point out the relevance of previously unconsidered factors on the formation of Shiba bands and their topological classification.

cond-mat.supr-con↗

arXiv2020

Rotating edge-field driven processing of chiral spin textures in racetrack devices

Topologically distinct magnetic structures like skyrmions, domain walls, and the uniformly magnetized state have multiple applications in logic devices, sensors, and as bits of information. One of the most promising concepts for applying these bits is the racetrack architecture controlled by electric currents or magnetic driving fields. In state-of-the-art racetracks, these fields or currents are applied to the whole circuit. Here, we employ micromagnetic and atomistic simulations to establish a concept for racetrack memories free of global driving forces. Surprisingly, we realize that mixed sequences of topologically distinct objects can be created and propagated over far distances exclusively by local rotation of magnetization at the sample boundaries. We reveal the dependence between the chirality of the rotation and the direction of propagation and define the phase space where the proposed procedure can be realized. The advantages of this approach are the exclusion of high current and field densities as well as its compatibility with an energy-efficient three-dimensional design.

cond-mat.mes-hall↗

arXiv2020

Plumbene on a magnetic substrate: a combined STM and DFT study

As heavy analog of graphene, plumbene is a two-dimensional material with strong spin-orbit coupling effects. Using scanning tunneling microscopy (STM), we observe that Pb forms a flat honeycomb lattice on an Fe monolayer on Ir(111). In contrast, without the Fe layer, a c(2x4) structure of Pb on Ir(111) is found. We use density functional theory (DFT) calculations to rationalize these findings and analyze the impact of the hybridization on the plumbene band structure. In the unoccupied states the splitting of the Dirac cone by spin-orbit interaction is clearly observed while in the occupied states of the freestanding plumbene we find a band inversion that leads to the formation of a topologically non-trivial gap. Exchange splitting as mediated by the strong hybridization with the Fe layer drives a quantum spin Hall to quantum anomalous Hall state transition.

cond-mat.mtrl-sci↗

arXiv2020

Towards skyrmion-superconductor hybrid systems

Spin-polarized scanning tunneling microscopy is used to identify the magnetic state of different thin films on a Re(0001) substrate, which becomes superconducting below 1.7 K. All magnetic films contain an Fe/Ir interface, which is known to facilitate the emergence of non-collinear magnetic order. For Fe monolayers on ultra-thin Ir films of different thickness we find several different atomic-scale magnetic states. For Pd/Fe bilayers we find nano-scale spin spirals as magnetic ground states for Ir thicknesses of three and four atomic layers. In applied magnetic fields skyrmions emerge, and in remanence non-trivial magnetic textures survive. This demonstrates the possibility to prepare skryrmion-hosting magnetic films on superconducting substrates.

cond-mat.mtrl-sci↗

arXiv2020

Spectroscopic signature of the Stark-shifted Tamm-type surface state of La(0001)

We have studied the Tamm-type surface state of La(0001) by tunneling spectroscopy within a wide range of tunneling currents from 0.1 nA to 8000 nA, thereby tuning the electric-field strength in a tip-vacuum-sample tunnel junction. We observe a significant shift of the unoccupied Tamm-type surface state toward the Fermi energy with increasing electric-field strength, accompanied by a broadening of the width of the resonance peak indicating a decrease of the surface-state lifetime. Our experimental results are contrary to previous reports for Stark-shifted Shockley-type surface states of noble metal (111) surfaces.

cond-mat.mes-hall↗

arXiv2020

Long-range focusing of magnetic bound states in superconducting lanthanum

Quantum mechanical systems with long-range interactions between quasiparticles provide a promising platform for coherent quantum information technology. Superconductors are a natural choice for solid-state based quantum devices, while magnetic impurities inside superconductors give rise to quasiparticle excitations of broken Cooper pairs that provide characteristic information about the host superconductor. Here, we reveal that magnetic impurities embedded below a superconducting La(0001) surface interact via quasiparticles extending to very large distances, up to several tens of nanometers. Using low-temperature scanning probe techniques, we observe the corresponding anisotropic and giant oscillations in the local density of states. Theoretical calculations indicate that the quasi-two-dimensional surface states with their strongly anisotropic Fermi surface play a crucial role for the focusing and long-range extension of the magnetic bound states. The quasiparticle focusing mechanism should facilitate the design of versatile magnetic structures with tunable and directed magnetic interactions over large distances, thereby paving the way toward the design of low-dimensional magnet-superconductor hybrid systems exhibiting topologically non-trivial quantum states as possible elements of quantum computation schemes based on Majorana quasiparticles.

