arXiv subjects

Romain Bachelard

Publications and source records attributed to Romain Bachelard.

At least 19 recordsLinked to original sources

arXiv2026

Strong Collective Chiroptical Response from Electric-Dipole Interactions in Atomic Systems

Chiroptical responses in atomic systems are usually weak, as they arise from the interference between electric- and much weaker magnetic-dipole transitions. We show that atoms arranged in chiral geometries can instead exhibit a strong collective chiroptical response mediated entirely by electric-dipole interactions. Using a coupled-dipole framework, we identify a regime of pronounced chiroptical response emerging at subwavelength interatomic separations, which can be tuned by the probe frequency. This enhancement is directly linked to the formation of subradiant collective modes. Our results establish a fundamental connection between geometric chirality and collective light-matter interactions, opening new pathways for engineering and exploiting chiral optical responses in atomic systems.

physics.atom-ph↗

arXiv2026

Engineering Atom-Photon Hybridization with Density-Modulated Atomic Ensembles in Coupled Cavities

Radiation-matter hybridization allows atoms to serve as mediators of effective interactions between light modes and, conversely, to interact among themselves via light. Here we exploit the spatial structure of atomic ensembles to control the coupling between modes of distinct cavities, thereby reshaping the resulting atom-photon spectra. We show that extended homogeneous clouds suppress mode-mode couplings through destructive interference, whereas grated clouds can preserve them under specific Bragg conditions. This leads to mode-mode spectral subsplittings, where collectivity arises not only from the atom number but also from the ability to tune modes of different cavities independently. Our results establish spatially engineered atomic ensembles as a pathway to selective photon transfer between modes and precise control of many-body complexity.

quant-ph↗

arXiv2026

Deviations from thermal light statistics in ensembles of independent two-level emitters

We investigate the light statistics of an ensemble of independent motionless two-level atoms in a product state. We identify the conditions under which the cold atomic ensemble emits thermal light statistics characterized by the Gaussian Moment Theorem. For the theorem to hold, we derive for each correlation order two conditions on the atom number and the ratio of coherent to incoherent light emission. We further discuss their validity for atoms either in a pure or mixed state. Our results contribute to the understanding of the generation of thermal light by two-level atoms without interactions among the emitters.

quant-ph↗

arXiv2026

Detecting multilevel entanglement from light-based entanglement witnesses

We introduce a set of electric-field based inequalities capable of detecting multilevel entanglement from a system of N quantum emitters. We determine that the polarization channel as well as the direction of detection can enhance entanglement detection, a feature specific to multilevel systems. We demonstrate the efficiency of the witnesses to detect genuine multipartite entanglement by applying it to families of paradigmatic quantum states, such as Dicke states, singlet states and W-like states. The detection is not only robust to noise, but also applies to mixed entangled states. Our findings open up possibilities for the detection of entanglement without local measurements in systems of multilevel emitters such as superconducting qubits, Rydberg atoms or quantum dots.

quant-ph↗

arXiv2026

Collective resonance displacement in strongly driven cold atoms

Cold atoms are promising platforms for metrology and quantum computation, yet their many-body dynamics remains largely unexplored. We here investigate Rabi oscillations from optically-thick cold clouds, driven by high-intensity coherent light. A dynamical displacement from the atomic resonance is predicted, which can be detected through the collective Rabi oscillations of the atomic ensemble. Different from linear-optics shifts, this dynamical displacement grows quadratically with the optical depth, yet it reduces with increasing pump power as dipole-dipole interactions are less effective.

physics.atom-ph↗

arXiv2025

Subradiant Decay in 2D and 3D Atomic Arrays

Subradiance is a phenomenon where coupled emitters radiate light at a slower rate than independent ones. While its observation was first reported in disordered cold atom clouds, ordered subwavelength arrays of emitters have emerged as promising platforms to design highly cooperative optical properties based on dipolar interactions. In this work we characterize the eigenmodes of 2D and 3D regular arrays, using a method which can be used for both infinite and very large systems. In particular, we show how finite-size effects impact the lifetimes of these large arrays. Our results may have interesting applications for quantum memories and topological effects in ordered atomic arrays.

quant-ph↗

arXiv2025

Nonergodic extended phase for waves in three dimensions

Wave transport in complex media is determined by the nature of quasimodes at the microscopic level. In three dimensional disordered media, waves generally undergo a phase transition from diffusion to Anderson localization, characterized by exponentially localized modes. A remarkable exception are electromagnetic waves, whose vector-like nature prevents Anderson localization to occur. Here we demonstrate that both scalar and vector (electromagnetic) waves exhibit a non-ergodic extended phase characterized by fractal quasimodes, for a broad range of disorder strengths. While electromagnetic waves remain in the non-ergodic extended phase at high disorder strength, scalar waves eventually enter a localized regime. These results pave the way for the engineering of anomalous wave transport phenomena in disordered media without spatial correlations.

