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Romain Pierrat

Publications and source records attributed to Romain Pierrat.

34 records · Page 2Linked to original sources

Mean path length invariance in multiple light scattering

Our everyday experience teaches us that the structure of a medium strongly influences how light propagates through it. A disordered medium, e.g., appears transparent or opaque, depending on whether its structure features a mean free path that is larger or smaller than the medium thickness. While the microstructure of the medium uniquely determines the shape of all penetrating light paths, recent theoretical insights indicate that the mean length of these paths is entirely independent of any structural medium property and thus also invariant with respect to a change in the mean free path. Here, we report an experiment that demonstrates this surprising property explicitly. Using colloidal solutions with varying concentration and particle size, we establish an invariance of the mean path length spanning nearly two orders of magnitude in scattering strength, from almost transparent to very opaque media. This very general, fundamental and counterintuitive result can be extended to a wide range of systems, however ordered, correlated or disordered, and has important consequences for many fields, including light trapping and harvesting for solar cells and more generally in photonic structure design.

physics.optics↗

Radiative transfer of acoustic waves in continuous complex media: Beyond the Helmholtz equation

Heterogeneity can be accounted for by a random potential in the wave equation. For acoustic waves in a fluid with fluctuations of both density and compressibility (as well as for electromagnetic waves in a medium with fluctuation of both permittivity and permeability) the random potential entails a scalar and an operator contribution. For simplicity, the latter is usually overlooked in multiple scattering theory: whatever the type of waves, this simplification amounts to considering the Helmholtz equation with a sound speed $c$ depending on position $\mathbf{r}$. In this work, a radiative transfer equation is derived from the wave equation, in order to study energy transport through a multiple scattering medium. In particular, the influence of the operator term on various transport parameters is studied, based on the diagrammatic approach of multiple scattering. Analytical results are obtained for fundamental quantities of transport theory such as the transport mean-free path $\ell^*$, scattering phase function $f$ and anisotropy factor $g$. Discarding the operator term in the wave equation is shown to have a significant impact on $f$ and $g$, yet limited to the low-frequency regime i.e., when the correlation length of the disorder $\ell_c$ is smaller than or comparable to the wavelength $λ$. More surprisingly, discarding the operator part has a significant impact on the transport mean-free path $\ell^*$ whatever the frequency regime. When the scalar and operator terms have identical amplitudes, the discrepancy on the transport mean-free path is around $300\,\%$ in the low-frequency regime, and still above $30\,\%$ for $\ell_c/λ=10^3$ no matter how weak fluctuations of the disorder are. Analytical results are supported by numerical simulations of the wave equation and Monte Carlo simulations.

physics.class-ph↗

Multiple scattering of polarized light in disordered media exhibiting short-range structural correlations

We develop a model based on a multiple scattering theory to describe the diffusion of polarized light in disordered media exhibiting short-range structural correlations. Starting from exact expressions of the average field and the field spatial correlation function, we derive a radiative transfer equation for the polarization-resolved specific intensity that is valid for weak disorder and we solve it analytically in the diffusion limit. A decomposition of the specific intensity in terms of polarization eigenmodes reveals how structural correlations, represented via the standard anisotropic scattering parameter $g$, affect the diffusion of polarized light. More specifically, we find that propagation through each polarization eigenchannel is described by its own transport mean free path that depends on $g$ in a specific and non-trivial way.

physics.optics↗

Spatial correlations of the spontaneous decay rate as a probe of dense and correlated disordered materials

We study theoretically and numerically a new kind of spatial correlation for waves in disordered media. We define $C_Γ$ as the correlation function of the fluorescent decay rate of an emitter at two different positions inside the medium. We show that the amplitude and the width of $C_Γ$ provide decoupled information on the structural correlation of the disordered medium and on the local environment of the emitter. This result may stimulate the emergence of new imaging and sensing modalities in complex media.

physics.optics↗

High-density hyperuniform materials can be transparent

We show that materials made of scatterers distributed on a stealth hyperuniform point pattern can be transparent at densities for which an uncorrelated disordered material would be opaque due to multiple scattering. The conditions for transparency are analyzed using numerical simulations, and an explicit criterion is found based on a perturbative theory. The broad applicability of the concept offers perspectives for various applications in photonics, and more generally in wave physics.

physics.optics↗

Time reversal sub-wavelength focusing in bubbly media

Thanks to a Multiple Scattering Theory algorithm, we present a way to focus energy at the deep subwavelength scale, from the far-field, inside a cubic disordered bubble cloud by using broadband Time Reversal (TR). We show that the analytical calculation of an effective wavenumber performing the Independant Scattering Approximation (ISA) matches the numerical results for the focal extension. Subwavelength focusings of lambda/100 are reported for simulations with perfect bubbles (no loss). A more realistic case, with viscous and thermal losses, allows us to obtain a $λ/14$ focal spot, with a low volume fraction of scatterers (phi = 0.01). Bubbly materials could open new perspective for acoustic actuation in the microfluidic context.

cond-mat.soft↗

Scattering mean-free path in continuous complex media: beyond the Helmholtz equation

We present theoretical calculations of the ensemble-averaged (a.k.a. effective or coherent) wavefield propagating in a heterogeneous medium considered as one realization of a random process. In the literature, it is usually assumed that heterogeneity can be accounted for by a random scalar function of the space coordinates, termed the potential. Physically, this amounts to replacing the constant wavespeed in Helmholtz' equation by a space-dependent speed. In the case of acoustic waves, we show that this approach leads to incorrect results for the scattering mean-free path, no matter how weak fluctuations are. The detailed calculation of the coherent wavefield must take into account both a scalar and an operator part in the random potential. When both terms have identical amplitudes, the correct value for the scattering mean-free paths is shown to be more than four times smaller (13/3, precisely) in the low frequency limit, whatever the shape of the correlation function. Based on the diagrammatic approach of multiple scattering, theoretical results are obtained for the self-energy and mean-free path, within Bourret's and on-shell approximations. They are confirmed by numerical experiments.

