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Rong Yu

Publications and source records attributed to Rong Yu.

At least 37 records · Page 2Linked to original sources

Theory of magnetism for rare-earth magnets on the Shastry-Sutherland lattice with non-Kramers ions

Motivated by the rapid experimental progress on the rare-earth Shastry-Sutherland lattice magnets, we propose a generic effective spin model that describes interacting non-Kramers local moments on the Shastry-Sutherland lattice. We point out that the local moments consist of both magnetic dipole and quadrupole components and the effective model turns out to be an extended XYZ model with an intrinsic field that accounts for the crystal field splitting. We then study the ground-state phase diagram of the model and find that pure quadrupole orders, which are invisible to conventional experimental probes, can be stabilized over a broad regime. In particular, we show that a hidden ``1/3 magnetization plateau'' with quadrupole orders generally exists and discuss its experimental signatures. Finally, we discuss the relevance of our results to the rare-earth Shastry-Sutherland lattice magnets Pr$_{2}$Ga$_{2}$BeO$_{7}$ and Pr$_{2}$Be$_{2}$GeO$_{7}$.

cond-mat.str-el

Two Plaquette-Singlet Phases and Emergent SO(5) Deconfined Quantum Criticality in SrCu2(BO3)2

The deconfined quantum critical point (DQCP) has become a central open concept in the physics of quantum matter, and its proposed presence in the Shastry-Sutherland model was followed by the experimental observation of at least a minimal DQC scenario induced by an applied magnetic field in SrCu$_2$(BO$_3$)$_2$. However, the nature of the plaquette-singlet phase in SrCu$_2$(BO$_3$)$_2$ remains unresolved, and with it the identification of the DQCP symmetry from among several theoretical scenarios. Here we perform detailed high-pressure $^{11}$B NMR studies to reveal the presence of both the full-plaquette (FP) and empty-plaquette (EP) phases in SrCu$_2$(BO$_3$)$_2$, phase-separated at a first-order, pressure-driven transition with a volume-fraction effect. The field-driven transition from the EP to the antiferromagnetic (AFM) phase complements our previous observations of the FP--AFM transition, with both showing deconfined quantum criticality, while the scaling of the spin-lattice relaxation rate near the EP--AFM transition, $1/T_1 \propto T^{0.6}$, suggests a DQCP governed by a different universality class. We discuss possible extensions to the Shastry-Sutherland model that account for these pressure and field effects. The expanded phase space we discover mandates an SO(5) DQCP symmetry, and hence our results take an important step towards a complete understanding of deconfined quantum criticality in SrCu$_2$(BO$_3$)$_2$.

cond-mat.str-el

Thermally activated detection of dark particles in a weakly coupled quantum Ising ladder

The Ising$_h^2$ integrable field theory emerges when two quantum critical Ising chains are weakly coupled. This theory possesses eight types of relativistic particles, among which the lightest one ($B_1$) has been predicted to be a dark particle, which cannot be excited from the ground state through (quasi-)local operations. The stability on one hand highlights its potential for applications, and on the other hand makes it challenging to be observed. Here, we point out that the mass of the $B_1$ dark particle $m_{B_1}$ appears as a thermally activated gap extracted from local spin dynamical structure factor at low frequency ($ω\ll m_{B_1}$) and low temperatures ($T \ll m_{B_1}$). We then further propose that this gapped behavior can be directly detected via the NMR relaxation rate measurement in a proper experimental setup. Our results provide a practical criterion for verifying the existence of dark particles.

cond-mat.str-el

Nematicity in iron pnictides: phase competition and emergent symmetry

The phase diagram of iron-based superconductors contains a host of electronic orders, which are intimately connected with their superconductivity. Here we analyze the fluctuations of one type of nematic order in another. Our analysis leads to an emergent U(1) symmetry at a first-order transition between a nematic phase and a $C_4$-symmetric charge-ordered phase. We characterize the continuous symmetry in terms of a certain hidden Lie algebra that links the different orders. This emergent symmetry leads to a Goldstone mode at the transition and causes softening of excitations in the nematic and charge sectors near the transition. The underlying physics bears a resemblance to the anisotropic XZ spin model, with the nematic order and charge $C_4$ order parameters playing the roles of the $x$ and $z$ components of the magnetization vector, respectively. We provide the experimental evidence in support of the proposed effects, and discuss the general implications of our results for the physics of iron-based superconductors and other correlated systems.