cond-mat.dis-nn↗

arXiv2025

Dimensional Control of the Coherence Time of Scattered Light in Cold Atom Clouds

Cold atomic clouds are promising platforms for generating correlated photons, but multiple scattering and associated Doppler broadening limit their temporal coherence. Here we demonstrate that cloud geometry provides a powerful means to extend the coherence time of scattered light. In the experiment, intensity-correlation measurements show that an elongated (quasi-1D) cloud exhibits systematically longer coherence times than a spherical (3D) cloud of the same on-axis optical thickness, as a direct consequence of the suppression of multiple scattering in the elongated geometry. Random-walk simulations reproduce this trend and further show that elongation drives the coherence time toward the single-scattering limit. The combined results establish cloud geometry as a robust control parameter for temporal coherence in cold-atom ensembles, with potential applications in quantum optics and communication.

physics.atom-ph↗

arXiv2025

Condensation of vanishing photon emission rates in random atomic clouds

In the collective photon emission from atomic clouds both the atomic transition frequency and the decay rate are modified compared to a single isolated atom, leading to the effects of superradiance and subradiance. In this article, we analyse the properties of the Euclidean random matrix associated to the radiative dynamics of a cold atomic cloud, previously investigated in the contexts of photon localization and Dicke super- and subradiance. We present evidence of a new type of phase transition, surprisingly controlled by the cooperativeness parameter, rather than the spatial density or the diagonal disorder. The numerical results corroborate the occurrence of such a phase transition at a critical value of the cooperativeness parameter, above which the lower edge of the spectrum vanishes exhibiting a macroscopic accumulation of eigenvalues. Independent evaluations based on the two phenomena provide the same value of the critical cooperativeness parameter.

quant-ph↗

arXiv2024

Detecting entanglement from macroscopic measurements of the electric field and its fluctuations

To address the outstanding task of detecting entanglement in large quantum systems, entanglement witnesses have emerged, addressing the separable nature of a state. Yet optimizing witnesses, or accessing them experimentally, often remains a challenge. We here introduce a family of entanglement witnesses for open quantum systems, based on the electric field -- its quadratures and the total fluorescence. More general than spin-squeezing inequalities, it can detect new classes of entangled states, as changing the direction for far-field observation opens up a continuous family of witnesses, without the need for a state tomography. Their efficiency is demonstrated by detecting, from almost any direction, the entanglement of collective single-photon states, such as long-lived states generated by cooperative spontaneous emission. Able to detect entanglement in large quantum systems, these electric-field-based witnesses can be used on any set of emitters described by the Pauli group, such as atomic systems (cold atoms and trapped ions), giant atoms, color centers, and superconducting qubits.

quant-ph↗

arXiv2024

Temporal coherences of atomic chaotic light sources: the Siegert relation and beyond

Light is characterized by its electric field, yet quantum optics has revealed the importance of monitoring photon-photon correlations at all orders. We here present a comparative study of two experimental setups, composed of cold and warm Rubidium atoms, respectively, which allow us to probe and compare photon correlations up to the fourth order. The former operates in the quantum regime where spontaneous emission dominates, whereas the latter exhibits a temperature-limited coherence time. While both setups present almost-chaotic light statistics, we discuss how the access to different orders of photon correlations allows one to better characterize the mechanisms responsible for deviations from those statistics.

physics.atom-ph↗

arXiv2024

Phononic bright and dark states: Investigating multi-mode light-matter interactions with a single trapped ion

Interference underpins some of the most practical and impactful properties of both the classical and quantum worlds. In this work we experimentally investigate a new formalism to describe interference effects, based on collective states which have enhanced or suppressed coupling to a two-level system. We employ a single trapped ion, whose electronic state is coupled to two of the ion's motional modes in order to simulate a multi-mode light-matter interaction. We observe the emergence of phononic bright and dark states for both a single phonon and a superposition of coherent states and demonstrate that a view of interference which is based solely on their decomposition in the collective basis is able to intuitively describe their coupling to a single atom. This work also marks the first time that multi-mode bright and dark states have been formed with the bounded motion of a single trapped ion and we highlight the potential of the methods discussed here for use in quantum information processing.