cond-mat.supr-con↗

arXiv2020

Atomic-scale spin-polarization maps using functionalized superconducting probes

A scanning tunneling microscope (STM) with a magnetic tip that has a sufficiently strong spin-polarization can be used to map the sample's spin structure down to the atomic scale but usually lacks the possibility to absolutely determine the value of the sample's spin-polarization. Magnetic impurities in superconducting materials give rise to pairs of perfectly, i.e. 100% spin-polarized sub-gap resonances. In this work, we functionalize the apex of a superconducting Nb STM-tip with such impurity states by attaching Fe atoms to probe the spin-polarization of atom-manipulated Mn nanomagnets on a Nb(110) surface. By comparison with spin-polarized STM measurements of the same nanomagnets using Cr bulk tips we demonstrate an extraordinary spin-sensitivity and the possibility to measure the sample's spin-polarization values quantitatively with our new functionalized probes.

cond-mat.supr-con↗

arXiv2020

Topological superconductivity induced by a triple-Q magnetic structure

We demonstrate that the recently discovered triple-Q (3Q) magnetic structure, when embedded in a magnet-superconductor hybrid (MSH) system, gives rise to the emergence of topological superconductivity. We investigate the structure of chiral Majorana edge modes at domain walls, and show that they can be distinguished from trivial in-gap modes through the spatial distribution of the induced supercurrents. Finally, we show that topological superconductivity in 3Q MSH systems is a robust phenomenon that does not depend on the relative alignment of the magnetic and superconducting layers, or on the presence of electronic degrees of freedom in the magnetic layer.

cond-mat.supr-con↗

arXiv2020

A cavity optomechanical locking scheme based on the optical spring effect

We present a novel locking scheme for active length-stabilization and frequency detuning of a cavity optomechanical device based on the optical spring effect. The scheme can be used as an alternative to the Pound-Drever-Hall locking technique but in contrast doesn't require signal processing on time-scales of the cavity decay rate. It is therefore particularly suited for stabilizing micro cavities, where this time-scale can be extremely fast. The error signal is generated through the optical spring effect, i.e. the detuning-dependent frequency-shift of a nanomechanical oscillator that is dispersively coupled to the intra-cavity light field. We explain the functional principle of the lock and characterize its performance in terms of bandwidth and gain profile. The optical spring locking scheme can be implemented without larger efforts in a wide variety of optomechanical systems in the unresolved sideband regime.

physics.ins-det↗

arXiv2020

Discovery of magnetic single- and triple-Q states in Mn/Re(0001)

We experimentally verify the existence of two model-type magnetic ground states which were previously predicted but so far unobserved. We find them in Mn monolayers on the Re(0001) surface using spin-polarized scanning tunneling microscopy. For fcc stacking of Mn the collinear row-wise antiferromagnetic state occurs, whereas for hcp Mn a three-dimensional spin structure appears, which is a superposition of three row-wise antiferromagnetic states and is known as triple-Q state. Density functional theory calculations elucidate the subtle interplay of different magnetic interactions to form these spin structures and provide insight into the role played by relativistic effects.

cond-mat.mes-hall↗

arXiv2020

Controlling in-gap end states by linking nonmagnetic atoms and artificially-constructed spin chains on superconductors

Chains of magnetic atoms with either strong spin-orbit coupling or spiral magnetic order which are proximity-coupled to superconducting substrates can host topologically non-trivial Majorana bound states. The experimental signature of these states consists of spectral weight at the Fermi energy and spatially localized near the ends of the chain. However, topologically trivial Yu-Shiba-Rusinov in-gap states localized near the ends of the chain can lead to similar spectra. Here, we explore a protocol to disentangle these contributions by artificially augmenting a candidate Majorana spin chain with orbitally-compatible nonmagnetic atoms. Combining scanning tunneling spectroscopy with ab-initio and tight-binding calculations, we realize a sharp spatial transition between the proximity-coupled spiral magnetic order and the non-magnetic superconducting wire termination, with persistent zero-energy spectral weight localized at either end of the magnetic spiral. Our findings open a new path towards the control of the spatial position of in-gap end states, trivial or Majorana, via different chain terminations, and the realization of designer Majorana chain networks for demonstrating topological quantum computation.

cond-mat.supr-con↗

arXiv2020

Real-space imaging of atomic-scale spin textures at nanometer distances

Spin-polarized scanning tunneling microscopy (SP-STM) experiments on ultrathin films with non-collinear spin textures demonstrate that resonant tunneling allows for atomic-scale spin-sensitive imaging in real space at tip-sample distances of up to 8 nm. Spin-polarized resonance states evolving between the foremost atom of a magnetic probe tip and the opposed magnetic surface atom are found to provide a loophole from the hitherto existing dilemma of losing spatial resolution when increasing the tip-sample distance in a scanning probe setup. Bias-dependent series of SP-STM images recorded via resonant tunneling reveal spin sensitivity at resonance conditions, indicating that the spin-polarized resonance states act as mediators for the spin contrast across the nm-spaced vacuum gap. With technically feasible distances in the nm regime, resonant tunneling in SP-STM qualifies for a spin-sensitive read-write technique with ultimate lateral resolution in future spintronic applications.