cond-mat.str-el

Spin dynamics and dark particle in a weak-coupled quantum Ising ladder with $\mathcal{D}_8^{(1)}$ spectrum

Emergent Ising$_h^2$ integrability is anticipated in a quantum Ising ladder composed of two weakly-coupled critical transverse field Ising chains. The system is remarkable for including eight types of massive relativistic particles, with their scattering matrix and mass spectrum characterized by the $\mathcal{D}_8^{(1)}$ Lie algebra. In this article, by computing the spin dynamical structure factors following analytical form factor approach, we clearly identify dispersive single-particle excitations of (anti-) soliton and breathers as well as their multi-particle continua in the spectra, which is further confirmed by the numerical simulations. We show that the selection rule inherent in the parity and topological charge of the theory, causes a significant result that charge-parity-odd particles, termed as dark particles, cannot be directly excited from the ground state through any local or quasi-local operations. This in turn suggests the long lifetime of the lightest dark particle.

cond-mat.str-el

Deconfined Quantum Critical Point: A Review of Progress

Deconfined quantum critical points (DQCPs) have been proposed as a class of continuous quantum phase transitions occurring between two ordered phases with distinct symmetry-breaking patterns, beyond the conventional framework of Landau-Ginzburg-Wilson (LGW) theory. At the DQCP, the system exhibits emergent gauge fields, fractionalized excitations, and enhanced symmetries. Here we review recent theoretical and experimental progress on exploring DQCPs in condensed matter systems. We first introduce theoretical advancements in the study of DQCPs over the past twenty years, particularly in magnetic models on square lattices, honeycomb lattices, kagome lattices, and one-dimensional spin chains. We then discuss recent progress on experimental realization of DQCP in quantum magnetic systems. Experimentally, the Shastry-Sutherland model, realized in SrCu$_2$(BO$_3$)$_2$, offers a particularly promising platform for realizing DQCPs. The magnetic frustration inherent to this model drives phase transitions between two distinct symmetry-breaking states: a valence bond solid (VBS) phase and a Néel antiferromagnetic phase. Remarkably, SrCu$_2$(BO$_3$)$_2$ has provided the first experimental evidence of a proximate DQCP through a field-induced Bose-Einstein condensation, transitioning from the VBS state to the Néel state. Nevertheless, the direct experimental realization of a DQCP remains a significant challenge. Despite this, it offers a promising platform for exploring emergent phenomena through quantum phase transition in low-dimensional quantum systems.

cond-mat.str-el

NMR study of supersolid phases in the triangular-lattice antiferromagnet Na2BaCo(PO4)2

We report ultra-low-temperature $^{23}$Na NMR measurements on the Ising triangular lattice antiferromagnet Na$_2$BaCo(PO$_4$)$_2$, which precisely resolve the phase diagram under magnetic field applied along the crystalline $c$ axis. With increasing field, the NMR spectra resolve three ordered phases with distinct spin configurations: the Y, up-up-down (UUD), and V phases. The spin-lattice relaxation rate $1/T_1$ data demonstrate gapless excitations in the Y and V phases, strongly supporting their supersolid nature. However, the phase transitions from the UUD phase to the two supersolid phases exhibit dramatically different behaviors upon cooling. Prior to entering the Y phase, $1/T_1$ identifies a gapless regime within the UUD phase, suggesting a Berezinskii-Kosterlitz-Thouless phase above a second-order phase transition. In contrast, the coexistence of the UUD and V phases observed in our experiments provides direct evidence of a first-order phase transition between these phases.