quant-ph↗

arXiv2023

Cooperative photon emission rates in random atomic clouds

We investigate the properties of the cooperative decay modes of a cold atomic cloud, characterized by a Gaussian distribution in three dimensions, initially excited by a laser in the linear regime. We study the properties of the decay rate matrix $S$, whose dimension coincides with the number of atoms in the cloud, in order to get a deeper insight into properties of cooperative photon emission. Since the atomic positions are random, $S$ is a Euclidean random matrix whose entries are function of the atom distances. We show that, in the limit of a large number of atoms in the cloud, the eigenvalue distribution of $S$ depends on a single parameter $b_0$, called the cooperativeness parameter, which can be viewed as a quantifier of the number of atoms that are coherently involved in an emission process. For very small values of $b_0$, we find that the limit eigenvalue density is approximately triangular. We also study the nearest-neighbour spacing distribution and the eigenvector statistics, finding that, although the decay rate matrices are Euclidean, the bulk of their spectra mostly behaves according to the expectations of classical random matrix theory. In particular, in the bulk there is level repulsion and the eigenvectors are delocalized, therefore exhibiting the universal behaviour of chaotic quantum systems.

quant-ph↗

arXiv2023

Multipartite entanglement encoded in the photon-number basis by sequential excitation of a three-level system

We propose a general scheme to generate entanglement encoded in the photon-number basis, via a sequential resonant two-photon excitation of a three-level system. We apply it to the specific case of a quantum dot three-level system, which can emit a photon pair through a biexciton-exciton cascade. The state generated in our scheme constitutes a tool for secure communication, as the multipartite correlations present in the produced state may provide an enhanced rate of secret communication with respect to a perfect GHZ state.

quant-ph↗

arXiv2023

Nonlinear effects in Anderson localization of light by two-level atoms

While Anderson is a single-particle wave effect, guaranteeing a single excitation in the system can be challenging. We here tackle this limitation in the context of light localization in three dimensions in disordered cold atom clouds, in presence of several photons. We show that the presence of these multiple excitations does not affect substantially the abnormal intensity fluctuations which characterize the Anderson localization transition, provided that the radiated light is frequency filtered. Due to their narrow linewidth, long-lived modes, and particularly the localized ones, are strongly saturated even for a weak resonant pump, leading to a large increase of the inelastic scattering and to reduced fluctuations in the total radiation. Yet the atomic coherences and the resulting elastic scattering remain a proper witness of the Anderson localization transition. Hence, frequency filtering allows one to investigate the single-excitation sector, dismissing the many-body effects showing up in the fluorescence spectrum.

physics.atom-ph↗

arXiv2023

Collateral coupling between superconducting resonators: Fast and high fidelity generation of qudit-qudit entanglement

Superconducting circuits are highly controllable platforms to manipulate quantum states, which make them particularly promising for quantum information processing. We here show how the existence of a distance-independent interaction between microwave resonators coupled capacitively through a qubit offers a new control parameter toward this goal. This interaction is able to induce an idling point between resonant resonators, and its state-dependent nature allows one to control the flow of information between the resonators. The advantage of this scheme over previous one is demonstrated through the generation of high-fidelity NOON states between the resonators, with a lower number of operations than previous schemes. Beyond superconducting circuits, our proposal could also apply to atomic lattices with clock transitions in optical cavities, for example.

quant-ph↗

arXiv2023

Single-shot measurements of phonon number states using the Autler-Townes effect

We present a single-shot method to measure motional states in the number basis. The technique can be applied to systems with at least three non-degenerate energy levels which can be coupled to a linear quantum harmonic oscillator, such as in trapped ion experiments. The method relies on probing an Autler-Townes splitting that arises when two levels are strongly coupled via a phonon-number changing transition. We demonstrate the method using a single trapped ion and show that it may be used in a non-demolition fashion to prepare phonon number states. We also show how the Autler-Townes splitting can be used to measure phonon number distributions.

quant-ph↗

arXiv2022

From classical to quantum loss of light coherence

Light is a precious tool to probe matter, as it captures microscopic and macroscopic information on the system. We here report on the transition from a thermal (classical) to a spontaneous emission (quantum) mechanism for the loss of light coherence from a macroscopic atomic cloud. The coherence is probed by intensity-intensity correlation measurements realized on the light scattered by the atomic sample, and the transition is explored by tuning the balance between thermal coherence loss and spontaneous emission via the pump strength. Our results illustrate the potential of cold atom setups to investigate the classical-to-quantum transition in macroscopic systems.

physics.atom-ph↗