physics.app-ph↗

arXiv2019

Probing weakly hybridized magnetic molecules by spin-polarized tunneling

Advances in molecular spintronics rely on the in-depth characterization of the molecular building blocks in terms of their electronic and, more importantly, magnetic properties. For this purpose, inert substrates that interact only weakly with adsorbed molecules are required in order to preserve their electronic states. Here, we investigate the magnetic-field response of a single paramagnetic 5,5-dibromosalophenatocobalt(II) (CoSal) molecule adsorbed on a weakly interacting magnetic substrate, namely Fe-intercalated graphene (GR/Fe) grown on Ir(111), by using spin-polarized scanning tunneling microscopy and spectroscopy (SP-STM/STS). We have obtained local magnetization curves, spin-dependent tunneling spectra, and spatial maps of magnetic asymmetry for a single CoSal molecule, revealing its magnetic properties and coupling to the local environment. The distinct magnetic behavior of the Co-metal center is found to rely strictly on its position relative to the GR/Fe moire structure, which determines the level of hybridization between the GR/Fe surface pi-system, the molecular ligand pi-orbitals and the molecular Co-ion d-orbital.

physics.app-ph↗

arXiv2019

Nano-scale magnetic skyrmions and target states in confined geometries

Research on magnetic systems with broken inversion symmetry has been stimulated by the experimental proof of particle-like configurations known as skyrmions, whose non-trivial topological properties make them ideal candidates for spintronic technology. This class of materials enables Dzyaloshinskii-Moriya interactions (DMI) which favor the stabilization of chiral configurations. Recent advances in material engineering have shown that in confined geometries it is possible to stabilize skyrmionic configurations at zero field. Moreover, it has been shown that in systems based on Pd/Fe bilayers on top of Ir(111) surfaces skyrmions can be as small as a few nanometres in diameter. In this work we present scanning tunneling microscopy measurements of small Pd/Fe and Pd$_2$/Fe islands on Ir(111) that exhibit a variety of different spin textures, which can be reproduced using discrete spin simulations. These configurations include skyrmions and skyrmion-like states with extra spin rotations such as the target state, which have been of interest due to their promising dynamic properties. Furthermore, using simulations we analyze the stability of these skyrmionic textures as a function of island size, applied field and boundary conditions of the system. An understanding of the parameters and conditions affecting the stability of these magnetic structures in confined geometries is crucial for the development of energetically efficient and optimally sized skyrmion-based devices.

cond-mat.mes-hall↗

arXiv2019

Stochastic dynamics and pattern formation of geometrically confined skyrmions

Ensembles of magnetic skyrmions in confined geometries are shown to exhibit thermally driven motion on two different time scales. The intrinsic fluctuating dynamics ($t\sim 1~$ps) is governed by short-range symmetric and antisymmetric exchange interactions, whereas the long-time limit ($t\gtrsim10\,$ns) is determined by the coaction of skyrmion-skyrmion-repulsion and the system's geometry. Micromagnetic simulations for realistic island shapes and sizes are performed and analyzed, indicating the special importance of skyrmion dynamics at finite temperatures. We demonstrate how the competition between skyrmion mobility and observation time directly affects the addressability of skyrmionic bits, which is a key challenge on the path of developing skyrmion-based room-temperature applications. The presented quasiparticle Monte Carlo approach offers a computationally efficient description of the diffusive motion of skyrmion ensembles in confined geometries, like racetrack memory setups.

cond-mat.mes-hall↗

arXiv2019

Magnetism and in-gap states of 3d transition metal atoms on superconducting Re

Magnetic atoms on heavy-element superconducting substrates are potential building blocks for realizing topological superconductivity in one- and two-dimensional atomic arrays. Their localized magnetic moments induce so-called Yu-Shiba-Rusinov (YSR) states inside the energy gap of the substrate. In the dilute limit, where the electronic states of the array atoms are only weakly coupled, proximity of the YSR states to the Fermi energy is essential for the formation of topological superconductivity in the band of YSR states. Here, we reveal via scanning tunnel spectroscopy and ab initio calculations of a series of 3d transition metal atoms (Mn, Fe, Co) adsorbed on the heavy-element superconductor Re that the increase of the Kondo coupling and sign change in magnetic anisotropy with d-state filling is accompanied by a shift of the YSR states through the energy gap of the substrate and a crossing of the Fermi level. The uncovered systematic trends enable the identification of the most promising candidates for the realization of topological superconductivity in arrays of similar systems.

cond-mat.supr-con↗