cond-mat.str-el

Nematic quantum disordered state in FeSe

The unusual quantum-disordered magnetic ground state intertwined with superconductivity and electronic nematicity in FeSe has been a research focus in iron-based superconductors. However, the intrinsic spin excitations across the entire Brillouin zone in detwinned FeSe, which forms the basis for a microscopic understanding of the magnetic state and superconductivity, remain to be determined. Here, we use inelastic neutron scattering to map out the spin excitations of FeSe dewtinned with a uniaxial-strain device. We find that the stripe spin excitations (Q=(1, 0)/(0, 1)) exhibit the $C_2$ symmetry up to $E\approx120$ meV, while the N{é}el spin excitations (Q=(1, 1)) retain their $C_4$ symmetry in the nematic state. The temperature dependence of the difference in the spin excitations at Q=(1, 0) and (0, 1) for temperatures above the structural phase transition unambiguously shows the establishment of the nematic quantum disordered state. The similarity of the Néel excitations in FeSe and NaFeAs suggests that the Néel excitations are driven by the enhanced electron correlations in the $3d_{xy}$ orbital. By determining the key features of the stripe excitations and fitting their dispersions using a Heisenberg Hamiltonian with biquadratic interaction ($J_1$-$K$-$J_2$), we establish a spin-interaction phase diagram and conclude that FeSe is close to a crossover region between the antiferroquadrupolar, Néel, and stripe ordering regimes. The results provide an experimental basis for establishing a microscopic theoretical model to describe the origin and intertwining of the emergent orders in iron-based superconductors.

cond-mat.supr-con

Imaging thick objects with deep-sub-angstrom resolution and deep-sub-picometer precision

Size effects are ubiquitous in the structural, mechanical, and physical properties of materials, making it highly desirable to study the intrinsic properties of thick objects through high-resolution structural analysis in transmission electron microscopy. Although deep-sub-angstrom resolution has been achieved with multislice electron ptychography, the sample thickness is typically very limited. By combining energy filtering and extended local-orbital ptychography (eLOP) that retrieves varying aberrations during electron scanning, here we report ptychographic reconstructions for silicon as thick as 85 nm, approximately three times larger than usual thickness threshold for conventional multislice electron ptychography. The elimination of aberration variations contributes to accurate reconstructions with an information limit of 18 pm and atomic position precision of 0.39 pm. Accurate ptychographic reconstructions for thick objects can facilitate the discovery or interpretation of intrinsic structural and physical phenomena in solids, which is of great significance in physics, chemistry, materials science, and semiconductor device engineering.

cond-mat.mtrl-sci

Orbital-selective correlation effects and superconducting pairing symmetry in a multiorbital $t$-$J$ model for bilayer nickelates

The recent discovery of superconductivity in La$_3$Ni$_2$O$_7$ raises key questions about its mechanism and the nature of pairing symmetry. This system is believed to be described by a bilayer two-orbital Hubbard model. The considerations of orbital-selective Mott correlations motivate a bilayer two-orbital $t$-$J$ model and, accordingly, we study the superconducting pairing in this model. We obtain an overall phase diagram of superconductivity, where the leading channel has either extended $s$-wave or $d_{x^2-y^2}$-wave symmetry. Our analysis highlights how the orbital-selective correlations affect the superconducting pairing via the interlayer exchange couplings and low-energy electronic structure. In particular, we find that the dominant orbital for the pairing may change between $z^2$ and $x^2-y^2$ when the position of the bonding $z^2$ band is varied by tuning either the $c$-axis lattice constant or electron concentration strength. We discuss the implications of these results for the superconductivity in both bulk La$_{3}$Ni$_{2}$O$_{7}$ and its thin film counterpart.

cond-mat.supr-con

Emergence of topological defects and spin liquid in a two-orbital spin-fermion model on the honeycomb lattice