physics.class-ph↗

Invariance property of wave scattering through disordered media

A fundamental insight in the theory of diffusive random walks is that the mean length of trajectories traversing a finite open system is independent of the details of the diffusion process. Instead, the mean trajectory length depends only on the system's boundary geometry and is thus unaffected by the value of the mean free path. Here we show that this result is rooted on a much deeper level than that of a random walk, which allows us to extend the reach of this universal invariance property beyond the diffusion approximation. Specifically, we demonstrate that an equivalent invariance relation also holds for the scattering of waves in resonant structures as well as in ballistic, chaotic or in Anderson localized systems. Our work unifies a number of specific observations made in quite diverse fields of science ranging from the movement of ants to nuclear scattering theory. Potential experimental realizations using light fields in disordered media are discussed.

physics.optics↗

Polarization and spatial coherence of electromagnetic waves in uncorrelated disordered media

Spatial field correlation functions represent a key quantity for the description of mesoscopic phenomena in disordered media and the optical characterization of complex materials. Yet many aspects related to the vector nature of light waves have not been investigated so far. We study theoretically the polarization and coherence properties of electromagnetic waves produced by a dipole source in a three-dimensional uncorrelated disordered medium. The spatial field correlation matrix is calculated analytically using a multiple scattering theory for polarized light. This allows us to provide a formal description of the light depolarization process in terms of "polarization eigenchannels" and to derive analytical formulas for the spatial coherence of multiply-scattered light.

physics.optics↗

Strong Coupling to Two-Dimensional Anderson Localized Modes

We use a scattering formalism to derive a condition of strong coupling between a resonant scatterer and an Anderson localized mode for electromagnetic waves in two dimensions. The strong coupling regime is demonstrated based on exact numerical simulations, in perfect agreement with theory. The strong coupling threshold can be expressed in terms of the Thouless conductance and the Purcell factor, thus connecting key concepts in transport theory and cavity quantum electrodynamics.

physics.optics↗

Towards a full characterization of a plasmonic nanostructure with a fluorescent near-field probe

We report on the experimental and theoretical study of the spatial fluctuations of the local density of states (EM-LDOS) and of the fluorescence intensity in the near-field of a gold nanoantenna. EM-LDOS, fluorescence intensity and topography maps are acquired simultaneously by scanning a fluorescent nanosource grafted on the tip of an atomic force microscope at the surface of the sample. The results are in good quantitative agreement with numerical simulations. This work paves the way for a full near-field characterization of an optical nanoantenna.

physics.optics↗

Subwavelength focusing inside an open disordered medium by time reversal at a single point antenna

We study theoretically light focusing at subwavelength scale inside a disordered strongly scattering open medium. We show that broadband time reversal at a single point antenna, in conjunction with near-field interactions and multiple scattering, produces spatial focusing with a quality comparable to that obtained in an ideal closed cavity. This gives new perspectives for super-resolved optical imaging and coherent control of single nanosources or absorbers in complex media.

physics.optics↗

Absorption by an optical dipole antenna in a structured environment

We compute generalized absorption and extinction cross-sections of an optical dipole nanoantenna in a structured environment. The expressions explicitly show the influence of radiation reaction and the local density of states on the intrinsic absorption properties of the antenna. Engineering the environment could allow to modify the overall absorption as well as the frequency and the linewidth of a resonant antenna. Conversely, a dipole antenna can be used to probe the photonic environment, in a similar way as a quantum emitter.

physics.optics↗

Coherent flash of light emitted by a cold atomic cloud

When a resonant laser sent on an optically thick cold atomic cloud is abruptly switched off, a coherent flash of light is emitted in the forward direction. This transient phenomenon is observed due to the highly resonant character of the atomic scatterers. We analyze quantitatively its spatio-temporal properties and show very good agreement with theoretical predictions. Based on complementary experiments, the phase of the coherent field is reconstructed without interferometric tools.

physics.atom-ph↗

Near-field interactions and non-universality in speckle patterns produced by a point source in a disordered medium

A point source in a disordered scattering medium generates a speckle pattern with non-universal features, giving rise to the so-called C_0 correlation. We analyze theoretically the relationship between the C_0 correlation and the statistical fluctuations of the local density of states, based on simple arguments of energy conservation. This derivation leads to a clear physical interpretation of the C_0 correlation. Using exact numerical simulations, we show that C_0 is essentially a correlation resulting from near-field interactions. These interactions are responsible for the non-universality of C_0, that confers to this correlation a huge potential for sensing and imaging at the subwavelength scale in complex media.

physics.optics↗

Enhancement of radiation trapping for quasi-resonant scatterers at low temperature

We present a transport equation for the incoherent propagation of radiation inside a quasi-resonant atomic gas at low temperature. The derivation is based on a generalized Bethe-Salpeter equation taking into account the motion of the atoms. The obtained equation is similar to the radiative transfer equation. It is solved numerically by an original Monte Carlo approach in the case of a slab geometry. The partial frequency redistribution caused by the small velocity of the scatterers make the emitted flux outside the system and the energy density inside the medium to behave differently than in the case of complete frequency redistribution. In particular, the long time dependence of the specific intensity (escape factor) is slightly different from the Holstein prediction.

cond-mat.dis-nn↗