Stabilizing exotic quantum phases of matter, e.g. spin liquid, is an attractive topic in condensed matter. Here, by a Monte Carlo study of a two-orbital spin-fermion model on a honeycomb lattice, we show the cooperative effects of the orbital degeneracy of itinerant electrons and the exchange interaction of localized spins can significantly suppress both ferromagnetic and antiferromagnetic orders by generating topological defects and give rise to an intermediate spin liquid state via continuous phase transitions. This phase competition can also be achieved by tuning the electron filling. These results shed new light on realizing spin liquids on geometrically non-frustrated lattices.

cond-mat.str-el

Haldane phase, field-induced magnetic ordering and Tomonaga-Luttinger liquid behavior in a spin-one chain compound NiC$_2$O$_4$$\cdot$2NH$_3$

We performed single-crystal magnetic susceptibility and $^1$H NMR measurements on a quasi-1D, spin-1 antiferromagnet NiC$_2$O$_4$$\cdot$2NH$_3$, with temperature down to 100 mK and with field up to 26 T. With field applied along the chain direction (crystalline $b$ direction), a spin gap is determined at low fields. Our susceptibility and spin-lattice relaxation measurements reveal a Haldane phase at low field, with an intrachain exchange coupling $J$ $\approx$ 35 K and an easy-plane single-ion anisotropy of 17 K. A field-induced antiferromagnetic (AFM) ordering emerges at fields of 2.1 T, which sets a three-dimensional (3D) quantum critical point (QCP). The high-temperature spin-lattice relaxation rates $1/T_1$ resolves an onset of Tomonaga-Luttinger liquid behavior at field above $3.5$ T, which characterizes a hidden 1D QCP.

cond-mat.str-el

Digital Twin-Empowered Task Assignment in Aerial MEC Network: A Resource Coalition Cooperation Approach with Generative Model

To meet the demands for ubiquitous communication and temporary edge computing in 6G networks, aerial mobile edge computing (MEC) networks have been envisioned as a new paradigm. However, dynamic user requests pose challenges for task assignment strategies. Most of the existing research assumes that the strategy is deployed on ground-based stations or UAVs, which will be ineffective in an environment lacking infrastructure and continuous energy supply. Moreover, the resource mutual exclusion problem of dynamic task assignment has not been effectively solved. Toward this end, we introduce the digital twin (DT) into the aerial MEC network to study the resource coalition cooperation approach with the generative model (GM), which provides a preliminary coalition structure for the coalition game. Specifically, we propose a novel network framework that is composed of an application plane, a physical plane, and a virtual plane. After that, the task assignment problem is simplified to convex optimization programming with linear constraints. And then, we also propose a resource coalition cooperation approach that is based on a transferable utility (TU) coalition game to obtain an approximate optimal solution. Numerical results confirm the effectiveness of our proposed approach in terms of energy consumption and utilization of resources.

cs.NI

Evidence for field induced quantum spin liquid behavior in a spin-1/2 honeycomb magnet

One of the most important issues in modern condensed matter physics is the realization of fractionalized excitations, such as the Majorana excitations in the Kitaev quantum spin liquid. To this aim, the 3d-based Kitaev material Na2Co2TeO6 is a promising candidate whose magnetic phase diagram of B // a* contains a field-induced intermediate magnetically disordered phase within 7.5 T < |B| < 10 T. The experimental observations, including the restoration of the crystalline point group symmetry in the angle-dependent torque and the coexisting magnon excitations and spinon-continuum in the inelastic neutron scattering spectrum, provide strong evidence that this disordered phase is a field induced quantum spin liquid with partially polarized spins. Our variational Monte Carlo simulation with the effective K-J1-Γ-Γ'-J3 model reproduces the experimental data and further supports this conclusion.

cond-mat.str-el

High-quality imaging of large areas through path-difference ptychography

Tilting planar samples for multi-zone-axes observation is a routine procedure in electron microscopy. However, this process invariably introduces optical path differences in the electron beam across different sample positions, significantly compromising image quality, particularly over large fields of view. To address this challenge, we developed path difference ptychography (PDP), a method capable of decoupling path differences from the four-dimensional data during reconstruction. This enables the acquisition of high-quality, large-scale images, facilitating a more comprehensive understanding and analysis of materials microstructure. Moreover, PDP has the potential to promote the widespread application of ptychographic tomography in the analysis of planar samples.

cond-mat.mtrl-sci

Quantum scaling of the spin lattice relaxation rate in the checkerboard $J$-$Q$ model

Motivated by recent progress on the experimental realization of proximate deconfined quantum critical point in a frustrated quantum magnet, we study the low-energy spin dynamics of a related checkerboard $J$-$Q$ model by using quantum Monte Carlo simulations. The ground state of this model undergoes a weakly first-order quantum phase transition with an emergent $O(4)$ symmetry between an antiferromagnetic state and a plaquette valence bond solid. The calculated spin lattice relaxation rate of nuclear magnetic resonance, $1/T_1$, exhibits distinct low-temperature behaviors depending on the ground states. With decreasing the temperature, $1/T_1$ rises up on the antiferromagnetic side, characterizing a crossover to the renormalized classical regime, whereas $1/T_1$ drops exponentially on the side of valence bond solid, reflecting the gap opening in the plaquette ordered phase. The extracted spin gap scales with the distance to the transition point as a power-law with an exponent $ϕ\approx0.3$, consistent with the scaling ansatz $ϕ=νz$ with $ν\approx0.3$ and $z=1$. Near the quantum phase transition, the temperature dependent $1/T_1$ shows a broad crossover regime where a universal scaling $1/T_1\sim T^η$ with $η\approx0.6$ is found. Our results suggest a quantum scaling regime associated with the emergent enhanced symmetry near this first-order quantum phase transition.

cond-mat.str-el

Semiclassical approach to spin dynamics of a ferromagnetic S=1 chain

Motivated by recent experimental progress in the quasi-one-dimensional quantum magnet NiNb$_2$O$_6$, we study the spin dynamics of an S=1 ferromagnetic Heisenberg chain with single-ion anisotropy by using a semiclassical molecular dynamics approach. This system undergoes a quantum phase transition from a ferromagnetic to a paramagnetic state under a transverse magnetic field, and the magnetic responses reflecting this transition is well described by our semiclassical method. We show that at low-temperature the transverse component of the dynamical structure factor depicts clearly the magnon dispersion, and the longitudinal component exhibits two continua associated with single- and two-magnon excitations, respectively. These spin excitation spectra show interesting temperature dependence as effects of magnon interactions.Our findings shed light on experimental detection of spin excitations in a large class of quasi-one-dimensional magnets.

cond-mat.str-el

Hybrid-Generative Diffusion Models for Attack-Oriented Twin Migration in Vehicular Metaverses

The vehicular metaverse is envisioned as a blended immersive domain that promises to bring revolutionary changes to the automotive industry. As a core component of vehicular metaverses, Vehicle Twins (VTs) are digital twins that cover the entire life cycle of vehicles, providing immersive virtual services for Vehicular Metaverse Users (VMUs). Vehicles with limited resources offload the computationally intensive tasks of constructing and updating VTs to edge servers and migrate VTs between these servers, ensuring seamless and immersive experiences for VMUs. However, the high mobility of vehicles, uneven deployment of edge servers, and potential security threats pose challenges to achieving efficient and reliable VT migrations. To address these issues, we propose a secure and reliable VT migration framework in vehicular metaverses. Specifically, we design a two-layer trust evaluation model to comprehensively evaluate the reputation value of edge servers in the network communication and interaction layers. Then, we model the VT migration problem as a partially observable Markov decision process and design a hybrid-Generative Diffusion Model (GDM) algorithm based on deep reinforcement learning to generate optimal migration decisions by taking hybrid actions (i.e., continuous actions and discrete actions). Numerical results demonstrate that the hybrid-GDM algorithm outperforms the baseline algorithms, showing strong adaptability in various settings and highlighting the potential of the hybrid-GDM algorithm for addressing various optimization issues in vehicular metaverses.

cs.AI